Copéret, Christophe - Eidgenössische Technische Hochschule Zürich - Department of Chemistry and Applied Biosciences

个人简介

Prof. Christophe Copéret (CCH) was trained in chemistry and chemical engineering in CPE Lyon (France) and then undertook a PhD in chemistry at Purdue University (USA), where he studied the development of highly efficient synthesis of complex molecules via Pd-catalyzed carbonylation reactions in the group of external pageProf. E. Negishicall_made (1991-1996). After a postdoctoral stay at the Scripps Research Institute (La Jolla, USA) in the group of external pageProf. K.B. Sharplesscall_made (1996-1997), where he developed oxidation reactions, CCH was offered in 1998 a permanent research position in CNRS in C2P2 (at the time LCOMS, directed by Dr. Jean-Marie Basset), a laboratory devoted to catalysis, chemistry of surfaces and polymers, and was promoted CNRS Research Director in 2008. Since Nov, 1st 2010, CCH is Professor in the Department of Chemistry and Applied Biosciences at ETH Zürich. His scientific interest lies at the frontiers of molecular, material and surface chemistry, with the aims to design functional materials with applications in catalysis (sustainable chemistry and energy), molecular recognition, imaging and microelectronics.

研究领域

Computational Chemistry Decoding NMR Chemical Shift Dynamic Nuclear Polarization (DNP) High Throughput Experimentation (HTE) Nanoscale Surface Organometallic Chemistry (SOMC) Automation and AI Team

近期论文

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Introduction: Bridging the Gaps: Learning from Catalysis across Boundaries Ward T.R. and Copéret C. Chemical Reviews, vol. 123: no. 9, pp. 5221-5224, 2023. DOI: 10.1021/acs.chemrev.3c00029 call_made Swiss CAT+, a Data-driven Infrastructure for Accelerated Catalysts Discovery and Optimization Paco Laveille, Pascal Miéville, Sourav Chatterjee, Elisa Clerc, Jean-Charles Cousty, Florian de Nanteuil, Erwin Lam, Edy Mariano, Adrian Ramirez, Urielle Randrianarisoa, Keyan Villat, Christophe Copéret and Nicolai Cramer Chimia, vol. 77: no. 3, pp. 154-158, Bern: Schweizerische Chemische Gesellschaft, 2023. DOI: 10.2533/chimia.2023.154 call_made Evaluating the stability of Ir single atom and Ru atomic cluster oxygen evolution reaction electrocatalysts Matej Zlatar, Darryl Nater, Daniel Escalera-López, Rani Mary Joy, Paulius Pobedinskas, Ken Haenen, Christophe Copéret and Serhiy Cherevko Electrochimica Acta, vol. 444, pp. 141982, Kidlington: Elsevier, 2023. DOI: 10.1016/j.electacta.2023.141982 call_made Assigning H-1 chemical shifts in paramagnetic mono- and bimetallic surface sites using DFT: a case study on the Union Carbide polymerization catalyst Anna Giorgia Nobile, David Trummer, Zachariah J. Berkson, Michael Wörle, Christophe Copéret and Pierre-Adrien Payard Chemical Science, vol. 14: no. 9, pp. 2361-2368, Cambridge: Royal Society of Chemistry, 2023. DOI: 10.1039/d2sc06827c call_made Surface organometallic and coordination chemistry approach to formation of single site heterogeneous catalysts Christophe Copéret and Maciej Damian Korzynski Comprehensive Inorganic Chemistry III (Third Edition). Volume 6: Heterogeneous Inorganic Catalysis, pp. 67-85, Amsterdam: Elsevier, 2023. DOI: 10.1016/B978-0-12-823144-9.00003-0 call_made Visualizing Structural and Chemical Transformations of an Industrial Cu/ZnO/Al2O3 Pre-catalyst during Activation and CO2 Reduction Xing Huang, Arik Beck, Alexey Fedorov, Hannes Frey, Bingsen Zhang, Bernhard Klötzer, Jeroen A. van Bokhoven, Christophe Copéret and Marc Willinger ChemCatChem, vol. 14: no. 24, pp. e202201280, Weinheim: Wiley-VCH, 2022. DOI: 10.1002/cctc.202201280 call_made Speciation and Structures in Pt Surface Sites Stabilized by N-Heterocyclic Carbene Ligands Revealed by Dynamic Nuclear Polarization Enhanced Indirectly Detected 195Pt NMR Spectroscopic Signatures and Fingerprint Analysis Zhuoran Wang, Laura A. Völker, Thomas C. Robinson, Nicolas Kaeffer, Georges Menzildjian, Ribal Jabbour, Amrit Venkatesh, David Gajan, Aaron J. Rossini, Christophe Copéret and Anne Lesage Journal of the American Chemical Society, vol. 144: no. 47, pp. 21530-21543, Washington, DC: American Chemical Society, 2022. DOI: 10.1021/jacs.2c08300 call_made Solid-state NMR spectra of protons and quadrupolar nuclei at 28.2 T: Resolving signatures of surface sites with fast magic angle spinning Zachariah J. Berkson, Snædís Björgvinsdóttir, Alexander Yakimov, Domenico Gioffrè, Maciej Damian Korzynski, Alexander B. Barnes and Christophe Copéret JACS Au, vol. 2: no. 11, pp. 2460-2465, Washington, DC: American Chemical Society, 2022. DOI: 10.1021/jacsau.2c00510 call_made Ga and Zn increase the oxygen affinity of Cu-based catalysts for the COx hydrogenation according to ab initio atomistic thermodynamics Andreas Müller, Aleix Comas Vives and Christophe Copéret Chemical Science, vol. 13: no. 45, pp. 13442-13458, Cambridge: Royal Society of Chemistry, 2022. DOI: 10.1039/d2sc03107h call_made Grafting of Group-10 Organometallic Complexes on Silicas: Differences and Similarities, Surprises and Rationale Domenico Gioffrè, Lukas Rochlitz, Pierre-Adrien Payard, Alexander Yakimov and Christophe Copéret Helvetica Chimica Acta, vol. 105: no. 10, pp. e202200073, New York, NY: Wiley-VCH, 2022. DOI: 10.1002/hlca.202200073 ca Classifying and Understanding the Reactivities of Mo-Based Alkyne Metathesis Catalysts from Mo-95 NMR Chemical Shift Descriptors Zachariah J. Berkson, Lukas Lätsch, Julius Hillenbrand, Alois Fürstner and Christophe Copéret Journal of the American Chemical Society, vol. 144: no. 33, pp. 15020-15025, Washington, DC: American Chemical Society, 2022. DOI: 10.1021/jacs.2c06252 call_made Correction to “Silica-Supported PdGa Nanoparticles: Metal Synergy for Highly Active and Selective CO2‑to-CH3OH Hydrogenation” Scott R. Docherty, Nat Phongprueksathat, Erwin Lam, Gina Noh, Olga V. Safonova, Atsushi Urakawa and Christophe Copéret JACS Au, vol. 2: no. 8, pp. 1946-1947, Washington, DC: American Chemical Society, 2022. DOI: 10.1021/jacsau.2c00421 call_made Elucidation of Metal Local Environments in Single-Atom Catalysts Based on Carbon Nitrides Simon Büchele, Alexander Yakimov, Sean M. Collins, Andrea Ruiz-Ferrando, Zupeng Chen, Elena Willinger, Demie M. Kepaptsoglou, Quentin M. Ramasse, Christoph R. Müller, Olga V. Safonova, Núria López, Christophe Copéret, Javier Pérez-Ramírez and Sharon Mitchell Small, vol. 18: no. 33, pp. 2202080, Weinheim: Wiley-VCH, 2022. DOI: 10.1002/smll.202202080 call_made Cationic molybdenum oxo alkylidenes stabilized by N-heterocyclic carbenes: from molecular systems to efficient supported metathesis catalysts Janis V. Musso, Jordan De Jesus Silva, Mathis J. Benedikter, Jonas Groos, Wolfgang Frey, Christophe Copéret and Michael R. Buchmeiser Chemical Science, vol. 13: no. 29, pp. 8649-8656, Cambridge: Royal Society of Chemistry, 2022. DOI: 10.1039/d2sc03321f call_made Molecular and Electronic Structure of Isolated Platinum Sites Enabled by the Expedient Measurement of 195Pt Chemical Shift Anisotropy Amrit Venkatesh, Domenico Gioffrè, Benjamin A. Atterberry, Lukas Rochlitz, Scott L. Carnahan, Zhuoran Wang, Georges Menzildjian, Anne Lesage, Christophe Copéret and Aaron J. Rossini Journal of the American Chemical Society, vol. 144: no. 30, pp. 13511-13525, Washington, DC: American Chemical Society, 2022. DOI: 10.1021/jacs.2c02300 call_made A Robust and Efficient Propane Dehydrogenation Catalyst from Unexpectedly Segregated Pt2Mn Nanoparticles Lukas Rochlitz, Quentin Pessemesse, Jorg W. A. Fischer, Daniel Klose, Adam H. Clark, Milivoj Plodinec, Gunnar Jeschke, Pierre-Adrien Payard and Christophe Copéret Journal of the American Chemical Society, vol. 144: no. 29, pp. 13384-13393, Washington, DC: American Chemical Society, 2022. DOI: 10.1021/jacs.2c05618 call_made Porous polyisothiocyanurates for selective palladium recovery and heterogeneous catalysis Kyung Seob Song, Timur Ashirov, Siddulu Naidu Talapaneni, Adam Hugh Clark, Alexander V. Yakimov, Maarten Nachtegaal, Christophe Copéret and Ali Coskun Chem, vol. 8: no. 7, pp. 2043-2059, Philadelphia, PA: Elsevier, 2022. DOI: 10.1016/j.chempr.2022.05.009 call_made Single-Site Iridium Picolinamide Catalyst Immobilized onto Silica for the Hydrogenation of CO2 and the Dehydrogenation of Formic Acid Leonardo Tensi, Alexander V. Yakimov, Caterina Trotta, Chiara Domestici, Jordan De Jesus Silva, Scott R. Docherty, Cristiano Zuccaccia, Christophe Copéret and Alceo Macchioni Inorganic Chemistry, vol. 61: no. 27, pp. 10575-10586, Washington, DC: American Chemical Society, 2022. DOI: 10.1021/acs.inorgchem.2c01640 call_made Atomic-scale changes of silica-supported catalysts with nanocrystalline or amorphous gallia phases: implications of hydrogen pretreatment on their selectivity for propane dehydrogenation Pedro Castro-Fernández, Alexander I. Serykh, Alexander V. Yakimov, Igor P. Prosvirin, Andrey V. Bukhtiyarov, Paula M. Abdala, Christophe Copéret, Alexey Fedorov and Christoph R. Müller Catalysis Science & Technology, vol. 12: no. 12, pp. 3957-3968, Cambridge: Royal Society of Chemistry, 2022. DOI: 10.1039/d2cy00074a call_made Multiple Surface Site Three-Dimensional Structure Determination of a Supported Molecular Catalyst Ribal Jabbour, Marc Renom-Carrasco, Ka Wing Chan, Laura A. Völker, Pierrick Berruyer, Zhuoran Wang, Cory M. Widdifield, Moreno Lelli, David Gajan, Christophe Copéret, Chloé Thieuleux and Anne Lesage Journal of the American Chemical Society, vol. 144: no. 23, pp. 10270-10281, Washington, DC: American Chemical Society, 2022. DOI: 10.1021/jacs.2c01013 Structure and Framework Association of Lewis Acid Sites in MOR Zeolite Alexander V. Yakimov, Manoj Ravi, René Verel, Vitaly L. Sushkevich, Jeroen A. van Bokhoven and Christophe Copéret Journal of the American Chemical Society, vol. 144: no. 23, pp. 10377-10385, Washington, DC: American Chemical Society, 2022. DOI: 10.1021/jacs.2c02212 call_made An Anionic Dinuclear Ruthenium Dihydrogen Complex of Relevance for Alkyne gem-Hydrogenation Tobias Biberger, Nils Nöthling, Markus Leutzsch, Christopher P. Gordon, Christophe Copéret and Alois Fürstner Angewandte Chemie. International Edition, vol. 61: no. 24, pp. e202201311, Weinheim: Wiley, 2022. DOI: 10.1002/anie.202201311 call_made Ethylene-to-propene (ETP) conversion over Ni(II) single sites on tailored silica-alumina supports Zixuan Chen, Scott Docherty, Christophe Copéret, Alexey Fedorov and Christoph R. Müller Online Abstracts: 27th North American Catalysis Society Meeting, s.l.: North American Catalysis Society, 2022. DNP NMR spectroscopy enabled direct characterization of polystyrene-supported catalyst species for synthesis of glycidyl esters by transesterification Shinji Tanaka, Yumiko Nakajima, Atsuko Ogawa, Takashi Kuragano, Yoshihiro Kon, Masanori Tamura, Kazuhiko Sato and Christophe Copéret Chemical Science, vol. 13: no. 16, pp. 4490-4497, Cambridge: Royal Society of Chemistry, 2022. DOI: 10.1039/d2sc00274d call_made HTE and Data Analysis for Discovery and Molecular-level Understanding of Catalysts Jordan De Jesus Silva and Christophe Copéret SCS Fall Meeting 2021, Online, pp.346-349, Bern: Schweizerische Chemische Gesellschaft, September 10, 2021. DOI: 10.2533/chimia.2022.346 call_made Olefin Metathesis Catalysts Generated In Situ from Molybdenum(VI)-Oxo Complexes by Tuning Pendant Ligands Darryl F. Nater, Christoph J. Kaul, Lukas Lätsch, Hayato Tsurugi, Kazushi Mashima and Christophe Copéret Chemistry - A European Journal, vol. 28: no. 22, pp. e202200559, Weinheim: Wiley-VCH, 2022. DOI: 10.1002/chem.202200559 call_made Revisiting Edge Sites of γ-Al2O3 Using Needle-Shaped Nanocrystals and Recoupling-Time-Encoded {27Al}-1H D-HMQC NMR Spectroscopy Laura A. Völker, Jordan Meyet, Zachariah J. Berkson, Lukas Rochlitz, Jeroen A. van Bokhoven and Christophe Copéret The Journal of Physical Chemistry C, vol. 126: no. 14, pp. 6351-6360, Washington, DC: American Chemical Society, 2022. DOI: 10.1021/acs.jpcc.2c00979 call_made Bulk and surface transformations of Ga2O3 nanoparticle catalysts for propane dehydrogenation induced by a H2 treatment Pedro Castro-Fernández, Deni Mance, Chong Liu, Paula Macarena Abdala, Elena Willinger, Aurelio A. Rossinelli, Alexander I. Serykh, Evgeny A. Pidko, Christophe Copéret, Alexey Fedorov and Christoph R. Müller Journal of Catalysis, vol. 408, pp. 155-164, San Diego, CA: Elsevier, 2022. DOI: 10.1016/j.jcat.2022.02.025 call_made W-oxo Adamantylidenes: Stable Molecular Precursors for Efficient Silica-Supported Metathesis Catalysts Darryl Nater, Maxime Boudjelel, Lukas Lätsch, Richard R. Schrock and Christophe Copéret Helvetica Chimica Acta, vol. 105: no. 4, pp. e202200013, New York, NY: Wiley-VCH, 2022. DOI: 10.1002/hlca.202200013 call_made Olefin-Surface Interactions: A Key Activity Parameter in Silica-Supported Olefin Metathesis Catalysts Zachariah J. Berkson, Moritz Bernhardt, Simon Laurenz Schlapansky, Mathis J. Benedikter, Michael R. Buchmeiser, Gregory A. Price, Glenn J. Sunley and Christophe Copéret JACS Au, vol. 2: no. 3, pp. 777-786, Washington, DC: American Chemical Society, 2022. DOI: 10.1021/jacsau.2c00052 c