个人简介
Education
09/1984-06/1988 B.S. in Physical Chemistry, Department of Chemistry, Chengdu University of Science and Technology (now Sichuan University), P. R. China
09/1988 -06/1991 M.S. in Nuclear Magnetic Resonance, Wuhan Institute of Physics, CAS (supervisor: Prof. Youru Du)
09/1993 - 06/1996 Ph.D in Nuclear Magnetic Resonance, Wuhan Institute of Physics, CAS (supervisor: Prof. Chaohui Ye and Prof. Youru Du)
Postdoctoral Training
10/1997-12/1998 Research Fellow, Chemistry Department, Texas A & M University, USA (with Prof. James F. Haw; In-situ solid-state NMR studies of heterogeneous catalytic reactions on zeolites)
Faculty Academic Appointments
07/1991-05/1993 Research assistant, Wuhan Institute of Physics, CAS
06/1993-06/1996 Assistant professor, Wuhan Institute of Physics, CAS
07/1996-11/1999 Associate professor, Wuhan Institute of Physics and Mathematics, CAS
12/1999-present Professor, Wuhan Institute of Physics and Mathematics, CAS; Group Leader of Solid-state NMR Spectroscopy and Heterogeneous Catalysis
09/2008-present Vice director of National Centre for Magnetic Resonance in Wuhan
04/2005-11/2016 Vice director of State Key Laboratory of Magnetic Resonance and Atomic and Molecular Physics
12/2016-present Director of State Key Laboratory of Magnetic Resonance and Atomic and Molecular Physics
近期论文
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Wang, C.; Chu, Y.Y.; Hu, M.; Cai, W.J.; Wang, Q.; Qi, G.D.; Li, S.H.; Xu, J.* ; Deng, F. Insight into carbocation induced non-covalent interactions in methanol-to-olefins reaction over ZSM-5 zeolite from solid-state NMR spectroscopy Angew. Chem. Int. Ed. 2021, DOI:10.1002/anie.202112948.
Wang, C ; Zhao, X.L.; Hu, M.; Qi, G.D.; Wang, Q.; Li, S.H.; Xu, J. * ; Deng, F. Unraveling hydrocarbon pool boosted propane aromatization on gallium/ZSM-5 zeolite by solid-state NMR spectroscopy Angew. Chem. Int. Ed. 2021, 60, 23630-23634.
Gao, W.; Qi, G.D.; Wang, Q.; Wang, W.Y.; Li, S.H.; Hung, I.; Gan, Z.H.; Xu, J. * ; Deng, F. Dual active sites on molybdenum/ZSM-5 catalyst for methane dehydroaromatization: insights From solid-state NMR spectroscopy Angew. Chem. Int. Ed. 2021, 60: 10709-10715.
Qi, G.D.; Wang, Q.; Xu, J. * ; Deng, F. Solid-state NMR studies of internuclear correlations for characterizing catalytic materials Chem. Soc. Rev. 2021, 50: 8382-8399.
Zheng, M.J.; Xin, S.H.; Wang, Q.* ; Trebosc, J.; Xu, J.; Qi, G.D.; Feng, N.D.; Lafon, O.* ;Deng, F.* Through-space 11B27Al correlation: influence of the recoupling channel Magn. Reson. Chem. 2021, 59:1062-1076.
Xiao, Y.Q.; Chu, Y.Y.; Li, S.H. * ; Chen, F.; Gao, W.; Xu, J.; Deng, F. * Host-guest interaction in ethylene and ethane separation on zeolitic imidazolate frameworks as revealed by solid-state NMR spectroscopy Chem. Eur. J. 2021, 27: 11303-11308.
Tang, J.; Chu, Y.Y.; Li, S.H. * ; Xu, J.; Xiong, W.P.; Wang, Q.; Deng, F. * Breathing effect via solvent inclusions on the linker rotational dynamics of functionalized MIL-53 Chem. Eur.J. 2021, 27: 14711-14720.
Wang, Y.X.; Xin, S.H.; Chu, Y.Y. * ; Xu, J.; Qi, G.D.; Wang, Q. * ; Xia, Q.H.; Deng, F. * Influence of trimethylphosphine oxide loading on the measurement of zeolite acidity by solidstate NMR spectroscopy J. Phys. Chem. C 2021, 125:9497-9506.
Wang, W.Y.; Wang, Q.; Chu, Y.Y.; Qi, G.D.; Li, S.H.; Xu, J. * ; Deng, F. Pairwise stereoselective hydrogenation of propyne on supported Pd-Ag catalysts investigated by parahydrogen-induced polarization J. Phys. Chem. C 2021, 125:17144-17154.
Qi, G.D.; Ye, X.D.; Xu, J. * ; Deng, F. * Progress in NMR studies of carbohydrates conversion on zeolites Chem. J. Chinese Universities-Chinese 2021, 42:148-164.
Feng, N.D. * ; Lin, H.W.; Song, H.; Yang, L.X.; Tang, D.M.; Deng, F.; Ye, J.H. * Efficient and selective photocatalytic CH4 conversion to CH3OH with O2 by controlling overoxidation on TiO2 Nat. Commun. 2021, 12: 4652.
Yang, L.; Wang, C.; Zhang, L.N.; Dai, W.L. * ; Chu, Y.Y.; Xu, J.; Wu, G.J.; Gao, M.B.; Liu, W.J.; Xu, Z.C.; Wang, P.F.; Guan, N.J.; Dyballa, M.; Ye, M.; Deng, F.; Fan, W.B.; Li, L.D. Stabilizing the framework of SAPO-34 zeolite toward long-term methanol-to-olefins conversion Nat. Commun. 2021, 12: 4661
Feng, N.D.; Lin, H.W.; Deng, F.; Ye, J.H. * Interfacial-bonding Ti-N-C boosts efficient photocatalytic H2 evolution in close coupling g-C3N4/TiO2 J. Phys. Chem. C 2021, 125:12012-12018.
Wang, Q.; Li, W.Z.; Hung, I.; Mentink-Vigier, F.; Wang, X.L.; Qi, G.D.; Wang, X.; Gan, Z.H.; Xu, J.* ; Deng, F. Mapping the oxygen structure of γ-Al2O3 by high field solid-state NMR spectroscopy Nat. Commun. 2020, 11:3620.
Wang, C.; Hu, M. ; Chu, Y.Y.; Zhou, X. ; Wang, Q.; Qi, G.; Li, S.H.; Xu, J. * ; Deng, F.-interaction between cyclic carbocations and aromatics causes zeolite deactivation in methanol-to-hydrocarbons conversion Angew. Chem. Int. Ed. 2020, 59:7198-7202.
Qi, G.D.; Chu,Y.Y.; Wang, Q.; Wang, X.X.; Li, Y.; Trebosc, J.; Lafon, O.; Xu, J* ; Deng, F. gem-diol-type intermediate in the activation of a ketone on Sn- zeolite as studied by solidstate NMR spectroscopy Angew. Chem. Int. Ed. 2020, 59:19532-19538.
Yan,W.; Li, S.H.* ; Yang,T.; Xia, Y.C.; Zhang, X.R.; Wang, C.; Yan, Z.; Deng, F. * ; Zhou, Q.H.; Deng, H.X.* Molecular vises for precisely positioning ligands near catalytic metal centers in metal-organic frameworks J. Am. Chem. Soc. 2020, 142:16182-16187.
Li, S. H.; Lafon, O.; Wang, W.Y.; Wang, Q,; Wang, X.X.; Li, Y.; Xu, J.* ; Deng, F. Recent advances of solid-state NMR spectroscopy for microporous materials Adv. Mater.2020, 32, 2002879.
Hu, M.; Wang, C.; Gao, X.Z.; Chu, Y.Y. ; Qi, G.D.; Wang, Q.; Xu, G.T.; Xu, J.* ; Deng F.* Establishing a link between the dual cycles in methanol-to-olefins conversion on HZSM-5: aromatization of cycloalkenes ACS Catal. 2020, 10:4299-4305.
Wang, C.; Xu J. * ; Deng, F.* The mechanism of methanol-to-hydrocarbon reactions over acidic zeolites: a solid-state NMR perspective ChemCatChem 2020, 12:965-980
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