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个人简介

教育背景 2001-10--2005-09 德国斯图加特大学 博士 1998-09--2001-06 北京大学 硕士 1994-09--1998-07 北京大学 学士 工作简历 2020-01~现在, 中国科学院大连化学物理研究所, 组长 2018-01~2019-12,德国马克思-普朗克煤炭研究所, 资深科学家 2011-08~2017-12,德国马克思-普朗克化学能源转化研究所, 资深科学家 2009-01~2011-07,德国波恩大学, 课题组组长 2006-08~2009-06,德国波恩大学, 博士后 2005-10~2006-08,德国马克思-普朗克生物无机化学研究所, 博士后

研究领域

主要进行金属酶及模拟金属配合物催化能源小分子活化和化学转化的反应机理的基础研究,为设计具有高度专一性的新型催化剂提供新思路

近期论文

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Angew. Chem. Int. Ed.null. 2024, [2] McWilliams, Sean F, Mercado, Brandon Q, MacLeod, K Cory, Fataftah, Majed S, Tarrago, Maxime, Wang, Xiaoping, Bill, Eckhard, Ye, Shengfa, Holland, Patrick L. Dynamic effects on ligand field from rapid hydride motion in an iron(ii) dimer with an S=3 ground state. CHEMICAL SCIENCE[J]. 2023, 14(9): 2303-2312, http://dx.doi.org/10.1039/d2sc06412j. Wei, XiangZhu, Ding, TianYu, Wang, Yang, Yang, Bing, Yang, QingQing, Ye, Shengfa, 佟振合, Wu, LiZhu. Tracking an Fe-V(O) Intermediate for Water Oxidation in Water. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION[J]. 2023, http://dx.doi.org/10.1002/anie.202308192. Mei, Tao, Zhang, Peng, Song, Zihe, Wang, Baomin, Qu, Jingping, Ye, Shengfa, Yang, Dawei. Unusual Hydrogenation Reactivities of a Thiolate-Bridged Dicobalt μ-Nitride Featuring a Bent {Co III -N-Co III } Core. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY[J]. 2023, 145(37): 20578-20587, http://dx.doi.org/10.1021/jacs.3c07254. Yang Liu, Stefan G. Resch, 陈浩玮, Sebastian Dechert, Serhiy Demeshko, Eckhard Bill, 叶生发, Franc Meyer. Fully Delocalized Mixed-Valent Cu1.5Cu1.5 Complex: Strong Cu-Cu interaction and Fast Electron Self-Exchange Rate Despite Large Structural Changes. Angew. Chem. Int. Ed.[J]. 2023 Dongmin Wang, Wang Chen, Cai Zhai, Lili Zhao, 叶生发, 谭庚文. Monosubstituted Doublet Sn(I) Radical Featuring Substantial Unquenched Orbital Angular Momentum. J. Am. Chem. Soc.[J]. 2023 Xiong, Jin, Liu, Qing, Lavina, Barbara, Hu, Michael Y, Zhao, Jiyong, Alp, Esen E, Deng, Liang, Ye, Shengfa, Guo, Yisong. Spin polarization assisted facile C-H activation by an S=1 iron(iv)-bisimido complex: a comprehensive spectroscopic and theoretical investigation. CHEMICAL SCIENCE[J]. 2023, 14(11): 2808-2820, http://dx.doi.org/10.1039/d2sc06273a. Shengfa Ye. Probing electronic structures of transition metal complexes using electron paramagnetic resonance spectroscopy. MAGNETIC RESONANCE LETTERS[J]. 2023, 3(1): 43-60, http://dx.doi.org/10.1016/j.mrl.2022.06.002. McWilliams, Sean F, Mercado, Brandon Q, MacLeod, K Cory, Fataftah, Majed S, Tarrago, Maxime, Wang, Xiaoping, Bill, Eckhard, Ye, Shengfa, Holland, Patrick L. Dynamic effects on ligand field from rapid hydride motion in an iron(ii) dimer with an S=3 ground state. CHEMICAL SCIENCE[J]. 2023, 14(9): 2303-2312, http://dx.doi.org/10.1039/d2sc06412j. Yang, Jianan, Ma, Yingjie, Liu, Qing, Leng, Xuebing, Zhou, Shuangliu, Ye, Shengfa, Deng, Liang, Wang, Shaowu. Noninnocent Behavior of a (3-Imino)indol-2-yl Ligand in Metal Complexes. ORGANOMETALLICS[J]. 2022, 41(4): 480-485, http://dx.doi.org/10.1021/acs.organomet.2c00003. Li, Yongxian, Chen, JiaYi, Miao, Qiyi, Yu, Xin, Feng, Lei, Liao, RongZhen, Ye, Shengfa, Tung, ChenHo, Wang, Wenguang. A Parent Iron Amido Complex in Catalysis of Ammonia Oxidation. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY[J]. 2022, 144(10): 4365-4375, http://dx.doi.org/10.1021/jacs.1c08609. Yixin Zhang, Jinfeng Zhao, Dawei Yang, Baomin Wang, Zhou Yuhan, Junhu Wang, Shengfa Ye. A thiolate-bridged FeIV FeIV μ-nitrido complex and its hydrogenation reactivity toward ammonia formation. Nature Chemistry[J]. 2022, Yang, Chengbo, Jiang, Xuebin, Chen, Qi, Leng, Xuebing, Xiao, Jie, Ye, Shengfa, Deng, Liang. Signet-Ring-Shaped Octaphosphorus-Cobalt Complexes: Synthesis, Structure, and Functionalization Reactions with Carbene Analogs. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY[J]. 2022, 144(45): 20785-20796, http://dx.doi.org/10.1021/jacs.2c08647. Cordes, Claudia, Klawitter, Iris, Rueter, Isabelle, Dechert, Sebastian, Demeshko, Serhiy, Ye, Shengfa, Meyer, Franc. Organometallic mu-Nitridodiiron Complexes in Oxidation States Ranging from (III/III) to (IV/IV). INORGANIC CHEMISTRY[J]. 2022, 61(18): 7153-7164, http://dx.doi.org/10.1021/acs.inorgchem.2c00685. Wang, GaoXiang, Chen, Wang, Yan, Xuechao, Xie, Fei, Wei, Junnian, Ye, Shengfa, Xi, Zhenfeng. Preparation and Characterization of a 19-Electron Ni(I) Complex Bearing a Cyclopentadienyl-Phosphine Ligand. ORGANOMETALLICS[J]. 2022, 41(15): 2227-2231, http://dx.doi.org/10.1021/acs.organomet.2c00304. Yao-Cheng Tian, 姜洋, Yen-Hao Lin, 张鹏, Chun-Chieh Wang, 叶生发, LEE WAY-ZEN. Hydrogen Atom Transfer Thermodynamics of Homologous Co(III)and Mn(III)-Superoxo Complexes: The Effect of the Metal Spin State. JACS Au[J]. 2022 Tarrago, Maxime, Ye, Shengfa, Neese, Frank. Electronic structure analysis of electrochemical CO2 reduction by iron-porphyrins reveals basic requirements for design of catalysts bearing non-innocent ligands. CHEMICAL SCIENCE[J]. 2022, 13(34): 10029-10047, http://apps.webofknowledge.com/CitedFullRecord.do?product=UA&colName=WOS&SID=5CCFccWmJJRAuMzNPjj&search_mode=CitedFullRecord&isickref=WOS:000840914900001. Monkcom, Emily C, de Bruin, Daniel, de Vries, Annemiek J, Lutz, Martin, Ye, Shengfa, Gebbink, Robertus J M Klein. Structurally Modelling the 2-His-1-Carboxylate Facial Triad with a Bulky N,N,O Phenolate Ligand. CHEMISTRY-A EUROPEAN JOURNAL[J]. 2021, 27(16): 5191-5204, https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8048785/. Zhe Huang, Yongliang Zhang, WenXiong Zhang, Junnian Wei, Shengfa Ye, Zhenfeng Xi. A tris-spiro metalla-aromatic system featuring Craig-Möbius aromaticity. NATURE COMMUNICATIONS[J]. 2021, 12(1): 1-7, https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7910433/. Xu, Sunlin, Yang, Dawei, Wang, Baomin, Chen, Yifeng, Ye, Shengfa, Qu, Jingping. Generation of a Sulfinamide Species from Facile N-O Bond Cleavage of Nitrosobenzene by a Thiolate-Bridged Diiron Complex. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY[J]. 2021, 143(42): 17374-17387, http://dx.doi.org/10.1021/jacs.1c03542. Huang, Zhe, Zhang, Yongliang, Zhang, WenXiong, Wei, Junnian, Ye, Shengfa, Xi, Zhenfeng. A tris-spiro metalla-aromatic system featuring Craig-Mobius aromaticity. NATURE COMMUNICATIONS[J]. 2021, 12(1): https://www.webofscience.com/wos/woscc/full-record/WOS:000624978300030. Qiao, Yunxiang, Theyssen, Nils, Spliethoff, Bernd, Folke, Jan, Weidenthaler, Claudia, Schmidt, Wolfgang, Prieto, Gonzalo, OchoaHernandez, Cristina, Bill, Eckhard, Ye, Shengfa, Ruland, Holger, Schueth, Ferdi, Leitner, Walter. Synthetic ferripyrophyllite: preparation, characterization and catalytic application. DALTON TRANSACTIONS[J]. 2021, 50(3): http://dx.doi.org/10.1039/d0dt03125a. Zhang, Yongliang, Yu, Chao, Huang, Zhe, Zhang, WenXiong, Ye, Shengfa, Wei, Junnian, Xi, Zhenfeng. Metalla-aromatics: Planar, Nonplanar, and Spiro. ACCOUNTS OF CHEMICAL RESEARCHnull. 2021, 54(9): 2323-2333, http://dx.doi.org/10.1021/acs.accounts.1c00146. Tarrago, Maxime, Roemelt, Christina, Nehrkorn, Joscha, Schnegg, Alexander, Neese, Frank, Bill, Eckhard, Ye, Shengfa. Experimental and Theoretical Evidence for an Unusual Almost Triply Degenerate Electronic Ground State of Ferrous Tetraphenylporphyrin. INORGANICCHEMISTRY[J]. 2021, 60(7): 4966-4985, http://dx.doi.org/10.1021/acs.inorgchem.1c00031. Huang, Zhe, Zheng, Yu, Zhang, WenXiong, Ye, Shengfa, Deng, Liang, Xi, Zhenfeng. Dinickelaferrocene: A Ferrocene Analogue with Two Aromatic Nickeloles Realized by Electron Back-Donation from Iron. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION[J]. 2020, 59(34): 14394-14398, Yu, Chao, Zhong, Mingdong, Zhang, Yongliang, Wei, Junnian, Ma, Wangyang, Zhang, WenXiong, Ye, Shengfa, Xi, Zhenfeng. Butadienyl Diiron Complexes: Nonplanar Metalla-Aromatics Involving sigma-Type Orbital Overlap. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION[J]. 2020, 59(43): 19048-19053, http://dx.doi.org/10.1002/anie.202008986. Roy, Lisa, Mondal, Bhaskar, Ye, Shengfa. Computational mechanistic insights into non-noble-metal-catalysed CO2 conversion. DALTON TRANSACTIONSnull. 2020, 49(46): 16608-16616, https://www.webofscience.com/wos/woscc/full-record/WOS:000597124500005. Chan, SiuChung, Ang, Zhi Zhong, Gupta, Puneet, Ganguly, Rakesh, Li, Yongxin, Ye, Shengfa, England, Jason. Carbodicarbene Ligand Redox Noninnocence in Highly Oxidized Chromium and Cobalt Complexes. INORGANIC CHEMISTRY[J]. 2020, 59(6): 4118-4128, http://dx.doi.org/10.1021/acs.inorgchem.0c00153. Mondal, Bhaskar, Ye, Shengfa. Hidden ligand noninnocence: A combined spectroscopic and computational perspective. COORDINATION CHEMISTRY REVIEWSnull. 2020, 405: http://apps.webofknowledge.com/CitedFullRecord.do?product=UA&colName=WOS&SID=5CCFccWmJJRAuMzNPjj&search_mode=CitedFullRecord&isickref=WOS:000509626700002. Chen, TingYi, Ho, PoHsun, Spyra, CanJerome, Meyer, Franc, Bill, Eckhard, Ye, Shengfa, Lee, WayZen. Ambiphilicity of a mononuclear cobalt(iii) superoxo complex. CHEMICAL COMMUNICATIONS[J]. 2020, 56(94): 14821-14824, http://dx.doi.org/10.1039/d0cc05337f. Wong, Joanne W L, Hua, ShaoAn, Demeshko, Serhiy, Dechert, Sebastian, Ye, Shengfa, Meyer, Franc. Bis(pyrazolato) Bridged Diiron Complexes: Ferromagnetic Coupling in a Mixed-Valent HS-Fe-II/LS-Fe-III Dinuclear Complex. EUROPEAN JOURNAL OF INORGANIC CHEMISTRY[J]. 2020, 2020(43): 4137-4145, https://www.webofscience.com/wos/woscc/full-record/WOS:000587674700001. Tarrago, Maxime, Ye, Shengfa. A Short Perspective on Electrochemical CO2 Reduction to CO. CHIMIA[J]. 2020, 74(6): 478-482, https://doaj.org/article/d2703a4260c2463d9b0d3e88bb910a5a. Lin, YenHao, Kutin, Yury, van Gastel, Maurice, Bill, Eckhard, Schnegg, Alexander, Ye, Shengfa, Lee, WayZen. A Manganese(IV)-Hydroperoxo Intermediate Generated by Protonation of the Corresponding Manganese(III)-Superoxo Complex. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY[J]. 2020, 142(23): 10255-10260, http://dx.doi.org/10.1021/jacs.0c02756. Cheng, Jun, Chen, Qj, Leng, Xuebing, Ye, Shengfa, Deng, Liang. Three-Coordinate Iron(0) Complexes with N-Heterocyclic Carbene and Vinyltrimethylsilane Ligation: Synthesis, Characterization, and Ligand Substitution Reactions. INORGANIC CHEMISTRY[J]. 2019, 58(19): 13129-13141, https://www.webofscience.com/wos/woscc/full-record/WOS:000489676400074. Cheng, Jun, Liu, Jian, Leng, Xuebing, Lohmiller, Thomas, Schnegg, Alexander, Bill, Eckhard, Ye, Shengfa, Deng, Liang. A Two-Coordinate Iron(II) Imido Complex with NHC Ligation: Synthesis, Characterization, and Its Diversified Reactivity of Nitrene Transfer and C-H Bond Activation. INORGANIC CHEMISTRY[J]. 2019, 58(11): 7634-7644, https://www.webofscience.com/wos/woscc/full-record/WOS:000470332200054. Chang, HaoChing, Mondal, Bhaskar, Fang, Huayi, Neese, Frank, Bill, Eckhard, Ye, Shengfa. Electron Paramagnetic Resonance Signature of Tetragonal Low Spin Iron(V)-Nitrido and -Oxo Complexes Derived from the Electronic Structure Analysis of Heme and Non-Heme Archetypes. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY[J]. 2019, 141(6): 2421-2434, https://www.webofscience.com/wos/woscc/full-record/WOS:000459222100035. Ghosh, Munmun, Cramer, Hanna H, Dechert, Sebastian, Demeshko, Serhiy, John, Michael, Hansmann, Max M, Ye, Shengfa, Meyer, Franc. A mu-Phosphido Diiron Dumbbell in Multiple Oxidation States. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION[J]. 2019, 58(40): 14349-14356, Keilwerth, Martin, Hohenberger, Johannes, Heinemann, Frank W, Sutter, Joerg, Scheurer, Andreas, Fang, Huayi, Bill, Eckhard, Neese, Frank, Ye, Shengfa, Meyer, Karsten. A Series of Iron Nitrosyl Complexes {Fe-NO}(6-9) and a Fleeting {Fe-NO}(10) Intermediate en Route to a Metalacyclic Iron Nitrosoalkane. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY[J]. 2019, 141(43): 17217-17235, Roy, Lisa, AlAfyouni, Malik H, DeRosha, Daniel E, Mondal, Bhaskar, DiMucci, Ida M, Lancaster, Kyle M, Shearer, Jason, Bill, Eckhard, Brennessel, William W, Neese, Frank, Ye, Shengfa, Holland, Patrick L. Reduction of CO2 by a masked two-coordinate cobalt(i) complex and characterization of a proposed oxodicobalt(ii) intermediate. CHEMICAL SCIENCE[J]. 2019, 10(3): 918-929, https://www.webofscience.com/wos/woscc/full-record/WOS:000457304200029. Moore, James T, Chatterjee, Sudipta, Tarrago, Maxime, Clouston, Laura J, Sproules, Stephen, Bill, Eckhard, Bernales, Varinia, Gagliardi, Laura, Ye, Shengfa, Lancaster, Kyle M, Lu, Connie C. Enhanced Fe-Centered Redox Flexibility in Fe-Ti Heterobimetallic Complexes. INORGANIC CHEMISTRY[J]. 2019, 58(9): 6199-6214, https://www.webofscience.com/wos/woscc/full-record/WOS:000467351100092. Chang, HaoChing, Lin, YenHao, Werle, Christophe, Neese, Frank, Lee, WayZen, Bill, Eckhard, Ye, Shengfa. Conversion of a Fleeting Open-Shell Iron Nitride into an Iron Nitrosyl. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION[J]. 2019, 58(49): 17589-17593, http://dx.doi.org/10.1002/anie.201908689. Lin, YenHao, Cramer, Hanna Hinrika, van Gastel, Maurice, Tsai, YiHsuan, Chu, ChiYi, Kuo, TingShen, Lee, IRen, Ye, Shengfa, Bill, Eckhard, Lee, WayZen. Mononuclear Manganese(III) Superoxo Complexes: Synthesis, Characterization, and Reactivity. INORGANIC CHEMISTRY[J]. 2019, 58(15): 9756-9765, http://dx.doi.org/10.1021/acs.inorgchem.9b00767. Zhang, Yongliang, Wei, Junnian, Zhu, Miaomiao, Chi, Yue, Zhang, WenXiong, Ye, Shengfa, Xi, Zhenfeng. Tetralithio Metalla-aromatics with Two Independent Perpendicular Dilithio Aromatic Rings Spiro-fused by One Manganese Atom. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION[J]. 2019, 58(28): 9625-9631, Chan, SiuChung, Gupta, Puneet, Engelmann, Xenia, Ang, Zhi Zhong, Ganguly, Rakesh, Bill, Eckhard, Ray, Kallol, Ye, Shengfa, England, Jason. Observation of Carbodicarbene Ligand Redox Noninnocence in Highly Oxidized Iron Complexes. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION[J]. 2018, 57(48): 15717-15722, http://dx.doi.org/10.1002/anie.201809158. Ye Shengfa. Electronic Structure Contributions of Non-Heme Oxo-Iron(V) Complexes to the Reactivity. Journal of the American Chemical Society. 2018, [42] Cheng, Jun, Chen, Qi, Leng, Xuebing, Ouyang, Zhongwen, Wang, Zhenxing, Ye, Shengfa, Deng, Liang. The Stabilization of Three-Coordinate Formal Mn(0) Complex with NHC and Alkene Ligation. CHEM[J]. 2018, 4(12): 2844-2860, http://dx.doi.org/10.1016/j.chempr.2018.09.002. Kupper, Claudia, Mondal, Bhaskar, SerranoPlana, Joan, Klawitter, Iris, Neese, Frank, Costas, Miguel, Ye, Shengfa, Meyer, Franc. Nonclassical Single-State Reactivity of an Oxo-Iron(IV) Complex Confined to Triplet Pathways. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY[J]. 2017, 139(26): 8939-8949, http://dx.doi.org/10.1021/jacs.7b03255.

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