个人简介

Andrew M. Beale is Professor of Inorganic Chemistry based at the Research Complex at Harwell, Rutherford Appleton Laboratories in Harwell, Didcot. The current group comprises 12 members (7 PhDs and 5 Post Docs). Current research interests fall mainly into the category of catalysis and solid-state chemistry particularly studied under dynamic or operando conditions. He was worked at UCL since 2013 (2013-2015: Lecturer; 2015: Professor). Before this, he was an Assistant Professor and postdoctoral research associate in the Department of Inorganic Chemistry and Catalysis at Utrecht University in the Netherlands, working with Professor Bert M. Weckhuysen.

研究领域

Materials and Inorganic Chemistry

X-ray absorption and scattering techniques Chemical imaging Materials/catalyst preparation Solid-state chemistry In situ/operando techniques Microspectroscopy Heterogeneous catalysis

近期论文

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Beale, A. M., Lezcano-Gonzalez, I., Slawinksi, W. A., & Wragg, D. S. (2016). Correlation between Cu ion migration behaviour and deNO x activity in Cu-SSZ-13 for the standard NH 3 -SCR reaction. Chem. Commun., 52 (36), 6170-6173. doi:10.1039/C6CC00513F Mohammed, K. M. H., Chutia, A., Callison, J., Wells, P. P., Gibson, E. K., Beale, A. M., . . . Raja, R. (2016). Design and control of Lewis acid sites in Sn-substituted microporous architectures. JOURNAL OF MATERIALS CHEMISTRY A, 4 (15), 5706-5712. doi:10.1039/c5ta10283a Lezcano-González, I., O'Brien, M. G., Počkaj, M., Sánchez-Sánchez, M., & Beale, A. M. (2016). Flexibility of the imidazolium based ionic liquids/water system for the synthesis of siliceous 10-ring containing microporous frameworks. Microporous and Mesoporous Materials, 240, 117-122. doi:10.1016/j.micromeso.2016.11.019 Vamvakeros, A., Jacques, S. D. M., Di Michiel, M., Senecal, P., Middelkoop, V., Cernik, R. J., & Beale, A. M. (2016). Interlaced X-ray diffraction computed tomography. JOURNAL OF APPLIED CRYSTALLOGRAPHY, 49, 485-496. doi:10.1107/S160057671600131X Lezcano-Gonzalez, I., Oord, R., Rovezzi, M., Glatzel, P., Botchway, S. W., Weckhuysen, B. M., & Beale, A. M. (2016). Molybdenum Speciation and its Impact on Catalytic Activity during Methane Dehydroaromatization in Zeolite ZSM-5 as Revealed by Operando X-Ray Methods. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 55 (17), 5215-5219. doi:10.1002/anie.201601357 Pilaski, M., Artz, J., Islam, H. -. U., Beale, A. M., & Palkovits, R. (2016). N-containing covalent organic frameworks as supports for rhodium as transition-metal catalysts in hydroformylation reactions. MICROPOROUS AND MESOPOROUS MATERIALS, 227, 219-227. doi:10.1016/j.micromeso.2016.03.010 Sandbrink, L., Klindtworth, E., Islam, H. -. U., Beale, A. M., & Palkovits, R. (2016). ReOx/TiO2: A Recyclable Solid Catalyst for Deoxydehydration. ACS CATALYSIS, 6 (2), 677-680. doi:10.1021/acscatal.5b01936 Sankar, M., He, Q., Dawson, S., Nowicka, E., Lu, L., Bruijnincx, P. C. A., . . . Weckhuysen, B. M. (2016). Supported bimetallic nano-alloys as highly active catalysts for the one-pot tandem synthesis of imines and secondary amines from nitrobenzene and alcohols. CATALYSIS SCIENCE & TECHNOLOGY, 6 (14), 5473-5482. doi:10.1039/c6cy00425c Hoekstra, J., Beale, A. M., Soulimani, F., Versluijs-Helder, M., van de Kleut, D., Koelewijn, J. M., . . . Jenneskens, L. W. (2016). The effect of iron catalyzed graphitization on the textural properties of carbonized cellulose: Magnetically separable graphitic carbon bodies for catalysis and remediation. CARBON, 107, 248-260. doi:10.1016/j.carbon.2016.05.065 Herbert, J. J., Senecal, P., Martin, D. J., Bras, W., Beaumont, S. K., & Beale, A. M. (2016). X-ray spectroscopic and scattering methods applied to the characterisation of cobalt-based Fischer-Tropsch synthesis catalysts. CATALYSIS SCIENCE & TECHNOLOGY, 6 (15), 5773-5791. doi:10.1039/c6cy00581k Egan, C. K., Jacques, S. D. M., Wilson, M. D., Veale, M. C., Seller, P., Beale, A. M., . . . Cernik, R. J. (2015). 3D chemical imaging in the laboratory by hyperspectral X-ray computed tomography. SCIENTIFIC REPORTS, 5, ARTN 15979. doi:10.1038/srep15979 Hoekstra, J., Beale, A. M., Soulimani, F., Versluijs-Helder, M., Geus, J. W., & Jenneskens, L. W. (2015). Base Metal Catalyzed Graphitization of Cellulose: A Combined Raman Spectroscopy, Temperature-Dependent X-ray Diffraction and High-Resolution Transmission Electron Microscopy Study. The Journal of Physical Chemistry C, 119 (19), 10653-10661. doi:10.1021/acs.jpcc.5b00477 Price, S. W. T., Ignatyev, K., Geraki, K., Basham, M., Filik, J., Vo, N. T., . . . Mosselmans, J. F. W. (2015). Chemical imaging of single catalyst particles with scanning mu-XANES-CT and mu-XRF-CT. PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 17 (1), 521-529. doi:10.1039/c4cp04488f Lezcano-Gonzalez, I., Wragg, D. S., Slawinski, W. A., Hemelsoet, K., Van Yperen-De Deyne, A., Waroquier, M., . . . Beale, A. M. (2015). Determination of the Nature of the Cu Coordination Complexes Formed in the Presence of NO and NH3 within SSZ-13. JOURNAL OF PHYSICAL CHEMISTRY C, 119 (43), 24393-24403. doi:10.1021/acs.jpcc.5b06875 Beale, A. M., Lezcano-Gonzalez, I., Maunula, T., & Palgrave, R. G. (2015). Development and characterization of thermally stable supported V–W–TiO 2 catalysts for mobile NH 3 –SCR applications. Catalysis, Structure & Reactivity, 1 (1), 25-34. doi:10.1179/2055075814Y.0000000005 Martin, D. J., Liu, G., Moniz, S. J. A., Bi, Y., Beale, A. M., Ye, J., & Tang, J. (2015). Efficient visible driven photocatalyst, silver phosphate: performance, understanding and perspective. Chem. Soc. Rev.. doi:10.1039/C5CS00380F Luo, W., Sankar, M., Beale, A. M., He, Q., Kiely, C. J., Bruijnincx, P. C. A., & Weckhuysen, B. M. (2015). High performing and stable supported nano-alloys for the catalytic hydrogenation of levulinic acid to gamma-valerolactone. NATURE COMMUNICATIONS, 6, ARTN 6540. doi:10.1038/ncomms7540 Price, S. W. T., Geraki, K., Ignatyev, K., Witte, P. T., Beale, A. M., & Mosselmans, J. F. W. (2015). In Situ Microfocus Chemical Computed Tomography of the Composition of a Single Catalyst Particle During Hydrogenation of Nitrobenzene in the Liquid Phase. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 54 (34), 9886-9889. doi:10.1002/anie.201504227 Vamvakeros, A., Jacques, S. D. M., Middelkoop, V., Di Michiel, M., Egan, C. K., Ismagilov, I. Z., . . . Beale, A. M. (2015). Real time chemical imaging of a working catalytic membrane reactor during oxidative coupling of methane. CHEMICAL COMMUNICATIONS, 51 (64), 12752-12755. doi:10.1039/c5cc03208c Beale, A. M., Gao, F., Lezcano-Gonzalez, I., Peden, C. H. F., & Szanyi, J. (2015). Recent advances in automotive catalysis for NOx emission control by small-pore microporous materials. CHEMICAL SOCIETY REVIEWS, 44 (20), 7371-7405. doi:10.1039/c5cs00108k Vamvakeros, A., Jacques, S. D. M., Di Michiel, M., Middelkoop, V., Egan, C. K., Cernik, R. J., & Beale, A. M. (2015). Removing multiple outliers and single-crystal artefacts from X-ray diffraction computed tomography data. JOURNAL OF APPLIED CRYSTALLOGRAPHY, 48, 1943-1955. doi:10.1107/S1600576715020701 Gibson, E. K., Beale, A. M., Catlow, C. R. A., Chutia, A., Gianolio, D., Gould, A., . . . Wells, P. P. (2015). Restructuring of AuPd Nanoparticles Studied by a Combined XAFS/DRIFTS Approach. CHEMISTRY OF MATERIALS, 27 (10), 3714-3720. doi:10.1021/acs.chemmater.5b00866 Hoekstra, J., Beale, A. M., Soulimani, F., Versluijs-Helder, M., Geus, J. W., & Jenneskens, L. W. (2015). Shell decoration of hydrothermally obtained colloidal carbon spheres with base metal nanoparticles. NEW JOURNAL OF CHEMISTRY, 39 (8), 6593-6601. doi:10.1039/c5nj00804b Martis, V., Beale, A. M., Detollenaere, D., Banerjee, D., Moroni, M., Gosselin, F., & Bras, W. (2014). A high-pressure and controlled-flow gas system for catalysis research. Journal of Synchrotron Radiation, 21 (2), 462-463. doi:10.1107/S1600577513031937 Beale, A. M., Newton, M. A., Nachtegaal, M., & Ferri, D. (2014). Advances in the use of X-rays for the characterization of functional catalytic materials. Catalysis Today, 229, 1. doi:10.1016/j.cattod.2014.03.001