谢作伟 - 南方科技大学 - 深圳格拉布斯研究院

个人简介

Education 1983 B.Sc. Hangzhou University 1986 M.Sc. Shanghai Institute of Organic Chemistry (SIOC), Chinese Academy of Sciences 1990 Ph.D. Shanghai Institute of Organic Chemistry, Chinese Academy of Sciences, working in a joint PhD program between Technische Universität Berlin and SIOC Position Since 2022 Chair Professor 讲席教授 Southern University of Science and Technology 2013-2022 Choh-Ming Li Professor of Chemistry 卓敏化学讲座教授 The Chinese University of Hong Kong 2006-2013 Professor of Chemistry 化学讲座教授 The Chinese University of Hong Kong 2002-2006 Professor, The Chinese University of Hong Kong 1998-2002 Associate Professor, The Chinese University of Hong Kong 1995-1998 Assistant Professor, The Chinese University of Hong Kong 1991-1995 Postdoctoral Fellow, University of Southern California 1990-1991 Research Associate, Shanghai Institute of Organic Chemistry

研究领域

Chemistry of low-valent boron compounds, carboranes and metallacarboranes Organometallic chemistry of f- and d-block transition metal complexes Homogenous catalysis Coordinative unsaturation and small molecule activation Development of drugs for Boron Neutron Capture Therapy (BNCT)

近期论文

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Directing-Group-Assisted Transition-Metal-Catalyzed Selective BH Functionalization of o-Carboranes Zhang, J.; Xie, Z.Synthesis, 2024, 56, A–AA. Metallaaromaticity involving a d0 early transition metal centre: synthesis, structure, and aromaticity of tantallapyridinazirine complexes Yang, J.;† Xu, X.;† Lin, Z.; Xie, Z.Chem. Sci., 2024, 15, 7943-7948. Cyclic (Alkyl)(Amino)Carbene-Iminoboryl Compounds with Three Formal Oxidation States Mao, X.;† Qiu, S.;† Guo, R.; Dai, Y.; Zhang, J.; Kong, L.; Xie, Z.J. Am. Chem. Soc. 2024, 146, 10917–10924. Palladium-Catalyzed Regioselective B(3,5)-Dialkenylation and B(4)-Alkenylation of o-Carboranes Yuan, S.; Zhang, H.; Qiu, Z.; Xie, Z.J. Org. Chem. 2024, 89, 2474–2479. Catalyst-Free Regioselective Diborylation of Aryllithium with Tetra(o-tolyl)diborane(4) Mao, X.; Lu, Z.; Zhang, J.; Xie, Z.Angew. Chem. Int. Ed. 2024, 63, e202317614. Visible-Light-Promoted Palladium-Catalyzed Cross-Coupling of Iodocarboranes with Disulfides and Phenylselenyl Chloride Li, S.; Liu, Y.; Xie, Z.Chin. J. Chem. 2024, 42, 129-134. Enantioselective Alkenylation of o-Carboranes via Ir-Catalyzed Asymmetric B–H Activation Zhang, H.; Zhang, J.; Qiu, Z.; Xie, Z.ACS Catal. 2023, 13, 13856–13862. 10B-labelled diboron(4) reagents: Applications and relevance to boron neutron capture therapy Xie, Z.; Marder, T. B.Chem. 2023, 9, 3015-3017. Ir-Catalyzed B(3)-Amination of o-Carboranes with Amines via Acceptorless Dehydrogenative BH/NH Cross-Coupling Au, Y.; Ma, Q.; Zhang, J.; Xie, Z.Chem. Asian J. 2023, 18, e202300611. Nickel-catalyzed regioselective B(3,4,5,6)-H tetra-alkylation of o-carboranes Zhao, J.; Xie, Z.Sci. China Chem. 2023, 66, 2836–2841. Reaction of 4-Bpin-o-Carborane with Ketones: Sequential Carbon Vertex Alkylation and B−B Bond Activation Nie, Z.; Cheng, R.; Qiu, Z.; Xie, Z.Chem. Asian J. 2023, 18, e202300598. A Strategy for Regioselective B−H Functionalization of o-Carboranes via Base Metal Catalysis Zhang, J.; Xie, Z.Org. Chem. Front. 2023, 10, 3074-3079. Direct regioselective nucleophilic cage B–H bond substitution in o-carboranes Zhang, J.; Xie, Z.Sci. Sin. Chim. 2023, 53, 312-319. Synthesis of Organotantalum Alkyne Complexes [{η5:σ-Me2C(C5H4)(C2B10H10)}TaMe(η2-R1C≡CR2)] and Their Reactions with Unsaturated Molecules Yang, J.; Xie, Z.Organometallics. 2023, 42, 1347–1359. Synthesis, Structure, and Reactivity of Rare-Earth Metal Carboryne Complexes Guo, L, Wang, S.; Xie, Z.Organometallics. 2023, 42, 581–587. Iridium-Catalyzed Regioselective B(3,6)-Dialkenylation or B(4)-Alkenylation of o-Carboranes via B–H Activation and 1,2-Carbon Migration of Alkynes Zhang, H.; Cheng, R.; Qiu, Z.; Xie, Z.Chem. Commun. 2023, 59, 740-743. Advances in transition metal catalyzed selective B-H functionalization of o-carboranes Zhang, J.; Xie, Z.Adv. Catal. 2022, 71, 91-167. Visible-Light-Induced Palladium-Catalyzed Cross-Coupling of Iodocarboranes with (Hetero)Arenes Li, S.; Zhang, J.; Xie, Z.Org. Lett. 2022, 24, 7497–7501. Iridium-Catalyzed Selective B(4)–H Amination of o-Carboranes with Anthranils Zhang, L.; Xie, Z.Org. Lett. 2022, 24, 7077–7081. Tantalum η2-Vinyl Complexes Bearing an [η5:σ-Me2C(C5H4)(C2B10H10)]2– Ligand: Syntheses and Structural Characterizations Yang, J.; Sun, Y.; Xie, Z.Organometallics. 2022, 41, 2580–2588. Iron-Catalyzed Selective B–H Activation for 4/5-fold Methylation and Arylation of Carboranes Zhou, P.; Chen, Y.; Xie, Z.ACS Catal. 2022, 12, 8761–8767. Transition Metal Catalyzed Selective B(3)-H or B(4)-H Amination of o-Carboranes via Dehydrogenative BH/NH Cross-Coupling Lyu, H.; Xie, Z.Chem. Commun. 2022, 58, 8392-8395. N-Ligand-Enabled Aromatic Nucleophilic Amination of 1,2-Diaryl-o-Carboranes with (R2N)2Mg for Selective Synthesis of 4-R2N-o-Carboranes and 2-R2N-m-Carboranes Zhang, J.; Xie, Z.Angew. Chem. Int. Ed. 2022, 61, e202202675. Visible-Light-Promoted Nickel-Catalyzed Cross-Coupling of Iodocarboranes with (Hetero)Arenes via Boron-Centered Carboranyl Radicals Li, S.; Xie, Z.J. Am. Chem. Soc. 2022, 144, 7960–7965. Functionalization of o-carboranes via carboryne intermediates Qiu, Z.; Xie, Z.Chem. Soc. Rev. 2022, 51, 3164-3180. Iridium-Catalyzed Selective B(4)–H Acylmethylation of o-Carboranes with Sulfoxonium Ylides Zhang, L.; Xie, Z.Org. Lett. 2022, 24, 1318–1322. A (µ-Hydrido)diborane(4) Anion and Its Coordination Chemistry with Coinage Metals Mao, X.; Zhang, J.; Lu, Z.; Xie, Z.Chem. Sci. 2022, 13, 3009-3013. Rhodium-catalyzed sequential B(3)-, B(4)-, and B(5)-trifunctionalization of o-carboranes with three different substituents Cheng, B.; Chen, Y.; Zhou, P., Xie, Z.Chem. Commun. 2022, 58, 629-632. Light-enabled alkenylation of iodocarboranes with unactivated alkenes Ni, H.; Lu, Z.; Xie, Z.Dalton Trans. 2022, 51, 104-110. Self-assembled dipoles of o-carborane on gate oxide tuning charge carriers in organic field effect transistors Chu, M.; Zhang, J.; Zeng, X.; Chen, Z.; Liu, D.; Chen, H.; Xie, Z., Xu, J.; Miao, Q. J. Mater. Chem. C. 2022, 10, 2690-2695. Ir-catalyzed enantioselective B−H alkenylation for asymmetric synthesis of chiral-at-cage o-carboranes Cheng, R.; Zhang, J.; Zhang, H.; Qiu, Z.; Xie, Z.Nat. Commun. 2021, 12, 7146. Diboration of Alkenes and Alkynes with a Carborane-Fused Four-Membered Boracycle Bearing an Electron-Precise B-B Bond Zhong, M.; Zhang, J.; Lu, Z.; Xie, Z.Dalton Trans. 2021, 50, 17150-17155. Synthesis and Reactivity of Carboranylsilylene Stabilized Boranes: Construction of Carborane-Fused Silaboracycles Wang, H.; Xie, Z.Organometallics. 2021, 40, 3819-3824. Synthesis, Characterization, and Catalytic Activity of Dinuclear Rare-Earth Metal Alkyl Complexes Bearing 2,6-Diisopropylphenylamidomethyl Functionalized Pyrrolyl Ligand Zhu, X.; Guo, D.; Yao, F.; Huang, Z; Li, Y.; Xie, Z.; Wang, S.Organometallics. 2021, 40, 1633–1641. A Strategy for Selective Catalytic B–H Functionalization of o-Carboranes Qiu, Z.; Xie, Z.Acc. Chem. Res. 2021, 54, 4065–4079. Ring-opening and ring-expansion reactions of carborane-fused borirane Wang, H.; Zhang, J.; Xie, Z.Chem. Sci. 2021, 12, 13187-13192. Synthesis and structure of metallacarboranes bearing carborane-fused cyclopentenyl and dicarbollyl-fused cyclopentene ligands Chan, T.; Lu, Z; Xie, Z.Dalton Trans. 2021, 50, 10615-10620. Rhodium catalyzed multicomponent dehydrogenative annulation: one-step construction of isoindole derivatives Lyu, H.; Quan, Y.; Cheng, B.; Xie, Z.Chem. Commun. 2021, 57, 7930-7933. Iridium-Catalyzed Annulation of o-Carboranyl Carboxylic Acids with Alkynes: Synthesis of Carborano-Isocoumarins Cheng, B.; Chen, Y.; Xie, Z.J. Org. Chem. 2021, 86 , 12412–12418. Pd-catalyzed selective tetrafunctionalization of diiodo-o-carboranes Ge, Y.; Qiu, Z.; Xie, Z.Chem. Commun. 2021, 57, 8071-8074. Fe-Catalyzed Intramolecular B–H/C–H Dehydrogenative Coupling: Synthesis of Carborane-Fused Nitrogen Heterocycles Chen, Y.; Lyu, H.; Quan, Y.; Xie, Z.Org. Lett. 2021, 23 , 4163–4167. Synthesis, Structure and Reactivity of Acid-Free Neutral Oxoborane Wang, H.; Zhang, J.; Yang, J.; Xie, Z.Angew. Chem. Int. Ed. 2021, 60 , 19008-19012. Ene Reaction of o-Carboryne with Alkynes and Alkenes at Room Temperature: Synthesis of o-Carboranyl Allenes and Alkenes Zhang, J.; Xie, Z.Org. Lett. 2021, 23 , 2971–2975. Ir-Catalyzed Selective B(3)-H Amination of o-Carboranes with NH3 Au, Y.; Zhang, J.; Quan, Y.; Xie, Z.J. Am. Chem. Soc. 2021, 143 , 4148–4153. Recent Advances in Transition Metal-Catalyzed Selective B-H Functionalization of o-Carboranes Au, Y.; Xie, Z.Bull. Chem. Soc. Jpn. 2021, 94, 879–899. Catalytic Cage BH Functionalization of Carboranes via "Cage Walking" Strategy Guo, C.; Qiu, Z; Xie, Z.ACS Catal. 2021, 11, 2134–2140. Pd-Catalyzed sequential B(3)-I/B(4)-H bond activation for the synthesis of 3,4-benzo-o-carboranes Ge, Y.; Zhang, J.; Qiu, Z; Xie, Z.Dalton Trans. 2021, 50, 1766-1773. Tandem [4 + 2]/[2 + 2] Cycloaddition of o-Carboryne with Enynes: Facile Construction of Carborane-fused Tricyclics Zhang, J.; Xie, Z.Chem. Sci. 2021, 12, 5616-5620. Tri-insertion with Dearomatization of Terminal Arylalkynes at Carborane Based Frustrated Lewis Pair Template Zhang, J.; Xie, Z.Chem. Sci. 2021, 12, 1745-1749. Light-promoted copper-catalyzed cage C-arylation of o-carboranes: facile synthesis of 1-aryl-o-carboranes and o-carborane-fused cyclics Ni, H.; Lu, Z.; Xie, Z.New J. Chem. 2021, 45, 14944-14948.