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个人简介

1993年 北海道大学 大学院理学研究科化学専攻 博士後期課程修了(指導教官:喜多英明教授) Ph.D. Hokkaido University (Prof. Hideaki KITA) 1993年 北海道大学 大学院理学研究科化学専攻・教務職員(物理化学講座 魚崎浩平教授) Assitant Professor, Department of Chemistry, Hokkaido University (Prof. Kohei UOSAKI) 1994年 同・助手 Assitant Professor, Department of Chemistry, Hokkaido University (Prof. Kohei UOSAKI) 1997年 カリフォルニア大学バークレー校物理学科・研究員(Y. R. Shen教授) Visiting Researcher, Department of Physics, University of California at Berkeley (Prof. Y. R. SHEN) 2000年 北海道大学 触媒化学研究センター・准教授(界面分子科学研究分野 大澤雅俊教授) Associate Professor, Catalysis Research Center, Hokkaido University (Prof. Masatoshi OSAWA) 2017年 東北大学 大学院理学研究科化学専攻・教授(物理化学講座・有機物理化学研究室) Professor, Department of Chemistry, Tohoku University 兼任・プロジェクト 1999~2002 JSTさきがけ研究「変換と制御」領域・研究員 (総括:合志陽一 教授) 2005~2009 JSTさきがけ研究「界面の構造と制御」領域・研究員 (総括:川合真紀 教授) 2009~ 中国科学技術大学(USTC)化学物理系・客員教授

研究领域

Many chemical reactions, including catalytic reactions, occur on the surface or interface of a substance. Therefore, microscopic structural evaluation and control at the surface and interface of substances are extremely important for the essential understanding of chemical reactions and the creation of new functional substances. Based on classical electrochemical, our laboratory makes full use of cutting-edge measurement technologies such as sum frequency generation (SFG) nonlinear vibration spectroscopy, single molecule spectroscopy, microspectroscopy, and scanning probe microscopes to create material surfaces. We aim to create new materials by surface structure design by grasping the dynamic behavior of chemical reactions occurring at the interface with high sensitivity and investigating the relationship between the surface / interface structure and the reaction activity.

近期论文

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Peng, Q.; Liu, H.; Ye, S. Adsorption of Organic Carbonate Solvents on a Carbon Surface Probed by Sum Frequency Generation (SFG) Vibrational Spectroscopy. J. Electroanal. Chem., 2017, 800, 134-143. Wei, J.; Zheng, Y.; Li, X.; Xu, M.; Chen, Y.X.; Ye, S. Electrochemistry of Oxygen at Ir Single Crystalline Electrodes in Acid. Electrochimica Acta, 2017, 246, 329-337. Saito, K.; Peng, Q.; Qiao, L.; Wang, L.; Joutsuka, T.; Ishiyama, T.; Ye, S.; Morita, A. Theoretical and Experimental Examination on SFG Polarization Analysis at Acetonitrile-Water Solution Surfaces. Phys. Chem. Chem. Phys., 2017, 19, 8941-8961. Sakamoto, N.; Onodera, T.; Dezawa, T.; Shibata, Y.; Oikawa, H.; Highly enhanced emission of visible light from core-dual shell type hybridized nanoparticles. Particle & Particle Systems Characterization, accepted (2017). Tahara, K.; Mohamed, A.; Kawahara, K.; Nagao, R.; Kato, Y.; Fukumura, H.; Shibata, Y.; Noguchi, T.; Fluorescence property of photosystem II protein complexes bound to a gold nanoparticle. Faraday Discussion, 2017, 198, 121-134. Koshima. H.; Iyotani, Y.; Peng, Q.; Ye, S. Study of Friction-Reduction Properties of Fatty Acids and Adsorption Structures of their Langmuir-Blodgett Monolayers using Sum-Frequency Generation Spectroscopy and Atomic Force Microscopy. Tribology Letter, 2016, 64, 34 Liu, C.; Ye, S. In situ Atomic Force Microscopy (AFM) Study of Oxygen Reduction Reaction on a Gold Electrode Surface in a Dimethyl Sulfoxide (DMSO) Based Electrolyte Solution. J. Phys. Chem. C, 2016, 120, 25246–25255 Wuttig, A.; Liu, C.; Peng, Q.; Yaguchi, M.; Hendon, C.; Motobayashi, K.; Ye, S.; Osawa, M.; Surendranath, Y. Tracking a Common Surface-Bound Intermediate during CO2-to-Fuels Catalysis. ACS Central Science, 2016, 2, 522-528. Wang, L.; Peng, Q.; Ye, S.; Morita, A. Surface Structure of Organic Carbonate Liquids Investigated by Molecular Dynamics Simulation and Sum Frequency Generation Spectroscopy. J. Phys. Chem. C, 2016, 120, 15185-15197. Ge, A.; Matsusaki, M.; Qiao, L.; Akashi, M.; Ye, S. Salt Effects on Surface Structures of Polyelectrolyte Multilayers (PEMs) Investigated by Vibrational Sum Frequency Generation (SFG) Spectroscopy. Langmuir, 2016, 32, 3803-3810 Qiao, Y.; Ye, S. Spectroscopic Investigation for Oxygen Reduction and Evolution Reactions on Carbon Electrodes in Li−O2 Battery J. Phys. Chem. C, 2016, 120, 8033-8047 Qiao, Y.; Ye, S. Spectroscopic Investigation for Oxygen Reduction and Evolution Reactions with TTF as a Redox Mediator in Li-O2 Battery. J. Phys. Chem. C, 2016, 120, 15830-15845 Wu, H.; Tong, Y.; Li, N.; Peng, Q.; Ye, S. Phase Transition Behaviors of the Supported DPPC Bilayer Investigated by Sum Frequency Generation (SFG) and Atomic Force Microscopy (AFM). (Selected as an Inside Front Cover) Phys. Chem. Chem. Phys., 2016, 18, 1411-1421. Mohamed, A.; Nagao, R.; Noguchi, T.; Fukumura, H.; Shibata, Y. Structure-based modelling of fluorescence kinetics of photosystem II: relation between its dimeric form and photoregulation. J. Phys. Chem B, 2016, 120, 365-376 Qiao, L.; Ge, A.; Liang, Y.; Ye, S. Oxidative Degradation of the Monolayer of 1-Palmitoyl-2-Oleoyl-sn-Glycero-3-Phosphocholine (POPC) in Low-level Ozone. J. Phys. Chem. B, 2015, 119, 14188-14199. Ge, A.; Seo, J.; Qiao, L; Yui, N.; Ye, S. Structural Reorganization and Fibrinogen Adsorption Behaviors on the Polyrotaxane Surfaces Investigated by Sum Frequency Generation (SFG) Spectroscopy. ACS Applied Materials & Interfaces, 2015, 7, 22709-22718. Ge, A.; Peng, Q.; Qiao, L.; Yepuri, N.; Darwish, T.; Matsusaki, M.; Akashi, M.; Ye, S. Molecular Orientation of Organic Thin Films on Dielectric Solid Substrates: A Phase-sensitive Vibrational SFG Study. Phys. Chem. Chem. Phys., 2015, 17, 18072-18078. Tong, Y.; Peng, Q.; Ma, T.; Nishida, T.; Ye, S. Photocatalytic Oxidation of the Organic Monolayers on TiO2 Surface Investigated by in-situ Sum Frequency Generation (SFG) Spectroscopy. APL Materials, 2015, 3, 104402. Zhang, H.; Sasaki, Y.; Abe, M.; Zhang, Y.; Ye, S.; Osawa, M. Preparation, Spectroscopy, and Electrochemistry of Cyano-bridged Bis(oxo-centered-hexa (μ-acetato)-triruthenium) Complexes" J. Organomet. Chem., 2015, 797, 29-36. Qiao, Y.; Ye, S. In-situ Study of Oxygen Reduction in DMSO Solution: A Fundamental Study for Development of Lithium-oxygen Battery. J. Phys. Chem. C, 2015, 119, 12236–12250.

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