方千荣 - 吉林大学

个人简介

Qianrong grew up in Jianou, Fujian, China. After he earned his B.S. degree from Jilin University in 2001, he continued to pursue graduate studies at Jilin University working under the direction of Professor Shilun Qiu. His doctoral research was focused on the structural design and synthetic development of inorganic porous materials, especially metal-organic frameworks (MOFs). Motivated by the deep interest in inorganic materials chemistry cultivated by his graduate studies, Qianrong then carried out postdoctoral studies with Professor Omar Yaghi at UCLA (2007-2008), Professor Hong-Cai Zhou at Texas A&M (2008-2009), Professor Yushan Yan at UC Riverside (2009-2012) and UDel (2012-2014). His postdoctoral research was focused on crystalline porous materials, such as MOFs and covalent organic frameworks. In the winter of 2014, Qianrong went back to Jilin University to start his independent career. Education 2001 - 2007 Jilin University, Ph.D. (2007), Advisor: Professor Shilun Qiu 1997 - 2001 Jilin University, B.S. (2001) Professional Appointments 2014 - present Professor, College of Chemistry, Jilin University 2014 Senior Research Fellow, University of Delaware, Advisor: Professor Yushan Yan 2012 - 2014 Postdoctoral Research Associate, University of Delaware, Advisor: Professor Yushan Yan 2009 - 2012 Postdoctoral Research Associate, University of California, Riverside, Advisor: Professor Yushan Yan 2008 - 2009 Postdoctoral Research Associate, Texas A&M University, Advisor: Professor Hong-Cai Zhou 2007 - 2008 Postdoctoral Research Fellow, University of California, Los Angeles, Advisor: Professor Omar Yaghi Honors & Awards 2020 The National Science Foundation for Distinguished Young Scholars

研究领域

I. Structural Design and Rational Synthesis of Covalent Organic Frameworks Based on reticular chemistry, our group has been devoted to the structural design and rational synthesis of covalent organic frameworks. Various novel covalent organic frameworks (COFs) have been prepared with new linkages or topologies. Moreover, we have also developed several new methods for COF preparation. II. Functional Regulation of Covalent Organic Frameworks With large surface areas, developed channels, and highly designable structure, COFs were perfect application platforms. Our group prepared various functional COFs, especially three-dimensional COFs, for applications such as gas storage and separation, heterogeneous catalysis, energy storage and conversion, drug delivery, etc. Both bottom-up (e.g. active linkages, active building blocks, in-situ loading, etc.) and post-functionalization approaches (e.g. covalent modification, metalation, etc.) were utilized for the introduction of active sites. III. Stability Engineering of Covalent Organic Frameworks For practical applications of covalent organic frameworks, we focused on improving the robustness of these materials. The chemical stabilities have been successfully enhanced via robust linkages, steric hindrance and hydrophobic engineering.

近期论文

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3D Thioether‐Based Covalent Organic Frameworks for Selective and Efficient Mercury Removal Zhang, Y.; Li, H.; Chang, J.; Guan, X.; Tang, L.; Fang, Q.*; Valtchev, V.; Yan, Y.; Qiu, S.* Small 2021, 2006112 Three-Dimensional Triptycene-Based Covalent Organic Frameworks with ceq or acs Topology Li, H.‡; Chen, F.‡; Guan, X.; Li, J.; Li, C.; Tang, B.*; Valtchev, V.; Yan, Y.; Qiu, S.; Fang, Q.* J. Am. Chem. Soc. 2021, 143, 2654-2659 ChemRxiv. Preprint. https://doi.org/10.26434/chemrxiv.13311602.v1 Recent advances in AIEgen‐based crystalline porous materials for chemical sensing Liu, Y.; Guan, X.; Fang, Q.* Aggregate 2021, e34 3D Covalent Organic Frameworks Based on Polycyclic Aromatic Hydrocarbons for Reversible Oxygen Capture Zhang, M.‡; Fang, J.‡; Liu, Y.; Wang, Y.; Liao, L.; Tang, L.; Zhu, L.; Qiu, S.; Fang, Q.* Small Struct. 2021, 2000108 Syntheses, Crystal Structures and NBO Calculation of Two New Zinc(II) Coordination Polymers Li, X.; Wang, Z.; Valtchev, V.*; Fang, Q.; Pan, Y. J. Chem. Crystallogr. 2020, 50, 155-163 Postsynthetic functionalization of covalent organic frameworks Yusran, Y.; Guan, X.; Li, H.; Fang, Q.*; Qiu, S. Natl. Sci. Rev. 2020, 7, 170-190 Three-Dimensional Large-Pore Covalent Organic Framework with stp Topology Li, H.; Ding, J.; Guan, X.; Chen, F.; Li, C.; Zhu, L.; Xue, M.; Yuan, D.; Valtchev, V.; Yan, Y.; Qiu, S.; Fang, Q.* J. Am. Chem. Soc. 2020, 142, 13334-13338 Electroactive Covalent Organic Frameworks: Design, Synthesis, and Applications Yusran, Y.; Fang, Q.*; Valtchev, V. Adv. Mater. 2020, 32, 2002038 Three‐Dimensional Chemically Stable Covalent Organic Frameworks through Hydrophobic Engineering Ma, Y.; Wang, Y.; Li, H.; Guan, X.; Li, B.; Xue, M.; Yan, Y.; Valtchev, V.; Qiu, S.; Fang, Q.* Angew. Chem. Int. Ed. 2020, 59, 19633-19638 Expanding the Synthesis Field of High-Silica Zeolites Shi, D.; Haw, K.-G.; Kouvatas, C.; Tang, L.; Zhang, Y.; Fang, Q.; Qiu, S.; Valtchev, V.* Angew. Chem. Int. Ed. 2020, 59, 19576-19581 Syntheses, Crystal Structures and Theoretical Calculations of Two Nickel, Zinc Coordination Polymers with 4-Nitrophthalic Acid and Bis(imidazol) Ligands Li, X.; Wang, Z.; Valtchev, V.*; Fang, Q.; Pan, Y. J. Inorg. Organomet. Polym. Mater. 2020, 30, 477-485 Synthesis of a Two-dimensional Covalent Organic Framework with the Ability of Conducting Proton along Skeleton Wang, Z.; Li, H.; Yan, S.; Fang, Q.* Acta Chim. Sinica 2020, 78, 63-68 Covalent Organic Frameworks for Catalysis Yusran, Y.; Li, H.; Guan, X.; Fang, Q.*; Qiu, S.* EnergyChem 2020, 2, 100035 Metal-Free Thiophene-Sulfur Covalent Organic Frameworks: Precise and Controllable Synthesis of Catalytic Active Sites for Oxygen Reduction Li, D.; Li, C.; Zhang, L.; Li, H.; Zhu, L.; Yang, D.; Fang, Q.*; Qiu, S.; Yao, X.* J. Am. Chem. Soc. 2020, 142, 8104-8108 Binder-free preparation of ZSM-5@silica beads and their use for organic pollutant removal He, P.; Ding, J.; Qin, Z.; Tang, L.; Haw, K.-G.; Zhang, Y.; Fang, Q.; Qiu, S.; Valtchev, V.* Inorg. Chem. Front. 2020, 7, 2080-2088 A sponge-like small pore zeolite with great accessibility to its micropores Haw, K.-G.; Moldovan, S.; Tang, L.; Qin, Z.; Fang, Q.; Qiu, S.; Valtchev, V.* Inorg. Chem. Front. 2020, 7, 2154-2159 Crystalline, porous, covalent polyoxometalate-organic frameworks for lithium-ion batteries Yu, X.; Li, C.; Ma, Y.; Li, D.*; Li, H.; Guan, X.; Yan, Y.; Valtchev, V.; Qiu, S.; Fang, Q.* Microporous Mesoporous Mater. 2020, 299, 110105 Design and applications of three dimensional covalent organic frameworks Guan, X.; Chen, F.; Fang, Q.*; Qiu, S.* Chem. Soc. Rev. 2020, 49, 1357-1384 Three-Dimensional Mesoporous Covalent Organic Frameworks through Steric Hindrance Engineering Wang, Y.‡; Liu, Y.‡; Li, H.; Guan, X.; Xue, M.; Yan, Y.; Valtchev, V.; Qiu, S.; Fang, Q.* J. Am. Chem. Soc. 2020, 142, 3736-3741 Exfoliated Mesoporous 2D Covalent Organic Frameworks for High‐Rate Electrochemical Double‐Layer Capacitors Yusran, Y.; Li, H.; Guan, X.; Li, D.; Tang, L.; Xue, M.; Zhuang, Z.; Yan, Y.; Valtchev, V.; Qiu, S.; Fang, Q.* Adv. Mater. 2020, 32, 1907289 Bimetallic ZIF derived Co nanoparticle anchored N-doped porous carbons for an efficient oxygen reduction reaction Li, K.; Li, D.; Zhu, L.; Gao, Z.; Fang, Q.; Xue, M.*; Qiu, S.; Yao, X. Inorg. Chem. Front. 2020, 7, 946-952 2D Mesoporous Covalent Organic Framework with High Iodine Capture Capability Xu, G.; Chang, J.; Fang, Q.* Chem. J. Chinese Universities 2020, 41, 2667-2672 Quinone-based Covalent Organic Frameworks for Efficient Oxygen Evolution Reaction Chang, J.; Xu, G.; Li, H.; Fang, Q.* Chem. J. Chinese Universities 2020, 41, 1609-1614 A Photoresponsive Azobenzene-functionalized Covalent Organic Framework Li, S.; Zhao, W.; Li, H.; Fang, Q.* Chem. J. Chinese Universities 2020, 41, 1384-1390 Solvent-Free Crystallization of Zeolitic Imidazolate Framework Membrane via Layer-by-Layer Deposition Yang, P.; Li, Z.; Gao, Z.; Song, M.; Zhou, J.; Fang, Q.; Xue, M.*; Qiu, S. ACS Sustainable Chem. Eng. 2019, 7, 4158-4164 Three-dimensional Salphen-based Covalent Organic Frameworks as Catalytic Antioxidants Yan, S.; Guan, X.; Li, H.; Li, D.; Xue, M.; Yan, Y.; Valtchev, V.; Qiu, S.; Fang, Q. J. Am. Chem. Soc. 2019, 141, 2920-2924 From ZIF nanoparticles to hierarchically porous carbon: toward very high surface area and high-performance supercapacitor electrode materials Wang, F.; Zhu, L.; Pan, Y.; Li, Z.; Yang, P.; Song, M.; Gao, Z.; Fang, Q.; Xue, M.*; Qiu, S. Inorg. Chem. Front. 2019, 6, 32-39 Fast and efficient synthesis of SSZ-13 by interzeolite conversion of Zeolite Beta and Zeolite L Tang, L.; Haw, K.-G.; Zhang, Y.; Fang, Q.; Qiu, S.; Valtchev, V.* Microporous Mesoporous Mater. 2019, 280, 306-314 Synthesis of zeolite SSZ-24 using a catalytic amount of SSZ-13 seeds Tang, L.; Haw, K.-G.; He, P.; Fang, Q.; Qiu, S.; Valtchev, V.* Inorg. Chem. Front. 2019, 6, 3097-3103 A stable ZIF-8-coated mesh membrane with micro-/nano architectures produced by a facile fabrication method for high-efficiency oil-water separation Song, M.; Zhao, Y.; Mu, S.; Jiang, C.; Li, Z.; Yang, P.; Fang, Q.; Xue, M.*; Qiu, S.Sci. China Mater. 2019, 62, 536-544 One-pot cascade syntheses of microporous and mesoporous pyrazine-linked covalent organic frameworks as Lewis-acid catalysts Ma, Y.‡; Liu, X.‡; Guan, X.; Li, H.; Yusran, Y.; Xue, M.; Fang, Q.*; Yan, Y.; Qiu, S.; Valtchev, V.* Dalton Trans. 2019, 48, 7352-7357 Ambient aqueous-phase synthesis of covalent organic frameworks for degradation of organic pollutants Liu, Y.‡; Wang, Y.‡; Li, H.; Guan, X.; Zhu, L.; Xue, M.; Yan, Y.; Valtchev, V.; Qiu, S.; Fang, Q.* Chem. Sci. 2019, 10, 10815-10820 A Robust Zeolitic Imidazolate Framework Membrane with High H-2/CO2 Separation Performance under Hydrothermal Conditions Li, Z.; Yang, P.; Yan, S.; Fang, Q.; Xue, M.*; Qiu, S.* ACS Appl. Mater. Interfaces 2019, 11, 15748-15755 A new ZIF molecular-sieving membrane for high-efficiency dye removal Li, Z.; Yang, P.; Gao, Z.; Song, M.; Fang, Q.; Xue, M.*; Qiu, S. Chem. Commun. 2019, 55, 3505-3508 Three-Dimensional Tetrathiafulvalene-Based Covalent Organic Frameworks for Tunable Electrical Conductivity Li, H.; Chang, J.; Li, S.; Guan, X.; Li, D.; Li, C.; Tang, L.; Xue, M.; Yan, Y.; Valtchev, V.; Qiu, S.; Fang, Q.* J. Am. Chem. Soc. 2019, 141, 13324-13329 Hydrothermal synthesis and crystal structure of three-dimensional supramolecular zinc, manganese coordination polymers Wang, Z.; Valtchev, V.; Fang, Q.; Li, X.*; Pan, Y. Inorg. Nano-Metal Chem. 2019, 49, 44-50 Carbon beads with a well-defined pore structure derived from ion-exchange resin beads He, P.; Haw, K.-G.; Yan, S.; Tang, L.; Fang, Q.; Qiu, S.; Valtchev, V.* J. Mater. Chem. A 2019, 7, 18285-18294 Chemically stable polyarylether-based covalent organic frameworks Guan, X.; Li, H.; Ma, Y.; Xue, M.; Fang, Q.*; Yan, Y.*; Valtchev, V.*; Qiu, S. Nat. Chem. 2019, 11, 587-594 A Covalent Organic Framework with High Surface Area for Drug Delivery Liu, X.; Wang, Y.; Liu, Y.; Li, Z.; Li, H.; Fang, Q.; Jin, Y.* Chem. J. Chinese Universities 2019, 40, 1813-1817 Three-dimensional Covalent Organic Frameworks Synthesized by Room Temperature Ionic Liquid Method Liu, X.; Guan, X.; Fang, Q.; Jin, Y.* Chem. J. Chinese Universities 2019, 40, 1341-1344 Preparation, Characterization and Gas Adsorption Properties of Metal-Organic Aerogels Li, Z.; Shan, X.*; Yang, P.; Gao, Z.; Fang, Q.; Xue, M.*; Qiu, S. Chem. J. Chinese Universities 2019, 40, 1116-1120 MXene-Coated Mesh Membrane with Underwater Superoleophobicity for High-efficiency Oil-water Separation Zhang, J.; Zhou, J.; Lin, H.; Li, Z.; Fang, Q.; Xue, M.*; Qiu, S. Chem. J. Chinese Universities 2019, 40, 624-631 Highly Stable Fluorine Containing Hierarchical Porous Covalent Organic Framework Chen, Q.; Tang, J.; Fang, Q.* Chem. J. Chinese Universities 2018, 39, 2357-2362 Synthesis of Zeolite β@IISERP-COF2 Core-shell Hybrid Materials Huang, W.; Ren, J.; Fang, Q.; Valtchev, V.* Chem. J. Chinese Universities 2018, 39, 1127-1131 UiO-66-Coated Mesh Membrane with Underwater Superoleophobicity for High-Efficiency Oil-Water Separation Zhang, X.; Zhao, Y.; Mu, S.; Jiang, C.; Song, M.; Fang, Q.; Xue, M.*; Qiu, S.; Chen, B.* ACS Appl. Mater. Interfaces 2018, 10, 17301-17308 Postsynthetic Covalent Modification in Covalent Organic Frameworks Yusran, Y.; Fang, Q.; Qiu, S.* Isr. J. Chem. 2018, 58, 971-984 Postsynthetic Functionalization of Three-Dimensional Covalent Organic Frameworks for Selective Extraction of Lanthanide Ions Lu, Q.; Ma, Y.; Li, H.; Guan, X.; Yusran, Y.; Xue, M.; Fang, Q.*; Yan, Y.; Qiu, S.; Valtchev, V.* Angew. Chem. Int. Ed. 2018, 57, 6042-6048 Made in Water: A Stable Microporous Cu(I)-carboxylate Framework (CityU-7) for CO2, Water, and Iodine Uptake Liu, J.; Xiao, R.; Wong, Y.-L.; Zhou, X.-P.; Zeller, M.; Hunter, A. D.; Fang, Q.; Liao, L.; Xu, Z.* Inorg. Chem. 2018, 57, 4807-4811 MOF-cation exchange resin composites and their use for water decontamination He, P.; Haw, K.-G.; Ren, J. W.; Fang, Q.; Qiu, S.; Valtchev, V.* Inorg. Chem. Front. 2018, 5, 2784-2791 Fast, Ambient Temperature and Pressure lonothermal Synthesis of Three-Dimensional Covalent Organic Frameworks Guan, X.; Ma, Y.; Li, H.; Yusran, Y.; Xue, M.; Fang, Q.*; Yan, Y.; Valtchev, V.; Qiu, S. J. Am. Chem. Soc. 2018, 140, 4494-4498 Coordination-supported organic polymers: mesoporous inorganic-organic materials with preferred stability Chen, D.; Zhang, P.; Fang, Q.; Wan, S.; Li, H.; Yang, S.; Huang, C.; Dai, S. Inorg. Chem. Front. 2018, 5, 2018-2022