Hardacre, Christopher - University of Manchester - School of Chemical Engineering and Analytical Science

个人简介

Biography B.A. in Natural Sciences – University of Cambridge (1990) PhD – University of Cambridge (1994) Fellow of the Royal Society of Chemistry, CChem Fellow of the Institute of Chemical Engineers, CEng Elected Member of the Royal Irish Academy Background Chris Hardacre is Head of the School of Chemical Engineering and Analytical Science at the University of Manchester. He obtained a PhD from Cambridge University in 1994 and was an SERC/junior research fellow at Emmanuel College, Cambridge. He moved to Queen’s University, Belfast (QUB) in 1995 as a lecturer in Physical Chemistry and in 2003, he was appointed as Professor of Physical Chemistry. In 2016, he moved to the University of Manchester. In 2004 he was awarded a USAF, Window on Science visiting research fellowship. He was awarded the Royal Society of Chemistry Encouraging Innovation Award with Merck Chemicals Ltd in 2005 for is work in ionic liquids and the US R and D 100 award for the development of spatially resolved measurements in catalytic monoliths with Alex Goguet (QUB) and colleagues from the Oak Ridge National Lab in 2008. In 2013 he was the inaugural winner of the IChemE’s Andrew Medal for catalysis. He has published over 350 papers, 9 patents, 6 book chapters and has an H-index of 57.

研究领域

We have strong research interests in catalysis and ionic liquids. Current catalytic projects range from water gas shift and emission control catalysis using thermal and plasma activation to the use of transients to determine gas and liquid phase reaction mechanisms to liquid phase hydrogenations under batch and flow conditions to low temperature fuel cells and clean energy conversion. In addition, our research in ionic liquids includes their use in modifying the properties of heterogeneous catalysts, structural determination of ionic liquids, and species dissolved therein, electrochemistry and prediction of physical properties of ionic liquids. In both aspects of the research, the group has developed a number of state-of-the-art techniques both within the University as well as using synchrotron and neutron central facilities. Much of the work is collaborative and industrially related involving a combination of modelling and experimental studies. Our group is also strongly involved in the EPSRC funded UK Catalysis Hub (http://www.rc-harwell.ac.uk/UKCatalysisHub) as well as the 4CU (http://4cu.org.uk/) project on carbon capture and utilisation

近期论文

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Gibson, G., Wang, Z., Hardacre, C., & Wen-Feng Lin (2017). Insights into the Mechanism of Electrochemical Ozone Production via Water Splitting on the Ni and Sb Doped SnO2 Catalyst. Physical Chemistry Chemical Physics: high quality research in physical chemistry, chemical physics and biophysical chemistry. . Publication link: efb03750-931a-44ab-8210-f464787d96fb Morgan, K., Touitou, J., Choi, J-S., Coney, C., Hardacre, C., Pihl, J. A., ... Partridge, W. P. (2016). Evolution and Enabling Capabilities of Spatially Resolved Techniques for the Characterization of Heterogeneously Catalyzed Reactions. A C S Catalysis, 6(2), 1356-1381. DOI: 10.1021/acscatal.5b02602. Publication link: ecda49cb-1a49-48c1-854d-27a43ccc3dcc McCrellis, C., Taylor, R., Jacquemin, J., & Hardacre, C. (2016). Effect of the Presence of MEA on the CO2 Capture Ability of Superbase Ionic Liquids. Journal of Chemical & Engineering Data, 61(3), 1092-1100. DOI: 10.1021/acs.jced.5b00710. Publication link: d2fc3409-3b68-417b-9e63-de1f8cc6f0f7 Goodrich, P., Gunaratne, H. Q. N., Hall, L., Wang, Y., Jin, L., Muldoon, M. J., ... Hardacre, C. (2016). Using Chiral Ionic Liquid Additives to Enhance Asymmetric Induction in a Diels-Alder Reaction. Dalton Transactions. . Publication link: c91fb4cc-f630-4602-b07f-520ba0180c44 Neale, A., Li, P., Jacquemin, J., Goodrich, P., Ball, S., Compton, R. G., & Hardacre, C. (2016). Effect of cation structure on the oxygen solubility and diffusivity in a range of bis{(trifluoromethyl)sulfonyl}imide anion based ionic liquids for lithium-air battery electrolytes. Physical Chemistry Chemical Physics, 18, 11251. DOI: 10.1039/C5CP07160G. Publication link: aea974e5-80e4-4319-b8ad-60aa6ebdfc8e Almantariotis, D., Pensado, A. S., Gunaratne, H. Q. N., Hardacre, C., Pádua, A. A. H., Coxam, J-Y., & Costa Gomes, M. F. (2016). Influence of Fluorination on the Solubilities of Carbon Dioxide, Ethane and Nitrogen in 1-n-Fluoro-alkyl-3-methylimidazolium Bis(n-fluoroalkylsulfonyl)amide Ionic Liquids. The Journal of Physical Chemistry Part B. . Publication link: a3c563d5-cc2b-4c2a-888b-c6fee9c37e93 D'Agostino, C., Chansai, S., Bush, I., Gao, C., Mantle, M. D., Hardacre, C., ... Gladden, L. F. (2016). Assessing the effect of reducing agents on the selective catalytic reduction of NOx over Ag/Al2O3 catalysts. Catalysis Science & Technology, 6(6), 1661-1666. DOI: 10.1039/c5cy01508a. Publication link: a68813d5-cd60-4da0-93d3-5623bc7d18a1 Cuellar-Franca, R., Garcia-Gutierrez, P., Taylor, R., Hardacre, C., & Azapagic, A. (2016). FDCCS16 A novel methodology for assessing the environmental sustainability of ionic liquids used for CO2 capture. Faraday Discussions, -. DOI: 10.1039/C6FD00054A. Publication link: 8c1a6e9f-1b4b-472e-b3a5-2398c6ba43bd Allampally, N. K., Mayoral, M. J., Chansai, S., Lagunas, M. C., Hardacre, C., Stepanenko, V., ... Fernández, G. (2016). Control over the Self-Assembly Modes of PtII Complexes by Alkyl Chain Variation: From Slipped to Parallel π-Stacks. Chemistry - A European Journal, 22(23), 7810-7816. DOI: 10.1002/chem.201600176. Publication link: 96d506a0-a891-4545-907c-0153b6891c3c Wang, S., Liu, J., Hembre, R., Barnicki, S., Goodrich, P., Hughes, T-L., ... Hardacre, C. (2016). Liquid-Liquid Equilibria of Ionic Liquids-Water-Acetic Acid Mixtures. Journal of Chemical & Engineering Data. . Publication link: 9846d2e6-dfd3-4440-8d74-6501a3ed6f41 Schutter, C., Neale, A. R., Wilde, P., Goodrich, P., Hardacre, C., Passerini, S., ... Balducci, A. (2016). The use of binary mixtures of 1-butyl-1-methylpyrrolidinium bis{(trifluoromethyl)sulfonyl}imide and aliphatic nitrile solvents as electrolyte for supercapacitors. Electrochimica Acta. . Publication link: 90fc3243-94d7-48c0-8f5b-a820944d8cb0 Boada, R., Cibin, G., Coleman, F., Diaz-Moreno, S., Gianolio, D., Hardacre, C., ... Swadzba-Kwasny, M. (2016). Mercury capture on a supported chlorocuprate(II) ionic liquid adsorbent studied using operando synchrotron X-ray absorption spectroscopy. Dalton Transactions. DOI: 10.1039/C6DT03014A. Publication link: 53a5a7b1-02b4-459c-a73e-4dc40efa18f8 Caravaca, A., Daly, H., Smith, M., Mills, A., Chansai, S., & Hardacre, C. (2016). Continuous flow gas phase photoreforming of methanol at elevated reaction temperatures sensitised by Pt/TiO2. Reaction Chemistry & Engineering. . Publication link: 575992b7-e908-4160-ad6f-1e831a74ae36 Falkowska, M., Bowron, D. T., Manyar, H. G., Hardacre, C., & Youngs, T. G. A. (2016). Neutron Scattering of Aromatic and Aliphatic Liquids. ChemPhysChem. DOI: 10.1002/cphc.201600149. Publication link: 14056d18-8879-4033-b21a-c513a3d04b8f Caravaca, A., Jones, W., Hardacre, C., & Bowker, M. (2016). H2 production by the photocatalytic reforming of cellulose and raw biomass using Ni, Pd, Pt and Au on titania. Proceedings of the Royal Society A: Mathematical, Physical and Engineering Sciences, 472(2191), [20160054]. DOI: 10.1098/rspa.2016.0054. Publication link: 036ca447-4f3b-4a7f-b807-fa52a73c06ec Neale, A. R., Schutter, C., Wilde, P., Goodrich, P., Hardacre, C., Passerini, S., ... Jacquemin, J. (2016). Physical-Chemical Characterization of Binary Mixtures of 1-Butyl-1-methylpyrrolidinium Bis{(trifluoromethyl)sulfonyl}imide and Aliphatic Nitrile Solvents as Potential Electrolytes for Electrochemical Energy Storage Applications. Journal of Chemical & Engineering Data. . Publication link: 0344542e-f832-460e-9275-0215f4006034 Garcia-Gutierrez, P., Jacquemin, J., McCrellis, C., Dimitriou, I., Taylor, R., Hardacre, C., & Allen, R. W. K. (2016). Techno-Economic Feasibility of Selective CO2 Capture Processes from Biogas Streams using Ionic Liquids as Physical Absorbents. Energy & Fuels , null. DOI: 10.1021/acs.energyfuels.6b00364. Publication link: 1b1740c8-984d-4363-a1c6-59218bcc1ced Hutchings, G. J., Catlow, C. R. A., Hardacre, C., & Davidson, M. G. (2016). Catalysis making the world a better place: Satellite meeting. Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences, 374(2061), [20150358]. DOI: 10.1098/rsta.2015.0358. Publication link: 1fdf5ef2-ba20-431f-966b-d36bfdcb3105 Coadou, E., Goodrich, P., Neale, A., Timperman, L., Hardacre, C., Jacquemin, J., & Anouti, M. (2016). Synthesis and Thermophysical Properties of Ether Functionalized Sulfonium Ionic Liquids as Potential Electrolytes for Electrochemical Applications. ChemPhysChem. . Publication link: 4fb1baf3-7ed4-450b-aa1b-326ce33d4c58 Puthiyapura, V. K., Dan J. L. Brett, Andrea E. Russell, Wen-Feng Lin, & Hardacre, C. (2016). Biobutanol as fuel for direct alcohol fuel cells - Investigation of Sn-modified Pt catalyst for butanol electro-oxidation. ACS Applied Materials and Interfaces, 8(20), 12859–12870. DOI: 10.1021/acsami.6b02863. Publication link: 4e8f4fb8-d646-489d-872c-9550ead14d86 Falkowska, M., Chansai, S., Manyar, H. G., Gladden, L. F., Bowron, D. T., Youngs, T. G. A., & Hardacre, C. (2016). Determination of toluene hydrogenation kinetics with neutron diffraction. Physical Chemistry Chemical Physics, 18(26), 17237-17243. DOI: 10.1039/c6cp01494a. Publication link: 38d485b1-823c-44a7-a484-e8b586c200f2 Hardacre, C., Cunningham, R., Forero-Martinez, N., Youngs, T. G. A., & Migaud, M. E. (2016). Solubility study of tobramycin in room temperature ionic liquids: An experimental and computational based study . RSC Advances. DOI: 10.1039/C6RA23078D. Publication link: 368624f6-d8cb-4624-b329-d4424c88f227 Bersani, M., Gupta, K., Mishra, A. K., Lanza, R., Taylor, R., Islam, H-U., ... Darr, J. A. (2016). Combined EXAFS, XRD, DRIFTS, and DFT Study of Nano Copper-Based Catalysts for CO2 Hydrogenation. ACS Catalysis, 5823-5833. DOI: 10.1021/acscatal.6b01529. Publication link: 31d3bba5-f936-40fd-b419-556dbbe942b8