Oteyza, Dimas G. de - Universidad del Pais Vasco - Donostia International Physics Center

个人简介

Dimas performed his PhD studies at the Max-Planck Institute for Metals Research (Germany) and obtained the degree from the Universidad Autónoma de Madrid in 2007. Thereafter he has worked at the National Institute for Materials Science (Japan), Donostia International Physics Center (DIPC, Spain), Molecular Foundry of the Lawrence Berkeley National Lab (USA), University of California at Berkeley (USA) and Centro de Fisica de Materiales (Spain). He is currently an Ikerbasque Research Professor at DIPC.

研究领域

Our scientific efforts are focused mainly on physico-chemical phenomena ocurring in organic materials, including thin-film growth, self-assembly, interface electronics and, lately most of all, chemical reactions. In particular the surface-supported synthesis of functional materials from molecular precursors under ultra-high-vacuum is the true origin of this laboratory and its most pursued research line. However, we also maintain our interest in non-covalently bonded structures, their assembly and properties, as for example with molecular blends. In general, a multi-technique surface science approach is applied. The heart of the lab is a low-temperature scanning probe microscope (LT-SPM), determining our particular emphasis on scanning probe microscopy and spectroscopy. In addition, electron spectroscopies are also applied at synchrotron light sources.

近期论文

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T. Wang, A. Berdonces-Layunta, N. Friedrich, M. Vilas-Varela, J. P. Calupitan, J. I. Pascual, D. Casanova, D. Peña, M. Corso, D. G. de Oteyza, Aza-triangulene: On-Surface Synthesis, Electronic and Magnetic Properties, Journal of the American Chemical Society, 2022, 144, 4522−4529 Z. Zeng, D. Guo , T. Wang, Q. Chen, A. Matej, J. Huang, D. Han, Q. Xu, A. Zhao, P. Jelinek, D. G. de Oteyza, J.-S. McEwen, J. Zhu, Chemisorption Induced Formation of Biphenylene Dimer on Surfaces, Journal of the American Chemical Society, 2022, 144, 723–732 T. Wang, S. Sanz, J. Castro-Esteban, J. Lawrence, A. Berdonces-Layunta, M. S. G. Mohammed, M. Vilas-Varela, M. Corso, D. Peña, T. Frederiksen, D. G. de Oteyza, Magnetic interactions between radical pairs in chiral graphene nanoribbons, Nano Letters 2022, 22, 164−171 M. Corso, R. E. Menchón, I. Piquero-Zulaica, M. Vilas-Varela, J. E. Ortega, D. Peña, A. Garcia-Lekue, D. G. de Oteyza, Band structure and energy level alignment of chiral graphene nanoribbons on silver surfaces, Nanomaterials 2021, 11, 3303 A. Berdonces-Layunta, F. Schultz, F. Aguilar, J. Lawrence, J. Lobo-Checa, M. S. G. Mohammed, P. Liljeroth, D. G. de Oteyza, Order from a mess: the growth of 5-armchair graphene nanoribbons, ACS Nano 2021, 15, 16552–16561 J. Li, S. Sanz, N. Merino-Díez, M. Vilas-Varela, A. Garcia-Lekue, M. Corso, D. G. de Oteyza, T. Frederiksen, D. Peña, J. I. Pascual, Topological phase transition in chiral graphene nanoribbons: from edge bands to end states, Nature Communications 2021, 12, 5538 K. Ali, L. Fernández, A. A. Makarova, I. Pis, F. Bondini, J. Lawrence, D. G. de Oteyza, F. J. G. de Abajo, Z. Abd el-Fattah, J. E. Ortega, F. Schiller, Atomically-precise texturing of hexagonal boron nitride nanostripes, Advanced Science 2021, 8, 2101455 T. Wang, J. Lawrence, R. Robles, M. S. G. Mohammed, A. Berdonces-Layunta, D. Peña, N. Lorente, M. Corso, D. G. de Oteyza, Challenges in the surface-supported synthesis of corannulene-based non-planar nanographenes, Physical Chemistry Chemical Physics 2021, 23, 10845 -10851 M. S. G. Mohammed, J. Lawrence, F. García, P. Brandimarte, A. Berdonces-Layunta, D. Pérez, D. Sánchez-Portal, D. Peña, D. G. de Oteyza, From starphenes to non-benzenoid linear conjugated polymers by substrate templating, Nanoscale Advances 2021, 3, 2351–2358 A. Berdonces-Layunta, J. Lawrence, S. Edalatmanesh, J. Castro-Esteban, T. Wang, M. S. G. Mohammed, L. Colazzo, D. Peña, P. Jelinek, D. G. de Oteyza, Chemical Stability of (3,1)-Chiral Graphene Nanoribbons, ACS Nano 2021, 15, 5610−5617 J. Lawrence, M. S. G. Mohammed, D. Rey, F. Aguilar-Galindo, A. Berdonces-Layunta, D. Peña, D. G. de Oteyza, Reassessing Alkyne Coupling Reactions While Studying the Electronic Properties of Pyrene Linkages at Surfaces, ACS Nano 2021, 15, 4937− 4946 M. Abadia, J. Brede, A. Verdini, L. Floreano, P. Nita, D. G. de Oteyza, J. E. Ortega, M. Corso, C. Rogero, Why a Good Catalyst Can Turn Out Detrimental to Good Polymerization, The Journal of Physical Chemistry C 2021, 125, 5066-5075 J. Holec, B. Cogliati, J. Lawrence, A. Berdonces-Layunta, P. Herrero, Y. Nagata, M. Banasiewicz, B. Kozankiewicz, M. Corso, D. G. de Oteyza, A. Jancarik, A. Gourdon, A large starphene comprising pentacene branches, Angewandte Chemie International Edition 2021, 60, 7752–7758 A. S. Sinitsa, I. V. Lebedeva, Y. G. Polynskaya, D. G. de Oteyza, S. V. Ratkevich, A. A. Knizhnik, A. M. Popov, N. A. Poklonski, Y. E. Lozovik, Transformation of a graphene nanoribbon into a 1D nanoobject with alternating double chains and polycyclic regions, Physical Chemistry Chemical Physics 2021, 23, 425-441 M. S. G. Mohammed, L. Colazzo, R. Robles, R. Dorel, A. M. Echavarren, N. Lorente, D. G. de Oteyza, Electronic decoupling of polyacenes from the underlying metal substrate by sp3 carbon atoms, Communications Physics 2020, 3, 159-1-8 T. Wang, Y. Pan, W. Zhang, J. Lawrence, M. S. G. Mohammed, J. Huang, L. Feng, A. Berdonces-Layunta, D. Han, Q. Xu, X. Wu, S. L. Tait, D. G. de Oteyza, J. Zhu, On-Surface Synthesis of Five-membered Carbon Ring from a Terminal Alkynyl Bromide: a [4+1] Annulation, The Journal of Physical Chemistry Letters 2020, 11, 5902-5907 A. El-Sayed, I. Piquero-Zulaica, Z. M. Abd El-Fattah, L. Kormos, K. Ali, A. Weber, J. Brede, D. G. de Oteyza, J. Lobo-Checa, J. E. Ortega, M. Corso, Synthesis of graphene nanoribbons on a kinked Au surface: revealing the frontier valence band at the Brillouin zone center, The Journal of Physical Chemistry C 2020, 124, 15474-15480 M. S. G. Mohammed, L. Colazzo, A. Gallardo, J. Pomposo, P. Jelinek, D. G. de Oteyza, Steering alkyne homocoupling with on-surface synthesized metal-organic complexes, Chemical Communications 2020, 56, 8659-8662 N. Merino-Díez, M. S. G. Mohammed, J. Castro-Esteban, L. Colazzo, A. Berdonces-Layunta, J. Lawrence, J. I. Pascual, D. G. de Oteyza, D. Peña, Transferring axial molecular chirality through a sequence of on-surface reactions, Chemical Science 2020, 11, 5441-5446 C. C. Leon, O. Gunnarsson, D. G. de Oteyza, A. Roslawska, P. Merino, A. Grewal, K. Kuhnke, K. Kern, Photon antibunching and Coulomb blockade from STM-induced quantum-dot-like states, ACS Nano 2020, 14, 4216-4223 J. Lawrence, P. Brandimarte, A. Berdonces-Layunta, M. S. G. Mohammed, A. Grewal, C. C. Leon, D. Sánchez-Portal, D. G. de Oteyza, Probing the magnetism of topological end-states in 5-armchair graphene nanoribbons, ACS Nano 2020, 14, 4499-4508 M. Corso, D. G. de Oteyza, Topological engineering of organic polymers, Nature Nanotechnology 2020, 15, 421-423 R. Costantini, L. Colazzo, L. Batini, M. Stredansky, M. S. G. Mohammed, S. Achilli, L. Floreano, G. Fratesi, D. G. de Oteyza, A. Cossaro, Keto-enol tautomerization drives self-assembly of Leucoquinizarin on Au(111), Chemical Communications 2020, 56, 2833-2836 J. Li, P. Brandimarte, M. Vilas-Varela, N. Merino-Díez, C. Moreno, A. Mugarza, J. Saez Mollejo, D. Sánchez-Portal, D. G. de Oteyza, M. Corso, A. Garcia-Lekue, D. Peña, J. I. Pascual, Band depopulation of graphene nanoribbons induced by chemical gating with amino groups, ACS Nano 2020, 14, 1895−1901 A. Gourdon, D. G. de Oteyza, J. Zhu, On-Surface Synthesis, ChemPhysChem 2019, 20, 2249-2250 L. Colazzo, M. S. G. Mohammed, A. Gallardo, Z. M. Abd El-Fattah, J. Pomposo, P. Jelinek, D. G. de Oteyza, Controlling the stereospecific bonding motif of Au-thiolate links, Nanoscale 2019, 11, 15567-15575 N. Merino-Díez, A. Perez-Paz, J. Li, J. Castro-Esteban, M. S. G. Mohammed, J. Lawrence, A. Berdonces-Layunta, A. Barragán, J. I. Pascual, J. Lobo-Checa, D. Peña, D. G. de Oteyza, Hierarchy in the halogen activation during surface-promoted Ullmann coupling, ChemPhysChem 2019, 20, 2305-2310 J. Li, N. Friedrich, N. Merino-Díez, D. G. de Oteyza, D. Peña, D. Jacob, J. I. Pascual, Spin excitation of a magnetic porphyrin by electrons through graphene nanoribbon electrodes, Nano Letters 2019, 19, 3288-3294 S. Clair, D. G. de Oteyza, Controlling a chemical coupling reaction on a surface: tools and strategies for on-surface synthesis, Chemical Reviews 2019, 119, 4717-4776 I. Palacio, L. Aballe, M. Foerster, D. G. de Oteyza, M. García-Hernández, J.A. Martín-Gago, Reversible graphene decoupling by NaCl photo-dissociation, 2D Materials 2019, 6, 025021-1-5 I. Piquero, A. García-Lekue, L. Colazzo, C. K. Krug, M. S. G. Mohammed, Z. M. Abd El-Fattah, M. Gottfried, D. G. de Oteyza, J. E. Ortega, J. Lobo-Checa, Electronic structure tunability by periodic meta-ligand spacing in one-dimensional organic semiconductors, ACS Nano 2018, 12, 10537–10544 L. Colazzo, M. S. G. Mohammed, R. Dorel, P. Nita, C. García Fernández, P. Abufager, N. Lorente, A. Echavarren, D. G. de Oteyza, On-Surface Synthesis of Heptacene on Ag(001) from Brominated and Non-Brominated Tetrahydroheptacene Precursors, Chemical Communications 2018, 54, 10260-10263 E. Carbonell-Sanromà, A. Garcia-Lekue, M. Corso, G. Vasseur, P. Brandimarte, J. Lobo-Checa, D. G. de Oteyza, J. Li, S. Kawai, S. Saito, S. Yamaguchi, J. E. Ortega, D. Sánchez-Portal, J. I. Pascual, Electronic properties of substitutionally boron-doped graphene nanoribbons on a Au(111) surface, The Journal of Physical Chemistry C 2018, 122, 16092-16099 N. Merino-Díez, J. Lobo-Checa, P. Nita, A. Garcia-Lekue, A. Basagni, G. Vasseur, F. Tiso, F. Sedona, P. K. Das, J. Fujii, I. Vobornik, M. Sambi, J. I. Pascual, J. E. Ortega, D. G. de Oteyza, Switching from reactant to substrate engineering in the selective synthesis of graphene nanoribbons, The Journal of Physical Chemistry Letters 2018, 9, 2510-2517 J. Li, N. Merino-Díez, E. Carbonell-Sanromà, M. Vilas-Varela, D. G. de Oteyza, D. Peña, M. Corso, J. I. Pascual, Survival of spin state in magnetic porphyrins contacted by graphene nanoribbons, Science Advances 2018, 4, eaaq0582-1-6 N. Merino-Díez, J. Li, A. García-Lekue, G. Vasseur, M. Vilas-Varela, E. Carbonell-Sanromà, M. Corso, J. E. Ortega, D. Peña, J. I. Pascual, D. G. de Oteyza, Unraveling the electronic structure of narrow atomically-precise chiral graphene nanoribbons, The Journal of Physical Chemistry Letters 2018, 9, 25–30 P. Borghetti, A. Sarasola, N. Merino-Díez, G. Vasseur, L. Floreano, J. Lobo-Checa, A. Arnau, D. G. de Oteyza, J. E. Ortega, Symmetry, shape, and energy variations in frontier molecular orbitals at organic/metal interfaces: the case of F4TCNQ, The Journal of Physical Chemistry C 2018, 121, 28412-28419 N. Merino-Díez, A. García-Lekue, E. Carbonell-Sanromà, J. Li, M. Corso, L. Colazzo, F. Sedona, D. Sánchez-Portal, J. I. Pascual, D. G. de Oteyza, Width-dependent band gap in armchair graphene nanoribbons reveals Fermi level pinning on Au(111), ACS Nano 2017, 11, 11661-11668 M. Ilyn, A. Magaña, A. L. Walter, J. Lobo-Checa, D. G. de Oteyza, F. Schiller, J. E. Ortega, Step-doubling at vicinal Ni(111) surfaces investigated with a curved crystal, The Journal of Physical Chemistry C 2017, 121, 3880–3886 D. G. de Oteyza, A. García-Lekue, M. Vilas-Varela, N. Merino-Díez, E. Carbonell-Sanromà, M. Corso, G. Vasseur, C. Rogero, E. Guitián, J. I. Pascual, J.E. Ortega, Y. Wakayama, D. Peña, Substrate-independent growth of atomically precise chiral graphene nanoribbons, ACS Nano 2016, 10, 9000-9008 D. G. de Oteyza, A. Pérez Paz, Y.-C. Chen, Z. Pedramrazi, A. Riss, S. Wickenburg, H.-Z. Tsai, F. R. Fischer, M. F. Crommie, A. Rubio, Non-covalent dimerization after enediyne cyclization on Au(111), Journal of the American Chemical Society 2016, 138, 10963-10967 G. Vasseur, M. Abadia, L. A. Miccio, J. Brede, A. Garcia-Lekue, D. G. de Oteyza, C. Rogero, J. Lobo-Checa, J.E. Ortega, On-surface synthesis of poly-p-phenylene nanowires evidenced by electron spectroscopy on a semiconductor TiO2(110). Journal of the American Chemical Society 2016, 138, 5685-5692 P. Borghetti, D. G. de Oteyza, C. Rogero, E. Goiri, L. Floreano, A. Verdini, A. Cossaro, J. E. Ortega, Molecular-level realignment in donor-acceptor bilayer blends on metals, The Journal of Physical Chemistry C 2016, 120, 5997-6005 A. Basagni, G. Vasseur, C. Pignedoli, M. Vilas-Varela, D. Peña, L. Nicolas, L. Vitali, J. Lobo-Checa, D. G. de Oteyza, F. Sedona , M. Casarin, J. E. Ortega, M. Sambi, Tunable band alignment with unperturbed carrier mobility of on-surface synthesized organic semiconducting wires, ACS Nano 2016, 10, 2644-2651 A. Riss, S. Wickenburg, A. Paz, H.-Z. Tsai, P. Gorman, D. G. de Oteyza, A. Bradley, M. M. Ugeda, G. Etkin, A. Rubio, F. R. Fischer, M. F. Crommie, Imaging single-molecule intermediates for chemical reactions quenched by surface energy-dissipation, Nature Chemistry 2016, 8, 678-683 E. Goiri, P. Borghetti, A. El-Sayed, J. E. Ortega, D. G. de Oteyza, Multicomponent Organic Layers on Metal Surfaces, Advanced Materials 2016, 28, 1340-1368 D. G. de Oteyza, J. M. Garcia-Lastra, F. M. Toma, P. Borghetti, L. Floreano, A. Verdini, A. Cossaro, T. V. Pho, F. Wudl, J. E. Ortega, Decacyclene-tri-anhydride (DTA) at Functional Interfaces: An Ideal Electron Acceptor Material for Organic Electronics, The Journal of Physical Chemistry Letters 2016, 7, 90-95 D.L. Olynick, P. Perera, A. Schwartzberg, P. Kulshrethshta, D. G. de Oteyza, N. Jarnagin, C. Henderson, Z. Sun, I. Gunkel, T. Russell, M. Budden, I. W. Rangelow, Selective Laser Ablation in Resists and Block Copolymers for High Resolution Lithographic Patterning, Journal of Photopolymer Science and Technology 2015, 28, 663-668 Y.-C. Chen, T. Cao, C. Chen, Z. Pedramrazi, D. Haberer, D. G. de Oteyza, F. Fischer, S. Loiue, M. F. Crommie, Bandgap Engineering of Bottom-Up Synthesized Graphene Nanoribbons by Controlled Heterojunctions, Nature Nanotechnology 2015, 10, 156-160