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个人简介

Tao Yao, Professor of University of Science and Technology of China and PI of the group of ' Synchrotron Radiation and Energy Material '. Yao received his PhD degree in National Synchrotron Radiation Laboratory, University of Science and Technology of China in 2011. He has published more than 100 SCI papers in high-impact journals, including: Nature, Nature Catalysis, Nature Communications, J. Am. Chem. Soc., Angew. Chem. Int. Ed., which have been cited more than 3500 times. Prof. Yao received Excellent Youth Fund of the National Natural Science Foundation of China (2014), National Science Fund for Distinguished Youth Scholars(2020) and is member of the Youth Innovation Promotion Association of the Chinese Academy of Sciences (2015). Prof. Yao undertakes the 'Fourteenth Five-Year' National Key R&D Program 'Frontier Research of Large Scientific Devices' key project 'multi-scale in situ synchrotron radiation research platform for key catalytic processes of hydrogen energy' as project leader (2021YFA1600800), 2022-2026.

研究领域

SynchrotronRadiation X-ray Spectroscopy Synchrotron radiation based spectroscopies, such as X-ray Adsorption Spectroscopy(XAS) and X-ray Emission Spectroscopy (XES) Developing Novel Catalysts for Energy Conversion Design and synthesis novel catalysts for energy conversions, including (photo-/electro-/photoelectro-) water splitting and CO2 reduction. Especially focus on unraveling the correlation between atomic/electronic structures and properties of catalysts on atomic scale. Operando/Time-resolved Spectroscopy Structural characterization of the catalysts under real reaction conditions, and superfast investigation into the atomic/electronic structures of catalysts during reaction.

近期论文

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Wensheng Fang, Wei Guo, Ruihu Lu, Ya Yan, Xiaokang Liu, Dan Wu, Fu Min Li, Yansong Zhou, Chaohui He, Chenfeng Xia, Huiting Niu, Sicong Wang, Youwen Liu, Yu Mao, Chengyi Zhang, Bo You, Yuanjie Pang, Lele Duan, Xuan Yang, Fei Song, Tianyou Zhai, Guoxiong Wang, Xingpeng Guo, Bien Tan, Tao Yao*, Ziyun Wang*, Bao Yu Xia* Durable CO2 conversion in the proton-exchange membrane system Nature. 2024, 626, 86–91. Sicheng Li, Tong Liu, Wei Zhang*, Mingzhen Wang, Huijuan Zhang, Chunlan Qin, Lingling Zhang, Yudan Chen, Shuaiwei Jiang, Dong Liu, Xiaokang Liu, Huijuan Wang, Qiquan Luo, Tao Ding*, Tao Yao* Highly efficient anion exchange membrane water electrolyzers via chromium-doped amorphous electrocatalysts Nat. Commun. 2024, 15, 3416. Airong Xu, Tong Liu, Dong Liu, Wenzhi Li, Hui Huang, Sicong Wang, Li Xu, Xiaokang Liu, Shuaiwei Jiang, Yudan Chen, Mei Sun, Qiquan Luo, Tao Ding*, Tao Yao* Edge-Rich Pt-O-Ce Sites in CeO2 Supported Patchy Atomic-Layer Pt Enable a Non-CO Pathway for Efficient Methanol Oxidation Angew. Chem. Int. Ed. 2024, e202410545. Xue Zhang, Xiaokang Liu, Dan Wu, Longfei Hu, Huijuan Zhang, Zhiguo Sun, Shiting Qian, Zhiyuan Xia, Qiquan Luo*, Linlin Cao*, Jinlong Yang, Tao Yao* Self-Assembly Intermetallic PtCu3 Core with High-Index Faceted Pt Shell for High-Efficiency Oxygen Reduction Nano Lett. 2024, 24, 10, 3213–3220. Li Xu, Tong Liu, Dong Liu, Airong Xu, Sicong Wang, Hui Huang, Xiaokang Liu, Mei Sun, Qiquan Luo, Xusheng Zheng, Tao Ding*, Tao Yao* Boosting Electrocatalytic Ammonia Synthesis via Synergistic Effect of Iron-Based Single Atoms and Clusters Nano Lett. 2024, 24, 4, 1197–1204. Dong Liu, Li Xu, Sicheng Li, Airong Xu, Yuanhua Sun, Tong Liu, Mengyuan Liu, Huijuan Wang, Xiaokang Liu, Tao Yao, Tao Ding* Atomically precise Ru-O-Ru clusters for enhanced water dissociation in alkaline hydrogen evolution Nano Res. 2024. Zihang Chen, Tong Liu, Huijuan Zhang, Beibei Pang, Yuanhua Sun, Longfei Hu, Qiquan Luo, Xiaokang Liu*, Linlin Cao*, Tao Yao Laser-assisted synthesis of PtPd alloy for efficient ethanol oxidation Nano Res. 2024, 17, 6032–6037. Huijuan Zhang, Minyuan Tan, Longfei Hu, Renjie Gui, Xiaokang Liu, Xue Zhang, Zhiguo Sun, Linlin Cao*, Tao Yao Uncovering Structural Evolution during the Dealloying Process in Pt-Based Oxygen-Reduction Catalyst J. Phys. Chem. Lett. 2024, 15, 11, 3071–3077. Zhiguo Sun, Yuanhua Sun, Xue Zhang, Xiaokang Liu, Shuaiwei Jiang, Qiquan Luo, Faqiang Xu*, Linlin Cao*, Tao Yao Regulating the Local Microenvironment of an Fe−N4 Single-Atom Catalyst for Enhanced Oxygen Reduction Reaction J. Phys. Chem. C 2024, 128, 18, 7463–7471 Lingling Zhang, Tong Liu, Xiaokang Liu, Sicheng Li, Xue Zhang, Qiquan Luo, Tao Ding*, Tao Yao*, Wei Zhang* Highly dispersed ultrafine PtCo alloy nanoparticles on unique composite carbon supports for proton exchange membrane fuel cell Nanoscale, 2024, 16, 2868-2876. Tong Liu, Yudan Chen, Airong Xu, Xiaokang Liu, Dong Liu, Sicheng Li, Hui Huang, Li Xu, Shuaiwei Jiang, Qiquan Luo, Tao Ding*, Tao Yao* Regulating atomic Fe–Rh site distance for efficient oxygen reduction reaction Sci. China Chem. 2024, 67, 1352–1359. Hong Chen, Chaohui He, Huiting Niu, Chenfeng Xia, Fu-Min Li, Wenshan Zhao, Fei Song, Tao Tao, Yu Chen*, Yaqiong Su*, Wei Guo*, Bao Yu Xia* Surface Redox Chemistry Regulates the Reaction Microenvironment for Efficient Hydrogen Peroxide Generation J. Am. Chem. Soc. 2024, 146, 22, 15356–15365. Wensheng Fang, Ruihu Lu, Fu-Min Li*, Chaohui He, Dan Wu, Kaihang Yue, Yu Mao, Wei Guo, Bo You, Fei Song, Tao Yao, Ziyun Wang*, Bao Yu Xia* Low-coordination Nanocrystalline Copper-based Catalysts through Theory-guided Electrochemical Restructuring for Selective CO2 Reduction to Ethylene Angew. Chem. Int. Ed. 2024, 63, e202319936. Haoran Zhang, Feng Wu, Rui Huang, Xiaokang Liu, Zhiwen Zhang, Tao Yao, Yu Zhang*, Yuen Wu* Symmetry Evolution Induced 2D Pt Single Atom Catalyst with High Density for Alkaline Hydrogen Oxidation Adv. Mater. 2024, 2404672. Mengzhao Zhu, Huijuan Zhang, Yanmin Hu, Fangyao Zhou, Xiaoping Gao, Dayin He, Xuyan Zhao, Chao Zhao, Jing Wang*, Wenan Tie, Xiaoyan Tian, Bo Wang, Tao Yao, Huang Zhou, Zhe Wang*, Jin Wang*, Wenxin Guo*, Yuen Wu* In Situ Nitrogen Infiltration into an Ordered Pt3Co Alloy with sp–d Hybridization to Boost Fuel Cell Performance ACS Catal. 2024, 14, 8, 5858–5867. Wengang Fu, Yapei Yun, Hongting Sheng*, Xiaokang Liu, Tao Ding, Shuxian Hu, Tao Yao, Binghui Ge, Yuanxin Du, Didier Astruc*, Manzhou Zhu* Design of bifunctional single-atom catalysts NiSA/ZIF-300 for CO2 conversion by ligand regulation strategy Nano Res.2024, 17, 3827–3834. Dong Liu, Tao Ding*, Lifeng Wang, Huijuan Zhang, Li Xu, Beibei Pang, Xiaokang Liu*, Huijuan Wang, Junhui Wang, Kaifeng Wu, Tao Yao* In situ constructing atomic interface in ruthenium-based amorphous hybrid-structure towards solar hydrogen evolution Nat Commun. 2023, 14, 1720. Beibei Pang, Chuanyi Jia, Sicong Wang, Tong Liu, Tao Ding, Xiaokang liu, Dong Liu, Linlin Cao Mengzhao Zhu, Changhao liang*, Yuen Wu, Zhaoliang Liao* Jun Jiang*, Tao Yao* Self-Optimized Ligand Effect of Single-Atom Modifier in Ternary Pt-Based Alloy for Efficient Hydrogen Oxidation Nano Lett. 2023, 23, 9, 3826–3834. Sicong Wang, Tao Ding*, Tong Liu, Yanan Zhu, Zhinan Tao, Beibei Pang, Xiaokang Liu*, Qiquan Luo, Mei Sun, Hongting Sheng,Manzhou Zhu*, Tao Yao* Ligand Assisted Thermal Atomization of Palladium Clusters: An Inspiring Approach for the Rational Design of Atomically Dispersed Metal Catalysts Angew. Chem.Int. Ed.2023, 62, e202218630. Zhiguo Sun, Huijuan Zhang, Linlin Cao*, Xiaokang Liu, Dan Wu, Xinyi Shen, Xue Zhang, Zihang Chen, Sen Ru, Xiangyu Zhu, Zhiyuan Xia, Qiquan Luo*, Faqiang Xu, Tao Yao* Understanding Synergistic Catalysis on Cu-Se Dual Atom Sites via Operando X-ray Absorption Spectroscopy in Oxygen Reduction Reaction Angew. Chem.Int. Ed.2023, 135, e202217719. Wei Zhang, Dong Liu*, Tong Liu, Chenglong Ding, Tao Chen, Yanming Li, Xiaokang Liu, Lan Wang, Changli Li, Jingfu He*, Tao Ding*, Tao Yao Coordinately unsaturated nickel single atom electrocatalyst for efficient CO2 conversion Nano Res. 2023, 16, 10873–10880. Lan Wang, Honglei Chen, Yi Wang, Xiaokang Liu*, Changli Li*, Jingfu He*, Tao Yao Recent advances in regulating the local environment of M-N4 structure for tailored chemical reactions Nano Res. 2023, 16, 8596–8613. Lingxiao Wang, Xiaoping Gao, Sicong Wang, Cai Chen, Jia Song, Xianhui Ma, Tao Yao, Huang Zhou* , Yuen Wu* Axial Dual Atomic Sites Confined by Layer Stacking for Electroreduction of CO2 to Tunable Syngas J. Am. Chem. Soc. 2023, 145, 24, 13462–13468. Yapei Yun, Haitao Zeng, Lin Li, Haifeng Li, Shen Cheng, Ningning Sun, Meng Li, Hongting Sheng*, Shuxian Hu*, Tao Yao, Manzhou Zhu* Matching Bidentate Ligand Anchoring: an Accurate Control Strategy for Stable Single-Atom/ZIF Nanocatalysts Adv. Mater. 2023, 35, 2209561. Qingyu Wang, Yida Zhang, Minxi Lin, Hengwei Wang, Yu Bai, Chengyuan Liu, Junling Lu,Qiquan Luo, Gongming Wang, HaiLong Jiang, Tao Yao, Xusheng Zheng* Photoinduced Metastable Asymmetric Cu Single Atoms for Photoreduction of CO2 to Ethylene Adv. Energy Mater. 2023, 2302692. Yechuang Han, Jun Yi, Beibei Pang, Ning Wang, Xucheng Li, Tao Yao, Kostya S. Novoselov* Zhongqun Tian* Graphene-confined ultrafast radiant heating forhigh-loading subnanometer metal cluster catalysts Natl Sci Rev. 2023, 10, 6, nwad081. Fanying Meng, Wei Liu*, Azizur Rahman, Jing Zhang, Jiyu Fan, Chunlan Ma, Min Ge, Tao Yao, Li Pi, Lei Zhang*, Yuheng Zhang Crossover of critical behavior and nontrivial magnetism in the chiral soliton lattice host Cr1/3TaS2 Phys. Rev. B. 107, 144425. Sicong Wang, Tong Liu, Yanan Zhu, Xiaokang Liu*, Qiquan Luo, Manzhou Zhu, Tao Ding*, Tao Yao Structure–Activity Relationship of Continuous Transformed Palladium Nanoclusters and Single Atoms for Selective Phenylacetylene Hydrogenation J. Phys. Chem. C. 2023, 127, 12, 5911–5919. Xinyi Shen, Dan Wu, Hujuan Zhang, Xiaokang Liu*, Linlin Cao*, Tao Yao Application of Time-Resolved Synchrotron X-ray Absorption Spectroscopy in an Energy Conversion Reaction J. Phys. Chem. Lett. 2023, 14, 3, 645–652. Fangyao Zhou, Yaner Ruan, Mengzhao Zhu, Xiaoping Gao, Wenxin Guo, Xiaokang Liu, Wenyu Wang, Min Chen, Geng Wu, Tao Yao, Huang Zhou*, Yuen Wu* Coupling Single-Atom Sites and Ordered Intermetallic PtM Nanoparticles for Efficient Catalysis in Fuel Cells Small. 2023, 2302328. Tao Chen, Tong Liu, Beibei Pang, Tao Ding, Wei Zhang, Xinyi Shen, Dan Wu, Lan Wang, Xiaokang Liu, Qiquan Luo, Wenkun Zhu*, Tao Yao* Actinide-uranium single-atom catalysis for electrochemical nitrogenfixation Sci Bull. 2022, 67, 2001-2012. Linlin Cao, Xiaokang Liu, Xinyi Shen, Dan Wu, Tao Yao* Uncovering the Nature of Active Sites during Electrocatalytic Reactions by In Situ Synchrotron-Based Spectroscopic Techniques Acc. Chem. Res. 2022, 55, 18, 2594–2603. Sicong Wang, Beibei Pang, Xiaokang Liu*, Tao Ding*, Tao Yao* Application of XAFS Technique in Single-atom Electrocatalysis Chem. J. Chinese Universities, 2022, 43(9), 20220487. Lan Wang, Ya Pan, Dan Wu, Xiaokang Liu, Linlin Cao, Wei Zhang, Honglei Chen, Tong Liu, Dong Liu, Tao Chen, Tao Ding, Yi Wang, Chenglong Ding, Caitao Kang, Changli Li*, Jingfu He*, Tao Yao* The in situ formation of defective CoOOH catalysts from semi-oxidized Co for alkaline oxygen evolution reaction J. Mater. Chem. A. 2022, 10, 20011-20017. Beibei Pang, Xiaokang Liu, Tianyang Liu, Tao Chen, Xinyi Shen, Wei Zhang, Sicong Wang, Tong Liu, Dong Liu, Tao Ding, Zhaoliang Liao, Yafei Li*, Changhao Liang*, Tao Yao* Laser-assisted High-performance PtRu Alloy for pH-Universal Hydrogen Evolution Energy Environ. Sci. 2022, 15, 102. Lingxiao Wang, Jing Wang, Xiaoping Gao, Cai Chen, Yunli Da, sicong Wang, Jia Yang, Zhiyu Wang, Jia Song, Tao Yao, Wu Zhou*, Huang Zhou*, Yuen Wu* Periodic One-Dimensional Single-Atom Arrays J. Am. Chem. Soc. 2022, 144, 35, 15999–16005. Zhenyu Wu, Hang Nan, Shancheng Shen, Mingxi Chen, Haiwei Liang*, Chuanqi Huang*, Tao Yao, Shengqi Chu, Weixue Li, Shuhong Yu* Incorporating Sulfur Atoms intoPalladium Catalysts by ReactiveMetal–Support Interaction forSelective Hydrogenation CCS Chem. 2022, 4, 3051–3063. Junhua Liu, Xinxin Zhang, Yaoyao Ji, Xiaofei Gao, Jiating Wu, Minjie Zhang, Lin Li, Xiaokang Liu, Wensheng Yan, Tao Yao, Yuewei Yin, Lingfei Wang, Hangwen Guo, Guanglei Cheng, Zhaosheng Wang, Peng Gao, Yilin Wang*, Kai Chen*, Zhaoliang Liao* Controllable Itinerant Ferromagnetism in Weakly Correlated 5d SrIrO3 J. Phys. Chem. Lett. 2022, 13, 51, 11946–11954. Qiuping Wang, Tianyang Liu, Kui Chen, Dan Wu, Cai Chen, Min Chen, Xianhui Ma, Jie Xu, Tao Yao, Yafei Li*, Huang Zhou*, Yuen Wu* Precise Regulation of Iron Spin States in Single Fe-N4 Sites for Efficient Peroxidase-Mimicking Catalysis Small. 2022, 18, 2204015. Ziyao Fang, Wei Liu, Tao Yao, Gentao Zhou, Shiqiang Wei, Liping Qin* Experimental study of chromium (III) coprecipitation with calcium carbonate Geochim Cosmochim Ac. 2022, 322, 94–108. Tong Liu, Wei Zhang*, Tao Chen, Dong Liu, Linlin Cao, Tao Ding, Xiaokang Liu, Beibei Pang, Sicong Wang, LanWang, Qiquan Luo*, Tao Yao* Regulating the Coordination Environment of Ruthenium Cluster Catalysts for the Alkaline Hydrogen Evolution Reaction J. Phys. Chem. Lett. 2021, 12, 8016−8023 Dan Wu, Xinyi Shen, Xiaokang Liu, Tong Liu, Qiquan Luo, Dong Liu, Tao Ding, Tao Chen, LanWang, Linlin Cao*, Tao Yao* Insight into Fe Activating One-Dimensional alpha-Ni(OH)2 Nanobelts for Efficient Oxygen Evolution Reaction J. Phys. Chem. C 2021, 125, 20301-20308 Meng Gu, Dong Liu, Tao Ding, Xiaokang Liu, Tao Chen, Xinyi Shen, Tao Yao* Plasmon-assisted photocatalytic CO2 reduction on Au decorated ZrO2 catalysts Dalton Trans. 2021, 50, 6076 Tao Ding, Xiaokang Liu, Zhinan Tao, Tianyang Liu, Tao Chen, Wei Zhang, Xinyi Shen, DongLiu, Sicong Wang, Beibei Pang, Dan Wu, Linlin Cao, Lan Wang, Tong Liu, YafeiLi*, Hongting Sheng, Manzhou Zhu*, Tao Yao* Atomically Precise Dinuclear Site Active toward Electrocatalytic CO2 Reduction J. Am. Chem. Soc. 2021, 143, 11317−11324 Tao Chen,Tianyang Liu, Xinyi Shen, Wei Zhang, Tao Ding, Lan Wang, Xiaokang Liu, LinlinCao, Wenkun Zhu*, Yafei Li*, Tao Yao* Synergistically electronic tuning of metalloid CdSe nanorods for enhanced electrochemical CO2 reduction Sci China Mater 2021, 64(12): 2997–3006 Tao Chen, TongLiu, Tao Ding, Beibei Pang, Lan Wang, Xiaokang Liu, Xinyi Shen, Sicong Wang, Dan Wu, Dong Liu, Linlin Cao, Qiquan Luo, Wei Zhang*, Wenkun Zhu*, Tao Yao* Surface Oxygen Injection in Tin Disulfide Nanosheets for Efficient CO2 Electroreduction to Formate and Syngas Nano-Micro Lett. 2021, 13:189 Wei Zhang, Xiaokang Liu, Tong Liu, Tao Chen, Xinyi Shen, Tao Ding, Linlin Cao, Lan Wang, Qiquan Luo, Tao Yao* In Situ Investigation on Doping Effect in Co-Doped Tungsten Diselenide Nanosheets for Hydrogen Evolution Reaction J. Phys. Chem. C 2021, 125, 6229-6236 Xinyi Shen, Xiaokang Liu, Sicong Wang, Tao Chen, Wei Zhang, Linlin Cao*, Tao Ding, Yue Lin, Dong Liu, Lan Wang, Wei Zhang*, Tao Yao* Synergistic Modulation at Atomically Dispersed Fe/Au Interface for Selective CO2 Electroreduction Nano Lett. 2021, 21, 1, 686-692 Xi Kang, Xiao Wei, Xiaokang Liu, Sicong Wang, Tao Yao*, Shuxin Wang*, Manzhou Zhu* A reasonable approach for the generation of hollowicosahedral kernels in metal nanoclusters Nat. Comm. 2021 12:6186 Guokang Han, Xue Zhang, Wei Liu, Qinghua Zhang, Zhiqiang Wang, Jun Cheng, Tao Yao, Lin Gu, Chunyu Du*, Yunzhi Gao, Geping Yin Substrate strain tunes operando geometricdistortion and oxygen reduction activity of CuN2C2single-atom sites Nat. Comm. 2021, 12:6335 Ziyao Fang, Liping Qin*, Wei Liu, Tao Yao, Xiaoyan Chen, Shiqiang Wei Absence of hexavalent chromium in marine carbonates:implications for chromium isotopes as paleoenvironmentproxy Natl Sci Rev, 2021, Vol. 8, nwaa090 Songlin Yu, Yingjie Sun, Lixian Song, Xuan Cao, Le Chen, Xingtao An, Xiaohong Liu, Wenlong Cai, Tao Yao, Yingze Song*, Wei Zhang* Vanadium atom modulated electrocatalyst for accelerated Li-S chemistry Nano Energy. 2021, 89, 106414 Zhen Yu, Fanghua Ning, Huaifang Shang, Jin Song, Tao Yao, Zhe Sun, Wangsheng Chu*, Dingguo Xia* Relationship between Voltage Hysteresis and Voltage Decay in Lithium-Rich Layered Oxide Cathodes J. Phys. Chem. C 2021, 125, 16913-16920 Yida Zhang, Tingting Hou, Quan Xu, Qingyu Wang, Yu Bai, Shaokang Yang, Dewei Rao*, Lihui Wu, Haibin Pan*, Jiafu Chen, Gongming Wang, Junfa Zhu, Tao Yao, Xusheng Zheng* Dual-Metal Sites Boosting Polarization of Nitrogen Molecules for Efficient Nitrogen Photofixation Adv. Sci. 2021, 8, 2100302 Yafei Zhao, Huang Zhou, Xiaorong Zhu, Yunteng Qu, Can Xiong, Zhenggang Xue, Qingwei Zhang, Xiaokang Liu, Fangyao Zhou, Xiaoming Mou, Wenyu Wang, Min Chen, Ya Xiong, Xingen Lin, Yue Lin, Wenxing Chen, Hui-Juan Wang, Zheng Jiang, Lirong Zheng, Tao Yao, Juncai Dong, Shiqiang Wei, Weixin Huang, Lin Gu, Jun Luo, Yafei Li*, Yuen Wu* Simultaneous oxidative and reductive reactions in one system by atomic design Nat. Catal. 2021, 4, 134-143 Mengzhao Zhu, Chao Zhao, Xiaokang Liu, Xiaolin Wang, Fangyao Zhou, Jing Wang, Yanmin Hu, Yafei Zhao, Tao Yao, Li-Ming Yang*, Yuen Wu* Single Atomic Cerium Sites with a High Coordination Number for Efficient Oxygen Reduction in Proton-Exchange Membrane Fuel Cells ACS Catal. 2021, 7, 3923-3929

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