研究领域
Molten salt electrochemistry is a classic topic with a history backdated to the isolation of alkaline metal by the electrolysis of molten alkaline hydroxide in 1807 (discovered by Humphry Davy), which is now shining in commercial production of metallic materials (e.g. for massive production of metallic Al with the annual yields as high as several hundred million tons). Molten salt is a unique reaction medium, which could offer unusual capability for chemical reactions, heat storage/transfer and energy storage/conversion. Therefore, molten salt electrochemistry becomes a research hotspot for controllable preparation of functional nanomaterials, carbon capture/utilization, molten salt nuclear reactor, and deep space exploration.
The general goal of our group is to develop novel technologies contributing to energy, environmental and resource sustainability by (1) developing affordable, high-efficiency and controllable preparation of materials and (2) deep understanding physicochemical properties of materials in molecular levels for diverse applications including energy storage/conversion, Fischer-Tropsch synthesis, indoor-air purification, water treatment, etc.
近期论文
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M Jiang, CP Fu,* PY Meng, JM Ren, J Wang, JF Bu, AP Dong,* J Zhang, W Xiao,* BD Sun, Challenges and Strategies of Low-cost Aluminum Anodes for High-performance Al-based Batteries, Adv. Mater. 2021, 2102026.Link
W.Weng, JX Xiao, YJ Shen, XX Liang, T Lv, W Xiao*, Molten Salt Electrochemical Modulation of Iron-Carbon-Nitrogen for Lithium-Sulfur Batteries. Angew. Chem. Int. Ed. 2021.
ZY Fan, W Xiao*, Electrochemical splitting of methane in molten salts to produce hydrogen. Angew. Chem. Int. Ed. 2021, 60, 7664.
XX Liang, JX Xiao, W Weng, W Xiao*, Electrochemical Reduction of Carbon Dioxide and Iron Oxide in Molten Salts to Fe/Fe3C Modified Carbon for Electrocatalytic Oxygen Evolution. Angew. Chem. Int. Ed. 2021, 60, 2120.
ZY Fan, W Weng, J Zhou, D Gu, W Xiao*, Catalytic decomposition of methane to produce hydrogen: a review. J. Energy Chem. 2021, 58, 415-430.
D Pang, W Weng, J Zhou, D Gu, W Xiao*, Controllable conversion of rice husks to Si/C and SiC/C composites in molten salts. J. Energy Chem. 2021, 55, 102-107.
SX Jing, MY Wang*, W Xiao*, Electrochemical conversion of carbon dioxide in molten salts: In-situ and beyond. J. Energy Chem. 2022, 64, 404-405.
HS Xiao, H Zhu, W Weng, KZ Li, W Li* and W Xiao*,Electrochemical fixation of CO2 over a Mo plate to prepare a Mo2C film for electrocatalytic hydrogen evolution. Mater. Chem. Front., 2021,5, 4963-4969.
T Lv, JX Xiao*, W Weng, W Xiao*, Electrochemical Fixation of Carbon Dioxide in Molten Salts on Liquid Zinc Cathode to Zinc@Graphitic Carbon Spheres for Enhanced Energy Storage. Adv. Energy Mater. 2020, 10, 2002241.
W Weng, SB Wang, W Xiao*, XW Lou*, Direct Conversion of Rice Husks to Nanostructured SiC/C for CO2 Photoreduction. Adv. Mater. 2020, 32, 2001560.
W Weng, JR Yang, J Zhou, D Gu, W Xiao*, Template-Free Electrochemical Formation of Silicon Nanotube from Silica. Adv. Sci. 2020, 2001492.
J Zhou, HS Xiao, W Weng*, D Gu, W Xiao*, Interfacial confinement of Ni-V2O3 in molten salts for enhanced electrocatalytic hydrogen evolution. J. Energy Chem. 2020, 50, 280-285. (Cover paper)
J Zhou, DD Nie, XB Jin, W Xiao*, Controllable nitridation of Ta2O5 in molten salts for enhanced photocatalysis. Int. J. Miner. Metall. Mater. 2020, 27, 1703-1710.
W Weng, BM Jiang, Z Wang, W Xiao*, In situ electrochemical conversion of CO2 in molten salts to advanced energy materials with reduced carbon emissions. Sci. Adv. 2020, 6, eaay9278.
W Weng, J Zhou, D Gu, W Xiao*, Thermoelectrochemical formation of Fe/Fe3C@hollow N-doped carbon in molten salts for enhanced catalysis. J. Mater. Chem. A, 2020, 8, 4800-4806.
T Lv, W Weng, J Zhou, D Gu*, W Xiao*, Effects of K and Mn promoters over Fe2O3 on Fischer-Tropsch synthesis. J. Energy Chem., 2020, 47, 118-127.
CF Zhong, W Weng, XX Liang, D Gu, W Xiao*, One-step molten-salt synthesis of anatase/rutile bi-phase TiO2@MoS2 hierarchical photocatalysts for enhanced solar-driven hydrogen generation. Appl. Surf. Sci., 2020, 507, 145072.
JR Yang, W Weng, W Xiao*, Electrochemical synthesis of ammonia in molten salts. J. Energy Chem., 2020, 43, 195–207.
XX Liang,a W Weng,a D Gub, WXiao*a, Nickel Based Oxides Film Formed in Molten Salts for Efficient Electrocatalytic Oxygen Evolution. J. Mater. Chem. A, 2019,7, 10514-10522.
W Weng, C Zeng, W Xiao*, In Situ Pyrolysis Concerted Formation of Si/C Hybrids during Molten Salt Electrolysis of SiO2@Polydopamine. ACS Appl. Mater. Interfaces., 2019, 11, 9156-9163.
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