个人简介
2009-2013, B.Sc., Chemistry, Sichuan University
2013-2017, Ph.D., Chemistry, Sichuan University
2017-2021, Postdoc, The University of Texas at Austin
2022-now, Professor, University of Electronic Science and Technology of China
研究领域
Materials Electrochemistry for Energy and Sustainability
A fundamental understanding of materials electrochemistry is of general significance for the development of high-efficient energy storage and conversion systems with environmental sustainability. We are establishing powerful electrochemical techniques for studying inherent properties and unusual effects in electrocatalysis and battery materials. We are also working on advanced electrosynthesis of renewable fuels, essential nutrients and natural organics from environmental wastes and pollutants.
In-Situ/Operando Characterization Techniques with Atomic Resolution
Electrochemical reactions, especially electrocatalysis, involve complicated and rapid processes of proton-coupled electron transfer. However, conventional ensemble measurements can hardly allow insights into ultrafast surface and interface interactions. The urgent need for the development of in situ characterization techniques with high spatial and time resolution would offer great opportunities to an understanding and guidance of materials designing. We are developing in situ electrochemical molecular probes and demonstrating one can measure catalytic kinetic rates of individual active sites with high accuracy. This emerging technique is being coupled with other spectroscopies to permit more important quantitative information associated to electrocatalysis and materials chemistry.
Computational Materials Science and Fundamental Electrochemistry
Materials physics is the fundamental for studying the solid-state electrochemistry that is processed on electrode surfaces. We are using computational modeling to predict and optimize physical properties of electrode materials for regulating the electrochemical behavior. Advanced machining technologies, including deep learning and AI assist, are being complemented to facilitate the discovery of outstanding materials, which effectively instruct the experimental synthesis. In addition, finite element simulations are also supported in the group to configure and tailor electrochemical reactors as well as other continuum models.
近期论文
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P. Li*; L. Liao; Z. Fang; G. Su; Z. Jin*; G. Yu*, Proceedings of the National Academy of Sciences 2023, 120, e2305489120.
P. Li*; R. Li; Y. Liu; M. Xie; Z. Jin*; G. Yu*, Pulsed Nitrate-to-Ammonia Electroreduction Facilitated by Tandem Catalysis of Nitrite Intermediates. Journal of the American Chemical Society 2023, 145, 6471–6479.
M. Xie; S. Tang; Z. Li; M. Wang; Z. Jin; P. Li; X. Zhan; H. Zhou; G. Yu, Intermetallic Single-Atom Alloy In-Pd Bimetallene for Neutral Electrosynthesis of Ammonia from Nitrate. Journal of the American Chemical Society 2023, 145, 13957–13967.
T. Gao; X. Tang; X. Li; S. Wu; S. Yu; P. Li*; D. Xiao*; Z. Jin*, Understanding the Atomic and Defective Interface Effect on Ruthenium Clusters for the Hydrogen Evolution Reaction. ACS Catalysis 2023, 13, 49-59.
Z. Jin*, High-Spatiotemporal-Resolution Electrochemical Measurements of Electrocatalytic Reactivity. Analytical Chemistry 2023, 95, 6477–6489.
H. Li, Y. Guo*, Z. Jin*, Advanced electrochemical techniques for characterizing electrocatalysis at the single-particle level, Carbon Neutrality 2023, 2, 22.
Y. Liu, J. Mao, Y. Yuan, H. Huang, X. Ma, X. Li*, Z. Jin*, Accelerating corrosion of iron foam enables a bifunctional catalyst for overall water splitting, Materials Chemistry Frontiers 2023.
R. Li; T. Gao; P. Wang; W. Qiu; K. Liu; Y. Liu; Z. Jin; P. Li, The Origin of Selective Nitrate-to-Ammonia Electroreduction on Metal-Free Nitrogen-Doped Carbon Aerogel Catalysts. Applied Catalysis B: Environmental 2023, 331, 122677.
W. Qiu; M. Xie; P. Wang; T. Gao; R. Li; D. Xiao; Z. Jin; P. Li, Size-Defined Ru Nanoclusters Supported by TiO2 Nanotubes Enable Low-Concentration Nitrate Electroreduction to Ammonia with Suppressed Hydrogen Evolution. Small 2023, 19, 2300437.
R. Li, T. Gao, W. Qiu, M. Xie, Z. Jin, P. Li, Unveiling the size effect of nitrogen-doped carbon-supported copper-based catalysts on nitrate-to-ammonia electroreduction, Nano Research 2023, DOI: 10.1007/s12274-12023-16094-z.
Y. Liu, K. Liu, P. Wang, Z. Jin, P. Li, Electrocatalytic upcycling of nitrogenous wastes into green ammonia: advances and perspectives on materials innovation, Carbon Neutrality 2023, 2, 14.
T. Gao, L. Qiu, M. Xie, Z. Jin, P. Li, G. Yu, Defect-stabilized and oxygen-coordinated iron single-atomic sites facilitate hydrogen peroxide electrosynthesis, Materials Horizons 2023, DOI: 10.1039/D1033MH00882G.
Y. Liu, W. Qiu, P. Wang, R. Li, K. Liu, K. M. Omer, Z. Jin, P. Li, Pyridine-N-rich Cu single-atom catalyst boosts nitrate electroreduction to ammonia, Applied Catalysis B: Environmental 2024, 340, 123228.
M. Xie; B. Zhang; Z. Jin*; P. Li; G. Yu*, Atomically Reconstructed Palladium Metallene by Intercalation-Induced Lattice Expansion and Amorphization for Highly Efficient Electrocatalysis ACS Nano 2022, 16, 13715-13727.
W. Qiu; X. Chen; Y. Liu; D. Xiao*; P. Wang; R. Li; K. Liu; Z. Jin*; P. Li*, Confining Intermediates within A Catalytic Nanoreactor Facilitates Nitrate-to-Ammonia Electrosynthesis. Applied Catalysis B: Environmental, 2022, 315, 121548.
P. Wang; Z. Jin; P. Li; G. Yu, Design Principles of Hydrogen-Evolution-Suppressing Single-Atom Catalysts for Aqueous Electrosynthesis. Chem Catalysis, 2022, 2, 1277-1287.
Z. Jin*; P. Li; Z. Fang; G. Yu*, Emerging Electrochemical Techniques for Probing Site Behavior in Single-Atom Electrocatalysts, Accounts of Chemical Research 2022, 55, 759–769.
Y. Luo; P. Li*; Z.Jin*, Lithiated Interface of Pt/TiO2 Enables an Efficient Wire-Shaped Zn-Air Solar Micro-Battery. Chemical Communications, 2022, 58, 5988-5991.
Z. Fang; Z. Jin; S. Tang; P. Li; P. Wu; G. Yu, Porous Two-dimensional Iron-Cyano Nanosheets for High-rate Electrochemical Nitrate Reduction. ACS Nano 2022, 16, 1072–1081.
Z. Jin†; P. Li†; Y. Meng; Z. Fang; D. Xiao; G. Yu, Understanding the inter-site distance effect in single-atom catalysts for oxygen electroreduction. Nature Catalysis 2021, 4, 615-622.
P. Li; Z. Jin*; Z. Fang; G. Yu*, A single-site iron catalyst with preoccupied active center that achieves selective ammonia electrosynthesis from nitrate. Energy & Environmental Science 2021, 14, 3522-3531.
Z. Jin; A.J. Bard, Surface Interrogation of Electrodeposited MnOx and CaMnO3 Perovskites by Scanning Electrochemical Microscopy: Probing Active Sites and Kinetics for the Oxygen Evolution Reaction. Angewandte Chemie International Edition 2021, 60, 794-799.
X. Li; Y. Guo; T. Gao; P. Li*; Z. Jin*; D. Xiao*, Interconnecting 3D Conductive Networks with Nanostructured Iron/Iron Oxide Enables a High-Performance Flexible Battery. ACS Applied Materials & Interfaces 2021, 13, 57411-57421.
P. Li; Z. Jin*; Z. Fang; G. Yu*, Ammonia Electrosynthesis on Single-Atom Catalysts: Mechanistic Understanding and Recent Progress. Chemical Physics Reviews 2021, 2, 041305.Z.
Jin; A.J. Bard, Atom-by-atom electrodeposition of single isolated cobalt oxide molecules and clusters for studying the oxygen evolution reaction. Proceedings of the National Academy of Sciences 2020, 117, 12651-12656.
P. Li; Z. Jin*; Z. Fang; G. Yu*, A Surface-Strained and Geometry-Tailored Nanoreactor that Promotes Ammonia Electrosynthesis. Angewandte Chemie International Edition 2020, 59, 22610-22616.
P. Li†;Z. Jin†; Y. Qian; Z. Fang; D. Xiao; G. Yu, Supramolecular confinement of single Cu atoms in hydrogel frameworks for oxygen reduction electrocatalysis with high atom utilization. Materials Today 2020, 35, 78-86.
A.D. Klementiev; Z. Jin; M. Whiteley, Micron Scale Spatial Measurement of the O2 Gradient Surrounding a Bacterial Biofilm in Real Time. Mbio 2020, 11, e02536-20.
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