Wodtke, Alec - Georg-August-Universitäten Göttingen

个人简介

EDUCATION AND PROFESSIONAL PREPARATION 1986–8 Post-doctoral researcher, Max Planck Institute for Fluid Dynamics, Göttingen, Germany 1986 Ph.D. Department of Chemistry, University of California, Berkeley, Berkeley CA, USA 1981 Bachelor’s Degree, Department of Chemistry, University of Utah, Salt Lake City Utah,USA CURRENT POSITION(S) 2015– Professeur Titulaire, Ecole Polytechnique Fédérale Lausanne, Lausanne Switzerland 2010– Director, Max Planck Institute for Biophysical Chemistry, Göttingen Germany 2010– Professor, Institute for Physical Chemistry, University of Göttingen, Germany 2010– Research Professor, Department of Chemistry and Biochemistry, University of California Santa Barbara, Santa Barbara CA USA PREVIOUS POSITIONS 2016–18 Director, Institute for Physical Chemistry, University of Göttingen, Germany 2010 Professor Above-Scale, Department of Chemistry and Biochemistry, University of California Santa Barbara, Santa Barbara CA USA 1996-2010 Full Professor, Department of Chemistry and Biochemistry, University of California Santa Barbara, Santa Barbara CA USA 1993–96 Associate Professor, Department of Chemistry and Biochemistry, University of California Santa Barbara, Santa Barbara CA USA 1988–93 Assistant Professor, Department of Chemistry and Biochemistry, University of California Santa Barbara, Santa Barbara CA USA

研究领域

Overview and summary Dynamics at surfaces is the field where atomic-scale understanding emerges concerning the elementary events important to interfacial energy transfer and surface chemistry. Following the tradition of gas-phase chemical dynamics, a well proven strategy is employed, where quantum-state, angle (both incident and recoil) and speed resolved experiments are compared with first-principle theoretical simulations. Eventually, theoretical advances can be obtained that are sufficient to quantitatively describe a variety of highly sophisticated experimental results obtained over a wide range of experimental conditions. Where such agreement can be achieved, the validated first principle theory can be used to reveal an atomic level movie of interactions important in the molecule surface encounters. In a sense, this approach is capable of informing us of the complete range of atomic motions contributing to the processes of interest.

近期论文

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Choudhury, A.; Sinha, S.; Harlander, D.; DeVine, J.; Kandratsenka, A.; Saalfrank, P.; Schwarzer, D.; Wodtke, A. M.: Manipulating tunnelling gateways in condensed phase isomerization. Natural Sciences, in press (2023) Zhao, Z.; Wang, Y.; Yang, X.; Quan, J.; Krüger, B. C.; Stoicescu, P.; Nieman, R.; Auerbach, D. J.; Wodtke, A. M.; Guo, H. et al.: Spin-dependent reactivity and spin-flipping dynamics in oxygen atom scattering from graphite. Nature Chemistry (2023) Krüger, K.; Wang, Y.; Tödter, S.; Debbeler, F.; Matveenko, A.; Hertl, N.; Zhou, X.; Jiang, B.; Guo, H.; Wodtke, A. M. et al.: Hydrogen atom collisions with a semiconductor efficiently promote electrons to the conduction band. Nature Chemistry 15, pp. 326 - 331 (2023) Lau, J. A.; Verma, V. B.; Schwarzer, D.; Wodtke, A. M.: Superconducting single-photon detectors in the mid-infrared for physical chemistry and spectroscopy. Chemical Society Reviews 52, pp. 921 - 941 (2023) Fingerhut, J.; Lecroart, L.; Borodin, D.; Schwarzer, M.; Hoerandl, S.; Kandratsenka, A.; Auerbach, D. J.; Wodtke, A. M.; Kitsopoulos, T. N.: Binding Energy and Diffusion Barrier of Formic Acid on Pd(111). The Journal of Physical Chemistry A 127 (1), pp. 142 - 152 (2023) Golibrzuch, K.; Walpole, V.; Schönemann, A.-M.; Wodtke, A. M.: Generation of Sub-nanosecond H Atom Pulses for Scattering from Single-Crystal Epitaxial Graphene. The Journal of Physical Chemistry A 126 (43), pp. 8101 - 8110 (2022) Choudhury, A.; DeVine, J.; Sinha, S.; Lau, J. A.; Kandratsenka, A.; Schwarzer, D.; Saalfrank, P.; Wodtke, A. M.: Condensed-phase isomerization through tunnelling gateways. Nature 612, pp. 691 - 695 (2022) Zhang, Y.; Box, C. L.; Schäfer, T.; Kandratsenka, A.; Wodtke, A. M.; Maurer, R. J.; Jiang, B.: Stereodynamics of adiabatic and non-adiabatic energy transfer in a molecule surface encounter. Physical Chemistry Chemical Physics 24 (33), pp. 19753 - 19760 (2022) Schwarzer, M.; Hertl, N.; Nitz, F.; Borodin, D.; Fingerhut, J.; Kitsopoulos, T. N.; Wodtke, A. M.: Adsorption and Absorption Energies of Hydrogen with Palladium. The Journal of Physical Chemistry C 126 (34), pp. 14500 - 14508 (2022) Martin-Barrios, R.; Hertl, N.; Galparsoro, O.; Kandratsenka, A.; Wodtke, A. M.; Larregaray, P.: H atom scattering from W(110): A benchmark for molecular dynamics with electronic friction. Physical Chemistry Chemical Physics 24, pp. 20813 - 20819 (2022) Papendorf, K.; Golibrzuch, K.; Zhong, T.; Schwabe, S.; Kitsopoulos, T. N.; Wodtke, A. M.: Velocity‐resolved laser‐induced desorption for kinetics on surface adsorbates. Chemistry–Methods 2 (5), e202200017 (2022) DeVine, J.; Choudhury, A.; Lau, J. A.; Schwarzer, D.; Wodtke, A. M.: Spin-Forbidden Carbon–Carbon Bond Formation in Vibrationally Excited α-CO. The Journal of Physical Chemistry A 126 (14), pp. 2270 - 2277 (2022) Golibrzuch, K.; Schwabe, S.; Zhong, T.; Papendorf, K.; Wodtke, A. M.: Application of an event-based camera for real-time velocity resolved kinetics. The Journal of Physical Chemistry A 126 (13), pp. 2142 - 2148 (2022) Hertl, N.; Kandratsenka, A.; Wodtke, A. M.: Effective medium theory for bcc metals: Electronically non-adiabatic H atom scattering in full dimensions. Physical Chemistry Chemical Physics 24 (15), pp. 8738 - 8748 (2022) Dorst, A.C.; Güthoff, F.; Schauermann, D.; Wodtke, A. M.; Killelea, D. R.; Schäfer, T.: Velocity map images of desorbing oxygen from sub-surface states of Rh(111). Physical Chemistry Chemical Physics 24, pp. 26421 - 26427 (2022) Fingerhut, J.; Borodin, D.; Schwarzer, M.; Skoulatakis, G.; Auerbach, D. J.; Wodtke, A. M.; Kitsopoulos, T. N.: The barrier for CO2 functionalization to formate on hydrogenated Pt. Journal of Physical Chemistry A 125 (34), pp. 7396 - 7405 (2021) Lecroart, L.; Hertl, N.; Dorenkamp, Y.; Jiang, H.; Kitsopoulos, T. N.; Kandratsenka, A.; Bünermann, O.; Wodtke, A. M.: Adsorbate modification of electronic nonadiabaticity: H atom scattering from p(2 × 2) O on Pt(111). The Journal of Chemical Physics 155 (3), 034702 (2021) Hertl, N.; Kandratsenka, A.; Bünermann, O.; Wodtke, A. M.: Multibounce and subsurface scattering of H atoms colliding with a van der Waals solid. The Journal of Physical Chemistry A 125 (26), pp. 5745 - 5762 (2021) Hertl, N.; Martin-Barrios, R.; Galparsoro, O.; Larrégaray, P.; Auerbach, D. J.; Schwarzer, D.; Wodtke, A. M.; Kandratsenka, A.: Random force in molecular dynamics with electronic friction. The Journal of Physical Chemistry C 125 (26), pp. 14468 - 14473 (2021) Borodin, D.; Rahinov, I.; Fingerhut, J.; Schwarzer, M.; Hörandl, S.; Skoulatakis, G.; Schwarzer, D.; Kitsopoulos, T. N.; Wodtke, A. M.: NO binding energies to and diffusion barrier on Pd obtained with velocity-resolved kinetics. The Journal of Physical Chemistry C 125 (21), pp. 11773 - 11781 (2021) Auerbach, D. J.; Tully, J. C.; Wodtke, A. M.: Chemical dynamics from the gas-phase to surfaces. Natural Sciences 1 (1), e10005 (2021) Bünermann, O.; Kandratsenka, A.; Wodtke, A. M.: Inelastic scattering of H atoms from surfaces. Journal of Physical Chemistry A 125 (15), pp. 3059 - 3076 (2021) Jiang, H.; Tao, X.; Kammler, M.; Ding, F.; Wodtke, A.; Kandratsenka, A.; Miller III, T. F.; Bünermann, O.: Small nuclear quantum effects in scattering of H and D from graphene. Journal of Physical Chemistry Letters 12 (7), pp. 1991 - 1996 (2021) Lau, J. A.; Chen, L.; Choudhury, A.; Schwarzer, D.; Verma, V. B.; Wodtke, A. M.: Transporting and concentrating vibrational energy to promote isomerization. Nature 589 (7842), pp. 391 - 395 (2021) Borodin, D.; Schwarzer, M.; Hahn, H. W.; Fingerhut, J.; Wang, Y.; Auerbach, D. J.; Guo, H.; Schroeder, J.; Kitsopoulos, T. N.; Wodtke, A. M.: The puzzle of rapid hydrogen oxidation on Pt(111). Molecular Physics 119 (17-18), e1966533 (2021) Wille, S.; Jiang, H.; Bünermann, O.; Wodtke, A. M.; Behler, J.; Kandratsenka, A.: An experimentally validated neural-network potential energy surface for H-atom on free-standing graphene in full dimensionality. Physical Chemistry Chemical Physics 22 (45), pp. 26113 - 26120 (2020) Geweke, J.; Wodtke, A. M.: Vibrationally inelastic scattering of HCl from Ag(111). Journal of Chemical Physics 153 (16), 164703 (2020) Lau, J. A.; Schönemann, A.-M.; Schwarzer, D.; Wodtke, A. M.: The coverage dependence of the infrared absorption of CO adsorbed to NaCI(100). The Journal of Chemical Physics 153 (15), 154703 (2020) Galparsoro, O.; Kaufmann, S.; Auerbach, D. J.; Kandratsenka, A.; Wodtke, A. M.: First principles rates for surface chemistry employing exact transition state theory: application to recombinative desorption of hydrogen from Cu(111). Physical Chemistry Chemical Physics 22 (31), pp. 17532 - 17539 (2020) Gerrits, N.; Geweke, J.; Smeets, E. W. F.; Voss, J.; Wodtke, A. M.; Kroes, G.-J.: Closing the gap between experiment and theory: Reactive scattering of HCl from Au(111). Journal of Physical Chemistry C 124 (29), pp. 15944 - 15960 (2020) Lau, J. A.; Choudhury, A.; Chen, L.; Schwarzer, D.; Verma, V. B.; Wodtke, A. M.: Observation of an isomerizing double-well quantum system in the condensed phase. Science 367 (6474), pp. 175 - 178 (2020) Kumar, S.; Jiang, H.; Schwarzer, M.; Kandratsenka, A.; Schwarzer, D.; Wodtke, A. M.: Vibrational relaxation lifetime of a physisorbed molecule at a metal surface. Physical Review Letters 123 (15), 156101 (2019) Park, G. B.; Krüger, B. C.; Borodin, D.; Kitsopoulos, T.; Wodtke, A. M.: Fundamental mechanisms for molecular energy conversion and chemical reactions at surfaces. Reports on Progress in Physics 82 (9), 09640 (2019) Krüger, B. C.; Schäfer, T.; Wodtke, A. M.; Park, G. B.: Quantum-state resolved lifetime of triplet (ã3A2) formaldehyde. Journal of Molecular Spectroscopy 362, pp. 61 - 68 (2019) Lee, H. J.; Yang, U. J.; Kim, K. N.; Park, S.; Kil, K. H.; Kim, J. S.; Wodtke, A. M.; Choi, W. J.; Kim, M. H.; Baik, J. M.: Directional Ostwald ripening for producing aligned arrays of nanowires. Nano Letters 19 (7), pp. 4306 - 4313 (2019) Jiang, H.; Kammler, M.; Ding, F.; Dorenkamp, Y.; Manby, F. R.; Wodtke, A. M.; Miller, T. F.; Kandratsenka, A.; Bünermann, O.: Imaging covalent bond formation by H atom scattering from graphene. Science 364 (6438), pp. 379 - 382 (2019) Zhou, L.; Kandratsenka, A.; Campbell, C. T.; Wodtke, A. M.; Guo, H.: Origin of thermal and hyperthermal CO2 from CO oxidation on Pt surfaces: The role of post-transition-state dynamics, active sites, and chemisorbed CO2. Angewandte Chemie International Edition 58 (21), pp. 6916 - 6920 (2019)