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研究领域

With a strong interest in materials and catalysis, the Lo group has been focussing on the fundamental aspects of zeolitic and MOF materials and their catalytic applications. We employ a new structural methodology in using state-of-the-art synchrotron X-ray facility that can: (i) directly visualised how reactant molecules behave and interact with zeolite catalysts, (ii) elucidated the ammonia desorption processes from zeolites, (iii) revealed the reaction mechanisms of existing industrial catalysis processes, (iv) explained the reaction kinetics of new catalysis reactions, and (v) designed and engineered a novel enzyme-mimic inorganic system.

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Xue, Qi, et al. “Controlled Synthesis of bi- and tri-nuclear Cu-oxo Nanoclusters on Metal-organic Frameworks and the Structure-reactivity Correlations” Chemical Science. Advanced article. Zhao, Zhenqing, et al. “Engineering Vacancy and Hydrophobicity of Two-Dimensional TaTe2 for Efficient and Stable Electrocatalytic N2 Reduction.” The Innovation. Liu, Qiong, et al. “Boosted CO desorption behaviors induced by spatial dyadic heterostructure in polymeric carbon nitride for efficient photocatalytic CO2 conversion.” Applied Catalysis B: Environmental 295 (2021): 120289. Duan, Xinping, et al. “Intercalating Lithium into Lattice of Silver Nanoparticles boosts Catalytic Hydrogenation of Carbon-Oxygen Bond.” Chemical Science 12 (2021): 8791-8802 Xue, Qi, et al. “Guest-Anion-Induced Rotation-Restricted Emission in UiO-66-NH2 and Advanced Structure Elucidation” Chemistry of Materials 33.13 (2021): 5422-5429. Chen, Tianxiang, Lin Ye, and Benedict Tsz Woon Lo. “Designing the Electronic and Geometric Structures of Single‐Atom and Nanocluster Catalysts.” Journal of Materials Chemistry A (2021). Xue, Qi, et al. “Recent Advances in the Engineering of Single-Atom Catalysts Through Metal–Organic Frameworks.” Topics in Current Chemistry 379.2 (2021): 1-22. DOI: 10.1007/s41061-021-00324-y Xue, Qi, et al. “A rational study on the geometric and electronic properties of single-atom catalysts for enhanced catalytic performance.” Nanoscale 12.45 (2020): 23206-23212. DOI: 10.1039/D0NR06006B Lin, Wei-Che, et al. “Cooperative catalytically active sites for methanol activation by single metal ion-doped H-ZSM-5.” Chemical Science (2020). DOI: 10.1039/D0SC04058D Yang, Lianghao, et al. “Single yttrium sites on carbon-coated TiO 2 for efficient electrocatalytic N 2 reduction.” Chemical Communications 56.74 (2020): 10910-10913. DOI: 10.1039/D0CC01136C Zhang, Jieru, et al. “Chemical State Tuning of Surface Ce Species on Pristine CeO2 with 2400% Boosting in Peroxidase-like Activity for Glucose Detection.” Chemical Communications (2020). DOI: 10.1039/D0CC02351E Zhai, Lingling, et al. “In Situ Phase Transformation on Nickel-Based Selenides for Enhanced Hydrogen Evolution Reaction in Alkaline Medium.” ACS Energy Letters (2020). DOI: 10.1021/acsenergylett.0c01385 Zhang, Jieru, et al. “Chemical State Tuning of Surface Ce Species on Pristine CeO2 with 2400% Boosting in Peroxidase-like Activity for Glucose Detection.” Chemical Communications (2020). DOI: 10.1039/D0CC02351E Chen, T., Xue, Q., Leung, K.C., Lo, B.T.W. “Recent advances of precise Cu nanoclusters in microporous materials.” Chemistry – An Asian Journal (Invited) (2020) DOI: 10.1002/asia.202000331 Yang, Benyong, et al. “Efficient TiO2-nanobelt-supported Ir catalysts for FCC-generated NOx and CO remediation.” Industrial & Engineering Chemistry Research (2020). https://doi.org/10.1021/acs.iecr.9b06656 Boles, S., et al. “In Situ Formation of Aluminum-Silicon-Lithium Active Materials in Aluminum Matrices for Lithium-Ion Batteries” Journal of Material Chemistry: A (2020) 2020, 8, 4877-4888 Chen, T., Wun, C.K.T., Day, S., Tang, C.C., Lo, B.T.W. “Enantiospecificity in achiral zeolites for asymmetric catalysis.” Physical Chemistry Chemical Physics (Invited) (2020) DOI: 10.1039/D0CP00262C Advanced Article Chen, T., Huang, B., Day, S., Tang, C. C., Tsang, S. C. E., Wong, K. Y., & Lo, T. W. B. “Differential adsorption of L‐and D‐lysine on achiral MFI zeolites as determined by synchrotron X‐ray powder diffraction and thermogravimetric analysis.” Angewandte Chemie 132(3) 2020, 1109-1113. Benedict T.W. Lo, Wei-Che Lin, Molly Meng Jung Li, Sarah Day, Chiu Tang, S. C. Edman Tsang “Evaluation of Brønsted and Lewis acid sites in H-ZSM-5 and H-USY with or without metal modification using probe molecule-synchrotron X-ray powder diffraction.” Applied Catalysis A: General (2020), 596, 117528. Chen, Tianyi, et al. “Interstitial Boron Atoms in Palladium Lattice of Industrial Type of Nano-catalyst: Properties and Structural Modifications.” Journal of the American Chemical Society 141.50 (2019), 19616-19624.

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