Jong, Krijn de - Utrecht University - Inorganic Chemistry and Catalysis

个人简介

Krijn P. de Jong (1954) obtained his MSc in chemistry (1978) and PhD degree in catalysis (1982), both degrees cum laude and at Utrecht University. In 1987 he obtained an MSc in chemical engineering from Twente University. From 1982-1997 he was with Shell Research working on catalyst synthesis, heavy oil conversion, environmental processes, zeolite catalysis and synthesis gas production and conversion. In 1997 he was appointed as full professor of inorganic chemistry and catalysis at Utrecht University. His current research interests are catalyst synthesis and assembly, hydrocarbon conversions over zeolites, solid catalysts for fine chemicals manufacture, conversion of synthesis gas and hydrogen storage. De Jong obtained the Unilever Chemistry Award in 1977, the Shell Patent Award in 1987 and 1991. Furthermore, he was the recipient of the international Award for Excellence in Natural Gas Conversion in 2013. From January 1st 2012 until February 1st 2015, he was appointed as Scientific Director of the Debye Institute for Nanomaterials Science of Utrecht University. He is currently a member of the Technology Advisory Council (TAC) of BP and since October 2015, elected member of the Academia Europaea. In May 2016, de Jong was appointed member of the International Advisory Committee (IAC) at the Key State Laboratory ‘Physical Chemistry of Solid Surfaces’ (PCOSS) of Xiamen University – China.

研究领域

Research interests involve a fundamental understanding of the synthesis of catalysts and functional materials with particular interest in zeolites, mesoporous materials, carbon nanofibers, supported metals and metal oxides, and solid base materials such as hydrotalcites. The work on zeolites comprises generation of mesopores, characterization using electron tomography (3D-TEM) and catalysis. Carbon nanofibers are investigated for their potential as catalysts support materials. Mesoporous materials (e.g. MCM-41, SBA-15) are used as support materials for fundamental studies on catalyst preparation. Most recently we have focused on control of the location of metal nanoparticles in bifunctional catalysts such as Pt/alumina/zeolite catalysts. The approach in our research is to combine the outcome of several techniques into a unifying picture of the complex nanomaterials that are synthesized. The in-house techniques are a.o. in situ XRD, IR, physisorption, TPR-TPD-TPO, TGA, SEM and TEM. As special competencies Electron Tomography, STEM-EDX and Liquid-Phase TEM (Dr. Jovana Zecevic) and high-throughput catalyst testing using a 16-reactor Flowrence set up of Avantium are mentioned. Catalytic studies involve (hydro-)isomerisation of hydrocarbons, selective hydrogenations, aldol-condensation and synthesis gas conversion (paraffins, olefins and alcohols).

近期论文

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Harmel, J; Wal, Van Der L I; Zečević, J; Jongh, De P E; Jong, De K P Influence of intimacy for metal-mesoporous solid acids catalysts for: N -alkanes hydro-conversion Journal Article Catalysis Science and Technology, 10 (7), pp. 2111-2119, 2020. van Deelen, T W; Yoshida, H; Oord, R; Zečević, J; Weckhuysen, B M; de Jong, K P Cobalt nanocrystals on carbon nanotubes in the Fischer-Tropsch synthesis: Impact of support oxidation Journal Article Applied Catalysis A: General, 593 , 2020. Mejía, Hernández C; Vogt, C; Weckhuysen, B M; de Jong, K P Stable niobia-supported nickel catalysts for the hydrogenation of carbon monoxide to hydrocarbons Journal Article Catalysis Today, 343 , pp. 56-62, 2020. Cheng, K; van der Wal, L I; Yoshida, H; Oenema, J; Harmel, J; Zhang, Z; Sunley, G; Zečević, J; de Jong, K P Impact of the Spatial Organization of Bifunctional Metal–Zeolite Catalysts on the Hydroisomerization of Light Alkanes Journal Article Angewandte Chemie - International Edition, 59 (9), pp. 3592-3600, 2020. Weber, J L; Krans, N A; Hofmann, J P; Hensen, E J M; Zecevic, J; de Jongh, P E; de Jong, K P Effect of proximity and support material on deactivation of bifunctional catalysts for the conversion of synthesis gas to olefins and aromatics Journal Article Catalysis Today, 342 , pp. 161-166, 2020. Krans, N A; Weber, J L; Bosch, Van Den W; Zečević, J; Jongh, De P E; Jong, De K P Influence of Promotion on the Growth of Anchored Colloidal Iron Oxide Nanoparticles during Synthesis Gas Conversion Journal Article ACS Catalysis, 10 (3), pp. 1913-1922, 2020. Meijerink, M J; Jong, De K P; Zečević, J Growth of Supported Gold Nanoparticles in Aqueous Phase Studied by in Situ Transmission Electron Microscopy Journal Article Journal of Physical Chemistry C, 124 (3), pp. 2202-2212, 2020. Oenema, J; Hofmann, J P; Hensen, E J M; Zečević, J; de Jong, K P Assessment of the Location of Pt Nanoparticles in Pt/zeolite Y/γ-Al2O3 Composite Catalysts Journal Article ChemCatChem, 12 (2), pp. 615-622, 2020. Keijzer, P H; Donoeva, B; de Jong, K P; de Jongh, P E Supported silver catalysts prepared via melt infiltration: Synthesis, characterization and performance in selective hydrogenation Journal Article Catalysis Today, 2020. Donoeva, B; de Jong, K P Torn between two sites Journal Article Nature Materials, 19 (1), pp. 5-6, 2020. van Deelen, T W; Harmel, J M; Nijhuis, J J; Su, H; Yoshida, H; Oord, R; Zečević, J; Weckhuysen, B M; de Jong, K P Disk-Shaped Cobalt Nanocrystals as Fischer–Tropsch Synthesis Catalysts Under Industrially Relevant Conditions Journal Article Topics in Catalysis, 63 (15-18), pp. 1398-1411, 2020. van Deelen, T W; Yoshida, H; Oord, R; Zečević, J; Weckhuysen, B M; de Jong, K P Cobalt nanocrystals on carbon nanotubes in the Fischer-Tropsch synthesis: Impact of support oxidation Journal Article Applied Catalysis A: General, 593 , 2020. Mejía, Hernández C; Vogt, C; Weckhuysen, B M; de Jong, K P Stable niobia-supported nickel catalysts for the hydrogenation of carbon monoxide to hydrocarbons Journal Article Catalysis Today, 343 , pp. 56-62, 2020. Rivera-Torrente, M; Mejía, Hernández C; Hartman, T; de Jong, K P; Weckhuysen, B M Impact of Niobium in the Metal–Organic Framework-Mediated Synthesis of Co-Based Catalysts for Synthesis Gas Conversion Journal Article Catalysis Letters, 149 (12), pp. 3279-3286, 2019. Xie, J; Paalanen, P P; van Deelen, T W; Weckhuysen, B M; Louwerse, M J; de Jong, K P Promoted cobalt metal catalysts suitable for the production of lower olefins from natural gas Journal Article Nature Communications, 10 (1), 2019. van den Reijen, J E; Versluis, W C; Kanungo, S; d'Angelo, M F; de Jong, K P; de Jongh, P E From qualitative to quantitative understanding of support effects on the selectivity in silver catalyzed ethylene epoxidation Journal Article Catalysis Today, 338 , pp. 31-39, 2019. van Deelen, T W; Mejía, Hernández C; de Jong, K P Control of metal-support interactions in heterogeneous catalysts to enhance activity and selectivity Journal Article Nature Catalysis, 2 (11), pp. 955-970, 2019. Ismail, A S M; Casavola, M; Liu, B; Gloter, A; Deelen, Van T W; Versluijs, M; Meeldijk, J D; Stéphan, O; Jong, De K P; Groot, De F M F Atomic-Scale Investigation of the Structural and Electronic Properties of Cobalt-Iron Bimetallic Fischer-Tropsch Catalysts Journal Article ACS Catalysis, 9 (9), pp. 7998-8011, 2019. Meijerink, M J; de Jong, K P; Zečević, J Assessment of oxide nanoparticle stability in liquid phase transmission electron microscopy Journal Article Nano Research, 12 (9), pp. 2355-2363, 2019. van der Wal, L I; de Jong, K P; Zečević, J The Origin of Metal Loading Heterogeneities in Pt/Zeolite Y Bifunctional Catalysts Journal Article ChemCatChem, 11 (16), pp. 4081-4088, 2019.