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个人简介

仲崇立,教授,博士生导师,天津工业大学省部共建分离膜与膜过程国家重点实验室主任、化学工程与技术学院院长。1993年获北京化工大学工学博士学位,先后在日本广岛大学和荷兰Delft University of Technology任助理教授、博士后研究员,1999年9月至2018年12月任北京化工大学化工学院教授,2019年1月至今,任职于天津工业大学。曾任国家自然科学基金项目会评专家、科技部“973计划”项目复评专家。

研究领域

长期从事面向化工、环境与能源等领域应用的纳微结构材料的分子设计、合成与性能研究,特别是MOF/COF及其复合材料的吸附分离与膜分离性能研究。

近期论文

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J. Li, M. Du, Z. Wu, X. Zhang, W. Xue, H. Huang, C. Zhong, Engineering single-atom sites with the Irving-Williams series for the simultaneous co-photocatalytic CO2 reduction and CH3CHO oxidation, Angew. Chem. Int. Ed., 2024, 63, 202407975. Y, Liang, Z. Zhang, A. Chen, C. Yu, Y. Sun, J. Du, Z. Qiao, Z. Wang, M. D. Guiver, C. Zhong, Large-area ultrathin metal-organic framework membranes fabricated on flexible polymer supports for gas separations, Angew. Chem. Int. Ed., 2024, e202404058. D. Ao, Z. Yang, A. Chen, Y. Sun, M. Ye, L. Tian, X. Cen, Z. Xie, J. Du, Z. Qiao, A. K. Cheetham, J. Hou, C. Zhong, Effective C4 separation by zeolite metal-organic framework composite membranes, Angew. Chem. Int. Ed., 2024, DOI: 10.1002/anie.202401118. M. Zheng, W. Xue, T. Yan, Z. Jiang, Z. Fang, H. Huang, C. Zhong, Fluorinated MOF-based hexafluoropropylene nanotrap for highly efficient purification of octafluoropropane electronic specialty gas, Angew. Chem. Int. Ed., 2024, DOI: 10.1002/anie.202401770. G. Han, H. Huang, M. Guo, F. Li, H. Fan, Q. Guo, C. Zhong, Rational design of the double hydrogen-bonds sites in IL@MOF composites for efficient and selective formaldehyde capture, Sep. Purif. Technol., 2024,  328, 125116. X. Cen, Y. Sun, C. Yu, C. Geng, Z. Gu, D. Ao, Z. Zhang, Z. Qiao, C. Zhong, A facile synthesis of monolithic MOF single crystal for gas separation via a supersaturation strategy, Sep. Purif. Technol., 2024, 334, 125995. F. Zhou, Y. Chen, Z. Zhang, Z. Gu, Y. Sun, M. Tong, Q. Yang, W. Dong, Y. Pan, Z. Qiao, C. Zhong, The effect of different solvents on the formation of large-area MOF membranes, AIChE J., 2024, DOI: 10.1002/AIC.18455. K. Wang, L. Si, Y. Tian, F. Yang, Ionization of a neutral MOF to disperse and anchor acid for boosting anhydrous proton conductivity, Micropor. Mesopor. Mater., 2024, 363, 112825. Z. Jiang, L. Wang, W. Xue, M. Zheng, X. Guo, H. Huang, C. Zhong, Adenine-based metal-organic framework with 1 D narrow channel for molecular-sieving separation of n-Butane and Isobutane, Sep. Purif. Technol., 2024, 328, 125025. Y. Sun, Q. Yu, C. Geng, G.-R. Zhang, Z. Zhang, Z. Qiao, C. Zhong, Ethane-selective permeation in mixed matrix membranes containing fluorinated carboxylic acid functionalized metal-organic frameworks, Chem. Eng. J. 2024, 479, 147656. W. Wang, M. Wu, W. Xue, X. Zhao, Z. Fang, L. Nie, Y. Heng, H. Huang, C. Zhong, A robust cationic covalent triazine framework-based nanotrap for fast and efficient recovery of gold from electronic waste, Chem. Eng. J., 2024, 483, 149208. Z. Yang, Y. Belmabkhout, L. N. McHugh, D. Ao, Y. Sun, S. Li, Z. Qiao, T. D. Bennett, M. D. Guiver, C. Zhong, ZIF-62 glass foam self-supported membranes to address CH4/N2 separations, Nat. Mater., 2023, 22, 888-894. C. Yu, X. Cen, Z. Zhang, Y. Sun, W. Xue , Z. Qiao, M. D. Guiver, C. Zhong, Step-nucleation in situ self-repair to prepare rollable large-area ultrathin MOF membranes, Adv. Mater., 2023, 35, 2307013. D. Ao, Z. Yang, Z. Qiao, Y. Sun, Z. Zhang, M. D. Guiver, C. Zhong, Metal–organic framework crystal–glass composite membranes with preferential permeation of ethane, Angew. Chem. Int. Ed., 2023, 62, e202304535. L. Wang, W. Xue, H. Zhu, X. Guo, H. Huang, C. Zhong, Stepwise engineering of a cage-like MOF pore aperture for the efficient separation of isomeric C4 paraffins under humid conditions, Angew. Chem. Int. Ed., 2023, 62, e202218596. N. Li, C. Ma, M. Ye, X. Guo, Z. Qiao, C. Zhong, Mechanochemical synthesized amino-functionalized ultramicroporous ZIF based mixed-matrix membranes for CO2 separation, J. Membr. Sci., 2023, 680, 121733. F. Yang, J. Sun, Y. Sun, Z. Qiao, C. Zhong, Homoelemental effect boosted stable ZIF-8 membrane with super high H2 permeance, Sep. Purif. Technol., 2023, 325, 124751. D. Li, N. Li, W. Liu, S. Xu, Y. Sun, Z. Qiao, C. Zhong, Highly water-stable MOF-74 synthesized by in-situ trace polymer modification, Polymer, 2023, 281, 126112. H. Zhu, W. Xue, H. Huang, Z. Jiang, M. Zheng, C. Zhong, Twisted pore aperture of MOF induced three-dimensional restricted sieving separation for CO2 and C2H2 mixtures, Sci. Bull., 2023, 68, 2531–2535. Y. Sun, Y. Gao, C. Geng, Z. Zhang, Z. Qiao, C. Zhong, Improved CO2/N2 separation performance by relatively continuous and defect-free distribution of IL-encapsulated ZIF-67 in ion gel membranes, J. Membr. Sci. 2023, 683, 121818. C. Geng, Y. Sun, Z. Zhang, Z. Qiao, C. Zhong, Mixed matrix metal–organic framework membranes for efficient CO2/N2 separation under humid conditions, AIChE J., 2023, 69, e18025. S. Zhang, Y. He, S. Liu, Z. Zhang, C. Zhong, Metal–organic framework membrane constructor: a tool for high-throughput construction of metal–organic framework membrane models, J. Chem. Inf. Model., 2023, 63, 23, 7476–7486. H. Huang, Z. Jiang, L. Wang, Z. Fang, W. Xue, X. Guo, C. Zhong, Guest molecule engineered pore aperture of a yttrium-based metal–organic framework for efficient 1,3-butadiene separation from C4 hydrocarbons, Sep. Purif. Technol., 2023, 327, 124949. S. Xu, X. Guo, Z. Qiao, C. Zhong, Facile in situ polymer functionalization approach for constructing water-resistant metal−organic frameworks, Ind. Eng. Chem. Res., 2023, 62, 1899−1905. Z. Jiang, W. Xue, H. Huang, H. Zhu, Y. Sun, C. Zhong, Mechanochemistry-assisted linker exchange of metal-organic framework for efficient kinetic separation of propene and propane, Chem. Eng. J., 2023, 454, 140093. X. Cen, Y. Sun, C. Yu, Z. Qiao, C. Zhong, Metal confined in metal-organic framework-based mixed matrix membranes for efficient butadiene recognition separation, Aggregate, 2023, 4, e361. C. Ma, N. Li, W. Xue, X. Guo, Z. Qiao, C. Zhong, Polarization enhanced CH4/N2 separation in bromine functionalized ZIF-62 based mixed-matrix membranes, J. Membr. Sci., 2023, 683, 121829. Y. He, X. Cao, Z. Zhang, Z. Jiang, H. Huang, S. Zhang, Q. Han, C. Zhong, Discovery of high-performing metal−organic frameworks for efficient SF6/N2 separation: a combined computational screening, machine learning, and experimental study, Ind. Eng. Chem. Res., 2023, 62, 7642−7649. C. Ma, N. Li, D. Li, Z. Gu, Z. Qiao, C. Zhong, A self-supported agZIF-UC-4 glass membrane for gas separation, J. Membr. Sci., 2023, 683, 121873. M. Zheng, Z. Fang, Y. Heng, W. Wang, H. Zhu, H. Huang, C. Zhong, Robust hierarchical-pore covalent triazine framework for efficient iodine capture and ammonia adsorption, Sep. Purif. Technol., 2023, 322, 124338. Z. Jiang, W. Wang, W. Xue, H. Zhu, M. Zheng, H. Huang, C. Zhong, Construction of π back donation active site in metal-organic framework for dense packing of C2H2 and efficient C2H2/CO2 separation, Sep. Purif. Technol., 2023, 322, 124345. W. Wang, W. Xue, F. Yang, J. Li, L. Nie, H. Huang, C. Zhong, Ligand polarity regulated metal-support charge transfer over Pd@MOFs for direct H2O2 synthesis: A structure-property relationship study, Ind. Eng. Chem. Res., 2023, 62, 11840-11850. Y. Chang, H. Huang, H. Zhu, Y. Zhao, L. Wang, Y. Sun, C. Zhong, Robust carbazole-based covalent triazine frameworks with defective ultramicropore structure for efficient ethane-selective ethane-ethylene separation, Chem. Eng. J., 2022, 427, 131726. X. Liang, H. Wu, H. Huang, X. Wang, M. Wang, H. Dou, G. He, Y. Ren, Y. Liu, Y. Wu, S. Wang, H. Ge, C. Zhong, Y. Chen, Z. Jiang, Efficient ethylene/ethane separation through ionic liquid-confined covalent organic framework membranes, J. Mater. Chem. A, 2022, 10, 5420-5429. Z. Zhang, X. Cao, C. Geng, Y. Sun, Y. He, Z. Qiao, C. Zhong, Machine Learning Aided High-throughput Prediction of Ionic Liquid@MOF Composites for Membrane-based CO2 Capture, J. Membr. Sci., 2022, 650, 120399. Y. Sun, L. Tian, Z. Qiao, C. Geng, X. Guo, C. Zhong, Surface modification of bilayer structure on metal-organic frameworks towards mixed matrix membranes for efficient propylene/propane separation, J. Membr. Sci., 2022, 648, 120350. Z. Yang, D. Li, D. Ao, C. Ma, N. Li, Y. Sun, Z. Qiao, C. Zhong, M.D. Guiver, Self-supported membranes fabricated by a polymer-hydrogen bonded network with a rigidified MOF framework, J. Membr. Sci., 2022, 650, 120427. N. Li, W. Wang, C. Ma, L. Zhu, X. Chen, B. Zhang, C. Zhong, A novel conductive rGO/ZnO/PSF membrane with superior water flux for electrocatalytic degradation of organic pollutants, J. Membr. Sci., 2022, 641, 119901. C.Yu, Y.Liang, X.Guo, Z.Qiao, C.Zhong, Fabrication of metal-organic framework-mixed matrix membranes with abundant open metal sites through dual-induction mechanism, Sep. Purif. Rev., 2022, 290, 120850. C. Geng, Y. Sun, Z. Zhang, Z. Qiao, C. Zhong, Mitigated aging in a defective metal–organic framework pillared polymer of an intrinsic porosity hybrid membrane for efficient gas separation, ACS Sustain. Chem. Eng., 2022, 10, 3643–3650. S. Xu, S. Li, X. Guo, H. Huang, Z. Qiao, C. Zhong, Co-assembly of soluble metal–organic polyhedrons for high-flux thin-film nanocomposite membranes, J. Colloid Interf. Sci., 2022, 615, 10-18. Y. Liang, R. Zhang, Z. Qiao, C. Zhong, Regulating interface nucleus growth of CuTCPP membranes via polymer collaboration method, Sep. Purif. Tech., 2022, 282, 120045. F. Yang, R. Shi, H. Huang, Z. Zhang, C. Zhong, Nano-channel engineering in a metal-organic frameworks by grafting sulfonic groups for boosting proton conductivity, ACS Appl. Energy Mater., 2022, 5, 3, 3235–3241. Y. Zhao, H. Huang, H. Zhu, C. Zhong, Design and synthesis of novel pyridine-rich cationic covalent triazine framework for CO2 capture and conversion, Micropor. Mesopor. Mater., 2022, 329, 111526. L. Wang, H. Huang, H. Zhu, Y. Chang, X. Guo, F. Yang, C. Zhong, Efficient separation of 1,3-butadiene from C4 hydrocarbons by flexible metal-organic framework with gate-opening effect, AIChE J., 2022, e17568. Y. Li, Q. Wang, Z. Ding, D. Wan, X. Nie, C. Zhong, A functionalized magnetic graphene-based MOFs platform as the heterogeneous mimic enzyme sensor for glucose detection, Catal. Lett., 2022, 152, 2375–2385. M. Zheng, H. Huang, Z. Jiang, Y. Zhao, Y. Sun, C. Zhong, Superhydrophobic conjugated porous organic polymer coated polyurethane sponge for efficient oil/water separating, J. Porous Mater., 2022, 29, 433-444 X. Cao, Y. He, Z. Zhang, Y. Sun, Q. Han, Y. Guo, C. Zhong, Predicting of covalent organic frameworks for membrane-based isobutene/1,3-butadiene separation: combining molecular simulation and machine learning, Chem. Res. Chinese Universities. 2022, 38, 421-427. X. Jia, D. Ao, Z. Yang, Z. Qiao, Y. Sun, M. D. Guiver, C. Zhong, Condensability sieving porous coordination polymer membranes for preferential permeation of C1–C4 alkanes over H2, Adv. Membr., 2022, 2, 100044. B. Yang, W. Xue, X. Zhao, W. Wang, H. Zhu, L. Luo, H. Huang, C. Zhong, Synergistic dicarboxylate sites of natural citric acid modified MOF-808 for the deep removal of Pb2+ in water, J. Mol. Liq., 2022, 366, 120235. L. Luo, H. Huang, Y. Heng, R. Shi, W. Wang, B. Yang, C. Zhong, Hierarchical-pore UiO-66-NH2 xerogel with turned mesopore size for highly efficient organic pollutants removal, J. Colloid Interf. Sci., 2022, 628, 705-716. J. Li, X. Yu, W. Xue, L. Nie, H. Huang, C. Zhong, Engineering the direct Z-scheme systems over lattice intergrown of MOF-on-MOF for selective CO2 photoreduction to CO, AIChE J., 2022, e17906. R. Shi, Z. Zhang, F. Yang, C. Zhong, Simultaneously anchoring free carboxyl and sulfonate groups into a metal-organic framework for high proton conductivity, Micropor. Mesopor. Mater., 2022, 343, 112192. C. Ma, Z. Yang, X. Guo, Z. Qiao, C. Zhong, Size-reduced low-crystallinity ZIF-62 for the preparation of mixed-matrix membranes for CH4/N2 separation, J. Membr. Sci., 2022, 663, 121069. H. Zhu, W, Xue, H. Huang, L. Chen, H. Liu, C. Zhong, Water boosted CO2/C2H2 separation in L-arginine functionalized metal—organic framework, Nano Res., 2023, 16, 6113–6119. Y. Sun, C. Geng, Z. Zhang, Z. Qiao, C. Zhong, Two-dimensional basic cobalt carbonate supported ZIF-67 composites towards mixed matrix membranes for efficient CO2/N2 separation, J. Membr. Sci., 2022, 661, 120928. Y. Peng, Q. Tan, H. Huang, Q. Zhu, X. Kang, C. Zhong, B. Han, Customization of functional MOFs by a modular design strategy for target applications, Chem. Synth., 2022, 2, 15. Z. Zhang, Q. Han, S. Zhang, X. Guo, H. Huang, F. Yang, C. Zhong, Abundant hydrophilic atoms enhanced high proton conductivity of a stable metal-organic framework at wide relative humidity range, ACS Sustainable Chem. Eng., 2022, 10, 11867-11874. Z. Gu, Z. Yang, Y. Sun, Z. Qiao, C. Zhong, Large-area vacuum-treated ZIF-8 mixed-matrix membrane for highly efficient CH4/N2 separation, AIChE J., 2022, 68, e17749. F. Yang, R. Shi, H. Huang, Z. Zhang, X. Guo, Z, Qiao, C. Zhong, Nanochannel engineering in metal−organic frameworks by grafting sulfonic groups for boosting proton conductivity, ACS Appl. Energy Mater., 2022, 5, 3235−3241. X. Cao, Z. Zhang, Y. He, W. Xue, H. Huang, C. Zhong, Machine-learning-aided computational study of covalent organic frameworks for reversed C2H6/C2H4 separation, Ind. Eng. Chem. Res. 2022, 61, 30, 11116-11123.

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