Fayer, Michael D. - Stanford University

个人简介

Education University of California at Berkeley, 1969-1974, Ph.D. Chemistry - 1974 Advisor: Professor Charles B. Harris University of California at Berkeley, 1965-1969, B. S. Chemistry - 1969 Undergraduate National Science Foundation Fellow Phi Beta Kappa Academic Positions David Mulvane Ehrsam and Edward Curtis Franklin Professor of Chemistry Stanford University, 2000 - on Professor of Chemistry Stanford University, 1984 - 2000 Associate Professor of Chemistry Stanford University, 1980 - 1984 Assistant Professor of Chemistry Stanford University, 1974 - 1980 Awards and Honors National Academy of Sciences of the United States of America (since 2007) American Academy of Arts and Sciences (since 1999) Peter Debye Award in Physical Chemistry – American Chemical Society (2021) Pittsburgh Spectroscopy Award –Spectroscopy Society of Pittsburgh (2018) Ahmed Zewail Award in Ultrafast Science and Technology – American Chemical Society (2014) Arthur L. Schawlow Prize in Laser Science – American Physical Society (2012) Ellis R. Lippincott Award – Optical Society of America (2009) E. Bright Wilson Award for Spectroscopy – American Chemical Society (2007) Earl K. Plyler Prize for Molecular Spectroscopy – American Physical Society (2000) Optical Society of America Fellow (since 2009) Royal Society of Chemistry Fellow (since 2008) Guggenheim Foundation Fellow (1983) American Physical Society Fellow (since 1982) Camille & Henry Dreyfus Foundation Fellow (1977) Alfred P. Sloan Foundation Fellow (1977) Stanford University Dean's Award for Distinguished Teaching (1986)

研究领域

The Fayer group is involved in research on the dynamics and interactions of molecules in complex molecular materials. Systems that have mesoscopic structure and other types of complex structures and dynamics are common in nature and have properties that are distinct from a typical bulk material. For example, water in a nanoscopic pool of several hundred water molecules behaves very differently from bulk water. To study such systems, we are applying a variety of ultrafast nonlinear experiments including two dimensional infrared vibrational echo spectroscopy, other ultrafast IR methods, and ultrafast visible and UV experiments. We are exploring dynamics and intermolecular interactions of molecules in liquids, liquids in nanoscopic environments, room temperature ionic liquids, polymers, polymer membranes, and perovskites.We are also studying solute-solvent dynamics and interactions such as complex formation and dissociation and isomerization. A prominent area of our research is the dynamics of water in nanoconfinement, interacting with interfaces, and with ions, as well as dynamics of biological membranes. Proton transfer in water and other liquids and in nanoscopic systems. We are also investigating highly concentrated aqueous salt solutions. We develop methodologies and theory of ultrafast multidimensional vibrational spectroscopy and other ultrafast optical methods for general probes of structural dynamics in complex molecular systems. We also develop and apply statistical mechanics theory of molecular systems and experimental observables.

近期论文

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"Poly (ether imide) Alumina Nanocomposites: Interphase Properties Determined from Free Volume Element Radius Distributions"Junkun Pan, Aaron P. Charnay, Michael D. Fayer Macromolecules 57, 6492–6501 (2024). "Enhanced Menshutkin SN2 Reactivity in Mesoporous Silica: The Influence of Surface Catalysis and Confinement"Weizhong Zheng, Steven A. Yamada, Samantha T. Hung, Weizhen Sun, Ling Zhao, and Michael D. Fayer, J. Am. Chem. Soc. 142, 5636-5648 (2020). "Structural Dynamics in Ionic Liquid Thin Films: The Effect of Cation Chain Length"Boning Wu, John P. Breen, and Michael D. Fayer, J. Phys. Chem. C 124, 4179-4189 (2020). "Microstructural and Dynamical Heterogeneities in Ionic Liquids"Yong-Lei Wang, Bin Li, Sten Sarman, Francesca Mocci, Zhong-Yuan Lu, Jiayin Yuan, Aatto Laaksonen, and Michael D. Fayer, Chem. Rev. 120, 5798-5877 (2020). "Effects of Pore Size on Water Dynamics in Mesoporous Silica"Steven A. Yamada, Samantha T. Hung, Ward H. Thompson, and Michael D. Fayer, J. Chem. Phys. 152, 154704 (2020). "Amorphous Polymer Dynamics and Free Volume Element Size Distributions from Ultrafast IR Spectroscopy"David J. Hoffman, Sebastian M. Fica-Contreras, and Michael D. Fayer, Proc. Nat. Acad. Sci. U.S.A. 117, 13949-13958 (2020). "Controlling the Dynamics of Ionic Liquid Thin Films via Multilayer Surface Functionalization"Boning Wu, John P. Breen, Xiangyu Xing and Michael D. Fayer, J. Am. Chem. Soc. 142, 9482-9492 (2020). "CLS Next Gen: Accurate Frequency-Frequency Correlation Functions from Center Line Slope Analysis of 2D Correlation Spectra using Artificial Neural Networks"David J. Hoffman and Michael D. Fayer, J. Phys. Chem. A 124, 5979-5992 (2020). [SI2 (.xlsx)] "Single Ensemble Nonexponential Photoluminescent Population Decays from a Broadband White-Light-Emitting Perovskite"Joseph E. Thomaz, Kurt P. Lindquist, Hemamala I. Karunadasa, and Michael D. Fayer, J. Am. Chem. Soc. 142, 16622−16631 (2020). "Proton Transfer Dynamics in the Aprotic Proton Accepting Solvent 1-Methylimidazole"Joseph E. Thomaz, Alice R. Walker, Stephen J. Van Wyck, Jan Meisner, Todd J. Martinez, and Michael D. Fayer, J. Phys. Chem. B 124, 7897−7908 (2020). "Pulse-Shaped Chopping: Eliminating and Characterizing Heat Effects in Ultrafast Infrared Spectroscopy"David J. Hoffman, Sebastian M. Fica-Contreras, Junkun Pan, and Michael D. Fayer, J. Chem. Phys. 153, 204201 (2020). "Orientational Pair Correlations and Local Structure of Benzonitrile from Molecular Dynamics Simulations with Comparisons to Experiments"Maolin Sha, Steven A. Yamada, and Michael D. Fayer, J. Phys. Chem. B 125, 3163-3177 (2021) "Free Volume Element Sizes and Dynamics in Polystyrene and Poly(methyl methacrylate) Measured with Ultrafast Infrared Spectroscopy"Sebastian M. Fica-Contreras, David J. Hoffman, Junkun Pan, Chungwen Liang, and Michael D. Fayer, J. Am. Chem. Soc. 143, 3583-3594 (2021) "Complex Formation and Dissociation Dynamics on Amorphous Silica Surfaces"Steven A. Yamada, Samantha T. Hung, Jae Yoon Shin, and Michael D. Fayer, J. Phys. Chem. B 125, 4566-4581 (2021) "Distinguishing Steric and Electrostatic Molecular Probe Orientational Ordering Via Their Effects on Reorientation-Induced Spectral Diffusion"David J. Hoffman, Sebastian M. Fica-Contreras, Junkun Pan, and Michael D. Fayer, J. Chem. Phys. 154, 244104 (2021). "Ultrafast Dynamics and Liquid Structure in Mesoporous Silica: Propagation of Surface Effects in a Polar Aprotic Solvent"Samantha T. Hung, Steven A. Yamada, Weizhong Zheng, and Michael D. Fayer, J. Phys. Chem. B 125, 10018-10034 (2021) "Long Vibrational Lifetime R-selenocyanate Probes for Ultrafast Infrared Spectroscopy: Properties and Synthesis"Sebastian M. Fica-Contreras, Robert Daniels, Omer Yassin, David J. Hoffman, Junkun Pan, Gregory Sotzing, and Michael D. Fayer, J. Phys. Chem. B 125, 8907-8918 (2021) "Identical Water Dynamics in Acrylamide Hydrogels, Polymers, and Monomers in Solution: Ultrafast IR Spectroscopy and Molecular Dynamics Simulations"Sean A. Roget, Zeke A. Piskulich, Ward H. Thompson, and Michael D. Fayer, J. Am. Chem. Soc. 143, 14855-14868 (2021) "Proton Transfer from a Photoacid to Water: First Principles Simulations and Fast Fluorescence Spectroscopy"Alice R. Walker, Boning Wu, Jan Meisner, Michael D. Fayer, and Todd J. Martínez, J. Phys. Chem. B 125, 12539-12551 (2021) "Water Dynamics and Structure of Highly Concentrated LiCl Solutions Investigated using Ultrafast IR Spectroscopy"Sean A. Roget, Kimberly A. Carter-Fenk, and Michael D. Fayer, J. Am. Chem. Soc. 144, 4233-4243 (2022). "Probing Lattice Dynamics in Two-Dimensional Inorganic Pseudohalide Perovskites with Ultrafast Infrared Spectroscopy"Xiangyu Xing, Jiayi Li, John P. Breen, Jun Nishida, Hemamala I. Karunadasa, and Michael D. Fayer, J. Phys. Chem. C 126, 10145-10158 (2022). "Water Dynamics in Aqueous Poly-N-Isopropylacrylamide through the Lower Critical Solution Temperature Phase Transition"Sean A. Roget, Kimberly A. Carter-Fenk, and Michael D. Fayer J. Phys. Chem. B 126, 7066-7075 (2022). "Vibrational Stark Spectroscopy: Peak Shifts, Linewidths and the Role of Non-Stark Solvent Coupling"Sebastian M. Fica-Contreras, Aaron P. Charnay, Junkun Pan, and Michael D. Fayer J. Phys. Chem. B 127, 717-731 (2023). "Synthetically Tunable Polymers, Free Volume Element Size Distributions, and Dielectric Breakdown Field Strengths"Sebastian M. Fica-Contreras, Zongze Li, Abdullah Alamri, Aaron P. Charnay, Junkun Pan, Chao Wu, Jeffery Lockwood, Omer Yassin, Gregory Sotzing, Yang Cao, and Michael D. Fayer Materials Today 67, 57-67 (2023). "Dynamics of Acrylamide Hydrogels, Polymers, and Monomer in Water Measured with Optical Heterodyne Detected Optical Kerr Effect Spectroscopy"Stephen J. Van Wyck and Michael D. Fayer J. Phys. Chem. B 127, 1276-1286 (2023). "Ion/Water Network Structural Dynamics in Highly Concentrated Lithium Chloride and Lithium Bromide Solutions Probed with Ultrafast IR Spectroscopy"Sean A. Roget, Tristan R. Heck, Kimberly A. Carter-Fenk, and Michael D. Fayer, J. Phys. Chem. B 127, 4532-4543 (2023). "Concentration Dependence of Dynamics and Structure among Hydrated Magnesium Ions: An Ultrafast Infrared Study"Samantha T. Hung, Sean A. Roget, Weizhong Zheng, and Michael D. Fayer J. Phys. Chem. B 127, 3278-3290 (2023). "Dynamics of Concentrated Aqueous Lithium Chloride Solutions Investigated with Optical Kerr Effect Experiments"Stephen J. Van Wyck and Michael D. Fayer J. Phys. Chem. B 127, 3488-3495 (2023). "Structural Dynamics of a Novel Pseudohalide Perovskite Cs2Pb(SeCN)2Br2 Investigated with Nonlinear Infrared Spectroscopy"Xiangyu Xing, Jiayi Li, John P. Breen, Hemamala I. Karunadasa, and Michael D. Fayer J. Phys. Chem. C 127 4283-14292 (2023). "Long-Range Interface Effects in Room Temperature Ionic Liquids: Vibrational Lifetime Studies of Thin Films"John P. Breen, Laura C. Leibfried, Xiangyu Xing, and Michael D. Fayer J. Phys. Chem. B published (2023). "Water-in-salt: fast dynamics, structure, thermodynamics, and bulk properties"Laura Kacenauskaite, Stephen J. Van Wyck, Max Moncada Cohen, Michael D. Fayer J. Phys. Chem. B 128, 291-302 (2023). "Restricted Orientation Anisotropy Method for FVE Radii Characterization: Confirmed and Refined via the Study of Six Vibrational Probes"Junkun Pan, Aaron P. Charnay, Sebastian M. Fica-Contreras, Michael D. Fayer Macromolecules 57, 903-915 (2024). "Fast Structural Dynamics in Concentrated HCl Solutions: From Proton Hopping to the Bulk Viscosity"Laura Kacenauskaite, Max Moncada Cohen, Stephen J. Van Wyck, Michael D. Fayer J. Am. Chem. Soc. 146, 12355-12364 (2024). "Influence of Internal Bond Rotation on Ultrafast IR Anisotropy Measurements and the Internal Rotational Potential"Aaron P. Charnay, Junkun Pan, Michael D. Fayer J. Phys. Chem. B 128, 280-286 (2023). "Pendant Group Functionalization of Cyclic Olefin for High Temperature and High‐Density Energy Storage"Stuti Shukla, Chao Wu, Ankit Mishra, Junkun Pan, Aaron P Charnay, Ashish Khomane, Ajinkya Deshmukh, Jierui Zhou, Madhubanti Mukherjee, Rishi Gurnani, Pragati Rout, Riccardo Casalini, Rampi Ramprasad, Michael D Fayer, Priya Vashishta, Yang Cao, Gregory Sotzing Adv. Mater. e2402133 (2024). "Effects of Nanoconfinement on Dynamics in Concentrated Aqueous Magnesium Chloride Solutions"Samantha T. Hung, Sean A. Roget, Michael D. Fayer J. Phys. Chem. B 128, 5513-5527 (2024).