We use supervised machine learning together with the concepts of classical density functional theory to investigate the effects of interparticle attraction on the pair structure, thermodynamics, bulk liquid-gas coexistence, and associated interfacial phenomena in many-body systems. Local learning of the one-body direct correlation functional is based on Monte Carlo simulations of inhomogeneous systems

X-ray spectroscopy has been a key method to determine ground- and excited-state properties of quantum materials with atomic specificity. Now, new x-ray facilities are opening the door to the study of pump-probe x-ray spectroscopy—specifically, time-resolved x-ray absorption (trXAS) and time-resolved resonant inelastic x-ray scattering (trRIXS). In this paper, we will present simulations of each of

We propose a novel approach to generate, protect, and control Gottesman-Kitaev-Preskill (GKP) qubits. It employs a microwave frequency comb parametrically modulating a Josephson circuit to enforce a dissipative dynamics of a high-impedance circuit mode, autonomously stabilizing the finite-energy GKP code. The encoded GKP qubit is robustly protected against all dominant decoherence channels plaguing

Active agents are capable of exerting nonreciprocal forces upon one another. For instance, one agent, say A, may attract another agent B while B repels A. These antagonistic nonreciprocal interactions have been extensively studied in classical systems, revealing a wealth of exciting phenomena such as novel phase transitions and traveling-wave states. Whether these phenomena can originate in quantum

Highly excited Rydberg states and their interactions play an important role in quantum computing and simulation. These properties can be predicted accurately for alkali atoms with simple Rydberg level structures. However, an extension of these methods to more complex atoms such as alkaline-earth atoms has not been demonstrated or experimentally validated. Here, we present multichannel quantum defect

The detailed understanding of electronic coherence in quantum systems requires measurements on the attosecond timescale. Attosecond x-ray pulses enable the study of electronic coherence in core-excited molecular systems. Here we report on the coherent motion of electrons in the 1,1-difluoroethylene ion following ionization of the K shell of the two nonequivalent carbon sites with a subfemtosecond x-ray

Charge order pervades the phase diagrams of quantum materials where it competes with superconducting and magnetic phases, hosts electronic phase transitions and topological defects, and couples to the lattice generating intricate structural distortions. Incommensurate charge order is readily stabilized in manganese oxides, where it is associated with anomalous electronic and magnetic properties, but

The extremely low superfluid density and unprecedented tunability of oxide interface superconductors provide an ideal platform for studying fluctuations in two-dimensional superconductors. In this work, we fabricate an LaAlO3/KTaO3 interface superconductor patterned with a nanohoneycomb array of insulating islands. Little-Parks-like magnetoresistance oscillations are observed, which are dictated by

Two-dimensional materials subject to long-wavelength modulations have emerged as novel platforms to study topological and correlated quantum phases. In this article, we develop a versatile and computationally inexpensive method to predict the topological properties of materials subjected to a superlattice potential by combining degenerate perturbation theory with the method of symmetry indicators.

Unmeasured causal forces influence diverse experimental time series, such as the transcription factors that regulate genes or the descending neurons that steer motor circuits. Combining the theory of skew-product dynamical systems with topological data analysis, we show that simultaneous recurrence events across multiple time series reveal the structure of their shared unobserved driving signal. We

Natural communities display a rich variety of dynamics, including global stability, multistability, periodic oscillations, and chaotic fluctuations in species abundances. While phenomenological models (e.g., generalized Lotka-Volterra dynamics) can replicate these dynamic behaviors, understanding biological reasons behind the phenomena requires modeling mechanistic interactions. In this study, we employ

Networks of interconnected materials permeate throughout nature, biology, and technology due to exceptional mechanical performance. Despite the importance of failure resistance in network design and utility, no existing physical model effectively links strand mechanics and connectivity to predict bulk fracture. Here, we reveal a scaling law that bridges these levels to predict the intrinsic fracture

We explore the relationship between higher-form symmetries and entanglement properties in lattice gauge theories with discrete gauge groups, which can exhibit both topologically ordered phases and higher-form symmetry-protected topological (SPT) phases. Our study centers on a generalization of the Fradkin-Shenker model describing Z2 lattice gauge theory with matter, where the Gauss law constraint can

The Hebel-Slichter coherence peak, observed in the spin-lattice relaxation rate 1/T1 just below the critical temperature Tc, serves as a crucial experimental validation of the Bardeen-Cooper-Schrieffer pairing symmetry in conventional superconductors. However, no coherence peak in 1/T1 has been observed in unconventional superconductors like cuprates. In this study, an unconventional coherence peak

Among the wealth of single fluorescent defects recently detected in silicon, the G center catches interest for its telecom single-photon emission that could be coupled to a metastable electron spin triplet. The G center is a unique defect where the standard Born-Oppenheimer approximation used in solid-state physics breaks down as one of its atoms, a silicon atom in interstitial position Si(i), can

The capacity to custom tailor the properties of quantum matter and materials is a central requirement for enlarging their range of possible functionalities. A particularly promising route is the use of driving protocols to engineer specific desired properties with a high degree of control and flexibility. Here, we present such a program for the tunable generation of sequences of symmetries on controllable

We study quantum many-body scars (QMBS) in the language of commutant algebras, which are defined as symmetry algebras of of local Hamiltonians. This framework explains the origin of dynamically disconnected subspaces seen in models with exact QMBS, i.e., the large “thermal” subspace and the small “nonthermal” subspace, which are attributed to the existence of unconventional nonlocal conserved quantities

Quantum complexity is a measure of the minimal number of elementary operations required to approximately prepare a given state or unitary channel. Recently, this concept has found applications beyond quantum computing—in studying the dynamics of quantum many-body systems and the long-time properties of anti–de Sitter black holes. In this context, Brown and Susskind [] conjectured that the complexity

Masers once represented the state of the art in low-noise microwave amplification technology but eventually became obsolete due to their need for cryogenic cooling. Masers based on solid-state spin systems perform most effectively as amplifiers, since they provide a large density of spins and can, therefore, operate at relatively high powers. While solid-state maser oscillators have been demonstrated

We perform extensive molecular dynamics simulations of an ensemble of realistic microgel particles in swollen conditions in a wide range of packing fractions ζ. We compare neutral and charged microgels, where we consider charge distribution adherent to experimental conditions. Through a detailed analysis of single-particle behavior, we are able to identify the different regimes occurring upon increasing

Understanding quantum materials—solids in which interactions among constituent electrons yield a great variety of novel emergent quantum phenomena—is a forefront challenge in modern condensed matter physics. This goal has driven the invention and refinement of several experimental methods, which can spectroscopically determine the elementary excitations and correlation functions that determine material

Magnetoresistance (MR) oscillations serve as a hallmark of intrinsic quantum behavior, traditionally observed only in conducting systems. Here we report the discovery of MR oscillations in an insulating system, the vertical junctions of CrPS4 which is a two-dimensional A-type antiferromagnetic semiconductor. Systematic investigations of MR peaks under varying conditions, including electrode materials

Quantum Darwinism is a paradigm to understand how classically objective reality emerges from within a fundamentally quantum universe. Despite the growing attention that this field of research has been enjoying, it is currently not known what specific properties a given Hamiltonian describing a generic quantum system must have to allow the emergence of classicality. Therefore, in the present work, we

Computational modeling of assembly is challenging for many systems, because their timescales can vastly exceed those accessible to simulations. This article describes the multiMSM, which is a general framework that uses Markov state models (MSMs) to enable simulating self-assembly and self-organization of finite-sized structures on timescales that are orders of magnitude longer than those accessible

While data qubits with a long coherence time are essential for the storage of quantum information, ancilla qubits are pivotal in quantum error correction (QEC) for fault-tolerant quantum computing. The recent development of optical tweezer arrays, such as the preparation of large-scale qubit arrays and high-fidelity gate operations, offers the potential for realizing QEC protocols, and one of the important

In living cells, proteins self-assemble into large functional structures based on specific interactions between molecularly complex patches. Because of this complexity, protein self-assembly results from a competition between a large number of distinct interaction energies, of the order of one per pair of patches. However, current self-assembly models typically ignore this aspect, and the principles

We present a unifying framework that allows us to study the mixed crystalline-electromagnetic responses of topological semimetals in spatial dimensions up to D=3 through dimensional augmentation and reduction procedures. We show how this framework illuminates relations between the previously known topological semimetals and use it to identify a new class of quadrupolar nodal line semimetals for which

Despite its long history, a canonical formulation of quantum ergodicity that applies to general classes of quantum dynamics, including driven systems, has not been fully established. Here we introduce and study a notion of quantum ergodicity for closed systems with time-dependent Hamiltonians, defined as statistical randomness exhibited in their longtime dynamics. Concretely, we consider the temporal

Quantum sensing promises to revolutionize sensing applications by employing quantum states of light or matter as sensing probes. Photons are the clear choice as quantum probes for remote sensing because they can travel to and interact with a distant target. Existing schemes are mainly based on the quantum illumination framework, which requires quantum memory to store a single photon of an initially

Topological semimetals with massless Dirac and Weyl fermions represent the forefront of quantum materials research. In two dimensions, a peculiar class of fermions that are massless in one direction and massive in the perpendicular direction was predicted 16 years ago. These highly exotic quasiparticles—the semi-Dirac fermions—ignited intense theoretical and experimental interest but remain undetected

Decoherence in qubits, caused by their interaction with a noisy environment, poses a significant challenge to the development of reliable quantum processors. A prominent source of errors arises from noise in coupled ancillas, which can quickly spread to qubits. By actively monitoring these noisy ancillas, it is possible to not only identify qubit decoherence events but also to correct these errors

When an ensemble of quantum emitters couples to a common radiation field, their polarizations can synchronize and a collective emission termed superfluorescence can occur. Entering this regime in a free-space setting requires a large number of emitters with a high spatial density as well as coherent optical transitions with small inhomogeneity. Here, we show that, by coupling nitrogen-vacancy centers

We present a new numerical tool designed to probe the dense layers of neutron star crusts. It is based on the time-dependent Hartree-Fock-Bogoliubov theory with generalized Skyrme nuclear energy-density functionals of the Brussels-Montreal family. We use it to study the time evolution of a nucleus accelerating through superfluid neutron medium in the inner crust of a neutron star. We extract an effective

Materials-realistic microscopic theoretical descriptions of copper-based superconductors are challenging due to their complex crystal structures combined with strong electron interactions. Here, we demonstrate how density functional theory can accurately describe key structural, electronic, and magnetic properties of the normal state of the prototypical cuprate Bi2Sr2CaCu2O8+x (Bi-2212). We emphasize

The observation of unexpected polarization textures such as vortices, skyrmions, and merons in various oxide heterostructures has challenged the widely accepted picture of ferroelectric domain walls as being Ising-like. Bloch components in the 180° domain walls of PbTiO3 have recently been reported in PbTiO3/SrTiO3 superlattices and linked to domain wall chirality. While this opens exciting perspectives

We report universal statistical properties displayed by ensembles of pure states that naturally emerge in quantum many-body systems. Specifically, two classes of state ensembles are considered: those formed by (i) the temporal trajectory of a quantum state under unitary evolution or (ii) the quantum states of small subsystems obtained by partial, local projective measurements performed on their complements

Striving for higher gate fidelity is crucial not only for enhancing existing noisy intermediate-scale quantum devices, but also for unleashing the potential of fault-tolerant quantum computation through quantum error correction. A recently proposed theoretical scheme, the double-transmon coupler (DTC), aims to achieve both suppressed residual interaction and a fast high-fidelity two-qubit gate simultaneously

The Kerr-cat qubit is a bosonic qubit in which multiphoton Schrödinger cat states are stabilized by applying a two-photon drive to an oscillator with a Kerr nonlinearity. The suppressed bit-flip rate with increasing cat size makes this qubit a promising candidate to implement quantum error correction codes tailored for noise-biased qubits. However, achieving strong light-matter interactions necessary

Topologically protected edge channels show prospects for quantum devices. They have been found experimentally in two-dimensional quantum spin Hall insulators (QSHIs), weak topological insulators, and higher-order topological insulators, but the number of materials realizing these topologies is still quite limited. Here, we provide evidence for topological edge states within a novel topology named three-dimensional

We consider a dynamic system that is driven by an intensity-modulated Poisson process with intensity Λ(t)=λ(t)+ϵν(t). We derive an exact relation between the input-output cross-correlation in the spontaneous state (ϵ=0) and the linear response to the modulation (ϵ>0). If ϵ is sufficiently small, linear-response theory captures the full response. The relation can be regarded as a variant of the Furutsu-Novikov

In recent demonstrations of the quantum charge-coupled device computer architecture, circuit times are dominated by cooling. Some motional modes of multi-ion crystals take orders of magnitude longer to cool than others because of low coolant ion participation. Here we demonstrate a new technique, that solves this issue by coherently exchanging the thermal populations of selected modes on timescales

The ground state of an homogeneous electron gas is a paradigmatic state that has been used to model and predict the electronic structure of matter at equilibrium for nearly a century. For half a century, it has been successfully used to predict ground states of quantum systems via the local density approximation (LDA) of density functional theory (DFT), and systematic improvements in the form of generalized

Phosphorescent organic light-emitting devices (PHOLEDs) suffer from destructive molecular processes due to triplet-polaron and triplet-triplet annihilation. These processes are energetically driven and hence are particularly active in decreasing the lifetime of blue PHOLEDs. It has recently been shown that increasing triplet radiative rates via the Purcell effect effectively extends the device operational

Attosecond physics enables the study of ultrafast coherent electron dynamics in matter upon photoexcitation and photoionization, revealing spectacular effects such as hole migration and coherent Auger dynamics in molecules. In the photoionization scenario, there has been a strong focus on probing the physical manifestations of internal quantum coherence within the individual parent ion and photoelectron

We report on broad instantaneous bandwidth microwave spectrum analysis with hot Rb87 atoms in a microfabricated vapor cell in a large magnetic field gradient. The sensor is a MEMS atomic vapor cell filled with isotopically pure Rb87 and N2 buffer gas to localize the motion of the atoms. The microwave signals of interest are coupled through a coplanar waveguide to the cell, inducing spin-flip transitions

We study a model of electrons moving in a parent band of uniform Berry curvature. At sufficiently high parent Berry curvature, we show that strong repulsive interactions generically lead to the formation of an anomalous Hall crystal: a topological state with spontaneously broken continuous translation symmetry. Our results are established via a mapping to a problem of Wigner crystallization in a regular

Topology, like symmetry, is a fundamental concept in understanding general properties of physical systems. In condensed matter, nontrivial topology may manifest itself as singular features in the energy spectrum or the quantization of electrical properties such as conductance and magnetic flux. Using microwave spectroscopy, we determine that a superconducting circuit with three Josephson tunnel junctions