Dai, Sheng - Oak Ridge National Laboratory - Chemical Sciences Division

个人简介

Dr. Sheng Dai is currently a corporate fellow and section head overseeing four research groups in the areas of separations and polymer chemistry at Chemical Sciences Division, Oak Ridge National Laboratory (ORNL) and a Professor of Chemistry at the University of Tennessee, Knoxville (UTK). His current research interests include ionic liquids, porous materials, and their applications for separation sciences and energy storage as well as catalysis by nanomaterials. He was named US DOE Distinguished Scientist Fellow for pioneering advances in development of functional materials in 2022. His research has led to the 2020 Max Bredig Award for Ionic Liquids and Molten Salts, the 2019 ACS Award in Separation Science and Technology, 2018 IMMA Award given by International Mesostructured Materials Association, Battelle Distinguished Inventor Award in 2016, and six R&D100 Awards. He is a Fellow of Material Research Society and Fellow of the American Association for the Advancement of Science.

研究领域

His current research interests include ionic liquids, porous materials, and their applications for separation sciences and energy storage as well as catalysis by nanomaterials.

近期论文

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Molten salt electrochemical upcycling of CO2 to graphite for high performance battery anodes... Journal: Carbon August, 2023 Selective deconstruction of mixed plastics by a tailored organocatalyst... Journal: Materials Horizons July, 2023 A one-pot synthesis of high-density biofuels through bifunctional mesoporous zeolite-encapsulated Pd catalysts... Journal: Applied Catalysis B June, 2023 Expeditious Coordination-Driven Construction of Hierarchically Nanoporous Barium Salts... Journal: CCS Chemistry June, 2023 High-performance CO2 Capture from Air by Harnessing the Power of CaO- and Superbase Ionic Liquid-Engineered Sorbents... Journal: ChemSusChem June, 2023 High-performance CO2 Capture from Air by Harnessing the Power of CaO- and Superbase Ionic Liquid-Engineered Sorbents... Journal: ChemSusChem June, 2023 Construction of Boron- and Nitrogen-Enriched Nanoporous π-Conjugated Networks Towards Enhanced Hydrogen Activation... Journal: Angewandte Chemie International Edition May, 2023 Construction of conjugated scaffolds driven by mechanochemistry towards energy storage applications... Journal: Green Chemical Engineering April, 2023 Ionothermally Synthesized Nanoporous Ti0.95W0.05Nb2O7: a Novel Anode Material for High-Performance Lithium-Ion Batteries... Journal: Batteries & Supercaps April, 2023 Mechanochemistry-Induced Strong Metal–Support Interactions Construction toward Enhanced Hydrogenation... Journal: ACS Catalysis April, 2023 Probing sub-5 Ångstrom micropores in carbon for precise light olefin/paraffin separation... Journal: Nature Communications March, 2023 Electrochemical CO2-to-ethylene conversion on metal-free covalent quinazoline network-derived electrodes... Journal: Chem Catalysis February, 2023 Nonclassical Strong Metal–Support Interactions for Enhanced Catalysis... Journal: The Journal of Physical Chemistry Letters February, 2023 In-situ synthesis of porous metal fluoride@carbon composite via simultaneous etching/fluorination enabled superior Li storage... Journal: Nano Energy December, 2022 Construction of Nitrogen-abundant Graphyne Scaffolds via Mechanochemistry-Promoted Cross-Linking of Aromatic Nitriles with Ca... Journal: Small December, 2022 Strategies for design and synthesis of porous liquids toward carbon capture and separation... Journal: Current Opinion in Green and Sustainable Chemistry December, 2022 Complete Description of the LaCl3–NaCl Melt Structure and the Concept of a Spacer Salt That Causes Structural Heterogeneity... Journal: Journal of the American Chemical Society November, 2022 CO2 Chemisorption Behavior in Conjugated Carbanion-Derived Ionic Liquids via Carboxylic Acid Formation... Journal: Journal of the American Chemical Society November, 2022 Engineering Nanostructured Interfaces of Hexagonal Boron Nitride-Based Materials for Enhanced Catalysis... Journal: Accounts of Chemical Research November, 2022 Electrochemical noise studies on localized corrosion of Ni and Ni-20Cr in molten ZnCl2... Journal: Electrochimica Acta November, 2022 Conformal LiF Stabilized Interfaces via Electrochemical Fluorination on High Voltage Spinel Cathodes (≈4.9 V) for Lithium-... Journal: Advanced Materials Interfaces October, 2022 Enhanced Carbon Capture Behavior of Carbon Fibers via Ionic Liquid Modification... Journal: ChemNanoMat October, 2022 Computational Insights into Malononitrile-Based Carbanions for CO2 Capture... Journal: The Journal of Physical Chemistry B September, 2022 Prospective Life Cycle Assessment of Synthetic Graphite Manufactured via Electrochemical Graphitization... Journal: ACS Sustainable Chemistry & Engineering September, 2022 Construction of Fluorine- and Piperazine-Engineered Covalent Triazine Frameworks Towards Enhanced Dual-Ion Positive Electrode... Journal: ChemSusChem August, 2022 Enhanced Oxygen Activation Achieved by Robust Single Chromium Atom-Derived Catalysts in Aerobic Oxidative Desulfurization... Journal: ACS Catalysis July, 2022 Insight into the Fast-Rechargeability of a Novel Mo 1.5 W 1.5 Nb 14 O 44 Anode Material for High-Performance Lithium-Ion Batt... Journal: Advanced Energy Materials July, 2022 Fully Conjugated Poly(phthalocyanine) Scaffolds Derived from a Mechanochemical Approach Towards Enhanced Energy Storage... Journal: Angewandte Chemie International Edition July, 2022 Design of a multi-functional gel polymer electrolyte with a 3D compact stacked polymer micro-sphere matrix for high-performan... Journal: Journal of Materials Chemistry A June, 2022 Two Ligands of Interest in Recovering Uranium from the Oceans: The Correct Formation Constants of the Uranyl(VI) Cation with ... Journal: Inorganic Chemistry June, 2022 Mechanochemistry-driven phase transformation of crystalline covalent triazine frameworks assisted by alkaline molten salts... Journal: Journal of Materials Chemistry A June, 2022 Defect Engineering of Ceria Nanocrystals for Enhanced Catalysis via a High-Entropy Oxide Strategy... Journal: ACS Central Science June, 2022 Real-Space Local Dynamics of Molten Inorganic Salts Using Van Hove Correlation Function... Journal: The Journal of Physical Chemistry Letters June, 2022 Ionic liquids for carbon capture... Journal: MRS Bulletin May, 2022 Mechanochemistry-Driven Construction of Aza-fused π-Conjugated Networks Toward Enhanced Energy Storage... Journal: Advanced Functional Materials May, 2022 Ultrasound-mediated synthesis of nanoporous fluorite-structured high-entropy oxides toward noble metal stabilization... Journal: iScience May, 2022 Defect-Regulated Frustrated-Lewis-Pair Behavior of Boron Nitride in Ambient Pressure Hydrogen Activation... Journal: Journal of the American Chemical Society May, 2022 Single Atoms Anchored in Hexagonal Boron Nitride for Propane Dehydrogenation from First Principles... Journal: ChemCatChem May, 2022 Mechanochemically Assisted Synthesis of High-Entropy Layer-Structured Dittmarite Analogues... Journal: ACS Applied Energy Materials March, 2022 Direct Correlation of the Salt-Reduced Diffusivities of Organic Solvents with the Solvent’s Mole Fraction... Journal: The Journal of Physical Chemistry Letters March, 2022 Ionothermal Synthesis of Carbon/TiO 2 Nanocomposite for Supercapacitors... Journal: ChemNanoMat February, 2022 Flux upcycling of spent NMC 111 to nickel-rich NMC cathodes in reciprocal ternary molten salts... Journal: iScience February, 2022 Enhancing Cycling Stability and Capacity Retention of NMC811 Cathodes by Reengineering Interfaces via Electrochemical Fluorin... Journal: Advanced Materials Interfaces February, 2022 Beyond Simple Dilution: Superior Conductivities from Cosolvation of Acetonitrile/LiTFSI Concentrated Solution with Acetone... Journal: The Journal of Physical Chemistry C January, 2022 Intra-crystalline mesoporous zeolite encapsulation-derived thermally robust metal nanocatalyst in deep oxidation of light alk... Journal: Nature Communications January, 2022 Beyond Simple Dilution: Superior Conductivities from Cosolvation of Acetonitrile/LiTFSI Concentrated Solution with Acetone... Journal: The Journal of Physical Chemistry C January, 2022 Highly Perfluorinated Covalent Triazine Frameworks Derived from a Low-Temperature Ionothermal Approach Towards Enhanced CO 2 ... Journal: Angewandte Chemie International Edition December, 2021 A High Temperature Cell for Investigating Interfacial Structure on the Molecular Scale in Molten Salt/Alloy Systems... Journal: Review of Scientific Instruments December, 2021 Surpassing the Organic Cathode Performance for Lithium-Ion Batteries with Robust Fluorinated Covalent Quinazoline Networks... Journal: ACS Energy Letters December, 2021 New-Generation Carbon-Capture Ionic Liquids Regulated by Metal-Ion Coordination... Journal: ChemSusChem December, 2021 FTIR investigation of the interfacial properties and mechanisms of CO2 sorption in porous ionic liquids... Journal: Green Chemical Engineering December, 2021 Challenges in engineering the structure of ionic liquids towards direct air capture of CO2... Journal: Green Chemical Engineering December, 2021 Operando Analysis of Gas Evolution in TiNb2O7 (TNO)-Based Anodes for Advanced High-Energy Lithium-Ion Batteries under Fast Ch... Journal: ACS Applied Materials & Interfaces November, 2021 Visualizing time-dependent microstructural and chemical evolution during molten salt corrosion of Ni-20Cr model alloy using c... Journal: Corrosion Science November, 2021 Benchmark CO2 separation achieved by highly fluorinated nanoporous molecular sieve membranes from nonporous precursor via in ... Journal: Journal of Membrane Science November, 2021 Benchmark CO2 separation achieved by highly fluorinated nanoporous molecular sieve membranes from nonporous precursor via in ... Journal: Journal of Membrane Science November, 2021 Strategies toward the Synthesis of Advanced Functional Sorbent Performance for Uranium Uptake from Seawater... Journal: Industrial & Engineering Chemistry Research October, 2021 A bifunctional zeolitic porous liquid with incompatible Lewis pairs for antagonistic cascade catalysis... Journal: Chem September, 2021 A Holistic Approach for Elucidating Local Structure, Dynamics, and Speciation in Molten Salts with High Structural Disorder... Journal: Journal of the American Chemical Society September, 2021 High-Entropy Catalysts: Supremacy of Diversity... Journal: Chem Catalysis August, 2021