Wang, Lei - National University of Singapore - Department of Chemical and Biomolecular Engineering

个人简介

Postdoc, Stanford University, California, U.S. Postdoc, Uppsala University, Uppsala, Sweden PhD, KTH Royal Institute of Technology, Stockholm, Sweden MS, Dalian University of Technology, Dalian, China BS, Dalian University of Technology, Dalian, China

研究领域

Our research interests lie primarily in understanding the structure-function relationships of catalytic materials, working fundamentals and establishing effective design principles for efficient, high-selectivity electrocatalytic processes, with the goal of large-scaled chemical transformations in renewable energy applications. CO2 reduction for fuels and chemicals production Water splitting for H2 production and its reverse reaction Electrochemical organic transformations

近期论文

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Preserving molecular tuning for enhanced electrocatalytic CO2-to-ethanol conversion Weiwei Fu, Yuke Li, Jiayi Chen, Jingyi Chen, Shibo Xi, Jia Zhang, Lei Wang* Angewandte Chemie International Edition, 2024. Energy-efficient CO(2) conversion to multicarbon products at high rates on CuGa bimetallic catalys Lei Chen, Junmei Chen, Weiwei Fu, Jiayi Chen, Di Wang, Yukun Xiao, Shibo Xi, Yongfei Ji*, Lei Wang* Nature Communication, 2024. Selective and stable CO2 electroreduction at high rates via control of local H2O/CO2 ratio Junmei Chen, Haoran Qiu, Yilin Zhao, Haozhou Yang, Lei Fan, Zhihe Liu, ShiBo Xi, Guangtai Zheng, Jiayi Chen, Lei Chen, Ya Liu, Liejin Guo, and Lei Wang* Nature Communication, 2024. Alkali cation-induced cathodic corrosion in Cu electrocatalysts Shikai Liu, Yuheng Li, Di Wang, Shibo Xi, Haoming Xu, Yulin Wang, Xinzhe Li, Wenjie Zang, Weidong Liu, Mengyao Su, Katherine Yan, Adam C. Nielander, Andrew B. Wong, Jiong Lu, Thomas F. Jaramillo, Lei Wang*, Pieremanuele Canepa*, and Qian He* Nature Communication, 2024. Revealing the Structure Evolution of CuAg Composites During Electrochemical Carbon Monoxide Reduction Di Wang, Hyun Dong Jung, Shikai Liu, Jiayi Chen, Haozhou Yang, Qian He*, Shibo Xi*, Seoin Back*, and Lei Wang* Nature Communication, 2024. Cu/LaF3 Interfaces Boost Electrocatalytic CO-to-Acetate Conversion Yilin Zhao, Yuke Li, Jingyi Chen, Buwei Sun, Lei Fan, Junmei Chen, Yukun Xiao, Haozhou Yang, Di Wang, Jiayi Chen, Xiaopeng Han, Shibo Xi, Jia Zhang*, and Lei Wang* ACS Catalysis, 2024. Enzyme-Inspired Ligand Engineering of Gold Nanoclusters for Electrocatalytic Microenvironment Manipulation Zhihe Liu, Junmei Chen, Bo Li, De-en Jiang*, Lei Wang*, Qiaofeng Yao*, and Jianping Xie* Journal of the American Chemical Society, 2024. Enhancing Cu-Ligand Interaction for Efficient CO2 Reduction towards Multi-Carbon Products Jingyi Chen, Lei Fan, Yilin Zhao, Haozhou Yang, Di Wang, Bihao Hu, Shibo Xi, Lei Wang*Chemical Communications, 2024. Tailoring the Chemical Environment of Ru-Mo Composites for Efficient Hydrogen and Oxygen Evolution Reaction Chunfeng Li, Jiayi Chen, Kok Chan Chong, Lei Wang*, Bin Liu*Small Structures, 2023. Enhancing CO Diffusion for Selective Acetate Production via CO Reduction on Copper Catalyst Junmei Chen, Lei Chen, Jingyi Chen, Di Wang, Yilin Zhao, Lan Wen, Shibo Xi, Lei Wang*Applied Catalysis B: Environmental, 2023. Multi-Shell Copper Catalysts for Selective Electroreduction of CO2 to Multicarbon Chemicals Yukun Xiao, Meng Wang, Haozhou Yang, Haoran Qiu, Haotian Lu, Yumin Da, Ganwen Chen, Tianyuan Jiang, Weiwei Fu, Bihao Hu, Junmei Chen, Lei Chen, Yishui Ding, Baihua Cui, Chonglai Jiang, Zejun Sun, Yu Long, Haotian Yang, Zhangliu Tian, Lei Wang*, Wei Chen* Advanced Energy Materials, 2023. Boosting Oxygen Reduction through Microenvironment Modulation to Enhance Mass Transportation Bihao Hu, Miao Wang, Danning Li, Jingyi Chen, Chunfeng Li, Lei Wang*Advanced Energy and Sustainability Research, 2023. Additive-Assisted Electrodeposition of Cu on Gas Diffusion Electrodes Enables Selective CO2 Reduction to Multicarbon Products Lei Chen, Jingyi Chen, Lei Fan, Jiayi Chen, Tianyu Zhang, Junmei Chen, Shibo Xi, Baoliang Chen*, and Lei Wang*ACS Catalysis, 2023. Selective production of ethylene glycol at high rate via cascade catalysis Lei Fan, Yilin Zhao, Lei Chen, Jiayi Chen, Junmei Chen, Haozhou Yang, Yukun Xiao, Tianyu Zhang, Jingyi Chen & Lei Wang*Nature Catalysis, 2023. Ligand effect on switching the rate-determining step of water oxidation in atomically precise metal nanoclusters Zhihe Liu, Hua Tan, Bo Li, Zehua Hu, De-en Jiang, Qiaofeng Yao*, Lei Wang* & Jianping Xie*Nature Communications, 2023. Promote electroreduction of CO2 via catalyst valence state manipulation by surface-capping ligand Yilin Zhao, Xiaoqing Liu, Jingyi Chen, Junmei Chen, Jiayi Chen, Lei Fan, Haozhou Yang, Shibo Xi, Lei Shen, and Lei Wang*PNAS, 2023. Electrocatalytic amino acid synthesis from biomass-derivable keto acids over ball milled carbon nanotubes Yiying Xiao, Chia Wei Lim, Jinquan Chang, Qixin Yuan,Lei Wang* and Ning Yan*Green Chemistry, 2023. Diversity of platinum-sites at platinum/fullerene interface accelerates alkaline hydrogen evolution Jiayi Chen, Mohammed Aliasgar, Fernando Buendia Zamudio, Tianyu Zhang, Yilin Zhao, Xu Lian, Lan Wen, Haozhou Yang, Wenping Sun*, Sergey M. Kozlov*, Wei Chen & Lei Wang*.Nature Communications, 2023. Directing oxygen reduction reaction selectivity towards hydrogen peroxide via electric double layer engineering Jingyi Chen, Yilin Zhao, Haozhou Yang, Tianyu Zhang, Lei Fan, Chunfeng Li and Lei Wang*.Nanoscale, 2023. Pinpointing the axial ligand effect on platinum single-atom-catalyst towards efficient alkaline hydrogen evolution reaction Tianyu Zhang, Jing Jin, Junmei Chen, Yingyan Fang, Xu Han, Jiayi Chen, Yaping Li, Yu Wang, Junfeng Liu* & Lei Wang*. Nature Communications, 2022. Functionalized Ag with Thiol Ligand to Promote Effective CO2 Electroreduction Junmei Chen, Xiaoqing Liu, Shibo Xi, Tianyu Zhang, Zhihe Liu, Jiayi Chen, Lei Shen,* Sibudjing Kawi,* and Lei Wang*. ACS Nano, 2022. Promoting oxygen reduction via coordination environment modulation through secondary metal-atom incorporation Haozhou Yang, Tianyu Zhang, Xiao Chi,Xiaojiang Yu, Junmei Chen, Jiayi Chen, Chunfeng Li, Shengdong Tan, Qian He, Xun Wang and Lei Wang. Journal of Materials Chemistry A, 2022. Vapor-Fed Electrolyzers for Carbon Dioxide Reduction Using Tandem Electrocatalysts: Cuprous Oxide Coupled with Nickel-Coordinated Nitrogen-Doped Carbon Yi-Rung Lin,Dong Un Lee,Shunquan Tan,David M. Koshy,Tiras Y. Lin,Lei Wang,Daniel Corral,Jaime E. Avilés Acosta,Jose A. Zamora Zeledon,Victor A. Beck,Sarah E. Baker,Eric B. Duoss,Christopher Hahn,Thomas F. Jaramillo. Advanced Functional Materials, 2022. A happy couple makes acetate from CO Lei Wang. Nature Catalysis, 2022. Using pH Dependence to Understand Mechanisms in Electrochemical CO Reduction Georg Kastlunge, Lei Wang, Nitish Govindarajan, Hendrik Heenen, Stefan Ringe, Thomas Jaramillo, Christopher Hahn, Chan Karen. ACS Catalysis, 2022. Designing a Zn–Ag Catalyst Matrix and Electrolyzer System for CO2 Conversion to CO and Beyond Sarah Lamaison, David Wakerley, Frauke Kracke, Thomas Moore, Lan Zhou, Dong Un Lee, Lei Wang, McKenzie A Hubert, Jaime E Aviles Acosta, John M Gregoire, Eric B Duoss, Sarah Baker, Victor A Beck, Alfred M Spormann, Marc Fontecave, Christopher Hahn, Thomas F Jaramillo. Advanced Materials, 2022. A perspective on the electrocatalytic conversion of carbon dioxide to methanol with metallomacrocyclic catalysts Xinyan Liu, Bo-Quan Li, Bing Ni, Lei Wang, Peng Hong-jie. Journal of Energy Chemistry, 2022. Effects of the Catalyst Dynamic Changes and Influence of the Reaction Environment on the Performance of Electrochemical CO2 Reduction Chen Jiayi, Lei Wang. Advanced materials, 2021. Guiding the Catalytic Properties of Copper for Electrochemical CO2 Reduction by Metal Atom Decoration Christopher Hahn Yusaku F. Nishimura, Hong-Jie Peng, Stephanie Nitopi, Michal Bajdich, Lei Wang, Carlos G. Morales-Guio, Frank Abild-Pedersen, Thomas F. Jaramillo. ACS Applied Materials & Interfaces, 2021. Electrolyte-Guided Design of Electroreductive CO Coupling on Copper Surfaces Sneha A Akhade, Buddhinie S Jayathilake, Stephen E Weitzner, Hannah V Eshelman, Julie Hamilton, Jeremy T Feaster, David W Wakerley, Lei Wang, Sarah Lamaison, Dong Un Lee, Christopher Hahn, Thomas F Jaramillo, Eric B Duoss, Sarah E Baker, Joel B Varley. ACS Applied Energy Materials 2021, 4(8), 8201-8210. Bimetallic effects on Zn-Cu electrocatalysts enhance activity and selectivity for the conversion of CO2 to CO Wang, L.; Peng, H.; Lamaison, S.; Qi, Z.; Koshy, M. D.; Stevens, M. B.; Wakerley, D.; Zamora Zeledo´, J.A.; King, L. A.; Zhou, L.; Lai, Y.; Fontecave, M.; Gregoire, J.; Abild-Pedersen, F.; Jaramillo, T. F.; Hahn, C. Chem Catalysis 2021, July 15, 1, 1-18. A perspective on the electrocatalytic conversion of carbon dioxide to methanol with metallomacrocyclic catalysts Liu, X.; Li, B.; Ni, B.; Wang, L.; Peng, H.* Journal of Energy Chemistry 2022, 64, 263-275. Electrolyte-Guided Design of Electroreductive CO Coupling on Copper Surfaces Akhade, S. A.; Jayathilake, B.S.; Weitzner, S. S.; Eshelman, H. V.; Hamilton, J.; Feaster, J. T.; Wakerley, D. W.; Wang, L.; Lamaison, S.; Lee. D. U.; Hahn, C.; Jaramillo, T. F.; Duoss, E. B.; Baker, S. E.; Varley, J. B.* ACS Appl. Energy Mater 2021, 10.1021/acsaem.1c01427. From Ru-bda to Ru-bds: a step forward to highly efficient molecular water oxidation electrocatalysts under acidic and neutral conditions Yang, J.;# Wang, L.;# Zhan, S.; Zou, H.; Chen, H.; Ahlquist, M. S. G.; Duan, L.;* Sun, L.* Nature Communications 2021, 12, Article number: 373 . Readily Constructed Glass Piston Pump for Gas Recirculation Nielander, A. C.; Blair, S. J.; McEnaney, J. M.; Schwalbe, J. A.; Adams, T.; Sawson Taheri, S.; Wang, L.; Sungeun Yang, S.; Cargnello, M.; Jaramillo, T. F.* ACS Omega 2020, 5, 27, 16455-16459. Selective reduction of CO to acetaldehyde with CuAg electrocatalysts Wang, L.; Higgins, D. C.; Ji, Y.; Morales-Guio, C. G.; Chan, K.; Hahn, C.*; Jaramillo, T. F.* PNAS 2020.