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Porous isoreticular non-metal organic frameworks Megan O’Shaughnessy, Joseph Glover, Roohollah Hafizi, Mounib Barhi, Rob Clowes, Samantha Y Chong, Stephen P Argent, Graeme M Day, Andrew I Cooper Nature, 2024, 630, 102, https://doi.org/10.1038/s41586-024-07353-9
Mixed‐Linker Strategy for the Construction of Sulfone‐Containing D–A–A Covalent Organic Frameworks for Efficient Photocatalytic Hydrogen Peroxide Production Chang Shu, Xiaoju Yang, Lunjie Liu, Xunliang Hu, Ruixue Sun, Xuan Yang, Andrew I Cooper, Bien Tan, Xiaoyan Wang Angewandte Chemie, 2024, 136 (22), e202403926, https://doi.org/10.1002/ange.202403926
Conjugated Polymer/Recombinant Escherichia coli Biohybrid Systems for Photobiocatalytic Hydrogen Production Ying Yang, Martijn A Zwijnenburg, Adrian M Gardner, Sylwia Adamczyk, Jing Yang, Yaqi Sun, Qiuyao Jiang, Alexander J Cowan, Reiner Sebastian Sprick, Lu-Ning Liu, Andrew I Cooper ACS Nano, 2024, 18, 21, 13484, https://doi.org/10.1021/acsnano.3c10668
2D to 3D Reconstruction of Boron-Linked Covalent–Organic Frameworks Xue Wang, Thomas Fellowes, Mounib Bahri, Hang Qu, Boyu Li, Hongjun Niu, Nigel D Browning, Weiwei Zhang, John W Ward, Andrew I Cooper J. Am. Chem. Soc.,2024, 146, 20, 14128, https://doi.org/10.1021/jacs.4c0267
Accelerated discovery of molecular nanojunction photocatalysts for hydrogen evolution by using automated screening and flow synthesis Weiwei Zhang, Miaojie Yu, Tao Liu, Muyu Cong, Xueyan Liu, Haofan Yang, Yang Bai, Qiang Zhu, Shuo Zhang, Hongxu Gu, Xiaofeng Wu, Zhiyun Zhang, Yongzhen Wu, He Tian, Xiaobo Li, Wei-Hong Zhu, Andrew I Cooper Nat. Synth., 2024, 3, 595, https://doi.org/10.1038/s44160-024-00494-9
Computationally guided synthesis of a hierarchical [4 [2+ 3]+ 6] porous organic ‘cage of cages’Qiang Zhu, Hang Qu, Gokay Avci, Roohollah Hafizi, Chengxi Zhao, Graeme M Day, Kim E Jelfs, Marc A Little, Andrew I Cooper Nat. Synth, 2024, https://doi.org/10.1038/s44160-024-00531-7
A soft cable loop based gripper for robotic automation of chemistry Lupo Manes, Sebastiano Fichera, Hatem Fakhruldeen, Andrew I Cooper, Paolo Paoletti Sci Rep., 2024, 14, 8899, https://doi.org/10.1038/s41598-024-59372-1
Polymer Photocatalysts with Side Chain Induced Planarity for Increased Activity for Sacrificial Hydrogen Production from Water Richard J Lyons, Ying Yang, Ewan McQueen, Liang Luo, Andrew I Cooper, Martijn A Zwijnenburg, Reiner Sebastian Sprick Adv. Energy Mater., 2024, 14, 2303680, https://doi.org/10.1002/aenm.202303680
Screening potential dye sensitizers for water splitting photocatalysts using a Genetic Algorithm Tao Liu, Linjiang Chen, Xiaoyan Wang, Andrew Cooper Phys. Chem. Chem. Phys., 2024, https://doi.org/10.1039/D4CP01487A
Exploration of the polymorphic solid-state landscape of an amide-linked organic cage using computation and automation Caitlin Elise Shields, Thomas Fellowes, Anna Grace Slater, AI Cooper, Keith G Andrews, Filip Tomasz Szczypiński Chem. Commun., 2024, 60, 6023, https://doi.org/10.1039/d4cc01407c
Fine-tuning GPT-3 for machine learning electronic and functional properties of organic molecules Zikai Xie, Xenophon Evangelopoulos, Ömer H Omar, Alessandro Troisi, Andrew I Cooper, Linjiang Chen Chem. Sci., 2024, 15, 500, https://doi.org/10.1039/D3SC04610A
Modular, multi-robot integration of laboratories: an autonomous workflow for solid-state chemistry Amy M Lunt, Hatem Fakhruldeen, Gabriella Pizzuto, Louis Longley, Alexander White, Nicola Rankin, Rob Clowes, Ben Alston, Lucia Gigli, Graeme M Day, Andrew I Cooper, Samantha Y Chong Chem. Sci., 2024, 15, 2456, https://doi.org/10.1039/D3SC06206F
Machine Learning Accelerated Exploration of Ternary Organic Heterojunction Photocatalysts for Sacrificial Hydrogen Evolution H Yang, Y Che, AI Cooper, L Chen, X Li J. Am. Chem. Soc., 2023, 145 (49), 27038, https://doi.org/10.1021/jacs.3c10586
Domain Knowledge Injection in Bayesian Search for New Materials Z Xie, X Evangelopoulos, J Thacker, A Cooper arXiv preprint arXiv:2311.15162, https://doi.org/10.3233/FAIA230587
Go with the flow: deep learning methods for autonomous viscosity estimations M Walker, G Pizzuto, H Fakhruldeen, AI Cooper Digital Discovery,2023, 2 (5), 1540https://doi.org/10.1039/D3DD00109A
Soft Hydrogen-Bonded Organic Frameworks Constructed Using a Flexible Organic Cage Hinge Qiang Zhu, Lei Wei, Chengxi Zhao, Hang Qu, Bowen Liu, Thomas Fellowes, Siyuan Yang, Alexandra Longcake, Michael J. Hall, Michael R. Probert, Yingbo Zhao, Andrew I. Cooper*, and Marc A. Little* .J. Am. Chem. Soc., 2023, https://doi.org/10.1021/jacs.3c09246
Powder-Bot: A Modular Autonomous Multi-Robot Workflow for Powder X-Ray Diffraction Amy M. Lunt, Hatem Fakhruldeen, Gabriella Pizzuto, Louis Longley, Alexander White, Nicola Rankin, Rob Clowes, Ben M. Alston, Andrew I. Cooper, Samantha Y. Chong .arXiv preprint arXiv:2309.00544, https://doi.org/10.48550/arXiv.2309.00544
Controlling the Crystallisation and Hydration State of Crystalline Porous Organic Salts Megan O'Shaughnessy, Alex C. Padgham, Rob Clowes, Marc A. Little, Michael C. Brand, Hang Qu, Anna G. Slater, Andrew I. Cooper .Chemistry–A European Journal, 2023, e202302420
Fine-tuning GPT-3 for machine learning electronic and functional properties of organic molecules Zikai Xie, Xenophon Evangelopoulos, Ömer Omar, Alessandro Troisi, Andrew I. Cooper, Linjiang Chen .ChemRxiv preprint, https://doi.org/10.26434/chemrxiv-2023-h02j4
HypBO: Expert-Guided Chemist-in-the-Loop Bayesian Search for New Materials Abdoulatif Cisse, Xenophon Evangelopoulos, Sam Carruthers, Vladimir V. Gusev, Andrew I. Cooper .arXiv preprint arXiv:2308.11787, https://doi.org/10.48550/arXiv.2308.11787
Leveraging Multi-modal Sensing for Robotic Insertion Tasks in R&D Laboratories Aaron Butterworth, Gabriella Pizzuto, Leszek Pecyna, Andrew I Cooper, Shan Luo .arXiv preprint arXiv:2307.00671, https://doi.org/10.48550/arXiv.2307.00671
Fluorinated covalent organic frameworks coupled with molecular cobalt cocatalysts for efficient photocatalytic CO2 reduction Zhiwei Fu, Chang Shu, Xiaoyan Wang, Linjiang Chen, Xue Wang, Lunjie Liu, Kewei Wang, Rob Clowes, Samantha Y Chong, Xiaofeng Wu, Andrew I Cooper, CSC Chemistry, 2023, https://doi.org/10.31635/ccschem.023.202202688
Experimental Confirmation of a Predicted Porous Hydrogen‐Bonded Organic Framework Caitlin E Shields, Xue Wang, Thomas Fellowes, Rob Clowes, Linjiang Chen, Graeme M Day, Anna G Slater, John W Ward, Marc A Little, Andrew I Cooper .Chem.Int., 2023, 62, e202303167, https://doi.org/10.1002/anie.202303167
Packing-induced selectivity switching in molecular nanoparticle photocatalysts for hydrogen and hydrogen peroxide production Haofan Yang, Chao Li, Tao Liu, Thomas Fellowes, Samantha Y Chong, Luca Catalano, Mounib Bahri, Weiwei Zhang, Yongjie Xu, Lunjie Liu, Wei Zhao, Adrian M Gardner, Rob Clowes, Nigel D Browning, Xiaobo Li, Alexander J Cowan, Andrew I Cooper .Nature Nanotechnology, 2023, 18 (3), 307, https://doi.org/10.1038/s41565-022-01289-9
Photoresponsive Type III Porous Liquids Michael C Brand, Nicola Rankin, Andrew I Cooper, Rebecca L Greenaway .Chemistry–A European Journal, 2023, 29 (4), e202202848, https://doi.org/10.1002/chem.202202848
Making the connections: Physical and electric interactions in biohybrid photosynthetic systems Ying Yang, Luning Liu, Haining Tian, Andrew Cooper, Reiner Sebastian Sprick .Energy Environ. Sci., 2023, https://doi.org/10.1039/D3EE01265D
Autonomous Biomimetic Solid Dispensing Using a Dual-Arm Robotic Manipulator Ying Jiang, Hatem Fakhruldeen, Gabriella Pizzuto, Louis Longley, Ai He, Tianwei Dai, Rob Clowes, Nicola Rankin, Andrew Cooper .Digital Discovery, 2023, https://doi.org/10.1039/D3DD00075C
Synthetic engineering of a new biocatalyst encapsulating [NiFe]-hydrogenases for enhanced hydrogen production Qiuyao Jiang, Tianpei Li, Jing Yang, Catherine M Aitchison, Jiafeng Huang, Yu Chen, Fang Huang, Qiang Wang, Andrew I Cooper, Lu-Ning Liu .J. Mater. Chem. B, 2023, 11, 2684, https://doi.org/10.1039/D2TB02781J
Investigating the factors that influence sacrificial hydrogen evolution activity for three structurally-related molecular photocatalysts: thermodynamic driving force, excited-state dynamics, and surface interaction with cocatalysts Tao Liu, Linjiang Chen, Xiaobo Li, Andrew I Coope .Phys. Chem. Chem. Phys., 2023, 25, 3494, https://doi.org/10.1039/D2CP04039E
Competitive aminal formation during the synthesis of a highly soluble, isopropyl-decorated imine porous organic cage Rachel J Kearsey, Andrew Tarzia, Marc A Little, Michael C Brand, Rob Clowes, Kim E Jelfs, Andrew I Cooper, Rebecca L Greenaway .Chem. Commun., 2023, 59, 3731, https://doi.org/10.1039/D3CC00072A
Reconstructed covalent organic frameworks .Weiwei Zhang, Linjiang Chen, Sheng Dai, Chengxi Zhao, Cheng Ma, Lei Wei, Minghui Zhu, Samantha Y Chong, Haofan Yang, Lunjie Liu, Yang Bai, Miaojie Yu, Yongjie Xu, Xiao-Wei Zhu, Qiang Zhu, Shuhao An, Reiner Sebastian Sprick, Marc A Little, Xiaofeng Wu, Shan Jiang, Yongzhen Wu, Yue-Biao Zhang, He Tian, Wei-Hong Zhu, Andrew I Cooper .Nature, 2022, 604, 72, https://doi.org/10.1038/s41586-022-04443-4
Using sound to synthesize covalent organic frameworks in water .Wei Zhao, Peiyao Yan, Haofan Yang, Mounib Bahri, Alex M James, Hongmei Chen, Lunjie Liu, Boyu Li, Zhongfu Pang, Rob Clowes, Nigel D Browning, John W Ward, Yue Wu, Andrew I Cooper .Nature Synthesis, 2022, 1, 87, https://doi.org/10.1038/s44160-021-00005-0
Accelerating Laboratory Automation Through Robot Skill Learning For Sample Scraping Gabriella Pizzuto, Hetong Wang, Hatem Fakhruldeen, Bei Peng, Kevin S Luck, Andrew I Cooper .arXiv preprint arXiv:2209.14875, https://doi.org/10.48550/arXiv.2209.14875
Ultrathin metal–organic framework nanosheets exhibiting exceptional catalytic activity Rong-Jia Wei, Pei-Ye You, Haiyan Duan, Mo Xie, Ri-Qin Xia, Xu Chen, Xiaoxu Zhao, Guo-Hong Ning, Andrew I Cooper, Dan L .J. Am. Chem. Soc., 2022, 144 (38), 17487, https://doi.org/10.1021/jacs.2c06312
Hydrogen isotope separation using a metal–organic cage built from macrocycles .Donglin He, Linda Zhang, Tao Liu, Rob Clowes, Marc A Little, Ming Liu, Michael Hirscher, Andrew I Cooper Angew. Chem. Int, 2022, 61, e202202450, https://doi.org/10.1002/anie.202202450
Discovery of a Covalent Triazine Framework Photocatalyst for Visible-Light-Driven Chemical Synthesis using High-Throughput Screening Sriram Vijayakrishnan, John W Ward, Andrew I Cooper ACS Catal., 2022, 12, 10057, https://doi.org/10.1021/acscatal.2c02743
Solis: Autonomous solubility screening using deep neural networks Gabriella Pizzuto, Jacopo De Berardinis, Louis Longley, Hatem Fakhruldeen, Andrew I Cooper 2022 International Joint Conference on Neural Networks (IJCNN), 1-7, 10.1109/IJCNN55064.2022.9892533
Photocatalytic overall water splitting under visible light enabled by a particulate conjugated polymer loaded with palladium and iridium Yang Bai, Chao Li, Lunjie Liu, Yuichi Yamaguchi, Mounib Bahri, Haofan Yang, Adrian Gardner, Martijn A Zwijnenburg, Nigel D Browning, Alexander J Cowan, Akihiko Kudo, Andrew I Cooper, Reiner Sebastian Sprick Angew. Chem.Int. Ed., 2022, 61, e202201299, https://doi.org/10.1002/ange.202201299
Accelerated synthesis and discovery of covalent organic framework photocatalysts for hydrogen peroxide production .Wei Zhao, Peiyao Yan, Boyu Li, Mounib Bahri, Lunjie Liu, Xiang Zhou, Rob Clowes, Nigel D Browning, Yue Wu, John W Ward, Andrew I Cooper .J. Am. Chem. Soc., 2022, 144, 9902, https://doi.org/10.1021/jacs.2c02666
Analogy powered by prediction and structural invariants: computationally led discovery of a mesoporous hydrogen-bonded organic cage crystal Qiang Zhu, Jay Johal, Daniel E Widdowson, Zhongfu Pang, Boyu Li, Christopher M Kane, Vitaliy Kurlin, Graeme M Day, Marc A Little, Andrew I Cooper .J. Am. Chem. Soc.,2022, 144, 9893, https://doi.org/10.1021/jacs.2c02653
Archemist: Autonomous robotic chemistry system architecture Hatem Fakhruldeen, Gabriella Pizzuto, Jakub Glowacki, Andrew Ian Cooper 2022 International Conference on Robotics and Automation (ICRA), 6013-6019, DOI: 10.1109/ICRA46639.2022.9811996
A Pyrene-4, 5, 9, 10-Tetraone-based covalent organic framework delivers high specific capacity as a Li-ion positive electrode Hui Gao, Alex R Neale, Qiang Zhu, Mounib Bahri, Xue Wang, Haofan Yang, Yongjie Xu, Rob Clowes, Nigel D Browning, Marc A Little, Laurence J Hardwick, Andrew I Cooper .J. Am. Chem. Soc.2022, 144, 9434, https://doi.org/10.1021/jacs.2c02196
Room temperature all-solid-state lithium batteries based on a soluble organic cage ionic conductor Jing Li, Jizhen Qi, Feng Jin, Fengrui Zhang, Lei Zheng, Lingfei Tang, Rong Huang, Jingjing Xu, Hongwei Chen, Ming Liu, Yejun Qiu, Andrew I Cooper, Yanbin Shen, Liwei Chen Nat. Commun., 2022, 13, 2031, https://doi.org/10.1038/s41467-022-29743-1
A smart and responsive crystalline porous organic cage membrane with switchable pore apertures for graded molecular sieving Ai He, Zhiwei Jiang, Yue Wu, Hadeel Hussain, Jonathan Rawle, Michael E Briggs, Marc A Little, Andrew G Livingston, Andrew I Cooper .Nature Materials, 2022, 21, 463, https://doi.org/10.1038/s41563-021-01168-z
Targeted design of porous materials without strong, directional interactions Megan O’Shaughnessy, Peter R Spackman, Marc A Little, Luca Catalano, Alex James, Graeme M Day, Andrew I Cooper .Chem. Commun., 2022, 58, 13254, https://doi.org/10.1039/D2CC04682B
Covalent triazine-based frameworks with cobalt-loading for visible light-driven photocatalytic water oxidation Hongmei Chen, Adrian M Gardner, Guoan Lin, Wei Zhao, Mounib Bahri, Nigel D Browning, Reiner Sebastian Sprick, Xiaobo Li, Xiaoxiang Xu, Andrew I Coope Catal. Sci. Technol., 2022, 12, 5442, https://doi.org/10.1039/D2CY00773H
Photoinduced inverse vulcanization Jinhong Jia, Jingjiang Liu, Zhi-Qiang Wang, Tao Liu, Peiyao Yan, Xue-Qing Gong, Chengxi Zhao, Linjiang Chen, Congcong Miao, Wei Zhao, Shanshan Cai, Xi-Cun Wang, Andrew I Cooper, Xiaofeng Wu, Tom Hasell, Zheng-Jun Quan .Nature Chemistry, 2022, 14, 1249, https://doi.org/10.1038/s41557-022-01049-1
Cage molecules stabilize lead halide perovskite thin films Shijing Sun, Ming Liu, Janak Thapa, Noor Titan Putri Hartono, Yicheng Zhao, Donglin He, Sarah Wieghold, Matthew Chua, Yue Wu, Vladimir Bulović, Sanliang Ling, Christoph J Brabec, Andrew I Cooper, Tonio Buonassisi .Chem. Mater., 2022, 34, 9384, https://doi.org/10.1021/acs.chemmater.2c01502
Why do sulfone-containing polymer photocatalysts work so well for sacrificial hydrogen evolution from water? Sam AJ Hillman, Reiner Sebastian Sprick, Drew Pearce, Duncan J Woods, Wai-Yu Sit, Xingyuan Shi, Andrew I Cooper, James R Durrant, Jenny Nelson J. Am. Chem. Soc.2022, 144, 19382, https://doi.org/10.1021/jacs.2c07103
Average Minimum Distances of periodic point sets-foundational invariants for mapping periodic crystals .Daniel Widdowson, Marco M Mosca, Angeles Pulido, Andrew I Cooper, Vitaliy Kurlin MATCH Commun. Math. Comput. Chem., 2022, 87, 529, 10.46793/match.87-3.529W
The changing state of porous materials Jing Li, Jizhen Qi, Feng Jin, Fengrui Zhang, Lei Zheng, Lingfei Tang, Rong Huang, Jingjing Xu, Hongwei Chen, Ming Liu, Yejun Qiu, Andrew I Cooper, Yanbin Shen and Liwei Chen Nat. Comm., 2022, 13, 9865, https://doi.org/10.1038/s41467-022-29743-1
Photocatalytic syngas production using conjugated organic polymers. Zhiwei Fu, Anastasia Vogel, Martijn A. Zwijnenburg, Andrew I. Cooper and Reiner Sebastian Sprick Journal of Materials Chemistry, 2021, DOI: 10.1039/D0TA09613J
Bottom-up wet-chemical synthesis of a two-dimensional porous carbon material with high supercapacitance using a cascade coupling/cyclization route Yongjie Xu, Reiner Sebastian Sprick, Nick J. Brownbill, Frédéric Blanc, Qingyin Li, John W. Ward, Shijie Ren and Andrew I. Cooper J. Mater. Chem. A, 2021, 9, 3303-3308 DOI: 10.1039/D0TA11649A
Melt-quenched porous organic cage glasses Michael C. Brand, Francesca Greenwell, Rob Clowes, Benjamin D. Egleston, Aiting Kai, Andrew I. Cooper, Thomas D. Bennett and Rebecca L. Greenaway J. Mater. Chem. A, 2021, 9, 19807-19816DOI: 10.1039/D1TA01906F
Creating porosity in a trianglimine macrocycle by heterochiral pairing Donglin He, Rob Clowes , Marc A. Little, Ming Liu and Andrew I. Cooper Chem. Commun., 2021, 57, 6141-6144, DOI: 10.1039/D1CC01650D
Combining machine learning and high-throughput experimentation to discover photocatalytically active organic molecules Xiaobo Li, Phillip M. Maffettone, Yu Che, Tao Liu, Linjiang Chen and Andrew I. Cooper Chem. Sci., 2021, 12, 10742-10754, DOI: 10.1039/D1SC02150H
Photocatalytic polymers of intrinsic microporosity for hydrogen production from water Yang Bai, Liam Wilbraham, Hui Gao, Rob Clowes, Haofan Yang, Martijn A. Zwijnenburg, Andrew I. Cooper and Reiner Sebastian Sprick J. Mater. Chem. A, J. Mater. Chem. A, 2021, 9, 19958-19964, DOI: 10.1039/D1TA03098A
Acetylene-linked conjugated polymers for sacrificial photocatalytic hydrogen evolution from water Lunjie Liu, Michał A. Kochman, Yongjie Xu, Martijn A. Zwijnenburg, Andrew I. Cooper and Reiner Sebastian Sprick J. Mater. Chem. A, 2021, 9, 17242-17248, DOI: 10.1039/D1TA04288B
Exploring cooperative porosity in organic cage crystals using in situ diffraction and molecular simulations Linjiang Chen, Yu Che, Andrew I. Cooper and Samantha Y. Chong Royal Society of Chemistry, Faraday Discuss., 2021, 225, 100
Digital navigation of energy–structure–function maps for hydrogen-bonded porous molecular crystals Chengxi Zhao, Linjiang Chen, Yu Che, Zhongfu Pang, Xiaofeng Wu, Yunxiang Lu, Honglai Liu , Graeme M. Day and Andrew I. Cooper Nature Communication, volume 12, Article number: 817, 2021,
Probing Dynamics of Water Mass Transfer in Organic Porous Photocatalyst Water-Splitting Materials by Neutron Spectroscopy Mohamed Zbiri, Catherine M. Aitchison, Reiner Sebastian Sprick, Andrew I. Cooper and Anne A. Y. Guilbert Chem. Mater. ,33, 1363-1372, 2021,
Crystallography companion agent for high-throughput materials discovery Phillip M. Maffettone, Lars Banko, Peng Cui, Yury Lysogorskiy, Marc A. Little, Daniel Olds, Alfred Ludwig and Andrew I. Cooper Nat. Comut. Sci. 1, 290, 2021 DOI: 10.1038/s43588-021-00059-2
The changing state of porous materials Thomas D. Bennett , François-Xavier Coudert , Stuart L. James and Andrew I. Cooper Nature Materials, VOL 20, 1179–1187, 2021,
Inherent Ethyl Acetate Selectivity in a Trianglimine Molecular Solid Donglin He, Chengxi Zhao, Linjiang Chen, Marc A. Little, Samantha Y. Chong, Rob Clowes, Katherine McKie, Mark G. Roper, Graeme M. Day, Ming Liu and Andrew I. Cooper Chem. Eur. J., 27, 10589 –10594, 2021,
SO2 Capture Using Porous Organic Cages Eva Martínez-Ahumada, Donglin He, Victoria Berryman, Alfredo López-Olvera, Magali Hernandez, Vojtech Jancik, Vladimir Martis, Marco A. Vera, Enrique Lima, Douglas J. Parker, Andrew I. Cooper, Ilich A. Ibarra and Ming Liu Angew.Chem. Int.Ed. 2021, 60,17556–17563,
Modular Type III Porous Liquids Based on Porous Organic Cage Microparticles Aiting Kai ,Benjamin D. Egleston, Andrew Tarzia, Rob Clowes, Michael E. Briggs, Kim E. Jelfs, Andrew I. Cooper and Rebecca L. Greenaway Adv. Funct. Mater. 202106116, 2021,
Dynamics in Flexible Pillar[n]arenes Probed by Solid-State NMR Ashlea R. Hughes, Ming Liu, Subhradip Paul, Andrew I. Cooper, and Frédéric Blanc J. Phys. Chem. 125, 13370−13381, 2021,