Qiao, Shizhang - University of Adelaide - School of Chemical Engineering

个人简介

Dr Qiao joined the School of Chemical Engineering of the University of Adelaide (UoA) in March 2012 as a professor (the inaugural Chair of Nanotechnology). He is the founding Director of Centre for Materials in Energy and Catalysis (CMEC) and Director of Australian Research Council (ARC) Industrial Transformation Training Centre for Battey Recycling. His research expertise is in nanostructured materials for new energy technologies (electrocatalysis, photocatalysis, batteries, fuel cell). He has co-authored more than 530 papers in refereed journals, including Nature, Nature Energy, Nature Nonotechnology, Nature Chemistry, Nature Materials, Nature Catalysis, Nature Communications, Science Advances, Angew Chem Int Ed, J. Am. Chem. Soc, Advanced Materials (over 105,986/122,858 citations, h-index: 166/179, Web of Sci./Google Scholar). He has filed seven patents on novel nanomaterials and attracted more than 35 million dollars in research grants from industrial partners and ARC. In recognition of his achievements in research, he was honoured with inaugural ARC Australian Industry Laureate Fellow (2023), Pioneers in Energy Research (Energy & Fuel, 2023), prestigious the South Australian Scientist of the Year (2021), inaugural UoA Vice-Chancellor's Award for Excellence in Research (2019), an Australian Star of Research (Lifetime Achievers Leaderboard, by "The Australian" 2019-2023), ARC Australian Laureate Fellow (2017), ExxonMobil Award (2016), ARC Discovery Outstanding Researcher Award (DORA, 2013), Emerging Researcher Award (2013, ENFL Division of the American Chemical Society) and UQ Foundation Research Excellence Award (2008). He has also been awarded an ARC ARF Fellowship, an ARC APD Fellowship and an inaugural UQ Mid-Career Research Fellowship. Dr Qiao is an elected Fellow of Australian Academy of Science (FAA), a Fellow of Institution of Chemical Engineers (FIChemE), Royal Society of Chemistry (FRSC) and Royal Australian Chemical Institute (FRACI). Dr Qiao is currently an Editor-in-Chief of EES Catalysis (RSC) and a Thomson Reuters/Clarivate Analytics Highly Cited Researcher (with 124 highly cited papers) in three categories of Chemistry, Materials Science, Environment and Ecology.

研究领域

Dr Qiao's research interests include synthesis, characterisation and simulation of nanomaterials as well as their applications in catalysis, energy storage (metal ion batteries, aqueous metal batteries, battery recycling) and conversion (production of fuels and chemicals by electrocatalysis and photocatalysis) Student projects (with Scholarships) available Nanostructured Electrocatalysts for Sustainable Clean Energy Generation Synthesis of Nanostructured Materials for High Performance Metal Ion Batteries and Advanced Aqueous Batteries Battery Recycling Nanostructured Materials for Photocatalysis AI-driven Discovery for Energy Materials (including Machine Learning)

近期论文

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Li H., Meng R.W., Ye C., Tadich A., Hua W., Gu Q.F., Johannessen B., Chen X., Davey K., Qiao S.Z., Developing High-power Li||S Batteries via Transition Metal/Carbon Nanocomposite Electrocatalysts Engineering, Nature Nanotechnology, 2024, DOI: 10.1038/s41565-024-01614-4 Ye C., Li H., Chen Y.J., Hao J.N., Liu J.H., Shan J.Q., Qiao S.Z., The Role of Electrocatalytic Materials for Developing Post-lithium Meta/Sulfur Batteries, Nature Communications, 2024, accepted Wu H., Hao J.N., Jiang Y.L., Jiao Y.R., Liu J.H., Xu X., Davey K., Wang C.S., Qiao S.Z., Akaline-based Aqueous Sodium-ion Battery for Large-scale Energy Storage, Nature Communications, 2024, 15, 575. DOI: 10.1038/s41467-024-44855-6. Hao J.N., Zhang S.J., Wu H., Yuan L.B., Davey K., Qiao S.Z., Advanced Cathodes for Aqueous Zn Batteries beyond Zn2+ Intercalation, Chemical Society Reviews, 2024, in press. Gao X.T., Zhang S., Wang P.T., Jaroniec M., Zheng Y., Qiao S.Z., Urea Catalytic Oxidation for Energy and Environmental Applications, Chemical Society Reviews, 2024, 53, 1552-1591. Chen C.J., Jin H.Y., Wang P.T., Sun X.G., Jaroniec M., Zheng Y., Qiao S.Z., Local Environment in Electrocatalysis, Chemical Society Reviews, 2024, 53, 2022-2055. Xu X., Ren S.Y., Wu H., Li H., Ye C., Davey K., Qiao S.Z., Establishing Exceptional Durability in Ultra-low-temperature Organic-sodium Batteries via Stabilized Multiphase Conversions, Journal of the American Chemical Society, 2024, 146(2), 1619-1626. Huang L.S., Bao D.Y., Jiang Y.L., Zheng Y., Qiao S.Z., Electrocatalytic Acetylene Hydrogenation in Concentrated Seawater at Industrial Current Densities, Angew. Chem. Int. Ed., 2024, 63, Chen Q.R., Hao J.N., Zhang S.J., Tian Z.H., Davey K., Qiao S.Z., High-reversibility Sulfur Anode for Advanced Aqueous Battery, Advanced Materials, 2024, 36(1), 2309038. Zheng M., Zhang J.Y., Wang P.T., Jin H.Y., Zheng Y., Qiao S.Z., Recent Advances in Electrocatalytic Hydrogenation Reactions on Copper-Based Catalysts, Advanced Materials, 2024, 36(14), 2307913. Ran J.R., Talebian-Kiakalaieh A., Qiao S.Z., Atomically-Scattered Active Centers Accelerating Photocatalytic Evolution of Ammonia, Advanced Energy Materials, 2024, DOI: 10.1002/aenm.202400650. Jiang Y.L., Li H.B., Chen C.J., Zheng Yao, Qiao S.Z., Dynamic Cu0/Cu+ Interface Promotes Acidic Co2 Electroreduction, ACS Catalysis, 2024, 14, Chen Y.J., Ye C., Zhang N.J., Liu J.H., Li H., Davey K., Qiao S.Z., Prospects of Practical Anode-free Sodium Batteries, Materials Today, 2024, 73, 260-274. Ran J.R., Talebian-Kiakalaieh A., Zhang S., Hashem E.M., Guo M.J., Qiao S.Z., Recent Advancement on Photocatalytic Plastic Upcycling, Chemical Science, 2024, 15, 1611-1637. Chen C.J., Huang L.S., Jiang Y.L., Zheng Y., Qiao S.Z., Modulating Local Environment for Electrocatalytic CO2 Reduction to Alcohol, Nano Energy, 2024, 126, 109656. Wu X.H., et al., Multi-site Catalysis of High-entropy Hydroxides for Sustainable Electrooxidation of Glucose to Glucaric Acid, Energy & Environmental Science, 2024, Guo J.X., Zheng Y., Hu Z.P., Zheng C., Mao J., Du K., Jaroniec M., Qiao S.Z., Ling T., Direct Seawater Electrolysis by Adjusting Catalyst's Local Reaction Environment, Nature Energy, 2023, DOI: 10.1038/s41560-023-01195-x Xie F.X., Cui X.L., Zhi X., Yao D.Z., Johannessen B., Zhang Q.H., Tang J., Woodfield T.B.T., Gu L., Qiao S.Z., A Beneral Approach to 3D Printed Single Atom Catalysts, Nature Synthesis, 2023, DOI: 10.1038/s44160-022-00193-3. Jin H.Y., Liu X.Y., Li H.J., Tang C., Yu H.M., Zhang Q.H., Dong J.C., Peng H.J., Gu L., Zheng Y., Song T., Davey K., Paik U., Qiao S.Z., Dynamic Rhenium Dopants boost Ruthenium Oxide for Durable Oxygen Evolution, Nature Communications, 2023, DOI: 10.1038/s41467-023-35913-6 Liu J.H., Ye C.,Wu H., Jaroniec M., Qiao S.Z., 2D Mesoporous Zincophilic Sieve for High-rate Sulfur-based Aqueous Zinc Battery, Journal of the American Chemical Society, 2023, 145, accepted Li H.B., Jiao Y., Davey K., Qiao S.Z., Machine Learning for Surface Structures of Heterogeneous Catalysts, Angew. Chem. Int. Ed., 2023, DOI:10.1002/anie.202216383 Yao D.Z., Tang C., Zhi X., Johannessen B., Slattery A., Jiao Y., Qiao S.Z., Inter-metal Interaction with a Threshold Effect in NiCu Dual-atom Catalysts for CO2 Electroreduction, Advanced Materials, 2023, DOI: 10.1002/adma.202209386. Zheng Y., Qiao S.Z., Direct Seawater Splitting to Hydrogen by a Membrane Electrolyser, Joule, 2023, 7(1), 20-22. Kao C.C., Ye C., Hao J.N., Shan J.Q., Li H., Qiao S.Z. Suppressing Hydrogen Evolution via Anticatalytic Interfaces towards Highly Efficient Aqueous Zn-ion-Batteries, ACS Nano, 2023, in press. Jiang Y.L., Shan J.Q., Wang P.T., Huang L.S., Zheng Y., Qiao S.Z., Stablizing Oxidation State of SnO2 for Highly Selective CO2 Electroreduction to Formate at Large Current Densities, ACS Catalysis, 2023, in press. Xu X., Ye C., Chao D.L., Davey K., Qiao S.Z., Initiating Jahn-Teller Effect in Vanadium Diselenide for High-performance Magnesium-based Hybrid Batteries Operated at -40 oC, Advanced Energy Materials, 2023, 13, DOI: 10.1002/aenm.202204344 Zheng Y., Qiao S.Z., Direct Seawater Splitting to Hydrogen by a Membrane Electrolyser, Joule, 2023, 7(1), 20-22. Yuan L.B., Hao J.N., Johannessen B., Ye C., Yang F., Wu C., Dou S.X., Liu H.K., Qiao S.Z., Hybrid Working Mechanism Enables Highly Reversible Zn Electrodes, eScience, 2023, DOI: 10.1016/j.esci.2023.100096. Shan J.Q., Ye C., Jiang Y.L., Jaroniec M., Zheng Y., Qiao S.Z., Metal-Metal Interactions in Correlated Single Atom Catalysts, Science Advances, 2022, 8(17), eabo0762. Liu X., Jiao Y., Zheng Y., Jaroniec M., Qiao S.Z., The Mechanism of C-N Bonds Formation in Electrocatalytic Urea Production Revealed by ab initio Molecular Dynamics Simulation", Nature Communications, 22, 13, 5471. DOI: 10.1038/s41467-022-33258-0. Wang P.T., Yang H., Tang C., Wu Y., Zheng Y., Cheng T., Davey K., Huang X.Q., Qiao S.Z., Boosting Electrocatalytic CO2-to-Ethanol Production via Asymmetric C-C Coupling, Nature Communications, 2022, 13, 3754. DOI: 10.1038/s41467-022-31427-9. Ran J.R., Zhang H.P., Fu S.J., Jaroniec M., Shan J.Q., Xia M.Q., Qu Y., Qu J., Chen S.M., Song L., Cairney J.M., Jing L.Q., Qiao S.Z., NiPS3 Ultrathin Nanosheets: A Versatile Platform for Highly Active Photocatalytic H2 Production, Nature Communications, 2022, 13, 4600. DOI: 10.1038/s41467-022-32256-6 Shan J.Q., Ye C., Zhu C.Z., Dong J.C., Xu W.J., Chen L., Jiao Y., Jiang Y.L., Song L., Zhang Y., Jaroniec M., Zhu Y.H., Zheng Y., Qiao S.Z., Integrating Interactive Noble Metal Single Atom Catalysts into Transition Metal Oxide Lattices, Journal of the American Chemical Society, 2022, 144 (50), 23214-23222. Zheng M., Wang P.T., Zhi X., Yang K., Jiao Y., Duan J.J., Zheng Y., Qiao S.Z., Electrocatalytic CO2-to-C2+ with Ampere-Level Current on Heteroatom Engineered Copper via Tuning *CO Intermediate Coverage, Journal of the American Chemical Society, 2022, 144(32), 14936-14944. Zhou X.L., Shan J.Q., Chen L., Xia B.Y., Ling T., Duan J.J., Jiao Y., Zheng Y., Qiao S.Z., Stabilizing Cu+2 Ions by Solid Solutions to Promote CO2 Electroreduction to Methane, Journal of the American Chemical Society, 2022, 144(5), 2079-2084. Li H., Meng R., Guo Y., Ye C., Kong D., Johannessen B., Jaroniec M., Qiao S.Z.,Unraveling the Catalyst-Solvent Interactions in Lean-Electrolyte Sulfur Reduction Electrocatalysis for Li-S Batteries, Angew. Chem. Int. Ed., 2022, 61(51), e202213863. Zhang Y.Z., Zhi X., Harmer J.R., Xu H., Davey K., Ran J.R., Qiao S.Z., Facet-specific Active Surface Regulation of BixMoy(M=Mo, V, W) Nanosheets for Boosted Photocatalytic CO2 Reduction, Angew. Chem. Int. Ed., 2022, 61(50), e202212355. Shan J.Q., Liao J.W., Ye C., Dong J.C., Zheng Y., Qiao S.Z., The Dynamic Formation from Metal-Organic Frameworks of High-Density Pt Single Atom Catalysts with Metal-Matel Interations, Angew. Chem. Int. Ed., 2022, 61(48), e202213412. Jin H.Y., Yu H.M., Li H.B., Davey K., Song T., Paik U., Qiao S.Z., MXene Analogue: A 2D Nitridene Solid Solution for High Rate Hydrogen Production, Angew. Chem. Int. Ed., 2022, 61(27), e202203850. Wang X.S., Jiao Y., Li L.Q., Zheng Y., Qiao S.Z., Local Environment Determined Reactant Adsorption Configuration for Enhanced Electrocatalytic Acetone Hydrogenation to Propane, Angew. Chem. Int. Ed., 2022, 61(5), e202114253. Hao J.N., Yuan L.B., Zhu Y.L., Jaroniec M., Qiao S.Z., Triple-function Electrolyte Regulation towards Advanced Zn-ion Batteries, Advanced Materials, 2022, 34(44), 2206963. Zhang S.J., Hao J.N., Li H., Zhang P. Yin Z., Li Y., Zhang B.K., Lin Z., Qiao S.Z., Polyiodide Confinement by Starch Enables Shuttle-Free Zn-Iodine Batteries, Advanced Materials, 2022, 34(23), 2201716. Xu X., Ye C., Chao D., Chen B., Li H., Tang C., Zhong X., Qiao S.Z., Synchrotron X-ray Spectroscopic Investigations of In-Situ Formed Alloy Anodes for Magnesium Batteries, Advanced Materials, 2022, 34(8), 2108688. Zhao E., Du K., Yin P.F., Ran J.R., Mao J., Ling T., Qiao S.Z., Advancing photoelectrochemical energy conversion through atomic design of catalysts, Advanced Science, 2022, 9(1), 2104363. Mao J.F., Ye C., Zhang S.L., Xie F.X., Zeng R., Davey K., Guo Z.P., Qiao S.Z., Toward Practical Lithium-ion Battery Recycling: Adding Value, Tackling Circularity and Recycling-oriented Design, Energy & Environmental Science, 2022, 15, 2732-2752. Xia B.Q., He B., Zhang J., Li L.Q., Zhang Y.Z., Yu J. G., Rang J.R., Qiao S.Z., TiO2/FePS3 S-scheme Heterojunction for Greatly Raised Potocatalytic Hydrogen Evolution, Advanced Energy Materials, 2022, 12(46), 2201449. Shan J.Q., Zheng Y., Qiao S.Z., Communications between Acive Sites Regulates Heterogeneous Catalysis, Chem, 2022, 8(11), 2897-2899. Zhang Y.Z., Yao D.Z., Xia B.Q., Jaroniec M., Ran J.R., Qiao S.Z., Photocatalytic CO2 Reduction: Identification and Elimination of False-Positive Results, ACS Energy Letters, 2022, 7, 1611-1617. Zhang S., Qiao S.Z., Mild Synthesis for Defect-switchable Photocatalysts for Hydrogen Evolution, Chem Catalysis, 2022, 2, 434-436. Xia B.Q., Yang Y., Zhang Y.Z., Xia Y., Jaroniec M., Yu J.G., Ran J.R., Qiao S.Z., Metal-organic framework with atomically dispersed Ni-N4 sites for greatly raised visible-light photocatalytic H2 production, Chemical Engineering Journal, 2022, 431(1), 133944. Yao D.Z., Tang C., Wang P.T., Cheng H., Jin H.Y., Ding L.X., Qiao S.Z., Electrocatalytic Green Ammonia Production beyond Ambient Aqueous Nitrogen Reduction, Chemical Engineering Science, 2022, 257, 117735. Geng S.K., Zheng Y., Li S.Q., Su H., Zhao X., Hu J., Shu H.B., Jaroniec M., Chen P., Liu Q.H., Qiao S.Z., Nickel Ferrocyanide as a High-performance Urea Oxidation Electrocatalyst, Nature Energy, 2021, 6, 904-912. Ye C., Jin H.Y., Shan J.Q., Jiao Y., Li H., Gu Q.F., Davey K., Wang H.H., Qiao S.Z., Catalyzing Na2S Electrodeposition for Efficient Room-Temperature Sodium-Sulfur Batteries, Nature Communications, 2021, 12, 7195. DOI: 10.1038/s41467-021-27551-7. Li H., Meng R.W., Guo Y., Chen B., Jiao Y., Ye C., Long Y., Yang Q.H., Jaroniec M., Qiao S.Z., Reversible Electrochemical Oxidation of Sulfur in Ionic Liquid for High-voltage Al-S Batteries, Nature Communications, 2021, 12, 5714. DOI: 10.1038/s41467-021-26056-7. Ye C., Shan J.Q., Chao D.L., Liang P., Hao J.N., Jiao Y., Davey K., Wang H.H., Qiao S.Z., Catalytic Oxidation of K2S via Atomic Co and Pyridinic N Synergy in Potassium-Sulfur Batteries, Journal of the American Chemical Society, 2021, 143, 16902-16907. Tang C., Chen L., Li H.J., Li L.Q., Jiao Y., Zheng Y., Xu H.L., Davey K., Qiao S.Z., Tailoring Acidic Oxygen Reduction-selectivity on Single-Atom Catalysts via Modification of First and Second Coordination Spheres, Journal of the American Chemical Society, 2021, 143, 7819-7827. Zhou X.L., Dong J.C., Zhu Y.H., Liu L.M., Jiao Y., Li H., Han Y., Davey K., Xu Q., Zheng Y., Qiao S.Z., A Molecular Scalpel to Chemically Cleave Metal-Organic Frameworks for Induced Phase Transition, Journal of the American Chemical Society, 2021, 143, 6681-6690. Shan J.Q., Ye C., Chen S.M., Sun Y.T., Jiao Y., Liu L.M., Zhu C.Z., Song L., Han Y., Jaroniec M., Zhu Y.H., Zheng Y., Qiao S.Z., Short-range Ordered Iridium Single Atoms Integrated into Cobalt Oxide Spinel Structure for Highly Efficient Electrocatalytic Water Oxidation, Journal of the American Chemical Society, 2021, 143, 5201-5211. Hao J.N., Yuan L.B., Johannessen B., Zhu Y.L., Jiao Y., Ye C., Xie F.X., Qiao S.Z., Studying Conversion Mechanism to Broaden Cathode Options in Aqueous Zn-ion Batteries, Angew. Chem. Int. Ed., 2021, 60, 25114-25121. Tang C., Zheng Y., Jaroniec M., Qiao S.Z., Electrocatalytic Refinery for Sustainable Production of Fuels and Chemicals, Angew. Chem. Int. Ed., 2021, 60, 19572-19590. Yao D.Z., Tang C., Vasileff A., Zhi X., Jiao Y., Qiao S.Z., The Controllable Reconstruction of Bi-MOFs for Electrochemical CO2 Reduction through Electrolyte and Potential Mediation, Angew. Chem. Int. Ed., 2021, 60, 18178-18184. Li L.Q., Tang C., Cui X.Y., Zheng Y., Wang X.S., Xu H.L., Zhang S., Shao T., Davey K., Qiao S.Z., Efficient Nitrogen Fixation to Ammonia through Integration of Plasma Oxidation with Electrocatalytic Reduction, Angew. Chem. Int. Ed., 2021, 60, 14131-14137. Hao J.N., Yuan L., Ye C., Chao D.L., Davey K., Guo Z.P., Qiao S.Z., Boosting Zn Electrode Reversibility in Aqueous Electrolyte Using Low-cost Antisolvents, Angew. Chem. Int. Ed., 2021, 60, 7366-7375. Zhou X.L., Jin H.Y., Xia B.Y., Davey K., Zheng Y., Qiao S.Z., Molecular Cleavage of Metal-Organic Frameworks and Application to Energy Storage and Conversion, Advanced Materials, 2021, 33(51), 2104341. Jin H.Y., Wang X.S., Tang C., Vasileff A., Li L.Q., Slattery A., Qiao S.Z., Stable and Highly Efficient Hydrogen Evolution from Seawater Enabled by an Unsaturated Nickel Surface Niride, Advanced Materials, 2021, 33(13), 20207508. Li L.Q., Tang C., Jin H.Y., Davey K., Qiao S.Z.,Main Group Elements Boost Electrochemical Nitrogen Fixation, Chem, 2021, 7(12), 3232-3255. DOI:10.1016/j.chempr.2021.10.008. Yuan L.B.,Hao J.N., Kao C.C., Wu C., Liu H.K., Dou S.X., Qiao S.Z., Regulation Methods for the Zn/electrolyte Interphase and the Effectiveness Evaluation in Aqueous Zn-Ion Batteries, Energy & Environmental Science, 2021, 14, 5669-5689. Zhi X., Vasileff A., Zheng Y., Jiao Y., Qiao S.Z., Role of Oxygen-Bound Reaction Intermediates in Selective Electrochmical CO2 Reduction, Energy & Environmental Science, 2021, 14, 3912-3930. Xia B.Q., Zhang Y.Z., Ran J.R., Jaroniec M., Qiao S.Z., Single-atom Photocatalysts for Emerging Reactions, ACS Central Science, 2021, 7, 39-54. Jin H.Y., Song T., Paik U., Qiao S.Z., Metastable Two-Dimensional Materials for Electrocatalytic Energy Conversion, Accounts of Materials Research, 2021, 2(7), 559-573. Zhang S.J., Hao J.N., Luo D., Zhang P.F., Zhang B.K., Davey K., Lin Z., Qiao S.Z., Dual-function Electrolyte Additive for Highly Reversible Zn Anode, Advanced Energy Materials, 2021, 11(37), 2102010. Xie F.X., Li H., Wang X.S., Zhi X., Chao D.L., Davey K., Qiao S.Z., Mechanism for Zincophilic Sites on Zinc-Metal Anode Hosts in Aqueous Batteries, Advanced Energy Materials, 2021, 11(9), 2003419. Zhi X., Jiao Y., Zheng Y., Davey K., Qiao S.Z., Directing Selectivity of CO2 Electroreduction to Target C2 Products via Non-metal Doping on Cu Surfaces, Journal of Materials Chemistry A, 2021, 9, 6345-6351. Ran J.R., Xia B.Q., Zhang Y.Z., Qiao S.Z., Two-dimensional Building Blocks for Photocatalytic Ammonia Production, Journal of Materials Chemistry A, 2021, 9, 18733-18745. Chen L., Tang C., Davey K., Zheng Y., Jiao Y., Qiao S.Z., Spatial-Confinement Induced Electroreduction of CO and CO2 to Diols on Densely-Arrayed Cu Nanopyramids, Chemical Science, 2021, 12, 8079-8087. Ran J.R., Zhang H.P., Qu J.T., Shan J.Q., Davey K., Cairney J.M., Jing L.Q., Qiao S.Z., Significantly Raised Visible-light Photocatalytic H2 Evolution on 2D/2D ReS2/In2ZnS4 van der Waals Heterostructure, Small, 2021, 17(32), 2100296. Zhang Y.Z., Yao D.Z., Xia B.Q., Xu H.L., Tang Y.H., Davey K., Ran J.R., Qiao S.Z., ReS2 Nanosheets with in situ Formed Sulfur Vacancies towards Efficient and Highly-selective Photocatalytic CO2 Reduction, Small Science, 2021, 1(2), 2000052. Xu C.C., Zhi X., Vasileff A., Wang D., Jin B., Jiao Y., Zheng Y., Qiao S.Z., Highly Selective Two-Electron Electrocatalytic CO2 Reduction on Single-Atom Cu Catalysts, Small Strucrures, 2021, 2(1), 2000058. Zhi X. Jiao Y., Zheng Y., Qiao S.Z., Key to C2 Production: Selective C-C Coupling for Electrochemical CO2 Reduction on Copper Alloy Surfaces, Chemical Communications, 2021, 57, 9526-9529. Xu C.C., Vasileff A., Zheng Y., Qiao S.Z., Recent Progress of 3d transition Metal Single-Atom Catalysts for Electrochemical CO2 Reduction, Advanced Materials Interface, 2021, 8(5), 2001904. You B., Qiao S.Z., Destabilizing Alkaline Water by 3d-Metal(Oxy)(Hydr)Oxides for Improved Hydrogen Evolution, Chemistry- A European Journal, 2021, 27, 553-564. Chao D.L.,Zhou W.H., Xie F.X., Ye C., Li H., Jaroniec M., Qiao S.Z., Roadmap for Advanced Aqueous Batteries: From Design of Materials to Applications, Science Advances, 2020, 6(21), eaba4098. Su D.W., Ran J.R., Zhuang Z.W., Chen C., Qiao S.Z., Li Y.D., Wang G.X., Atomically Dispersed Ni in Cadmium-Zinc Sulphide Quantum Dots for High-performance Visible-light Photocatalytic Hydrogen Production, Science Advances, 2020, 6(33), eaaz8447. Kuai C.G., Xu Z., Xi C., Hu A., Yang Z., Zhang Y., Sun C.J., Li L., Sokaras D., Dong C., Qiao S.Z., Du X.W., Lin F., Phase Segregation Reversibility in Mixed Metal Hydroxide Water Oxidation Catalysts, Nature Catalysis, 2020, 3, 743-753. Li H., Chao D.L., Chen B., Chen X., Chuah C., Tang Y., Jiao Y., Jaroniec M., Qiao S.Z., Revealing Principles for Design of Lean-electrolyte Lithium Metal Anode via in-situ Spectroscopy, Journal of the American Chemical Society, 2020, 142, 2012-2022. Xu X., Chao D.L., Chen B., Liang P., Li H., Xie F.X., Davey K., Qiao S.Z., Revealing the Magnesium Storage Mechanism in Mesoporous Bismuth via Spectroscopy and ab Initio Simulation, Angew. Chem. Int. Ed., 2020, 59, 21728-21735. Vasileff A., Zhu Y.P., Zhi X., Zhao Y.Q., Ge L., Chen H.M., Zheng Y., Qiao S.Z., Electrochemical Reduction of CO2 to Ethane through Stabilization of an Ethoxy Intermediate, Angew. Chem. Int. Ed., 2020, 59, 19649-19653. Tang C., Jiao Y., Liu J.N., Xie Z.H., Chen X., Zhang Q., Qiao S.Z., Coordination Tunes Selectivity: Two-Electron Oxygen Reduction on High-loading Molybdenum Single-Atom Catalysts, Angew. Chem. Int. Ed., 2020, 59, 9171-9176. Duan J.J., Chen S., Ledon C.O., Jaroniec M., Qiao S.Z., Phosphorus Vacancies Boost Electrocatalytic Hydrogen Evolution by Two Orders of Magnitude, Angew. Chem. Int. Ed., 2020, 59, 8181-8186. Yang Y.Y., Zhang L.F., Hu Z.P., Zheng Y., Tang C., Chen P., Wang R.G., Qiu K.W., Mao J., Ling T., Qiao S.Z., The Crucial Role of Charge Accumulation and Spin Polarization in Activating Carbon-based Catalysts for Electrocatalytc Nitrogen Reduction, Angew. Chem. Int. Ed., 2020, 59, 4525-4531. Ling T., Jaroniec M., Qiao S.Z., Recent Progress in Engineering Atomic and Electronic Structure of Electrocatalysts via Cation Exchange Reaction, Advanced Materials, 2020, 32(46), 2001866. Chao D.L., Ye C., Xie F.X., Zhou W.H., Zhang Q.H., Gu Q.F., Davey K., Gu L., Qiao S.Z., Atomic Engineering Catalyzed MnO2 Electrolysis Kinetics for Hybrid Aqueous Battery with High Power and Energy Density, Advanced Materials, 2020, 32(25), 2001894. Ye C., Jiao Y., Chao D.L., Ling T., Shan J.Q., Zhang B.W., Gu Q.F., Davey K., Wang H.H., Qiao S.Z., Electro-state Confinement of Polysulfides for Highly Stable Sodium-sulfur Batteries, Advanced Materials, 2020, 32(12), 1907557. Mu C., Mao J., Guo J.X., Guo Q.J., Li Z.Q., Qin W.J., Hu Z.P., Davey K., Ling T., Qiao S.Z., Rational Design of Spinel Cobalt Vanadate Oxide Co2VO4 for Superior Electrocatalysis, Advanced Materials, 2020, 32 (10), 1907168. Jin H.Y., Gu Q.F., Chen B., Tang C., Zheng Y., Zhang H., Jaroniec M., Qiao S.Z., Molten Salt-Directed Catalytic Synthesis of 2D Layered Transition Metal Nitrides for Efficient Hydrogen Evolution, Chem, 2020, 6(9), 2382-2394. Ye C., Chao D.L., Shan J.Q., Li H., Davey K., Qiao S.Z., Unveiling the Advances of 2D Materials for Li/Na-S Batteries Experimentally and Theoretically, Matter, 2020, 2(2), 323-344. Chao D.L., Qiao S.Z., Toward High-Voltage Aqueous Batteries: Super- or Low-Concentrared Electrolyte?, Joule, 2020, 4(9), 1846-1851. Chen B., Chao D.L., Liu E.Z., Jaroniec M., Zhao N.Q., Qiao S.Z., Transition Metal Dichalcogenide Anods for Aklali Metal Ion Batteries: Emerging Strategies at Atomic Level, Energy & Environmetal Science, 2020, 13, 1096-1131. Liu X., Jiao Y. Zheng Y., Qiao S.Z., Isolated Boron Sites for Electroreduction of Dinitrogen to Ammonia, ACS Catalysis, 2020, 10, 1847-1854. Ran J.R., Zhang H.P., Qu J.T., Shan J.Q., Chen S.M., Yang F., Zheng R.K., Cairney J., Song L., Jing L.Q., Qiao S.Z., Atomic-level Insights into the Edge Active ReS2 Ultrathin Nanosheets for High Effiviency Light-to-Hydrogen Conversion, ACS Materials Letters, 2020, 2, 1484-1494. 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