吴凯 - 北京大学 - 化学与分子工程学院

个人简介

1983－1987, Zhejiang University, B. S. in Chemistry 1987－1991, Dalian Institute of Chemical Physics, CAS, Ph. D in Physical Chemistry 1992－1995, State Key Laboratory of Catalysis, DICP, Assistant/Associate Researcher 1995－1998, Fritz-Haber-Institut der MPG, Germany, Visiting Scientist 1998－2000, Pacific Northwest National Laboratory, DOE, USA，Postdoctoral Associate 2000－Present, Professor, College of Chemistry and Molecular Engineering, Peking university 2011－2015, Dean, College of Chemistry and Molecular Engineering, Peking university 2016－2022, Vice Dean, Faculty of Science, Peking University

研究领域

Molecular Self-assembly and Surface Reactions Model Catalysis Ion Chemistry at Surfaces

近期论文

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Regioselective hydroformylation of propene catalyzed by 1 rhodium-zeolite, X.J. Zhang, T. Yan, H.M. Hou, J.Q. Yin, H.L. Wan, X.D. Sun, Q. Zhang, F.F. Sun, Y. Wei, M. Dong, W.B. Fan, J.G. Wang, Y.J. Sun, X. Zhou, K. Wu, Y. Yang, Y.W. Li, Z. Cao, Nature, 2024, 629, 597–602. Tuning Surface Organic Structures by Small Gas Molecules through Catassembly and Coassembly, J. Li, X.Y. Wang, Y. He, Z. Xu, X. Li, H.Y. Pan, Y.D. Wang, Y.Y. Dong, Q. Shen, Y.J. Zhang, S.M. Hou, K. Wu, Y.F. Wang, Journal of Physical Chemistry Letters, 2024, 15, 5564–5579. Selective Cleavage of α-Olefins to Produce Acetylene and Hydrogen, M.J. Xu, Z.-Y. Hu, X.Y. Liang, Y.F. Zhu, H.H. Ding, J. Hu, J.F. Xu, Z. Zhu, Z.-A. Wu, X.W. Zhao, W.J. Guo, K.Q. Nie, Y.F. Ye, J.F. Zhu, Z.-P. Liu, X. Zhou, K. Wu, Journal of American Chemical Society, 2024, 146, 12850–12856. Steering Electron-Induced Surface Reaction via a Molecular Assembly Approach, Y.X. Lin, J. Li, X.Y. Liang, T. Hu, Z.C. Huang, Z. Zhu, M.X. Diao, X.W. Zhao, Z.T. Peng, Y.F. Wang, Q.W. Chen, J. Liu, K. Wu, Journal of American Chemical Society, 2024, 146, 10150–10158. Surface-Confined Alternating Copolymerization with Molecular Precision by Stoichiometric Control, L.B. Xing, J. Li, Y.C. Bai, Y.X. Lin, L.H. Xiao, C.L. Li, D.H. Zhao, Y.F. Wang, Q.W. Chen, J. Liu, K. Wu, Nature Communications, 2024, 15, 666 (1-9). Unzipping Carbon Nanotubes to Sub-5-nm Graphene Nanoribbons on Cu(111) by Surface Catalysis, W.J. Dong, X. Li, S. Lu, J. Li, Y.S. Wang, M.J. Zhong, X. Dong, Z. Xu, Q. Shen, S. Gao, K. Wu, L.-M. Peng, S.M. Hou, Z.Y. Zhang, Y.J. Zhang, Y.F. Wang, Small, 2023, 2308430. Clustering-Evolved Frontier Orbital for Low-Temperature CO2 Dissociation, J.L. Pan, X.E. Li, Y.F. Zhu, J.Y. Zhou, Z. Zhu, C.L. Li, X.Z. Liu, X.Y. Liang, Z.X. Yang, Q.W. Chen, P.J. Ren, X.D. Wen, X. Zhou, K. Wu, Journal of the American Chemical Society, 2023, 145, 18748–18752. Diazulenorubicene as a Non-benzenoid Isomer of peri-Tetracene with Two Sets of 5/7/5 Membered Rings Showing Good Semiconducting Property, L.Y. Qin, Y.-Y. Huang, B.T. Wu, J.L. Pan, J.F. Yang, J. Zhang, G.C. Han, S.Y. Yang, L.L. Chen, Z. Yin, Y.L. Shu, L. Jiang, Y.P. Yi, Q. Peng, X. Zhou, C. Li, G.X. Zhang, X.-S. Zhang, K. Wu, D.Q. Zhang, Angewandte Chemie International Edition, 2023, doi: 10.1002/anie.202304632. Active Phase on Oxidized Pd(100) for Low-Temperature Propane Oxidation, M.J. Xu, Y.C. Zhang, Y.F. Zhu, C.L. Li, Z.-A. Wu, X. Zhou, K. Wu, Acta Physico-Chimica Sinica, doi: 10.3866/PKU.WHXB202305033. Assembling Surface Molecular Sierpiński Triangle Fractals via K+-Invoked Electrostatic Interaction, J.X. Dai, X.W. Zhao, Z.T. Peng, J. Li, Y.X. Lin, X.J. Wen, L.B. Xing, W.H. Zhao, J. Shang, Y.F. Wang, J. Liu, K. Wu, Physical Chemistry Chemical Physics, 2023, 145, 13531. Significantly enhanced photothermal catalytic CO2 reduction over TiO2/g-C3N4 composite with full spectrum solar light, X.Y. Bao, D.W. Lu, Z.N. Wang, H. Yin, B. Zhu, B. Chen, M.X. Shi, Y. Zhang, Q.X. Xu, Y.M. Qin, X.-C. Shen, K. Wu, Journal of Colloid and Interface Science, 2023, 638, 63. Molecular Insight into On-Surface Chemistry of an Organometallic Polymer, Y.X. Lin, M.X. Diao, J.X. Dai, Z. Xu, X.W. Zhao, X.J. Wen, L.B. Xing, X. Zhou, Q.W. Chen, J. Liu, K. Wu, Physical Chemistry Chemical Physics, 2023, 25，1006. Supramolecular Anisotropy in a Surface-Confined Bi-Component System, X.J. Wen, J. Li, Y.X. Lin, M.X. Diao, W.H. Zhao, B. Di, Z.T. Peng, D. Liu, X. Zhou, Q.W. Chen, Y.F. Wang, J. Liu, K. Wu, Journal of Physical Chemistry C, 2022, 126，20739. Flux-assisted growth of atomically thin materials, P. Zhang, X.G. Wang, H.N. Jiang, Y.W. Zhang, Q.Q. He, K.P. Si, B.X. Li, F.F. Zhao, A.Y. Cui, Y. Wei, L.X. Liu, H.F. Que, P.Z. Tang, Z.G. Hu, W. Zhou, K. Wu, Y.G. Gong, Nature Synthesis, 2022, 1, 864. Using Self-Assembly to Control On-Surface Reactions, Z.T. Peng, L.B. Xing, K. Wu, in Supramolecular Chemistry on Surfaces: 2D Networks and 2D Structures (Ed.: Neil Champness), 2022, pp. 103-134, Wiley-VCH. Self-assemblies and Properties of Side-on Picene Strips on Monolayered CuO Film, Z.T. Peng, B. Di, X.W. Zhao, Y.X. Lin, M.X. Diao, Z. Xu, W.J. Guo, X. Zhou, Q.W. Chen, Y.F. Wang, K. Wu, Journal of Physical Chemistry C, 2022, 126, 7753. Bidirectional modulation interaction between monatomic Pt and Tin+ sites on Ti4O7 for high-efficiency and durable oxygen reduction, Y.J. Luo, Y.W. Wang, X.T. Qin, Y.Y. Wang, K. Wu, H.J. Zhang, L. Zhang, H.M. Huang, W. Tian, Y. Wang, Journal of Catalysis, 2022, 411, 149. Observation of biradical spin coupling through hydrogen bonds, Y. He, N. Li, I.E. Castelli, R.N. Li, Y.J. Zhang, X. Zhang, C. Li, B.W. Wang, S. Gao, L.M. Peng, S.M. Hou, Z.Y. Shen, J.-T. Lü, K. Wu, P. Per P. Hedegård, Y.F. Wang, Physical Review Letters, 2022, 128, 236401. Single-Cation Catalyst: Ni Cation in Monolayered CuO for CO Oxidation, J.Y. Zhou, J.L. Pan, Y. Jin, Z.T. Peng, Z. Xu, Q.W. Chen, P.J. Ren, X. Zhou, K. Wu, Journal of American Chemical Society, 2022, 144, 8430. Visualization of on-surface ethylene polymerization through ethylene insertion, W.J. Guo, J.Q. Yin, Z. Xu, W.T. Li, Z.T. Peng, C. J. Weststrate, X. Yu, Y.R. He, Z. Cao, X.D. Wen, Y. Yang, K. Wu, Y.W. Li, J. W. Niemantsverdriet, X. Zhou, Science, 2022, 375, 1188. Spatially Resolved and Quantitatively Revealed Charge Transfer between Single Atoms and Catalyst Supports, B. Di, Z.T Peng, Z.Y. Wu, X. Zhou, K. Wu, Journal of Materials Chemistry A, 2022, 10, 5889. Carbon monoxide adsorption on cobalt overlayers on a Si(111) surface studied by STM and XPS, Y. He, C.J. Weststrate, Dan Luo, J.W. Niemantsverdriet, K. Wu, J. Xu, Y. Yang, Y.W. Li, X. D. Wen, Applied Surface Science, 2021, 569, 151045. Atomic and Electronic Edge Structures of Monolayer Ceria on Pt(111), Z.C. Huang, C. Han, Y.-Y. Sun, K. Wu, W. Chen, Journal of Physical Chemistry C, 2021, 125, 15599. Lattice-Directed Stabilization of Different Spin-State Phases in Metallo-Supramolecular Chains on Au Surfaces, J. Liu, J. Li, Q.W. Chen, Q. Xue, Y.F. Wang, B. Di, Y.F. Wang, K. Wu, Chemistry of Materials, 2021, 33, 6166. Atomic-Scale Local Work Function Characterizations of Br Islands on Cu(111), Z.C. Huang, Y.X. Lin, C. Han, Y.-Y. Sun, K. Wu, W. Chen, Journal of Physical Chemistry C, 2021, 125, 7944 Atomically Resolved Structure of Monolayered Ceria Island on Pt(111), H.R. Chen, Z.C Huang, W.H. Rong, J.Y. Zhou, Z. Xu, W.T. Li, Y.X. Lin, X. Zhou, K. Wu, Journal of Physical Chemistry C, 2020, 124, 28531 Steering Effect of Bromine on Intermolecular Dehydrogenation Coupling of Poly(P-Phenylene) on Cu(111), Y.X. Lin, Z.C. Huang, X.J. Wen, W.H. Rong, Z.T. Peng, M.X. Diao, L.B. Xing, J.X. Dai, X. Zhou, K. Wu, ACS Nano, 2020, 14, 17134. Surface-Mediated Ordering of Pristine Salen Molecules on Coinage Metals, D. Liu, B. Di , Z.T. Peng, C. Yin, H. Zhu, X.J. Wen, Q.W. Chen, J.F. Zhu, K. Wu, Inorganic Chemistry Frontiers, 2021, 8, 417. Packing Sierpiński Triangles into Two-Dimensional Crystals, Y.J Zhang, X. Zhang, Y.R. Li, S.T. Zhao, S.M. Hou, K. Wu, Y.F. Wang, Journal of American Chemical Society, 2020, 142, 17928. Selective Intramolecular Dehydrocyclization of Co-Porphyrin on Au(111), C. Yin, Z.T. Peng, D. Liu, H.J. Song, H. Zhu, Q.W. Chen, K. Wu, Molecules, 2020, 5, 3766. A perspective of oxide-supported single-atom catalysts, J.Y. Zhou, Z. Xu, M.J. Xu, X. Zhou, K. Wu, Nanoscale Advances, 2020, 2, 3624. Adsorption and Self-assembly of meso-tetra(p-methoxyphenyl)-porphyrinatocobalt(II) on Coinage Metal Surfaces, C. Yin, Z.K. Wang, D. Liu, Z.T. Peng, H,J, Song, H. Zhu, Q.W. Chen, K. Wu,, Acta Chim. Sinica, 2020, 78, 695. Reversibly Switching the Charge State and Adsorption Location of Single Potassium Atom on Ultrathin CuO Film, Z.T. Peng, B. Di, W.T. Li, D. Liu, X.J. Wen, H. Zhu, H.J. Song, Y.J. Zhang, C. Yin, X. Zhou, K. Wu, Angewandte Chemie International Edition, 2020, 58, 14321. One-step Fabrication of TiO2/Ti Foil Annular Photoreactor for Photocatalytic Degradation of Formaldehyde, Y.M. Qin, Z.N. Wang, J.T.Jiang, L.B. Xing, K. Wu, Chemical Engineering Journal, 2020, 394, 124917. Strain-induced Oxygen Vacancies in Monolayered CeO2(111) Islands Grown on Pt(111), W.H. Rong, H.R. Chen, Z.C. Huang, K. Wu, Journal of Physical Chemistry C, 2020, 124, 6284. Long-Range Ordered Structure of Corannulene Governed by Electrostactic Repulsion and Surface-State Mediation, X.J. Wen, Y.X. Lin, Z.C. Huang, M.X. Diao, W.H. Zhao, J.X. Dai, L.B. Xing, H. Zhu, Z.T. Peng, D. Liu, K. Wu, Journal of Physical Chemistry Letters, 2019, 10, 6800-6806. Atomic structure and local work electronic properties of K- and Rh-modified ceria/Pt(111) inverse model catalysts, H.R. Chen, W.H. Rong, Z.C. Huang, Z.T. Peng, Z. Xu, J.Y. Zhou, B. Di, X. Zhou, K. Wu, Journal of Chemical Physics, 2019, 151, 184703. Conformational Switching of Verdazyl Radicals on Au(111), Z.C. Huang, Y.Z. Dai, X.J. Wen, D. Liu, Y.X. Lin, Z. Xu, J. Pei, K. Wu, Acta Physico-Chimica, 2020, 36, 1907043(1-6). Local Work Function Measurements of Thin Oxide Films on Metal Substrates, Z.C. Huang, Z. Xu, J.Y. Zhou, H.R. Chen, W.H. Rong, Y.X. Lin, X.J. Wen, H. Zhu, K. Wu, Journal of Physical Chemistry C, 2019, 123, 17823. Chiral features of metal phthalocyanines sitting atop pre-assembled TiOPc monolayer on Ag(111), H. Zhu, H.J. Song, W.H. Zhao, Z.T. Peng, D. Liu, L.B. Xing, J.X. Dai, Z.C. Huang, P.L. Liao, Y. Wang, K. Wu, Physical Chemistry Chemical Physics, 2019, 21, 16323. . On-Surface Synthesis of Highly Ordered Covalent Sierpiński Triangle Fractals, Y.P. Mo, T. Chen, J.X. Dai, K. Wu, D. Wang, Journal of American Chemical Society, 2019, 141, 11378. Precursor Structures for Polymorphic Titanyl Phthalocyanine Crystal Phases on Au(111): A High-Resolution STM Study, H. Zhu, H.J. Song, W.H. Zhao, Z.T. Peng, D. Liu, B. Di, L.B. Xing, H.R. Chen, Z.C. Huang, Y. Wang, K. Wu, Journal of Physical Chemistry C, 2019, 123, 17390. Dechlorinated Ullmann Coupling Reaction of Aryl Chlorides on Ag(111): A Combined STM and XPS Study, J.X. Dai, W.H. Zhao, L.B. Xing, J. Shang, H.X. Ju, X. Zhou, J. Liu, Q.W. Chen, Y.F. Wang, J.F. Zhu, K. Wu, ChemPhysChem, 2019, 20, 2367 Two-sidedness of Surface Reaction Mediation, H.R. Chen, H. Zhu, Z.C. Huang, W.H. Rong, K. Wu, Advanced Materials, 2019, 1902080(1-16). Stepwise On-Surface Dissymmetric Reaction to Construct Binodal Organometallic Network, J. Liu, Q.W. Chen, K. Cai, J. Li, Y.R. Li, X. Yang, Y.J. Zhang, Y.F. Wang, H. Tang, D.H. Zhao, K. Wu, Nature Communications, 2019, 10, 2545. Steering the Achiral into Chiral with a Self-Assembly Strategy, H.J. Song, H. Zhu, Z.C. Huang, Y.J. Zhang, W.H. Zhao, J. Liu, Q.W. Chen, C. Yin, L.B. Xing, Z.T. Peng, P.L. Liao, Y.F. Wang, Y. Wang, K. Wu, ACS Nano, 2019, 13, 7202. On Controllability and Applicability of Surface Molecular Self-Assemblies, L.B. Xing, Z.T. Peng, W.T. Li, K. Wu, Accounts of Chemical Research, 2019, 52, 1048. Steering Two-Dimensional Porous Networks with σ-Hole Interactions of Br—S and Br—Br, L.B. Xing, W. Jiang, Z.C. Huang, J. Liu, H.J. Song, W.H. Zhao, J.X. Dai, H. Zhu, Z.H. Wang, P.S. Weiss, K. Wu, Chemistry of Materials, 2019, 31, 3041. Photocatalytic Degradation Kinetics of Gaseous Formaldehyde Flow Using TiO2 Nanowires, H.L. Dou, D. Long, X. Rao, Y.P. Zhang, Y.M. Qin, F. Pan, K. Wu, ACS Sustainable Chemistry & Engineering, 2019, 7, 4456. Probe the Catalytic Intermediates of CO2 Hydrogenation on Cu(111) by In-Operando Near-Ambient Pressure Technique, Y.J. Ren, K.D. Yuan, X. Zhou, H.C. Sun, K. Wu, S. L. Bernasek, W. Chen, G.Q. Xu, Chemistry – A European Journal, 2018, 34, 16097. Comparison Study of Structural Properties and CO Adsorption on the Cu/Au(111) and Au/Cu(111) Thin Films, W.Y. Wang, H.X. Shi, L. Wang, Z. Li, H. Shi, K. Wu, X. Shao, Journal of Physical Chemistry C, 2018, 122, 19551. Tuning the spin-related transport properties of FePc on Au(111) through single-molecule chemistry, 2. R.N. Li, N. Li, H. Wang, A. Weismann, Y.J. Zhang, S.M. Hou, K. Wu, Y.F. Wang, Chemical Communications, 2018, 54, 9135. Iron Carbidization on Thin-Film Silica and Silicon: A Near-Ambient-Pressure X-ray Photoelectron Spectroscopy and Scanning Tunneling Microscopy Study, X. Zhou, G. J. A. Mannie, J.Q. Yin, X. Yu, C. J. Weststrate, X.D. Wen, K. Wu, Y. Yang, Y.W. Li, and J. W. Niemantsverdriet, ACS Catalysis, 2018, 8, 7326. Adsorption and Assembly of Photoelectronic TiOPc Molecules on Coinage Metal Surfaces, W.H. Zhao, H. Zhu, H.J. Song, J. Liu, Q.W. Chen, Y. Wang, K. Wu, Journal of Physical Chemistry C, 2018, 122, 7695. Bromine Adatom Promoted C-H Bond Activation in Terminal Alkynes at Room Temperature on Ag(111), J. Liu, Q.W. Chen, Q.L. He, Y.J. Zhang, X.Y. Fu, Y.F. Wang, D.H. Zhao, W. Chen, G.Q. Xu, K. Wu, Physical Chemistry Chemical Physics, 2018, 20, 11081. Detection and Manipulation of Charge States for Double-Decker DyPc2 Molecules on Ultrathin CuO Films, Y.J. Zhang, Y.F. Wang, P.L. Liao, K. Wang, Z.C. Huang, J. Liu, Q.W. Chen, J.Z. Jiang, K. Wu, ACS Nano, 2018, 12, 2991. Unraveling Charge State of Supported Au Single-atoms during CO Oxidation, X. Zhou, Q. Shen, K.D. Yuan, W.S. Yang, Q.W. Chen, Z.H. Geng, J.L. Zhang, X. Shao, W. Chen, G.Q. Xu, X.M. Yang, K. Wu, Journal of American Chemical Society, 2018, 140, 554.