研究领域
Electronic Materials Processing
Our research interests are in the area of the thin film synthesis. Deposition techniques include plasma-enhanced chemical vapor deposition (PECVD), CVD, sputtering, and electrodeposition. A central theme is developing novel processing techniques that impart nanoscale control while retaining high rate for the efficient synthesis of mesoscale structures (50 - 1000 nm). Thin films are ubiquitous in advanced technology, and the materials we synthesize serve as integral components in photovoltaics, membranes, opto-electronics, electrochromics, thin film batteries, functional coatings, and catalysis. Investigation of these deposition processes is guided by detailed reactive flow modeling and experimental measures of both gas-phase and surface kinetics. In-situ process diagnostics and ex-situ materials characterization are used to gain a fundamental understanding of the process–structure–performance relationships in these systems.
近期论文
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D. M. Meysing, C. A. Wolden, M. M. Griffith, H. Mahabaduge, J. Pankow, M. O. Reese, J. M. Burst, W. L. Rance and T. M. Barnes, "Properties of reactively sputtered oxygenated cadmium sulfide (CdS:O) and their impact on CdTe solar cell performance", J. Vac. Sci. Technol. A 33, 021203 (2015). Journal Link
J. Li, D. R. Diercks, T. R. Ohno, C. W. Warren, M. C. Lonergan, J. D. Beach, and C. A. Wolden, "Controlled activation of ZnTe:Cu contacted CdTe solar cells using rapid thermal processing", Solar Energy Mater. Solar Cells 133, 208 (2015). Journal Link
A. W. Welch, P. P. Zawadzki, S. Lany, C. A. Wolden and A. Zakutayev, "Self-regulated growth and tunable properties of CuSbS2 solar absorbers", Solar Energy Mater. Solar Cells 132, 499 (2015). Journal Link
C.-P. Li, C. Engtrakul, R. C. Tenent, and C. A. Wolden, "Scalable synthesis of improved nanocrystalline, mesoporous tungsten oxide films with exceptional electrochromic performance", Solar Energy Mater. Solar Cells 132, 6 (2015). Journal Link
D. A. Cooney, J. D. Way, and C. A. Wolden, "A comparison of the performance and stability of Pd/BCC metal composite membranes for hydrogen purification", Int. J. Hydrogen Energy 39, 19009 (2014). Journal Link
A. Zakutayev, L. L. Baranowski, A.W. Welch, C. A. Wolden, E. S. Toberer, "Comparison of Cu-Sn-S and Cu-Sb-S as potential solar cell absorbers", Proceedings of the 40th IEEE Photovoltaic Specialists Conference, pp. 2360-2365 (2014). Journal Link
J. Li, J.D. Beach, and C. A. Wolden, "Rapid thermal processing of ZnTe:Cu contacted CdTe solar cells", Proceedings of the 40th IEEE Photovoltaic Specialists Conference, pp. 2436-2438 (2014). Journal Link
T. M Barnes, W. L. Rance, J. M Burst, M. O. Reese, D. M Meysing, C. A Wolden, T. A. Gessert, S. M Garner, P. Cimo, W. K Metzger, "High efficiency flexible CdTe superstrate devices", Proceedings of the 40th IEEE Photovoltaic Specialists Conference, pp. 2289-2292 (2014). Journal Link
J. M Burst, W. L. Rance, D. M Meysing, C. A Wolden, W. K Metzger, S. M Garner, P. Cimo, T. A. Gessert, T. M Barnes, M. O. Reese, "Performance of transparent conductors on flexible glass and plastic substrates for thin film photovoltaics", Proceedings of the 40th IEEE Photovoltaic Specialists Conference, pp. 1589-1592 (2014). Journal Link
D.M. Meysing, M.G. Griffith, M.O. Reese, J.M. Burst, W.L. Rance, W.K. Metzger, C.A. Wolden, T.M. Barnes, "Properties of oxygenated cadmium sulfide (CdS:O) and their impact on CdTe device performance", Proceedings of the 40th IEEE Photovoltaic Specialists Conference, pp. 0964-0967 (2014). Journal Link
D.R. Diercks, J. Li, J.P. Beach, C. A Wolden, B. P Gorman, "Atom probe tomography for nanoscale characterization of CdTe device absorber layers and interfaces", Proceedings of the 40th IEEE Photovoltaic Specialists Conference, pp. 0085-0089 (2014). Journal Link
M. O'Brien, K. Lee, R. Morrish, N. C. Berner, N. McEvoy, C. A. Wolden and G. S. Duesberg, "Plasma assisted synthesis of WS2 for gas sensing applications", Chem. Phys. Lett. 615, 6 (2014). Journal Link
S. S. Kelkar and C. A. Wolden, "Feature scale modeling of pulsed plasma-enhanced chemical vapor deposition", J. Vac. Sci. Technol. B 32, 052001(2014). Journal Link
R. Morrish, T. Haak, and C. A. Wolden, "Low temperature synthesis of n-type WS2 thin films via H2S plasma sulfurization of WO3", Chem. Mater. 26, 3986 (2014). Journal Link
A. E. Lewis, H. Zhao, H. Syed, C. A. Wolden and J. D. Way,, "PdAu and PdAuAg composite membranes for hydrogen separation from synthetic water-gas shift streams containing hydrogen sulfide", J. Membr. Sci. 465, 167 (2014). Journal Link
W. L. Rance, J. M. Burst, D. M. Meysing, C. A. Wolden, M. O. Reese, T. A. Gessert, W. K. Metzger, S. Garner, P. Cimo and T. M. Barnes, "14%-Efficient Flexible CdTe Solar Cells on Ultra-Thin Glass Substrates", Appl. Phys. Lett. 104, 143903 (2014). Journal Link
C.-P. Li, F. Lin, R. M. Richards, C. Engtrakul, R. C. Tenent and C. A. Wolden, "The influence of sol–gel processing on the electrochromic properties of mesoporous WO3 films produced by ultrasonic spray deposition", Solar Energy Mater. Solar Cells 121, 163 (2014). Journal Link
C.D. Sentman, M. O'Brien and C.A. Wolden, “Self limiting deposition of pyrite absorbers by pulsed PECVD”, J. Vac. Sci. Technol. A 32, 021201 (2014). Journal Link
S. K. Sahoo, R. P. Patel and C. A. Wolden, “Hybrid nanolaminate dielectrics engineered for frequency and bias stability", J. Appl. Phys. 114, 074101 (2013). Journal Link
D. M. Meysing, J. M. Burst, W. L. Rance, M. O. Reese, T. M. Barnes, T. A. Gessert and C. A. Wolden, "The influence of cadmium sulfide and contact annealing configuration on the properties of high-performance cadmium stannate", Solar Energy Mater. Solar Cells 117, 300-305 (2013). Journal Link