宋礼 - 中国科学技术大学 - 国家同步辐射实验室

个人简介

2001-2006，中国科学院物理研究所，硕/博士（导师：解思深院士） 2006-2008，德国慕尼黑大学，洪堡学者（合作导师：Katthaus 教授） 2008-2011，美国Rice大学，博士后（合作导师： Ajayan 教授） 2011-2012，日本信州大学，准教授 2012-至今，中国科学技术大学，教授

研究领域

Electrocatalysis The intermittency of energy supply from renewable and clean resources, such as solar, wind, geothermy, etc, has largely hampered the economic development and reduced the efficiency of energy utilization. Conversing these intermittent and localized energies into energy-dense molecules via electrocatalysis is regarded as a promising pathway to mitigate the intermittency problem. Among a series of electrochemical conversion reactions, water splitting and carbon dioxide reduction can produce clean hydrogen and reduce carbon dioxide emission respectively, therefore drawing a lot of attention from researchers. So far, precious metals are still the most active ones to catalyze the electrochemical conversion of reactants. One research interest of our group is to rationally design efficient non-precious catalysts or largely reduce the usage of precious metals while keeping or even improving the activity of catalysts. Energy storage system The development of electrochemical energy storage materials and the study of energy storage mechanism are very important for the sustainable development of new energy. Our research group focused on a variety of electrochemical energy storage devices such as Li+, Na+ battery; aqueous Zn2+ battery and supercapacitors, etc. We study on the design and development of two-dimensional electrode materials (transition metal sulfides, oxides and carbides, etc.) with promising energy storage performance. The structure of electrode materials was deeply studied by means of various synchrotron radiation spectroscopy (XAFS, XPS, XRD, etc.), and the energy storage mechanism was explored by ex/in situ XAFS, ex/in situ XRD and other characterization methods (ex/in situ Raman, etc.). Synthesis and device application Two-dimensional quantum materials, including graphene, h-BN, TMDCs, MXenes, etc., have shown abundance of exotic physical properties and are expected to be applied in electronics and photoelectronic devices with ultra-low power. The exploration of new materials is of importance to physical property engineering and device applications. By combination of theoretical calculations and predictions, we use a variety of growth means including CVD and CVT method to obtain high quality 2D materials, with the help of synchrotron radiation X-Ray absorption spectroscopy (XAS) and synchrotron radiation angular resolution photoelectron spectroscopy (ARPES) and other advanced characterization methods, we explore the basic physical properties of materials such as optical, electrical and magnetic properties. For 2D materials showing application potential, we further design and construct on-chip devices for optoelectronic response or electrocatalysis.

近期论文

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Synchrotron-radiation spectroscopic identification towards diverse local environments of single-atom catalysts Author(s): Sicong, Qiao; Qun, He; et al. Source: Journal of Materials Chemistry A. DOI: 10.1039/D1TA08254J Defect engineering on V2O3 cathode for long-cycling aqueous zinc metal batteries Author(s): Zhu, Kefu; Wei, Shiqiang;Shou, Hongwei; et al. Source: Nature communications. DOI: 10.1038/s41467-021-27203-w Carbon Nanotubes-Based Electrocatalysts: Structural Regulation, Support Effect, and Synchrotron-Based Characterization Author(s): Qun, He; Sicong Qiao;Yuzhu, Zhou; et al. Source: Advanced Functional Materials. DOI: 10.1002/adfm.202106684 Support induced phase engineering toward superior electrocatalyst Author(s): Sheng, Beibei; Cao, Dengfeng;Shou, Hongwei; et al. Source: Nano Research. DOI: 10.1007/s12274-021-3761-9 Robust and High Photoluminescence in WS2 Monolayer through In Situ Defect Engineering Author(s): Cui, Qilong; Luo, Ziyu; et al. Source: Advanced Functional Materials. DOI: 10.1002/adfm.202105339 HCl-Based Hydrothermal Etching Strategy toward Fluoride-Free MXenes Author(s): Wang, Changda; Shou, Hongwei; et al. Source: Advanced Materials. DOI: 10.1002/adma.202101015 Manganese buffer induced high-performance disordered MnVO cathodes in zinc batteries Author(s): Wei, Shiqiang; Chen, Shuangming; et al. Source: Energy Environ. Sci. DOI: 10.1039/d1ee00590a Short-Range Ordered Iridium Single Atoms Integrated into Cobalt Oxide Spinel Structure for Highly Efficient Electrocatalytic Water Oxidation Author(s): Shan, Jieqiong; Ye, Chao; et al. Source: Journal of the American Chemical Society DOI: 10.1021/jacs.1c01525 Interfacial engineering of heterogeneous catalysts for electrocatalysis Author(s): Zhang, Youkui; Lin, Yunxiang; et al. Source: Materials Today DOI: 10.1016/j.mattod.2021.02.004 Facile modulation of different vacancies in ZnS nanoplates for efficient solar fuel production Author(s): Li, Pan; Guo, Lingju; et al. Source: Journal of Materials Chemistry A DOI: 10.1039/D0TA12400A Probing self-optimization of carbon support in oxygen evolution reaction Author(s): Xu, Wenjie; Cao, Dengfeng et al. Source: Nano Research DOI: 10.1007/s12274-021-3368-1 Title: Ternary VOCl single-crystal as efficient gate dielectric for 2D field-effect transistors Author(s): Zhu, Wen; Cui, Qilong; et al. Source: 2D Materials DOI: 10.1088/2053-1583/abd288 Title: Operando X-ray spectroscopy visualizing the chameleon-like structural reconstruction on an oxygen evolution electrocatalyst Author(s): Cao, Dengfeng; Liu, Daobin; et al. Source: Energy Environ. Sci. DOI: 10.1039/D0EE02276D Title: Anomalous self-optimization of sulfate ions for boosted oxygen evolution reaction Author(s): Cao, Dengfeng; Oyawale Adetunji Moses; et al. Source: Science Bulletin DOI: 10.1016/j.scib.2020.09.037 Title: High-power lithium–selenium batteries enabled by atomic cobalt electrocatalyst in hollow carbon cathode Author(s): Tian, Hao; Tian, Huajun; et al. Source: Nature Communications DOI: 10.1038/s41467-020-18820-y Title: Atomic-Level Insights into the Edge Active ReS2 Ultrathin Nanosheets for High-Efficiency Light-to-Hydrogen Conversion Author(s): Ran, Jingrun; Zhang, Hongping; et al. Source: ACS Materials Letters DOI: 10.1021/acsmaterialslett.0c00205 Title: CdPS3 nanosheets-based membrane with high proton conductivity enabled by Cd vacancies Author(s): Qian, Xitang; Chen, Long; et al. Source: Science DOI: 10.1126/science.abb9704 Title: Multiphonon Raman Scattering and Strong Electron–Phonon Coupling in 2D Ternary Cu2MoS4 Nanoflakes Author(s): Qin, Liang; Wen, Zhilin; et al. Source: The Journal of Physical Chemistry Letters DOI: 10.1021/acs.jpclett.0c02530 Title: Computational Screening toward Hydrogen Evolution Reaction by the Introduction of Point Defects at the Edges of Group IVA Monochalcogenides: A First-Principles Study Author(s): Zhang, Bo; Fu, Xiuli; et al. Source: The Journal of Physical Chemistry Letters DOI: 10.1021/acs.jpclett.0c02047 Title: On the nature of Pt-carbon interactions for enhanced hydrogen generation Author(s): Chen, Wenyao; Chen, Shuangming; et al. Source: Journal of Catalysis DOI: 10.1016/j.jcat.2020.06.028 A Unique Ru-N4-P Coordinated Structure Synergistically Waking Up the Nonmetal P Active Site for Hydrogen Production Author(s): Wu, Chuanqiang; Ding, Shiqing; et al. Source: Research DOI: 10.34133/2020/5860712 Structural Regulation and Support Coupling Effect of Single‐Atom Catalysts for Heterogeneous Catalysis Author(s): Liu, Daobin; He, Qun; et al. Source: Advanced Energy Materials DOI: 10.1002/aenm.202001482 Structural Designs and in‐situ X‐ray Characterizations of Metal Phosphides for Electrocatalysis Author(s): Zhang, Youkui; Song, Li Source: ChemCatChem DOI: 10.1002/cctc.202000233 Electrochemical Conversion of CO2 to Syngas with Controllable CO/H2 Ratios over Co and Ni Single‐Atom Catalysts Author(s): He, Qun; Liu, Daobin; et al. Source: Angewandte Chemie International Edition DOI: 10.1002/anie.201912719 Tuning 2D MXenes by Surface Controlling and Interlayer Engineering: Methods, Properties, and Synchrotron Radiation Characterizations Author(s): Wang, Changda; Chen, Shuangming; et al. Source: Advanced Functional Materials DOI: 10.1002/adfm.202000869 Accelerating CO2 Electroreduction to CO Over Pd Single‐Atom Catalyst Author(s): Qun, He; Ji Hoon Lee; et al. Source: Advanced Functional Materials DOI: 10.1002/adfm.202000407 A Hydrogenated Metal Oxide with Full Solar Spectrum Absorption for Highly Efficient Photothermal Water Evaporation Author(s): Zhu, Qing; Ye, Ke; et al. Source: The Journal of Physical Chemistry Letters DOI: 10.1021/acs.jpclett.0c00592 Achieving Efficient Alkaline Hydrogen Evolution Reaction over a Ni5P4 Catalyst Incorporating Single‐Atomic Ru Sites Author(s): He, Qun; Tian, Dong; et al. Source: Advanced Materials DOI: 10.1002/adma.201906972 Dial the Mechanism Switch of VN from Conversion to Intercalation toward Long Cycling Sodium‐Ion Battery Author(s): Wei, Shiqiang; Wang, Changda; et al. Source: Advanced Energy Materials DOI: 10.1002/aenm.201903712