Brudvig, Gary W - Yale University - Biological & Biomedical Sciences

个人简介

A graduate of the University of Minnesota, Prof. Gary Brudvig earned his Ph.D. at the California Institute of Technology. He joined the Yale faculty in 1982. In addition to serving as a professor in and chair of the Department of Chemistry, he is also a professor of molecular biophysics and biochemistry and is affiliated with the Yale Center for Green Chemistry. Brudvig is the project leader of a team of Yale chemists and other scientists who, under the auspices of the U.S. Department of Energy, are hoping to improve the efficiency of solar-energy utilization. Its aim is to attach manganese complexes to titanium dioxide nanoparticles in order to develop a system that will efficiently produce renewable fuel using solar energy. From 1983 to 1986, Brudvig was a Searle Scholar at Yale. The Searle Scholarship program supports outstanding work by junior faculty members at select academic institutions. He was the Camille and Henry Dreyfus Teacher Scholar, a distinction given to “talented young faculty in the chemical sciences,” from 1985 to 1990. He was an Alfred P. Sloan Research Fellow 1986-1988. Brudvig was elected to the American Academy of Arts and Sciences in 1995. Miller Fellow University of California, Berkeley, CA

研究领域

Electron Spin Resonance Spectroscopy; Metalloproteins; Molecular Biology; Photosynthesis

近期论文

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Chloride Regulation of Enzyme Turnover: Application to the Role of Chloride in Photosystem II Pokhrel, R., McConnell, I.L. and Brudvig, G.W. (2011) Chloride Regulation of Enzyme Turnover: Application to the Role of Chloride in Photosystem II. Biochemistry 50, 2725–2734. Energy Conversion in Photosynthesis: A Paradigm for Solar Fuel Production Moore, G.F. and Brudvig, G.W. (2011) Energy Conversion in Photosynthesis: A Paradigm for Solar Fuel Production. Annu. Rev. Condensed Matter Phys. 2, 303-327. Quantum Mechanics/Molecular Mechanics Study of the Catalytic Cycle of Water Splitting in Photosystem II. Sproviero, E.M., Gascón, J.A., McEvoy, J.P., Brudvig, G.W. and Batista, V.S. (2008) Quantum Mechanics/Molecular Mechanics Study of the Catalytic Cycle of Water Splitting in Photosystem II. J. Am. Chem. Soc. 130, 3428-3442. Molecular recognition in the selective oxygenation of saturated C-H bonds by a dimanganese catalyst. Das, S., Incarvito, C.D., Crabtree, R.H., and Brudvig, G.W. (2006) Molecular recognition in the selective oxygenation of saturated C-H bonds by a dimanganese catalyst. Science 312:1119-1134. Water-splitting chemistry of Photosystem II. McEvoy, J.P. and Brudvig, G.W. (2006) Water-splitting chemistry of Photosystem II. Chem. Rev. 106:4455-4483. Determination of µ-oxo exchange rates in di-µ-oxo dimanganese complexes by electrospray ionization mass spectrometry. Tagore, R., Chen, H., Crabtree, R.H. and Brudvig, G.W. (2006) Determination of µ-oxo exchange rates in di-µ-oxo dimanganese complexes by electrospray ionization mass spectrometry. J. Am. Chem. Soc. 128, 9457-9465. Redox functions of carotenoids in photosynthesis. Frank, H.A. and Brudvig, G.W. (2004) Redox functions of carotenoids in photosynthesis. Biochemistry 43, 8607-8615. Vinyard DJ, Brudvig GW: Progress Toward a Molecular Mechanism of Water Oxidation in Photosystem II. Annu Rev Phys Chem. 2017 May 5; 2017 Feb 2. PMID: 28226223 Michaelos TK, Shopov DY, Sinha SB, Sharninghausen LS, Fisher KJ, Lant HMC, Crabtree RH, Brudvig GW: A Pyridine Alkoxide Chelate Ligand That Promotes Both Unusually High Oxidation States and Water-Oxidation Catalysis. Acc Chem Res. 2017 Apr 18; 2017 Mar 8. PMID: 28272869 Liu W, Jiang J, Yang KR, Mi Y, Kumaravadivel P, Zhong Y, Fan Q, Weng Z, Wu Z, Cha JJ, Zhou H, Batista VS, Brudvig GW, Wang H: Ultrathin dendrimer-graphene oxide composite film for stable cycling lithium-sulfur batteries. Proc Natl Acad Sci U S A. 2017 Apr 4; 2017 Mar 20. PMID: 28320950 Peper JL, Vinyard DJ, Brudvig GW, Mayer JM: Slow Equilibration between Spectroscopically Distinct Trap States in Reduced TiO2 Nanoparticles. J Am Chem Soc. 2017 Mar 1; 2017 Feb 13. PMID: 28177612 Wang J, Askerka M, Brudvig GW, Batista VS: Insights into Photosystem II from Isomorphous Difference Fourier Maps of Femtosecond X-ray Diffraction Data and Quantum Mechanics/Molecular Mechanics Structural Models. ACS Energy Lett. 2017 Feb 10; 2017 Jan 12. PMID: 28217747 Vinyard DJ, Khan S, Askerka M, Batista VS, Brudvig GW: Energetics of the S2 State Spin Isomers of the Oxygen-Evolving Complex of Photosystem II. J Phys Chem B. 2017 Feb 9; 2017 Jan 25. PMID: 28079373 Shopov DY, Rudshteyn B, Campos J, Vinyard DJ, Batista VS, Brudvig GW, Crabtree RH: A full set of iridium(iv) pyridine-alkoxide stereoisomers: highly geometry-dependent redox properties. Chem Sci. 2017 Feb 1; 2016 Nov 7. PMID: 28451293 Mohadjer Beromi M, Nova A, Balcells D, Brasacchio AM, Brudvig GW, Guard LM, Hazari N, Vinyard DJ: Mechanistic Study of an Improved Ni Precatalyst for Suzuki-Miyaura Reactions of Aryl Sulfamates: Understanding the Role of Ni(I) Species. J Am Chem Soc. 2017 Jan 18; 2017 Jan 10. PMID: 28009513 Askerka M, Brudvig GW, Batista VS: The O2-Evolving Complex of Photosystem II: Recent Insights from Quantum Mechanics/Molecular Mechanics (QM/MM), Extended X-ray Absorption Fine Structure (EXAFS), and Femtosecond X-ray Crystallography Data. Acc Chem Res. 2017 Jan 17; 2016 Dec 21. PMID: 28001034 Sharninghausen LS, Sinha SB, Shopov DY, Choi B, Mercado BQ, Roy X, Balcells D, Brudvig GW, Crabtree RH: High Oxidation State Iridium Mono-μ-oxo Dimers Related to Water Oxidation Catalysis. J Am Chem Soc. 2016 Dec 14; 2016 Dec 1. PMID: 27960326 Mi Y, Liu W, Yang KR, Jiang J, Fan Q, Weng Z, Zhong Y, Wu Z, Brudvig GW, Batista VS, Zhou H, Wang H: Ferrocene-Promoted Long-Cycle Lithium-Sulfur Batteries. Angew Chem Int Ed Engl. 2016 Nov 14; 2016 Oct 25. PMID: 27779359 Liu Y, Vinyard DJ, Reesbeck ME, Suzuki T, Manakongtreecheep K, Holland PL, Brudvig GW, Söll D: A [3Fe-4S] cluster is required for tRNA thiolation in archaea and eukaryotes. Proc Natl Acad Sci U S A. 2016 Oct 24; 2016 Oct 24. PMID: 27791189