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Rapid Construction of Polycyclic Skeletons via Brønsted Base-Catalyzed Annulations of Ethylidene 1,3-Indenediones and Vinyl 1,2-Diketones. Lixuan Zhu,§ Haotian Luo,§ Jinggong Liu,* Benlong Luo,* Shuang Yang, Xinqiang Fang,* Org. Lett. 2024, 10.1021/acs.orglett.4c01690.
Regio- and Stereoselective Transfer Hydrogenation of Aryloxy Group-Substituted Unsymmetrical 1,2-Diketones: Synthetic Applications and Mechanistic Studies. Wenjun Liu, Caiyi Ren, Liyuan Zhou, Haotian Luo, Xiangjian Meng, Peng Luo, Yingkun Luo, Wennan Dong, Shouang Lan, Jinggong Liu, Shuang Yang, Qi Zhang,* Xinqiang Fang,* J. Am. Chem. Soc. 2024, 10.1021/jacs.4c04171.
Catalytic Asymmetric Transfer Hydrogenation of Acylboronates: BMIDA as the Privileged Directing Group. Xiangjian Meng,§ Shouang Lan,§ Ting Chen, Haotian Luo, Lixuan Zhu, Nanchu Chen, Jinggong Liu, Shuang Yang, Andrej Emanuel Cotman, Qi Zhang,* Xinqiang Fang,* J. Am. Chem. Soc. 2024, 10.1021/jacs.4c05924.
Copper-catalyzed amine-mediated ynepropargylic substitution. Chunyun Jiang,§ Defu Luo,§ Xiangjian Meng, Qinqin Cui, Lili Zhao, Jinggong Liu,* Shuang Yang, Xinqiang Fang,* Org. Chem. Front. 2024, 11, 3946–3951.
Asymmetric Transfer Hydrogenation of Cyclobutenediones. Shouang Lan,§ Huangjiang Huang,§ Wenjun Liu, Chao Xu, Xiang Lei, Wennan Dong, Jinggong Liu, Shuang Yang, Andrej Emanuel Cotman, Qi Zhang,* and Xinqiang Fang,* J. Am. Chem. Soc. 2024, DOI: 10.1021/jacs.3c14239. (highlight: https://mp.weixin.qq.com/s/Cf-XheAGlA7KiIJqVy1xkw)
Kinetic Resolutions Enabled by N-Heterocyclic Carbene Catalysis: An Update. Shuang Yang*, Xinqiang Fang*, Chin. J. Org. Chem. 2024, DOI: 10.6023/cjoc202308023.
Transition-metal and base-free ether synthesis via alcohol-participated yne-allylic substitution. Chao Xu§, Yingkun Luo§, Shengtong Niu*, Fan Gong, Shouang Lan, Benlong Luo*, Jinggong Liu*, Shuang Yang, Xinqiang Fang*, Green Synth. Catal. 2024, DOI: 10.1016/j.gresc.2023.10.003
Copper-catalyzed Asymmetric Yne-allylic Substitution Using Electron-rich Arenes. Defu Luo§, Shengtong Niu§, Fan Gong, Chao Xu, Shouang Lan, Jinggong Liu*, Shuang Yang, Xinqiang Fang*, ACS Catal. 2024, 14, 2746–2757. (highlight: https://mp.weixin.qq.com/s/H-hNhsCvyTene8XnaydC0w )
Copper-catalyzed Umpolung Reactivity of Propargylic Carbonates in the Presence of Diboronates: One Stone Four Birds. Wennan Dong, Zhifei Zhao, Cheng-Zhi Gu*, Jing-Gong Liu, Shuang Yang, Xinqiang Fang*, J. Am. Chem. Soc. 2023, 145, 275395–27554. (highlight: https://mp.weixin.qq.com/s/hcabOgFBvztlHahP0b9kKg; https://mp.weixin.qq.com/s/AL1_iRMQbqpyoNJMz_bGVQ; https://mp.weixin.qq.com/s/J0PBtYRs9AnjwtgH-hk4Hg; https://mp.weixin.qq.com/s/rVHj1SoyR37F7ouZzgo_ig)
Carboxyl group assisted isodesmic meta-C–H iodination of phenethylamines, benzylamines, and 2-aryl anilines. Lei Yang, Lei Yang, Xinchao Wang, Meng Zhang, Shangda Li, Xinqiang Fang*, Gang Li *, Org. Chem. Front. 2023, 10, 3760–3765
Asymmetric Hydrogenation and Transfer Hydrogenation of Diketones. Shuang Yang, Xinqiang Fang*, Tetrahedron 2023, 145, 133609.
Copper-Catalysed Rearrangement of Cyclic Ethynylethylene Carbonates: Synthetic Applications and Mechanistic Studies, Chao Xu,§ Hao Zhang,§ Shouang Lan, Jinggong Liu, Shuang Yang, Qi Zhang,* Xinqiang Fang*, Angew. Chem. Int. Ed. 2023, e292219064. (highlight: https://mp.weixin.qq.com/s/hDLBalci4n-LIpm3jx0nhg; https://mp.weixin.qq.com/s/h1E-HKf6K0t-FrQjlG_qEA )
Dynamic Kinetic Resolution of β-Substituted α-Diketones via Asymmetric Transfer Hydrogenation, Ting Chen,§ Wenjun Liu,§ Wei Gu, Shengtong Niu, Shouang Lan, Zhifei Zhao, Fan Gong, Jinggong Liu, Shuang Yang, Andrej Emanuel Cotman, Jinshuai Song,* Xinqiang Fang*, J. Am. Chem. Soc. 2023, 145, 585–599. (highlight: https://mp.weixin.qq.com/s/aHyHQVVBAbssTksRPxqnzA)
Catalytic Synthesis of Seven-Membered Carbocycles via Ring Expansion of Cyclic β-Ketoesters, Li Chen,§ Huangjiang Huang,§ Benlong Luo,* Jinggong Liu,* Shuang Yang,* and Xinqiang Fang*, New J. Chem. 2023, 47, 41–45.
Oxa-Nazarov Cyclization-Michael Addition Sequence for the Rapid Construction of Dihydrofuranones, Ting Chen,§ Fan Gong,§ Sakkani Nagaraju,* Jinggong Liu,* Shuang Yang, Xingkuan Chen,* and Xinqiang Fang*, Org. Lett. 2022, 24, 8837–8842.
Asymmetric Semipinacol Rearrangement Enabled by Copper-Catalyzed Propargylic Alkylation, Fan Gong,§ Xiangjian Meng,§ Shouang Lan, Jinggong Liu, Shuang Yang, Xinqiang Fang,* ACS Catal. 2022, 12, 12036-12044.
Copper-Catalyzed Yne-Allylic Substitutions Using Stabilized Nucleophiles, Shengtong Niu, Yingkun Luo, Chao Xu, Jinggong Liu, Shuang Yang, Xinqiang Fang,* ACS Catal. 2022, 12, 6840–6850. (highlighted by Mark Lautens in Synfacts 2022, 18, 0982)
Organocatalyzed Trifunctionalization of Alkynyl 1,2-Diones for the Concise Synthesis of Acyloxy Allylidene Malonates and γ-Alkylidenebutenolides, Li Chen, Shengtong Niu, Shouang Lan, Wenjun Liu, Shuang Yang,* Xinqiang Fang,* Green Chem. 2022, 24, 3623–3628.
Access to Enantioenriched Molecules with Diverse Fluorinated Tetrasubstituted Stereocenters Using Hydroxy as Kinetic Resolution Auxiliary Group, Syeda Tazeen Zehra, Shouang Lan, Hao Zhang, Jinggong Liu,* Shuang Yang, and Xinqiang Fang,* Org. Chem. Front., 2022, 9, 1040–1047.
Copper-Catalyzed Diversified Annulations Between α-Diketones and Alkynyl α-Diketones, Xiangwen Kong, Fang Yu, Shengtong Niu, Fan Gong, Shuang Yang, Jinggong Liu, Benlong Luo,* Xinqiang Fang,* Chin. Chem. Lett. 2022, 33, 2997–3002.
Access to Enantioenriched Compounds Bearing Challenging Tetrasubstituted Stereocenters via Kinetic Resolution of Auxiliary Adjacent Alcohols, Shengtong Niu, Hao Zhang, Weici Xu,* Prasanta Ray Bagdi, Guoxiang Zhang, Jinggong Liu, Shuang Yang, Xinqiang Fang,* Nature Commun. 2021, 12: 3735. (Highlighted by X-MOL https://www.x-mol.com/news/682869).
N-Heterocyclic Carbene-Catalyzed Asymmetric Synthesis of Cyclopentenones, Zhizhou Chen, Xiangwen Kong, ShengtongNiu, Shuang Yang,*Jinggong Liu, BenlongLuo, and Xinqiang Fang*,Org. Lett. 2021, accepted.
Mechanistic Studies on N-Heterocyclic Carbene-Catalyzed Umpolung of β,γ-Unsaturated α-Diketones, Qi Zhang,Deb Kumar Das,Shuang Yang,Yao Fu,*Xinqiang Fang*,J. Org. Chem. 2021, accepted.
Catalytic chemodivergent annulations between α-diketones and alkynyl α-diketones, Xiangwen Kong, Fang Yu,Zhizhou Chen, Fan Gong, Shuang Yang, Jinggong Liu,BenlongLuo, Xinqiang Fang*, Sci. China Chem. 2021, DOI: 10.1007/s11426-021-9972-3.
Rapid Construction of Polycyclic Ketones and the Divergent Kinetic Resolution Using Ruthenium-Catalyzed Transfer Hydrogenation, ShouangLan,Hao Zhang, Zhizhou Chen, Shuang Yang,Xinqiang Fang*, Adv. Synth. Catal. 2021, DOI: 10.1002/adsc.202001594.
Ti(OiPr)4-Facilitated Formal Deoxygenative Annulation of Alkynyl 1,2-Diketones for the Synthesis of Highly Functionalized Furans, ShouangLan,§Rui Liu,§Xiangwen Kong, Jinggong Liu, BenlongLuo, Shuang Yang,*and Xinqiang Fang*, Org. Lett. 2021, DOI: 10.1021/acs.orglett.1c00291.
Divergent Synthesis of Bicyclo[3.2.1]octenes and Cyclohexenes via Catalytic Annulations of Nazarov Reagent and Vinyl 1,2-Diketones, Wenjun Liu,ShengtongNiu, Zhifei Zhao, Shuang Yang,Jinggong Liu,*Yongjin Li,* and Xinqiang Fang*, Org. Lett. 2020, 22, 7572-7576.
Lewis Acid-Catalyzed Asymmetric Alkynylation of Alkynyl 1,2-Diketones: Controllable Formation of 3(2H)-furanones and a-Hydroxy Ketones, Rui Liu, Shuang Yang, Zhizhou Chen, Xiangwen Kong, Houqiang Ding,* and Xinqiang Fang,* Org. Lett. 2020, 22, 6948-6953.
Asymmetric Catalytic Construction of Fully-Substituted Carbon Stereocenters Using Acyclic α-Branched β-Ketocarbonyls: The “Methyl Rule” Widely Exists, Deqian Sun,* Shuang Yang,* Xinqiang Fang,* Org. Chem. Front. 2020, 7, 3557-3577.
Catalytic Annulation of Alkynyl 1,2-Diketone Leading to Hydroxy Spirocyclopenteneindenedione: An Organic Dye with Strong Crystallization-Induced Emission and Data Storage Application, Zhizhou Chen, # Fang Yu, # Rui Liu, Xiangling Lin, Shuang Yang, Jinggong Liu,* Bolai Chen,* Sakkani Nagaraju, Min Zeng, Chenglin Ding, and Xinqiang Fang,* Org. Lett. 2020, 22, 2381？2385.
Organocatalyzed Kinetic Resolution of a-Functionalized Ketones: the Malonate Unit Leads the Way, Jian Liu,# Laxmaiah Vasamsetty,# Muhammad Anwar,# Shuang Yang,* Weici Xu, Jinggong Liu, Sakkani Nagaraju, and Xinqiang Fang,* ACS Catal. 2020, 10, 2882-2893.
Regioselectivity-Switchable Catalytic Annulations of Alkynyl α-Diketones and α-Cyanoketones, Sakkani Nagaraju,# Shuhua Liu,# Jinggong Liu,# Shuang Yang, Rui Liu, Zhizhou Chen, Banoth Paplal,and Xinqiang Fang,* Org. Lett. 2019, 21, 10075-10080.
Stereodivergent Access to Enantioenriched Epoxy Alcohols with Three Stereogenic Centers via Ruthenium-Catalyzed Transfer Hydrogenation, Zhifei Zhao, Prasanta Ray Bagdi, Shuang Yang, Jinggong Liu, Weici Xu,* and Xinqiang Fang,* Org. Lett. 2019, DOI: 10.1021/acs.orglett.9b01789.
Asymmetric Synthesis of Dihydronaphthalene-1,4-diones via Carbene-Catalyzed Stereodivergent Reaction, Zhifei Zhao, Shuang Yang, Shouang Lan, Jinggong Liu, Shuhua Liu,* and Xinqiang Fang,* Adv. Synth. Catal. 2019, DOI: 10.1002/adsc.201900506.
Carbene-Catalyzed Asymmetric Friedel-Crafts Alkylation-Annulation Sequence and Rapid Synthesis of Indole-Fused Polycyclic Alkaloids, Muhammad Anwar, Shuang Yang, Weici Xu, Jinggong Liu, Saima Perveen, Xiangwen Kong, Syeda Tazeen Zehra, and Xinqiang Fang,* Communications Chemistry 2019, DOI: 10.1038/s42004-019-0188-2.
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