全杨健 - 香港科技大学

个人简介

Education 2015 Ph.D. (Supervisor: Prof. Zuowei Xie), CUHK 2011 B.Sc. (Supervisor: Prof. Lin Dong), Nanjing University Professional Chronology 2019-2021 Postdoc Scholar (Wenbin Lin Group), UChicago 2015-2019 Research Assistant Professor, Chemistry, CUHK

研究领域

Our research is devoted towards innovative, energy-efficient, and sustainable catalytic systems by rational design and combination of boron catalysis, reticular materials, photochemistry, and electrochemistry. Our initial research efforts will focus on the following aspects: 1. Boron-based molecular catalyst and photosensitizer 2. Reticular materials (MOF&COF) featuring boron active center 3. Electroreductive small molecular activation 4. Photoinduced chemical transformations

近期论文

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Jiaxin Lin, Jing Ouyang, Tianyu Liu, Fengxing Li, Herman Ho-Yung Sung, Ian Williams, Yangjian Quan. Metal-Organic Framework Boosts Heterogeneous Electron Donor–Acceptor Photoactivation. Nat. Commun. 2023, DOI: 10.1038/s41467-023-43577-5. Guanwen Hu, Zhiyong Wang, Xinmou Wang, Yangjian Quan. Recent Advances in Borylation via Electron Donor-Acceptor Complex Photoactivation. ChemPhotoChem 2023, e202300041 (Invited Contribution). Feng-Xing Li, Xinmou Wang, Jiaxin Lin, Xiangyu Lou, Jing Ouyang, Guanwen Hu, and Yangjian Quan. Selective Multifunctionalization of N-Heterocyclic Carbene Boranes via the Intermediacy of Boron-Centered Radical. Chem. Sci. 2023, DOI: 10.1039/D3SC01132A. Shengxian Cheng, Jing Ouyang, Muqing Li, Yingxue Diao, Jiachen Yao, Fengxing Li, Yat-For Lee, Herman Ho-Yung SUNG, Ian Williams, Zhengtao Xu, and Yangjian Quan. Charge Separation in Metal-Organic Framework Enables Heterogeneous Thiol Catalysis. Angew. Chem. Int. Ed. 2023, DOI: 10.1002/anie.202300993. (Highlighted by WileyChem and X-mol) Zhiyong Wang, Jiaxin Chen, Zhenyang Lin, and Yangjian QUAN. Photoinduced Dehydrogenative Borylation via Dihydrogen Bond Bridged Electron Donor and Acceptor Complexes. Chem. Eur. J. 2022, 29, e2022030. (Highlighted by WileyChem) S. Chen, J. Tang, and Y. Quan. Metal-Organic Frameworks with Organic Photosensitizers in Organic Synthesis. Eur. J. Inorg. Chem.2022, e202200274. (Invited Contribution). Selected publications before joining HKUST: Y. K. Au, J. Zhang, Y. Quan,* Z. Xie,* Ir-Catalyzed Selective B(3)-H Amination of o-Carboranes with NH3. J. Am. Chem. Soc. 2021, 143, 4148–4153 (Highlighted in Chemistry Views). Y. Quan,† W. Shi,† Y. Song, X. Jiang, C. Wang, W. Lin* Bifunctional Metal-Organic Layer with Organic Dyes and Iron Centers for Synergistic Photoredox Catalysis. J. Am. Chem. Soc. 2021, 143, 3075–3080 (Highlighted in Matter, Matter 2021, 4, 2683-2685, and Synfacts). Y. Quan,† G. Lan,† W. Shi,† Z. Xu, Y. Fan, E. You, X. Jiang, C. Wang, W. Lin* Metal-Organic Layers Hierarchically Integrate Three Synergistic Active Sites for Tandem Catalysis. Angew. Chem. Int. Ed. 2021, 60, 3115–3120. Y. Quan,† Y. Song,† W. Shi, Z. Xu, J. S. Chen, X. Jiang, C. Wang, W. Lin,* Metal–Organic Framework with Dual Active Sites in Engineered Mesopores for Bioinspired Synergistic Catalysis. J. Am. Chem. Soc. 2020, 142, 8602–8607. Y. K. Au,† H. Lyu,† Y. Quan,* Z. Xie,* Copper-Catalyzed Electrochemical Selective B–H Oxygenation of o-Carboranes at Room Temperature. J. Am. Chem. Soc. 2020, 142, 6940–6945. Y. Quan,† G. Lan,† Y. Fan, W. Shi, E. You, W. Lin,* Metal–Organic Layers for Synergistic Lewis Acid and Photoredox Catalysis. J. Am. Chem. Soc. 2020, 142, 1746–1751. Y. K. Au, H. Lyu, Y. Quan,* Z. Xie,* Catalytic Cascade Dehydrogenative Cross-Coupling of BH/CH and BH/NH: One-Pot Process to Carborano-Isoquinolinone. J. Am. Chem. Soc. 2019, 141, 12855–12862 (JACS Cover Art). H. Lyu, J. Zhang, J. Yang, Y. Quan,* Z. Xie,* Catalytic Regioselective Cage B(8)–H Arylation of o-Carboranes via “Cage-Walking” Strategy. J. Am. Chem. Soc. 2019, 141, 4219–4224. H. Lyu, Y. Quan,* Z. Xie,* Transition Metal Catalyzed Direct Amination of Cage B(4)−H Bond in o-Carboranes: Synthesis of Tertiary, Secondary and Primary o-Carboranyl Amines. J. Am. Chem. Soc. 2016, 138, 12727–12730. Y. Quan, Z. Xie,* Palladium-Catalyzed Regioselective Diarylation of o-Carboranes via Direct Cage B-H Activation. Angew. Chem., Int. Ed. 2016, 55, 1295–1298. Y. Quan, Z. Xie,* Palladium-Catalyzed Regioselective Intramolecular Coupling of o-Carborane with Aromatics via Direct Cage B-H Activation. J. Am. Chem. Soc. 2015, 137, 3502–3505. Y. Quan, Z. Xie,* Iridium Catalyzed Regioselective Cage Boron Alkenylation of o-Carboranes via Direct Cage B-H Activation. J. Am. Chem. Soc. 2014, 136, 15513–15516 (Highlighted in JACS spotlights, J. Am. Chem. Soc. 2014, 136, 15807, and Synfacts). Y. Quan, Z. Qiu, Z. Xie,* Transition-Metal-Mediated Three-Component Cascade Cyclization: Selective Cage B–C(sp2) Coupling of Carborane with Aromatics and Synthesis of Carborane-Fused Tricyclics. J. Am. Chem. Soc. 2014, 136, 7599–7602. Y. Quan, J. Zhang, Z. Xie,* Three-Component [2+2+1] Cross-Cyclotrimerization of Carboryne, Unactivated Alkene, and Trimethylsilylalkyne Co-Mediated by Zr and Ni. J. Am. Chem. Soc. 2013, 135, 18742–18745.