Samorì, Paolo - University of Strasbourg -

个人简介

Prof. Paolo Samorì is Distinguished Professor at the Université de Strasbourg, Deputy Director of the Institut de Science et d’Ingénierie Supramoléculaires (ISIS) and Director of the Nanochemistry Laboratory. He is Fellow of the Royal Society of Chemistry (FRSC), Fellow of the European Academy of Sciences (EURASC), Member of the Academia Europaea, Foreign Member of the Royal Flemish Academy of Belgium for Science and the Arts (KVAB), Fellow of the University of Strasbourg Institute for Advanced Study (USIAS), Senior Member of the Institut Universitaire de France (IUF), Member of the National Academy of Technologies of France, and Member of the German National Academy of Science and Engineering (acatech). He has obtained a Laurea (master’s degree) in Industrial Chemistry at University of Bologna in 1995. In 2000, he has received his PhD in Chemistry from the Humboldt University of Berlin (Prof. J. P. Rabe). He has been permanent research scientist at Istituto per la Sintesi Organica e la Fotoreattività of the Consiglio Nazionale delle Ricerche of Bologna from 2001 to 2008 and Visiting Professor at ISIS from 2003 to 2008. He has published 460 papers on nanochemistry, supramolecular sciences, materials chemistry, and scanning probe microscopies with a specific focus on graphene and other 2D materials as well as functional organic/polymeric and hybrid nanomaterials for application in optoelectronics, energy and sensing. He has been awarded numerous prestigious prizes, including the E-MRS Graduate Student Award (1998), the MRS Graduate Student Award (2000), the IUPAC Prize for Young Chemists (2001), the Vincenzo Caglioti Award (2006), the Nicolò Copernico Award (2009), the Guy Ourisson Prize (2010), the ERC Starting Grant (2010), the CNRS Silver Medal (2012), the Catalán-Sabatier Prize (2017), the Grignard-Wittig Lectureship (2017), the ERC Proof of Concept Grant (2017), the RSC Surfaces and Interfaces Award (2018), the Blaise Pascal Medal in Materials Science (2018), the Pierre Süe Prize (2018), the ERC Advanced Grant (2019), the “Étoiles de l’Europe” Prize (2019), the ERC Proof of Concept Grant (2020), the RSC/SCF Joint Lectureship in Chemical Sciences (2020), and the André Collet Prize (2022). He is Associate Editor of ACS Nano and Member of the Advisory Boards of ACS Omega, Advanced Materials, Advanced Sensor Research, BMC Materials, Chemical Communications, Chemical Society Reviews, Chemistry Europe, ChemNanoMat, ChemPhysChem, ChemPlusChem, Journal of Materials Chemistry C, Materials Advances, MGE Advances, Nanoscale Horizons, Responsive Materials, RSC Applied Interfaces, Small, and SmartMat.

研究领域

The research of the Nanochemistry Laboratory is focused on unravelling and controlling the architecture vs. function relationship in complex and multicomponent supramolecular graphene-based and conjugated materials for organic electronics, to ultimately fabricate prototypes of (supra)molecular nanodevices operating at surfaces. The main research themes include: Scanning Probe Microscopies beyond imaging to gain insight into mechanical (AFM) and electronic/electrical properties (STM, C-AFM, KPFM) of nanostructures molecular materials with a nanoscale resolution. Achieving a full control over the formation of 2D multicomponent nanoscale architectures based on pre-programmed molecular modules. This requires the complete understanding over the kinetics and thermodynamics of the self-assembly process, by combining experimental and computational approaches. Nanoelectronics with single molecules or supramolecular assemblies to fabricate prototypes of 2- and 3-terminal nanocircuits. Nanoswitches and nanomotors operating at surfaces to construct responsive functional nanomaterials. Graphene chemistry and electronics.

近期论文

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G. Fu, H. Yang, W. Zhao, P. Samorì, T. Zhang, "2D Conjugated Polymer Thin Films for Organic Electronics: Opportunities and Challenges", Adv. Mater., 2024, in press. Featured in Hot Topic: Organic Electronics and Hot Topic: Surfaces and Interfaces. R.-R. Liang, S. Xu, Z. Han, Y. Yang, K.-Y. Wang, Z. Huang, J. Rushlow, P. Cai, P. Samorì, H.-C. Zhou, "Exceptionally High Perfluorooctanoic Acid Uptake in Water by a Zirconium-Based Metal–Organic Framework through Synergistic Chemical and Physical Adsorption", J. Am. Chem. Soc., 2024, in press (open access). C. Valentini, V. Montes-García, A. Ciesielski, P. Samorì, "Boosting Zinc Hybrid Supercapacitor Performance via Thiol Functionalization of Graphene-Based Cathodes", Adv. Sci., 2024, in press (open access). Featured in Hot Topic: Carbon, Graphite, and Graphene. H. Guo, V. Montes-García, H. Peng, P. Samorì, A. Ciesielski, "Molecular Connectors Boosting the Performance of MoS2 Cathodes in Zinc-Ion Batteries", Small, 2024, in press (open access). R. Hasler, G. E. Fenoy, A. Götz, V. Montes-García, C. Valentini, Z. Qiu, C. Kleber, P. Samorì, K. Müllen, W. Knoll, "“Clickable” graphene nanoribbons for biosensor interfaces", Nanoscale Horiz., 2024, 9, 598–608. Link to article (open access). Y. Lu, Z. Hu, P. Petkov, S. Fu, H. Qi, C. Huang, Y. Liu, X. Huang, M. Wang, P. Zhang, U. Kaiser, M. Bonn, H. I. Wang, P. Samorì, E. Coronado, R. Dong, X. Feng, "Tunable Charge Transport and Spin Dynamics in Two-Dimensional Conjugated Metal–Organic Frameworks", J. Am. Chem. Soc., 2024, 146, 2574–2582. Link to article and accepted manuscript (open access). R. C. Hensel, B. Di Vizio, V. Montes-García, J. Yang, G. G. Ilie, F. Sedona, M. Sambi, P. Samorì, A. Cester, S. Agnoli, S. Casalini, "Graphene Acetic Acid-Based Hybrid Supercapacitor and Liquid-Gated Transistor", Adv. Electron. Mater., 2024, 10, 2300685. Link to article (open access). Featured in Hot Topic: Batteries and Supercapacitors and Hot Topic: Carbon, Graphite, and Graphene. M. Sensi, R. Furlan de Oliveira, M. Berto, A. Paradisi, P. Greco, C. A. Bortolotti, P. Samorì, F. Biscarini, "How Biorecognition Affects the Electronic Properties of Reduced Graphene Oxide in Electrolyte-Gated Transistor Immunosensors", Adv. Funct. Mater., 2024, in press (open access). Y. Jeong, P. Samorì, "Functionalized 2D transition metal dichalcogenide inks via liquid-phase exfoliation for practical applications", Bull. Korean Chem. Soc., 2024, 45, 110–124. Link to article (open access). G. C. Lelis, W. T. Fonseca, A. H. de Lima, A. K. Okazaki, E. C. Figueiredo, A. Riul Jr, G. R. Schleder, P. Samorì, R. Furlan de Oliveira, "Harnessing Small-Molecule Analyte Detection in Complex Media: Combining Molecularly Imprinted Polymers, Electrolytic Transistors, and Machine Learning", ACS Appl. Mater. Interfaces, 2024, in press. D. Pakulski, V. Montes-García, W. Czepa, D. Marcinkowski, H. Peng, T. Chudziak, A. Gorczyński, W. Kukułka, C. Valentini, V. Patroniak, P. Samorì, A. Ciesielski, "MOF (UiO-66-NH2)@COF (TFP-TABQ) hybrids via on-surface condensation reactions for sustainable energy storage", Chem. Commun., 2024, 60, 412–415. Link to article and accepted manuscript (open access). D. Pakulski, V. Montes-García, A. Gorczyński, W. Czepa, T. Chudziak, M. Bielejewski, A. Musiał, I. Pérez-Juste, P. Samorì, A. Ciesielski, "Two-dimensional metal–organic polymers as cathode hybrid materials for high-performance Al-batteries", J. Mater. Chem. A, 2024, 12, 440–450. Link to article and accepted manuscript (open access). Y. Wang, B. Han, M. Mayor, P. Samorì, "Opto-Electrochemical Synaptic Memory in Supramolecularly Engineered Janus 2D MoS2", Adv. Mater., 2024, 36, 2307359. Link to article (open access). A. D. Sinnott, A. Kelly, C. Gabbett, J. Munuera, L. Doolan, M. Möbius, S. Ippolito, P. Samorì, J. N. Coleman, G. L. W. Cross, "Mechanical Properties of Conducting Printed Nanosheet Network Thin Films Under Uniaxial Compression", Adv. Mater., 2024, 36, 2306954. Link to article (open access). C. Wang, L. Cusin, C. Ma, E. Unsal, H. Wang, V. Girelli Consolaro, V. Montes-García, B. Han, S. Vitale, A. Dianat, A. Croy, H. Zhang, R. Gutierrez, G. Cuniberti, Z. Liu, L. Chi, A. Ciesielski, P. Samorì, "Enhancing the Carrier Transport in Monolayer MoS2 through Interlayer Coupling with 2D Covalent Organic Frameworks", Adv. Mater., 2024, 36, 2305882. Link to article (open access). Featured in Hot Topic: Surfaces and Interfaces. J. Sheng, J. Perego, S. Bracco, W. Czepa, W. Danowski, S. Krause, P. Sozzani, A. Ciesielski, A. Comotti, B. L. Feringa, "Construction of Multi-Stimuli Responsive Highly Porous Switchable Frameworks by In Situ Solid-State Generation of Spiropyran Switches", Adv. Mater., 2024, 36, 2305783. Link to article (open access). V. Montes-García, P. Samorì, "Humidity Sensing with Supramolecular Nanostructures", Adv. Mater., 2024, 36, 2208766. Link to article (open access). Featured in Special Issue: Hygroscopic Materials. T. Chudziak, V. Montes-García, W. Czepa, D. Pakulski, A. Musiał, C. Valentini, M. Bielejewski, M. Carlin, A. Tubaro, M. Pelin, P. Samorì, A. Ciesielski, "A comparative investigation of the chemical reduction of graphene oxide for electrical engineering applications", Nanoscale, 2023, 15, 17765–17775. Link to article (open access). Featured in Nanoscale Most Popular 2023 Articles. B. Tassignon, Z. Wang, A. Galanti, J. De Winter, P. Samorì, J. Cornil, K. Moth-Poulsen, P. Gerbaux, "Site Selectivity of Peptoids as Azobenzene Scaffold for Molecular Solar Thermal Energy Storage", Chem. Eur. J., 2023, 29, e202303168. Link to article and accepted manuscript (open access). Featured in Society Volumes: Belgium, Society Volumes: France, Society Volumes: Spain and Society Volumes: Sweden. M. Safuta, A. Ciesielski, P. Samorì, "Controlling the Formation of Electroactive Graphene-Based Cementitious Composites: Towards Structural Health Monitoring of Civil Structures", Chem. Eur. J., 2023, 29, e202301816. Link to article (open access). Featured in Hot Topic: Carbon, Graphite, and Graphene, Maurizio Prato’s 70th Birthday, Society Volumes: France and Society Volumes: Poland. B. Han, S. M. Gali, S. Dai, D. Beljonne, P. Samorì, "Isomer Discrimination via Defect Engineering in Monolayer MoS2", ACS Nano, 2023, 17, 17956–17965. Link to article and accepted manuscript (open access). S. Vitale, H. Puozzo, S. Saiev, L. Bonnaud, A. G. Ricciardulli, A. Ciesielski, D. Beljonne, P. Samorì, "Tuning the Piezoresistive Behavior of Graphene-Polybenzoxazine Nanocomposites: Toward High-Performance Materials for Pressure Sensing Applications", Chem. Mater., 2023, 35, 6909–6919. Link to article and accepted manuscript (open access). W. Drożdż, A. Ciesielski, A. R. Stefankiewicz, "Dynamic Cages—Towards Nanostructured Smart Materials", Angew. Chem. Int. Ed., 2023, 62, e202307552. Link to article (open access). Featured in Hot Topic: Surfaces and Interfaces. M. Sensi, R. Furlan de Oliveira, M. Berto, M. Palmieri, E. Ruini, P. A. Livio, A. Conti, M. Pinti, C. Salvarani, A. Cossarizza, J. M. Cabot, J. Ricart, S. Casalini, M. B. González-García, P. Fanjul-Bolado, C. A. Bortolotti, P. Samorì, F. Biscarini, "Reduced Graphene Oxide Electrolyte-Gated Transistor Immunosensor with Highly Selective Multiparametric Detection of Anti-Drug Antibodies", Adv. Mater., 2023, 35, 2211352. Link to article (open access). Y. Chen, H. Wang, H. Chen, W. Zhang, S. Xu, M. Pätzel, C. Ma, C. Wang, I. McCulloch, S. Hecht, P. Samorì, "Quasi-1D Polymer Semiconductor–Diarylethene Blends: High Performance Optically Switchable Transistors", Adv. Funct. Mater., 2023, 33, 2305494. Link to article (open access). N. Xu, L. Shi, X. Pei, W. Zhang, J. Chen, Z. Han, P. Samorì, J. Wang, P. Wang, Y. Shi, S. Li, "Oxidation kinetics and non-Marcusian charge transfer in dimensionally confined semiconductors", Nat. Commun., 2023, 14, 4074. Link to article (open access). H. Liu, Y. Yao, P. Samorì, "Taming Multiscale Structural Complexity in Porous Skeletons: From Open Framework Materials to Micro/Nanoscaffold Architectures", Small Methods, 2023, 7, 2300468. Link to article (open access). M. Volpi, R. Jouclas, J. Liu, G. Liu, L. Catalano, N. McIntosh, M. Bardini, C. Gatsios, F. Modesti, N. Turetta, D. Beljonne, J. Cornil, A. R. Kennedy, N. Koch, P. Erk, P. Samorì, G. Schweicher, Y. H. Geerts, "Enantiopure Dinaphtho[2,3-b:2,3-f]thieno[3,2-b]thiophenes: Reaching High Magnetoresistance Effect in OFETs", Adv. Sci., 2023, 10, 2301914. Link to article (open access). Featured in Hot Topic: Magnetic Materials. D. Pakulski, A. Gorczyński, D. Brykczyńska, V. Montes-García, W. Czepa, I. Janica, M. Bielejewski, M. Kubicki, V. Patroniak, P. Samorì, A. Ciesielski, "New Anderson-Based Polyoxometalate Covalent Organic Frameworks as Electrodes for Energy Storage Boosted Through Keto-Enol Tautomerization", Angew. Chem. Int. Ed., 2023, 62, e202305239. Link to article (open access). Selected as a Very Important Paper. Featured in Editors’ Choice: Spotlights. A. Boschi, A. Kovtun, F. Liscio, Z. Xia, K. H. Kim, S. Lara Avila, S. De Simone, V. Mussi, C. Barone, S. Pagano, M. Gobbi, P. Samorì, M. Affronte, A. Candini, V. Palermo, A. Liscio, "Mesoscopic 3D Charge Transport in Solution-Processed Graphene-Based Thin Films: A Multiscale Analysis", Small, 2023, 19, 2303238. Link to article (open access). Featured in Hot Topic: Carbon, Graphite, and Graphene. S. Crispi, G. Nocito, F. Nastasi, G. Condorelli, A. G. Ricciardulli, P. Samorì, S. Conoci, G. Neri, "Development of a novel C-dots conductometric sensor for NO sensing", Sens. Actuators B Chem., 2023, 390, 133957. Link to article and accepted manuscript (open access). A. Zhuravlova, A. G. Ricciardulli, D. Pakulski, A. Gorczyński, A. Kelly, J. N. Coleman, A. Ciesielski, P. Samorì, "High Selectivity and Sensitivity in Chemiresistive Sensing of Co(II) Ions with Liquid-Phase Exfoliated Functionalized MoS2: A Supramolecular Approach", Small, 2023, 19, 2208100. Link to article (open access). Featured in Special Issue: Biosensors. P. Pandey, L. Fijahi, N. McIntosh, N. Turetta, M. Bardini, S. Giannini, C. Ruzié, G. Schweicher, D. Beljonne, J. Cornil, P. Samorì, M. Mas-Torrent, Y. H. Geerts, E. Modena, L. Maini, "From synthesis to device fabrication: elucidating the structural and electronic properties of C7-BTBT-C7", J. Mater. Chem. C, 2023, 11, 7345–7355. Link to article (open access). S. Gullace, L. Cusin, F. Richard, N. Israfilov, A. Ciesielski, P. Samorì, "The Role of Superadsorbent Polymers on Covalent Organic Frameworks-Based Solid Electrolytes: Investigation of the Ionic Conductivity and Relaxation", Adv. Mater. Interfaces, 2023, 10, 2300124. Link to article (open access). W. Czepa, S. Witomska, P. Samorì, A. Ciesielski, "A Graphene Oxide–Thioamide Polymer Hybrid for High-Performance Supercapacitor Electrodes", Small Sci., 2023, 3, 2300013. Link to article (open access). M. Malaki, X. Jiang, H. Wang, R. Podila, H. Zhang, P. Samorì, R. S. Varma, "MXenes: from past to future perspectives", Chem. Eng. J., 2023, 463, 142351. Link to article and accepted manuscript (open access). S. Pilato, S. Moffa, G. Siani, F. Diomede, O. Trubiani, J. Pizzicannella, D. Capista, M. Passacantando, P. Samorì, A. Fontana, "3D Graphene Oxide-Polyethylenimine Scaffolds for Cardiac Tissue Engineering", ACS Appl. Mater. Interfaces, 2023, 15, 14077–14088. Link to article (open access). N. Turetta, W. Danowski, L. Cusin, P. A. Livio, R. Hallani, I. McCulloch, P. Samorì, "A photo-responsive organic electrochemical transistor", J. Mater. Chem. C, 2023, 11, 7982–7988. Link to article (open access). Selected as a Hot Paper. J. M. Buriak, D. Akinwande, N. Artzi, C. J. Brinker, C. Burrows, W. C. W. Chan, C. Chen, X. Chen, M. Chhowalla, L. Chi, W. Chueh, C. M. Crudden, D. Di Carlo, S. C. Glotzer, M. C. Hersam, D. Ho, T. Y. Hu, J. Huang, A. Javey, P. V. Kamat, I.-D. Kim, N. A. Kotov, T. R. Lee, Y. H. Lee, Y. Li, L. M. Liz-Marzán, P. Mulvaney, P. Narang, P. Nordlander, R. Oklu, W. J. Parak, A. L. Rogach, M. Salanne, P. Samorì, R. E. Schaak, K. S. Schanze, T. Sekitani, S. Skrabalak, A. K. Sood, I. K. Voets, S. Wang, S. Wang, A. T. S. Wee, J. Ye, "Best Practices for Using AI When Writing Scientific Manuscripts – Caution, Care, and Consideration: Creative Science Depends on It", ACS Nano, 2023, 17, 4091–4093. Link to editorial (free access). I. Janica, V. Montes-García, F. Urban, P. Hashemi, A. Shaygan Nia, X. Feng, P. Samorì, A. Ciesielski, "Covalently Functionalized MXenes for Highly Sensitive Humidity Sensors", Small Methods, 2023, 7, 2201651. Link to article (open access). Featured in Special Issue: MXene Chemistry and Applications. C. Valentini, V. Montes-García, P. A. Livio, T. Chudziak, J. Raya, A. Ciesielski, P. Samorì, "Tuning the electrical properties of graphene oxide through low-temperature thermal annealing", Nanoscale, 2023, 15, 5743–5755. Link to article (open access). H. Peng, V. Montes-García, J. Raya, H. Wang, H. Guo, F. Richard, P. Samorì, A. Ciesielski, "Supramolecular engineering of cathode materials for aqueous zinc-ion hybrid supercapacitors: novel thiophene-bridged donor–acceptor sp2 carbon-linked polymers", J. Mater. Chem. A, 2023, 11, 2718–2725. Link to article (open access). Selected as a Hot Paper. S. Ippolito, F. Urban, W. Zheng, O. Mazzarisi, C. Valentini, A. G. Kelly, S. M. Gali, M. Bonn, D. Beljonne, F. Corberi, J. N. Coleman, H. I. Wang, P. Samorì, "Unveiling Charge-Transport Mechanisms in Electronic Devices Based on Defect-Engineered MoS2 Covalent Networks", Adv. Mater., 2023, 35, 2211157. Link to article (open access). COVER PAGE. H. Peng, S. Huang, V. Montes-García, D. Pakulski, H. Guo, F. Richard, X. Zhuang, P. Samorì, A. Ciesielski, "Supramolecular Engineering of Cathode Materials for Aqueous Zinc-ion Energy Storage Devices: Novel Benzothiadiazole Functionalized Two-Dimensional Olefin-Linked COFs", Angew. Chem. Int. Ed., 2023, 62, e202216136. Link to article (open access). H. Zheng, C. Ou, X. Huang, B. Jiang, W. Li, J. Li, X. Han, C. Liu, Z. Han, T. Ji, P. Samorì, L. Zhang, "A Flexible, High-Voltage (>100 V) Generating Device Based on Zebra-Like Asymmetrical Photovoltaic Cascade", Adv. Mater., 2023, 35, 2209482. Link to article and accepted manuscript (open access). Featured in Hot Topic: Flexible Electronics. J. Miao, L. Wu, Z. Bian, Q. Zhu, T. Zhang, X. Pan, J. Hu, W. Xu, Y. Wang, Y. Xu, B. Yu, W. Ji, X. Zhang, J. Qiao, P. Samorì, Y. Zhao, "A “Click” Reaction to Engineer MoS2 Field-Effect Transistors with Low Contact Resistance", ACS Nano, 2022, 16, 20647–20655.