O'Hare, D.M. - University of Oxford - Department of Chemistry

个人简介

Professor Dermot O’Hare was born in Newry, Co Down and studied at Balliol College, Oxford University, where he obtained his B.Sc. in 1982 and his D. Phil in 1985, under the direction of Professor M.L.H Green. Subsequently, he was awarded a Royal Commission of 1851 Research Fellowship. He was a visiting research fellow at CR&D E.I. du Pont deNemours in Wilmington, Delaware in 1986/7 were he worked in the group lead by Prof J.S. Miller on molecular-based magnetic materials. In 1987 he returned to Oxford to a short term lectureship and in 1990 he was appointed to a permanent University position and a Septcentenary Tutorial Fellowship at Balliol College. In 1996 he was honoured by the Institüt de France, Académie des Sciences as one of the top 50 leading scientists in Europe under 40 yrs. He was the Royal Society of Chemistry Sir Edward Frankland Fellow in 1996/97. In 1997 he was awarded the Exxon European Chemical and Engineering Prize. In 1998 he became Professor. His interests are wide ranging, and include exploratory synthetic organometallic chemistry, intercalation chemistry, time-resolved, in situ diffraction studies and the synthesis of meso- and microporous solids. In 2010 he won the Royal Society of Chemistry’s Ludwig Mond award for outstanding research in Inorganic chemistry. In 2012, following the establishment of a mutually successful relationship with SCG Chemicals Co. Ltd, Dermot was instrumental in creating the SCG-Oxford Centre of Excellence for Chemistry (CoE) on which he serves as the Director. This is a unique collaboration between SCG and the University of Oxford with dedicated laboratories in the Department of Chemistry focusing on the research and development in the area of Nanomaterials and catalysis. It currently includes employs forty-five people, who work on 44 projects with total committed funds of over £10 million. The establishment of the CoE itself has strengthened scientific and commercial ties between the UK and Thailand leading to Professor Dermot O’Hare and SCG's presentation to HRH Princess Sirindhorn at the British Embassy, Bangkok in 2016, which was a tremendous honor. Also in recognition of the creation of the CoE he received an Impact Award from the University of Oxford. In 2016 he was awarded the RSC Tilden for his creative work on the synthesis, reactivity and advanced characterisation of molecular inorganic compounds and materials spanning organometallic chemistry to framework and layered materials.

研究领域

The O'Hare group's research interests covers a wide range of areas including novel ligand synthesis, transition metal organometallic chemistry and the synthesis of novel frustrated Lewis pair systems looking towards the activation of small molecules. We are also looking at the development of controlled synthesis of novel Layered Double Hydroxides (LDHs) and hybrid materials and their applications in catalysis and renewable feedstocks. Organometallics Frustrated Lewis Pairs (FLPs) Layered Double Hydroxides (LDHs) In-situ diffraction studies Heterogeneous catalysis

近期论文

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Molten salts−modified MgO−based adsorbents for intermediate-temperature CO2 capture: A review, Wanlin Gao, Tuantuan Zhou, Yanshan Gao, Benoît Louis, Dermot O’Hare, Qiang Wang, J. Energy Chem., (2017) on line. DOI: 10.1016/j.jechem.2017.06.005 The synthesis of CuyMnzAl1-zOx mixed oxide as low-temperature NH3-SCR catalyst with enhanced catalytic performance, Q. Yan, S. Chen, L. Qiu, Y. Gao, D. O’Hare, Q. Wang, Dalton Trans., (2017), on line. DOI: 10.1039/C7DT02000G Preparation of Two Dimensional Layered Double Hydroxides Nanosheets and Their Applications, J. Yu, Q. Wang, L. Sun, Chem. Soc. Rev., (2017), on line. Fabrication of Lithium Silicates As Highly Efficient High-Temperature CO2 Sorbents from SBA-15 Precursor Y. Pan, Y. Zhang, T. Zhou,B. Louis, D. O'Hare, Q. Wang, Inorg. Chem., (2017), 56, 7821-7834. DOI: 10.1021/acs.inorgchem.7b00559 Controlling the Surface Hydroxyl Concentration by Thermal Treatment of Layered Double Hydroxides C. M. R. Wright, K. Ruengkajorn, A. F. R. Kilpatrick, J.-C. Buffet, D. O'Hare, Dermot Inorg. Chem., (2017), 56, 7842-7850. DOI: 10.1021/acs.inorgchem.7b00582 Design of highly efficient NOx storage-reduction catalysts from layered double hydroxides for NOx emission control from naphtha cracker flue gases R. Yang, Y. Cui, Q. Yan, C. Zhang, L. Qiu, D. O'Hare, Q. Wang, Chem. Eng. J., (2017), 326, 656-666. DOI: 10.1016/j.cej.2017.06.016 High energy x-rays for following metal-organic framework formation: Identifying intermediates in interpenetrated MOF-5 crystallisation Y. Wu, M. I. Breeze, D. O'Hare, R. I. Walton, Microporous and Mesoporous Materials, (2017). DOI: 10.1016/j.micromeso.2017.04.043 Selective ethylene oligomerisation using supported tungsten mono-imido catalysts C. M. R. Wright, T. J. Williams, Z. R. Turner, J.-C. Buffet, D. O'Hare, Inorg. Chem. Front., (2017), 4, 1048-1060. DOI: 10.1039/c7qi00128b CuTi LDH derived NH3-SCR catalysts with highly dispersed CuO active phase and improved SO2 resistance Y. Nie, Q. Yan, S. Chen, D. O'Hare, Q. Wang, Cat. Commun. ,(2017), 97, 47-50. DOI: 10.1016/j.catcom.2017.04.014 Delaminated layered double hydroxide delivers DNA molecules as sandwich nanostructure into cells via a non-endocytic pathway, Y. Li, W. Bao, H. Wu, J. Wang, Y. Zhang. Y. Wan, D. Cao, D. O’Hare, Q. Wang, Sci. Bull., (2017), 62, 686-692. DOI: 10.1016/j.scib.2017.04.004 Highly dispersed CuyAlOx mixed oxides as superior low-temperature alkali metal and SO2 resistant NH3-SCR catalysts Q. Yan, Y. Nie, R. Yang, Y. Cui, D. O'Hare, Q. Wang, App. Cat. A, (2017), 538, 37-50. DOI: 10.1016/j.apcata.2017.03.021 Structural variety in ytterbium dicarboxylate frameworks and in situ study diffraction of their solvothermal crystallisation M. I. Breeze, T. W. Chamberlain, G. J. Clarkson, R. P. de Camargo, Y. Wu, Yue, J. F. de Lima, F. Millange, O. A. Serra, D. O'Hare, R. I. Walton, Cryst. Eng. Comm. ,(2017), 19, 2424-2433. DOI: 10.1039/C7CE00481H Bonding in Pentalene Complexes and Recent Applications, F.G.N. Cloke, J. C.Green, Alexander F. R. Kilpatrick, Dermot O’Hare, Coord. Chem. Rev., (2017). DOI: 10.1016/j.ccr.2016.12.006 Understanding Surface Interactions in Aqueous Miscible Organic Solvent Treated Layered Double Hydroxides, V. Erastova, M.T. Degiacomi, D. O’Hare, H.C. Greenwell, RSC Adv., (2017), 7, 5076-5083. DOI: 10.1039/C6RA26834J Time-Resolved In Situ X-ray Diffraction Reveals the Mechanisms of Molten Salt Synthesis, S. Moorhouse, Y. Wu, H. Buckley, D. O’Hare, Chem Comm., (2016), 13865 – 13868. DOI: 10.1039/c6cc08133a Layered double hydroxide-oxidized carbon nanotube hybrid as highly efficient flame retardant nanofillers for polypropylene, Y. Gao, Y. Zhang, G. Williams, D. O'Hare, Q. Wang, Scientific Reports, (2016), 6, 35502. DOI:10.1038/srep35502 Time-Resolved In Situ X-ray Diffraction Reveals Metal-Dependent Metal-Organic Framework Formation, Y. Wu, S. Henke, G. Kieslich, I. Schwedler, M. Yang, D.A.X. Fraser and D. O’Hare, Angew Chemie. Int Ed., (2016), 55(45), 14081–14084. DOI: 10.1002/anie.201608463 Synthesis and characterization of solid polymethylaluminoxane “sMAO”; a bifunctional activator and support for slurry-phase ethylene polymerization, A.F.R. Kilpatrick, J.-C. Buffet, S. Sripothongnak, P. Nørby, N.P. Funnell, and D. O’Hare, Chem Mater., (2016), 28(20), 7444-7450. DOI: 10.1021/acs.chemmater.6b03009 Simultaneous synchrotron X-ray diffraction – differential scanning calorimetry: A powerful technique for physical form characterisation in pharmaceutical materials, A. Clout, A.B.M. Buanz, T.J. Prior, C. Reinhard, Y. Wu, D. O’Hare, G.R. Williams and S. Gaisford, Anal. Chem., (2016), 88(20), 10111–10117. DOI: 10.1021/acs.analchem.6b02549 Polymethylaluminoxane supported zirconocene catalysts for polymerisation of ethylene, T.A.Q. Arnold, Z.R. Turner, J.-C. Buffet and D. O’Hare, J. Organomet. Chem., (2016), 822, 85-90. DOI: 10.1016/j.jorganchem.2016.08.015