个人简介
I received both my BSc (1992) and PhD (1995, supervised by Dr L.J. Yellowlees) at Edinburgh University. I then held post-doctoral positions with Drs F.E. Mabbs and D. Collison (Manchester, 1995-98) and with Profs. A.J. Thomson FRS and A.K. Powell (University of East Anglia, 1999) before returning to Manchester in 2000. I was promoted to a Chair of Inorganic Chemistry in 2007.
研究领域
Research interests in the Manchester Molecular Magnetism Group encompass synthetic coordination chemistry through to hard-core physical measurements on molecular magnetic materials. In particular we study d- and f-block coordination compounds where the paramagnetism gives rise to fascinating and potentially useful physical properties. The latter include magnetic memory effects ("single molecule magnets"), very large magnetocaloric effects which can be exploited for low temperature refrigeration, and materials that are potential elements in quantum information processing. We study the magnetic properties by magnetometry and EPR spectroscopic methods and collaborate widely with world-class physicists for further characterisation and exploitation.
I am Co-Director (with Prof David Collison) of the EPSRC-funded UK National EPR Facility and Service, which offers facilities and expertise for c.w. EPR at L, S, X, K, Q and W-band and pulsed EPR at S, X and Q-band to UK academics.
近期论文
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Cleaves P, King D, Kefalidis C, Maron L, Tuna F, McInnes E, McMaster J, Lewis W, Blake A, Liddle S. Two-Electron Reductive Carbonylation of Terminal Uranium(V) and Uranium(VI) Nitrides to Cyanate by Carbon Monoxide. Angewandte Chemie-International Edition. 2014; 53(39): 10412-10415. eScholarID:242055 | DOI:10.1002/anie.201406203
Gardner B, Balazs G, Scheer M, Tuna F, McInnes E, McMaster J, Lewis W, Blake A, Liddle S. Triamidoamine-Uranium( IV)-Stabilized Terminal Parent Phosphide and Phosphinidene Complexes**. Angewandte Chemie-International Edition. 2014; 53(17): 4484-4488. eScholarID:242057 | DOI:10.1002/anie.201400798
Garlatti E, Albring M, Baker M, Docherty R, Mutka H, Guidi T, Sakai V, Whitehead G, Pritchard R, Timco G, Tuna F, Amoretti G, Carretta S, Santini P, Lorusso G, Affronte M, McInnes E, Collison D, Winpenny R. A Detailed Study of the Magnetism of Chiral {Cr7M} Rings: An Investigation into Parametrization and Transferability of Parameters. Journal of the American Chemical Society. 2014; 136(27): 9763-9772. eScholarID:242041 | DOI:10.1021/ja5047445
Goodwin C, Tuna F, McInnes E, Liddle S, McMaster J, Vitorica-Yrezabal I, Mills D. U-III{N(SiMe(2)tBu)(2)}(3) : A Structurally Authenticated Trigonal Planar Actinide Complex. Chemistry-a European Journal. 2014; 20(45): 14579-14583. eScholarID:242054 | DOI:10.1002/chem.201404864
King D, McMaster J, Tuna F, McInnes E, Lewis W, Blake A, Liddle S. Synthesis and Characterization of an f-Block Terminal Parent Imido U=NH Complex: A Masked Uranium(IV) Nitride. Journal of the American Chemical Society. 2014; 136(15): 5619-5622. eScholarID:242050 | DOI:10.1021/ja502405e
Loughrey J, Sproules S, McInnes E, Hardie M, Halcrow M. Stable Mixed-Valent Radicals from Platinum( II) Complexes of a Bis( dioxolene) Ligand. Chemistry-a European Journal. 2014; 20(21): 6272-6276. eScholarID:242051 | DOI:10.1002/chem.201304848
Lu E, Cooper O, McMaster J, Tuna F, McInnes E, Lewis W, Blake A, Liddle S. Synthesis, Characterization, and Reactivity of a Uranium(VI) Carbene Imido Oxo Complex. Angewandte Chemie-International Edition. 2014; 53(26): 6696-6700. eScholarID:242048 | DOI:10.1002/anie.201403892
Magee S, Sproules S, Barra A, Timco G, Chilton N, Collison D, Winpenny R, McInnes E. Large Zero-Field Splittings of the Ground Spin State Arising from Antisymmetric Exchange Effects in Heterometallic Triangles. Angewandte Chemie-International Edition. 2014; 53(21): 5310-5313. eScholarID:242042 | DOI:10.1002/anie.201400655
Moreno Pineda E, Chilton N, Marx R, Dorfel M, Sells D, Neugebauer P, Jiang S, Collison D, van Slageren J, McInnes E, Winpenny R. Direct measurement of dysprosium(III)˙˙˙dysprosium(III) interactions in a single-molecule magnet. Nature communications. 2014; 5: 5243-5243. eScholarID:242043 | DOI:10.1038/ncomms6243
Moro F, de Miguel R, Jenkins M, Gomez-Moreno C, Sells D, Tuna F, McInnes E, Lostao A, Luis F, van Slageren J. Magnetic anisotropy of polycrystalline magnetoferritin investigated by SQUID and electron magnetic resonance. Journal of Magnetism and Magnetic Materials. 2014; 361: 188-196. eScholarID:242046 | DOI:10.1016/j.jmmm.2014.02.053
Moro F, Kaminski D, Tuna F, Whitehead G, Timco G, Collison D, Winpenny R, Ardavan A, McInnes E. Coherent electron spin manipulation in a dilute oriented ensemble of molecular nanomagnets: pulsed EPR on doped single crystals. Chemical Communications. 2014; 50(1): 91-93. eScholarID:242037 | DOI:10.1039/c3cc46326e
Pascu G, Deville C, Clifford S, Guenee L, Besnard C, Kraemer K, Liu S, Decurtins S, Tuna F, McInnes E, Winpenny R, Williams A. The coordination chemistry of tartronic acid with copper: magnetic studies of a quasi-equilateral tricopper triangle. Dalton Transactions. 2014; 43(2): 656-662. eScholarID:242053 | DOI:10.1039/c3dt51838h
Pineda E, Tuna F, Zheng Y, Teat S, Winpenny R, Schnack J, McInnes E. Iron Lanthanide Phosphonate Clusters: {Fe(6)Ln(6)P(6)} Wells-Dawson-like Structures with D-3d Symmetry. Inorganic Chemistry. 2014; 53(6): 3032-3038. eScholarID:242045 | DOI:10.1021/ic402839q
Sharples J, Collison D, McInnes E, Schnack J, Palacios E, Evangelisti M. Quantum signatures of a molecular nanomagnet in direct magnetocaloric measurements. Nature Communications. 2014; 5: eScholarID:242052 | DOI:10.1038/ncomms6321
Upadhyay A, Komatireddy N, Ghirri A, Tuna F, Langley S, Srivastava A, Sanudo E, Moubaraki B, Murray K, McInnes E, Affronte M, Shanmugam M. Synthesis and magnetothermal properties of a ferromagnetically coupled Ni-II-Gd-III-Ni-II cluster. Dalton Transactions. 2014; 43(1): 259-266. eScholarID:242049 | DOI:10.1039/c3dt52384e
Walsh J, Sproules S, Chilton N, Barra A, Timco G, Collison D, McInnes E, Winpenny R. On the Possibility of Magneto-Structural Correlations: Detailed Studies of Dinickel Carboxylate Complexes. Inorganic Chemistry. 2014; 53(16): 8464-8472. eScholarID:242047 | DOI:10.1021/ic501036h
Zangana K, Pineda E, McInnes E, Schnack J, Winpenny R. Centred nine-metal rings of lanthanides. Chemical Communications. 2014; 50(12): 1438-1440. eScholarID:242036 | DOI:10.1039/c3cc48708c
Zangana K, Pineda E, Vitorica-Yrezabal I, McInnes E, Winpenny R. Linking Cr-3 triangles through phosphonates and lanthanides: synthetic, structural, magnetic and EPR studies. Dalton Transactions. 2014; 43(35): 13242-13249. eScholarID:242044 | DOI:10.1039/c4dt01264j