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Synthesis of an All-Ferric Cuboidal Cluster [FeIII4S4(SAr)4], G. Moula, T. Matsumoto, M. E. Miehlich, K. Meyer, and K. Tatsumi*, Angew. Chem. Int. Ed., 2018, 57, 11594-11597. Structure and Reactivity of an Asymmetric Synthetic Mimic of Nitrogenase Cofacto, K. Tanifuji, N. Sickerman, C. C. Lee, T. Nagasawa, K. Miyazaki, Y. Ohki*, K. Tatsumi*, Y. Hu*, and M. W. Ribbe*, Angew. Chem. Int. Ed., 2016, 55, 15633-15636. Coupling of an N-Heterocyclic Carbene on Iron with Alkynes Forming 5-Cyclopentadienyl-Diimine Ligand, T. Hatanaka, Y. Ohki*, and K. Tatsumi*, Angew. Chem. Int. Ed., 2014, 53, 2727-2729. Catalytic Generation of Borenium Ions by Cooperative B–H Bond Activation: The Elusive Direct Electrophilic Borylation of Nitrogen Heterocycles with Pinacolborane, T. Stahl, K. Müther, Y. Ohki*, K. Tatsumi*, and M. Oestreich*, J. Am. Chem. Soc., 2013, 135, 10978-10981. Cooperative Catalytic Activation of Si-H Bonds by a Polar Ru-S Bond: Regioselective Low-Temperature C-H Silylation of Indoles under Neutral Conditions by a Friedel-Crafts Mechanism, H. F. T. Klare, M. Oestreich*, J. Ito, H. Nishiyama, Y. Ohki*, and K. Tatsumi*, J. Am. Chem. Soc., 2011, 133, 3312-3315. Synthetic analogues of [Fe4S4(Cys)3(His)] in hydrogenases and [Fe4S4(Cys)4] in HiPIP derived from all-ferric [Fe4S4{N(SiMe3)2}4, Y. Ohki, K. Tanifuji, N. Yamada, M. Imada, T. Tajima, and K. Tatsumi*, Proc. Natl. Acad. Sci. USA, 2011, 108, 12635-12640. A model for the CO-inhibited form of [NiFe] hydrogenase: synthesis of (CO)3Fe(μ-StBu)3Ni{SC6H3-2;6-(mesityl)2} and reversible CO addition at the Ni site, Y. Ohki, K. Yasumura, M. Ando, S. Shimokata, and K. Tatsumi*, Proc. Natl. Acad. Sci. USA, 2010, 107, 3994-3997. Synthesis, Structures, and Electronic Properties of [8Fe-7S] Cluster Complexes Modeling the Nitrogenase P-Cluster, Y. Ohki*, M. Imada, A. Murata, Y. Sunada, S. Ohta, M. Honda, T. Sasamori, N. Tokitoh, M. Katada, and K. Tatsumi*, J. Am. Chem. Soc., 2009, 131, 13168-13178. C-H Bond Activation of Heteroarenes Mediated by a Half-Sandwich Iron Complex of N-Heterocyclic Carbene, Y. Ohki*, T. Hatanaka, and K. Tatsumi*, J. Am. Chem. Soc., 2008, 130, 17174-17186. Reversible Heterolysis of H2 Mediated by an M-S(thiolate) Bond (M = Ir, Rh): A Mechanistic Implication for [NiFe] Hydrogenase, Y. Ohki*, M. Sakamoto, and K. Tatsumi*, J. Am. Chem. Soc., 2008, 130, 11610-11611. A Functional Hydrogenase Model: Reversible Interconversion of H2 and H2O by a Hydroxo/Sulfido-Bridged Dinuclear Ruthenium-Germanium Complex, T. Matsumoto, Y. Nakaya, N. Itakura, and K. Tatsumi*, J. Am. Chem. Soc., 2008, 130, 2458-2459. Heterolytic Dihydrogen Activation by a Sulfido- and Oxo-Bridged Dinuclear Germanium-Ruthenium Complex, T. Matsumoto, Y. Nakaya, and K. Tatsumi*, Angew. Chem. Int. Ed., 2008, 47, 1913-1915. Thiolate-bridged dinuclear iron(tris-carbonyl)–nickel complexes relevant to the active site of [NiFe] hydrogenase, Y. Ohki, K. Yasumura, K. Kuge, S. Tanino, M. Ando, Z. Li, and K. Tatsumi*, Proc. Natl. Acad. Sci. USA, 2008, 105, 7652-7657. Synthesis of New [8Fe-7S] Clusters: A Topological Link Between the Core Structures of P-Cluster, FeMo-co, and FeFe-co of Nitrogenases, Y. Ohki, Y. Ikagawa, and K. Tatsumi*, J. Am. Chem. Soc., 2007, 129, 10457-10465. Dithiolato-Bridged Dinuclear Iron-Nickel Complexes [Fe(CO)2(CN)2 (SCH2CH2CH2S)Ni(S2CNR2)] Modeling the Active Site of [NiFe] Hydrogenase, Z. Li, Y. Ohki, and K. Tatsumi*, J. Am. Chem. Soc., 2005, 127, 8950-8951. A half-sandwich ruthenium(II) complex containing a coordinatively unsaturated 2,6-dimesitylphenyl thiolate ligand, Y. Ohki, H. Sadohara, Y. Takikawa, and K. Tatsumi*, Angew. Chem. Int. Ed., 2004, 43, 2290-2293. Heterolytic Cleavage of Dihydrogen Promoted by Sulfido-Bridged Tungsten-Ruthenium Dinuclear Complexes, Y. Ohki, N. Matsuura, T. Marumoto, H. Kawaguchi, and K. Tatsumi*, J. Am. Chem. Soc., 2003, 125, 7978-7988. Synthesis of the P-Cluster Inorganic Core of Nitrogenases, Y. Ohki, Y. Sunada, M. Honda, M. Katada, and K. Tatsumi*, J. Am. Chem. Soc., 2003, 125, 4052-4053. Unusual Coordination Modes of Arylthiolates in Mo{5-SC6H3-2,6-(SiMe3)2}{7-SC6H3-2,6-(SiMe3)2}, T. Komuro, T. Matsuo, H. Kawaguchi*, and K. Tatsumi*, J. Am. Chem. Soc., 2003, 125, 2070-2071. Spontaneous Formation of a Diamond-crown Structure of Re8 Polyselenide and a Cage Structure of Re3 Polytelluride, G. X. Jin, Y. Arikawa, and K. Tatsumi*, J. Am. Chem. Soc., 2001, 123, 735-736.