Schneider, Sven - Georg-August-Universitäten Göttingen

个人简介

Ausbildung und Qualifikation seit 2012 W3-Professur, Georg-August-Universität Göttingen 2010 - 2012 W2-Professur, Friedrich-Alexander-Universität Nürnberg/Erlangen 2006 - 2010 Habilitation, TU München, Prof W A Herrmann 2003 - 2006 Postdoc, Northwestern University, USA, Prof T J Marks 1999 - 2003 Dissertation, Humboldt Universität zu Berlin, Prof A C Filippou 1999 Diplomarbeit (M.Sc.), TU Darmstadt, Prof H-F Klein 1995 - 1996 Chemiestudium, University of Bristol, UK 1993 - 1998 Chemiestudium, Technische Universität Darmstadt Auszeichnungen 2015 ERC Consolidator Grant 2010 Akademiepreis für Chemie der Akademie der Wissenschaften zu Göttingen 2009 Förderpreis der Otto Röhm Gedächtnis Stiftung 2006 Emmy-Noether Programm (DFG) 2006 Liebig Stipendium (FCI) 2004 Emmy-Noether Postdoc Stipendendium (DFG) 2003 Fischer-Nernst Preis (Humboldt Universität) 1999 Dr.-Anton-Keller Preis (TU Darmstadt)

研究领域

Our group examines challenging catalytic multielectron/multiproton redox transformations, such as (de-)hydrogenation reactions, CO2 reduction and specifically the direct use of dinitrogen as a chemical feedstock. For this purpose we develop functional ligands that serve as storage sites for redox equivalents and/or protons. These concepts of metal-ligand and multimetallic cooperativity are applied to homogeneous catalysis, electrocatalysis and photocatalyis relevant to chemical synthesis, chemical energy storage and material synthesis through chemical bottom-up approaches (Atomic Layer Deposition).

近期论文

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"Triplet Carbenes with Transition-Metal Substituents", Z.-J. Lv, K. A. Eisenlohr, R. Naumann, T. Reuter, H. Verplancke, S. Demeshko, R. Herbst-Irmer, K. Heinze, M. C. Holthausem, S. Schneider, Nat. Chem. 2024, accepted manuscript. "Isolation of an Osmium(III) Hydrido Complex", N. Alizadeh, J. Abbenseth, S. Bete, M. Finger, M. Otte, C. Würtele, S. Schneider, Z. anorg. allg. Chem. 2024, e202300249. "C–H Bond Activation by Iridium(III) and Iridium(IV) Oxo Complexes", M. A. Tepaske, A. Fitterer, H. Verplancke, D. Delony, M. C. Neben, B. de Bruin, M. C. Holthausen, S. Schneider, Angew. Chem. Int. Ed. 2024 e202316729. "Photoinduced Metallonitrene Formation by N2 Elimination from Azide Diradical Ligands", L. I. Domenianni, M. Bauer, T. Schmidt-Räntsch, J. Lindner, S. Schneider, P. Vöhringer, Angew. Chem. Int. Ed. 2023 e202309618. "Nitrides stepping up: Terminal nitrido complexes in nitrogen fixation and nitrogen atom transfer reactions", L. Alig, M. Finger, S. Schneider, Adv. Inorg. Chem. 2023, 82 , 1-40. "Linearly bridging N2 versus CO: Chemical bonding and spin-controlled reactivity", M. Fritz, S. Demeshko, C. Würtele, M. Finger, S. Schneider, Eur. J. Inorg. Chem. 2023 e202300011. "Stabilizing Doubly Deprotonated Diazomethane: Isolable Complexes with CN22– and CN2– Radical Ligands", Z.-J. Lv, P. D. Engel, L. Alig, S. Maji, M. Holthausen, S. Schneider, J. Am. Chem. Soc. 2022, 144, 21872–21877. Preview: "Carbynes reloaded: Isolation of singlet metallocarbenes", Z.-J. Lv, S. Schneider, Chem 2022, 8, 1-3.Main Paper: Crystalline monometal-substituted free carbenes "Halide Effects in Reductive Splitting of Dinitrogen with Rhenium Pincer Complexes", R. van Alten, P. A. Wieser, M. Finger, J. Abbenseth, S. Demeshko, C. Würtele, I. Siewert, S. Schneider, Inorg. Chem. 2022, 61, 11581-11591. "Photoelectrochemical Conversion of Dinitrogen to Benzonitrile: Selectivity Control by Electrophile- versus Proton-Coupled Electron Transfer", M. Fritz, S. Rupp, C.I. Kiene, S. Kisan, J. Telser, C. Würtele, V. Krewald, S. Schneider, Angew. Chem. Int. Ed. 2022, e202205922. "Facile Conversion of Ammonia to a Nitride in a Rhenium System that Cleaves Dinitrogen", G. P. Connor, D. Delony, J. E. Weber, B. Q. Mercado, J. B. Curley, S. Schneider, J. M. Mayer, P. L. Holland, Chem. Sci. 2022, 13, 4010-4018. "Nitrogen Atom Transfer Catalysis by Metallonitrene C–H Insertion: Photocatalytic Amidation of Aldehydes", T. Schmidt-Räntsch, H. Verplancke, J. N. Lienert, S. Demeshko, M. Otte, G. P. Van Trieste III, K. A. Reid, J. H. Reibenspies, D. C. Powers, M. C. Holthausen, S. Schneider, Angew. Chem. Int. Ed. 2022, 61, e202115626. "Rhenium-mediated Conversion of Dinitrogen and Nitric Oxide to Nitrous Oxide" L. Alig, K. A. Eisenlohr, Y. Zelenkova, S. Rosendahl, R. Herbst-Irmer, S. Demeshko, M. C. Holthausen, S. Schneider, Angew. Chem. Int. Ed. 2022, 61, e202113340. "Current Frontiers in Pincer Chemistry" N. Hazari, S. Schneider, Z. Anorg. Allg. Chem. 2021, 647, 1530. "Photo-Initiated Cobalt Catalyzed Radical Olefin Hydrogenation" S. Sang, T. Unruh, S. Demeshko, L. Domenianni, N. P. van Leest, P. Marquetand, F. Schneck, C. Würtele, F. J. de Zwart, B. de Bruin, L. González, P. Vöhringer, S. Schneider, Chem. Eur. J. 2021, 27, 16978-16989. "Stabilizing P≡P: P22– , P2•– and P20 as bridging Ligands" J. Sun, H. Verplancke, Julia I. Schweizer, M. Diefenbach, C. Würtele, M. Otte, I. Tkach, C. Herwig, C. Limberg, S. Demeshko, Max C. Holthausen, S. Schneider, Chem. 2021, 7, 1952-1962. "Cyanate Formation via Photolytic Splitting of Dinitrogen" B. Schluschaß, J.-H. Borter, S. Rupp, S. Demeshko, C. Herwig, C. Limberg, N. Maciulis, J. Schneider, C. Würtele, V. Krewald, D. Schwarzer, S. Schneider, JACS Au 2021, 1, 879-894. "Solvent dependent C-H Bond Strength in a Nickel Pincer Complex" F. Schneck, M. Finger, I. Siewert, S. Schneider, Z. Anorg. Allg. Chem. 2021, 647, 1478-1485. "Nitrogen Fixation via Splitting into Nitrido Complexes" S. Forrest, B. Schluschaß, E. Yuzik-Klimova, S. Schneider, Chem. Rev. 2021, 121, 6522-6587. "Exploring the coordination chemistry of N2 with technetium PNP pincer-type complexes" M. Besmer, H. Braband, S. Schneider, B. Spingler, R. Alberto, Inorg. Chem. 2021, 60, 6696-6701. "The Metaphosphite (PO2–) Anion as a Ligand" J. Abbenseth, F. Wätjen, M. Finger, S. Schneider, Angew. Chem. Int. Ed. 2020, 59, 23574-23578. "Examination of Protonation-Induced Dinitrogen Splitting by in situ EXAFS Spectroscopy" J. Abbenseth, J.-P. Oudsen, B. Venderbosch, S. Demeshko, M. Finger, C. Herwig, C. Würtele, M. Holthausen, C. Limberg, M. Tromp, S. Schneider, Inorg. Chem. 2020, 59, 14367-14375. "A Platinum(II) Metallonitrene with a Triplet Ground State" J. Sun, J. Abbenseth, H. Verplancke, M. Diefenbach, B. de Bruin, D. Hunger, C. Würtele, J. van Slageren, M. C. Holthausen, S. Schneider, Nature Chem. 2020, 12, 1054-1059. "Combined experimental and theoretical studies towards mutual osmium–bismuth donor/acceptor bonding" J. Ramler, K. Radacki, J. Abbenseth, C. Lichtenberg, Dalton Trans., 2020, 49, 9024-9034. "A Terminal Chlorophosphinidene Complex" J. Abbenseth, S. Schneider, Z. Anorg. Allg. Chem. 2020, 13, 565-569. "(Electro-)chemical Splitting of Dinitrogen with a Rhenium Pincer Complex" R. S. van Alten, F. Wätjen, S. Demeshko, A. J. M. Miller, C. Würtele, I. Siewert, S. Schneider, Eur. J. Inorg. Chem., 2020, 15-16, 1402-1410. "The Renaissance of Base Metal Catalysis Enabled by Functional Ligands" M. Fritz, S. Schneider, in: The Periodic Table II. Structure and Bonding (Eds.: D. Mingos), Springer, Cham, 2019, 182, pp. 1-36. "Selectivity of Tungsten Mediated Dinitrogen Splitting vs. Proton Reduction" B. Schluschaß, J. Abbenseth, S. Demeshko, M. Finger, A. Franke, C. Herwig, C. Würtele, I. Ivanovic-Burmazovic, C. Limberg, Joshua Telser, S. Schneider, Chem. Sci. 2019, 10, 10275-10280. "Oxidative Coupling of Terminal Rhenium Pnictide Complexes" J. Abbenseth, M. Diefenbach, A. Hinz, L. Alig, C. Würtele, J. M. Goicoechea, M. Holthausen, S. Schneider, Angew. Chem. Int. Ed. 2019, 58, 10971-10974. "A Terminal Iridium Oxo Complex with a Triplet Ground State" D. Delony, M. Kinauer, M. Diefenbach, S. Demeshko, C. Würtele, M. C. Holthausen, S. Schneider Angew. Chem. Int. Ed., 2019, 58, 10966-10970. "Interconversion of Phosphinyl Radical and Phosphinidene Complexes by Proton Coupled Electron Transfer" J. Abbenseth, D. Delony, M. C. Neben, C. Würtele, B. de Bruin, S. Schneider, Angew. Chem. Int. Ed. 2019, 58, 6338 –6341. "First-Row Transition Metal (De)hydrogenation Catalysis based on Functional Pincer Ligands" L. Alig, M. Fritz, S. Schneider Chem. Rev., 2019, 119, 2681-2751.. "Metal-Ligand Cooperative Synthesis of Benzonitrile via Electrochemical Reduction and Photolytic Splitting of Dinitrogen" F. Schendzielorz, M. Finger, J. Abbenseth, C. Würtele, V. Krewald, S. Schneider Angew. Chem. Int. Ed., 2019, 58, 830-834.