尚进 - 香港城市大学 - 能源与环境学院

个人简介

Dr. Jin Shang obtained his Bachelor (2007) and Master (2009) degrees both in Environmental Engineering at Northeastern University in China. He completed his PhD in Chemical Engineering at the University of Melbourne in 2013. His PhD thesis was on the separation of carbon dioxide from flue gas and natural gas streams using porous adsorbent materials. The study discovered a new separation mechanism (i.e., molecular trapdoor mechanism) which changed the conventional understanding of how these adsorbents discriminate between molecules in gases. After his PhD, he worked as research fellow on an Australian Research Council Discovery Project focusing on developing advanced adsorbents in Paul Webley Group at the University of Melbourne. Since 2015, as Co-chief Investigator of Australian Research Council Training Centre for Liquefied Natural Gas Futures, he has been actively participated in research along with major industry partners in oil and gas field. He then moved to Georgia Institute of Technology and worked as a postdoctoral fellow funded by ExxonMobil focusing on restricted gas diffusion in zeolites by advanced molecular simulation in David Sholl Group, prior to joining the City University of Hong Kong as an assistant professor in the School of Energy and Environment in September 2016.

研究领域

Molecular separation plays a key role in energy and environmental technologies. Notable examples are H2 and CH4 purifications, CO2 capture, volatile organic compounds (VOCs) removal, CO removal for fuel cell technology, flue gas purification, desulfurization of natural gas and transported fuels etc. Molecular separation is an important unit operation in chemical industry, accounting for more than 60% of the total cost in some processes. Of the adsorption-based molecular separations, molecular sieving is the most desirable separation mechanism because it affords unparalleled high-selectivity. Our research focus is on investigating and understanding the fundamental physical chemistry of gas adsorption and diffusion behaviour, using combined experimental and computational approaches to rationally design and synthesize “active” porous materials for gas separation and storage in environmental and energy applications. Some advanced experimental techniques applied include multiple component breakthrough and in situ synchrotron Powder X-ray Diffraction/Neutron Powder Diffraction/X-ray Absorption Spectroscopy of adsorption; some advanced computational techniques include ab initio density functional theory (DFT) and force field molecular simulations. We have broad interests in materials design and synthesis, particularly the study and design of stimuli responsive porous adsorbents to achieve controlled selective guest admission into host adsorbents through “smart” pore apertures. The stimuli can be guest molecules, temperature, pressure, light, electric field, etc

近期论文

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Wang, T., Wang, Y., Sun, M., Hanif, A., Wu, H., Gu, Q., Ok, Y. S., Tsang, D. C. W., Li, J., Yu, J., Shang, J.* “Thermally Treated Zeolitic Imidazolate Framework-8 (ZIF-8) for Visible Light Photocatalytic Degradation of Gaseous Formaldehyde”, Chemical Science 2020, in press. Wang, Z., Goyal, N., Liu, L., Tsang, D.C.W., Shang J., Liu, W., Li, G. “N-doped porous carbon derived from polypyrrole for CO2 capture from humid flue gases”, Chemical Engineering Journal 2020, 396, 125376. Chen, S. S., Cao, Y., Tsang, D. C. W., Tessonnier, J.-P., Shang, J., Hou, D., Shen, Z., Zhang, S., Ok, Y. S., Wu, K. C. W. “Effective Dispersion of MgO Nanostructure on Biochar Support as a Basic Catalyst for Glucose Isomerization”, ACS Sustainable Chemistry & Engineering 2020, 8 (18), 6990-7001. Cao, L., Yu, I. K. M., Xiong, X., Tsang, D. C. W., Zhang, S., Clark, J. H., Hu, C., Ng, Y. H., Shang, J., Ok, Y. S. “Biorenewable hydrogen production through biomass gasification: A review and future prospects”, Environmental Research 2020, 186, 109547. Shang, J.,* Hanif, A., Li, G., Xiao, G., Liu, J. Z., Xiao, P., Webley, P. A. “Separation of CO2 and CH4 by Pressure Swing Adsorption Using a Molecular Trapdoor Chabazite Adsorbent for Natural Gas Purification”, Industrial & Engineering Chemistry Research 2020, 59 (16), 7857-7865. Shang, S., Tao, Z., Yang, C., Hanif, A., Li, L., Tsang, D. C. W., Gu, Q., Shang, J.* “Facile synthesis of CuBTC and its graphene oxide composites as efficient adsorbents for CO2 capture”, Chemical Engineering Journal 2020, 393, 124666. Tian, M., Liu, S. J., Wang, L., Ding, H.,* Zhao, D., Wang, Y., Cui, J., Fu, J., Shang, J.,* Li, G. K.,* “Complete Degradation of Gaseous Methanol over Pt/FeOx Catalysts by Normal Temperature Catalytic Ozonation (NTCO)”, Environmental Science & Technology 2020, 54(3) 1938-1945. Xiao, K.M., Wang, T.Q., Sun, M.Z., Hanif, A., Gu, Q.F., Tian, B.B., Jiang, Z.F., Wang. B., Sun, H.L., Shang, J.,* Wong, P.K.,* “Photocatalytic Bacterial Inactivation by a Rape Pollen-MoS2 Biohybrid Catalyst: Synergetic Effects and Inactivation Mechanisms”, Environmental Science & Technology 2020, 54(1) 537-549. Li, B., Zheng, T., Ran, S., Sun, M., Shang, J., Hu, H., Lee, P.-H., Boles, S. T., “Performance recovery in degraded carbon-based electrodes for capacitive deionization”, Environmental Science & Technology 2020, 54(3), 1848-1856. Kumar, P., Kim, K.H., Lee, J., Shang, J., Khazi, M.I., Kumar, N., Lisak, G., “Metal-organic framework for sorptive/catalytic removal and sensing applications against nitroaromatic compounds”, Journal of Industrial and Engineering Chemistry 2020, 84, 87-95. Yu, I.K.M., Hanif, A., Tsang, D.C.W.,* Yip, A.C.K., Lin, K.Y.A., Gao, B., Ok, Y.S., Poon, C.S., Shang, J.,* “Tailoring Acidity and Porosity of Alumina Catalysts via Transition Metal Doping for Glucose Conversion in Biorefinery”, Science of The Total Environment 2020, 704, 135414. Yu, I.K.M., Hanif, A., Tsang, D.C.W.*, Shang, J.*, Su, Z.; Song, H., Ok, Y.S., Poon, C.S., “Tuneable functionalities in layered double hydroxide catalysts for thermochemical conversion of biomass-derived glucose to fructose”, Chemical Engineering Journal, 2020, 383, 122914. Igalavithana, A. D., Wan Choi, S., Dissanayake, P. D., Shang, J., Wang, C.-H., Yang, X., Kim, S., Tsang, D. C. W., Lee, K. B., Ok, Y. S., “Gasification biochar from biowaste (food waste and wood waste) for effective CO2 adsorption”, Journal of Hazardous Materials 2020, 39,121147. Vikrant, K., Kim, K.H.,* Szulejko, J. E., Boukhvalov, D., Shang J., Rinklebe, J., “Evidence of inter-species swing adsorption between aromatic hydrocarbons”, Environmental Research 2020, 181, 108814. Xiang, H., Ameen, A., Shang, J., Jiao, Y., Gorgojo, P., Siperstein, F. R., Fan, X., “Synthesis and modification of moisture-stable coordination pillared-layer metal-organic framework (CPL-MOF) CPL-2 for ethylene/ethane separation”, Microporous and Mesoporous Materials 2019, 293, 109784. Hanif, A., Sun, M., Tao, Z., Liu, L., Tsang, D. C. W., Gu, Q.,* Shang, J.,* “Silica Supported MgO as An Adsorbent for Pre-combustion CO2 Capture”, ACS Applied Nano Materials 2019, 2(10), 6565-6574. Tian, Y., Liang, G., Fan, T., Shang, J., Shang, S., Ma, Y., Matsuda, R., Liu, M., Wang, M., Li, L., Kitagawa, S., “Grafting free carboxylic acid groups onto pore surface of 3D porous coordination polymers for high proton conductivity”, Chemistry of Materials 2019, 31(20), 8494-8503. Iacomi, P., Formalik, F., Marreiros, J., Shang, J., Rogacka, J., Mohmeyer, A., Behrens, P., Ameloot, R., Kuchta, B., Llewellyn, P. L., “Role of structural defects in the adsorption and separation of C3 hydrocarbons in Zr-fumarate-MOF (MOF-801)”, Chemistry of Materials 2019, 31(20), 8413-8423. He, Y., Sun, M., Zhao, Q., Shang, J.,* Tian, Y., Xiao, P., Gu, Q.,* Li, L., Webley, P. A., “Effective Gas Separation Performance Enhancement Obtained by Constructing Polymorphous Core-Shell Metal-Organic Frameworks”, ACS Applied Materials & Interfaces 2019, 11(33), 30234-30239. Wang, S., Bai, P., Sun, M., Liu, W., Li, D., Wu, W., Yan, W., Shang, J.,* Yu, J.*, “Fabricating Mechanically Robust Binder-Free Structured Zeolites by 3D Printing Coupled with Zeolite Soldering: A Superior Configuration for CO2 Capture”, Advanced Science, 2019, 6(17), 1901317.