个人简介
2020 - present Professor, Shanghai Institute of Organic Chemistry, CAS
2015 - 2020 Assistant Professor, ShanghaiTech University
2013 - 2015 Postdoctoral Fellow, Princeton University Advisor: Professor David W. C. MacMillan
2007 - 2012 Ph.D., Chemistry, Shanghai Institute of Organic Chemistry, CAS Advisor: Professor Dawei Ma
2003 - 2007 B. S., Chemistry, Nanjing University Advisor: Professor Chengjian Zhu and Yixiang Chen
研究领域
The Zuo Group is interested in addressing long-standing synthetic challenges through the development of innovative catalytic platforms. We are particularly interested in the creative use of light energy and environmentally benign metals to achieve the direct activation of feedstock chemicals, including methane, light alkanes, and commonly occurring starting materials, for the syntheses of value-added products. We have been exploring ligand-to-metal charge transfer (LMCT) excitation of in situ formed metal complexes to generate various energetically challenging radicals and have achieved selective transformations of C(sp3)–H and C–C bonds. With powerful tools in organometallic chemistry, photochemistry, and photophysics, as well as flow technology, our group endeavors to develop practical synthetic processes for important basic chemicals and pharmaceuticals.
近期论文
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Multiplicative enhancement of stereoenrichment by a single catalyst for deracemization of alcohols Lu Wen†, Jia Ding†, Lingfei Duan†, Shun Wang, Qing An, Hexiang Wang, Zhiwei Zuo* Science, 2023, 382, 459- 464 DOI: 10.1126/science.adj0040
[INVITED PERSPECTIVE]Resurgence and advancement of photochemical hydrogen atom transfer processes in selective alkane functionalizations Liang Chang; Shun Wang; Qing An; Linxuan Liu; Hexiang Wang; Yubo Li; Kaixuan Feng; Zhiwei Zuo* Chem. Sci., 2023, 14, 6841- 6859 DOI: 10.1039/d3sc01118f
[INVITED THEME ISSUE]Selective oxidation of benzylic alcohols via synergistic bisphosphonium and cobalt catalysis Jia Ding†; Shuaishuai Luo†; Yuanli Xu; Qing An; Yi Yang; Zhiwei Zuo* Chem. Comm., 2023, 59, 4055- 4058 DOI: 10.1039/d3cc00532a
Identification of Alkoxy Radicals as Hydrogen Atom Transfer Agents in Ce-Catalyzed C–H Functionalization Qing An; Yang-Yang Xing; Ruihua Pu; Menghui Jia; Yuegang Chen; Anhua Hu; Shuo-Qing Zhang, Shuoqing Zhang; Na Yu, Jianbo Du, Yanxia Zhang, Jinquan Chen*, Weimin Liu*, Xin Hong*, and Zhiwei Zuo* J. Am. Chem. Soc., 2023, 145, 1, 359– 376. DOI: 10.1021/jacs.2c10126
[INVITED REVIEW]Alkoxy Radicals See the Light: New Paradigms of Photochemical Synthesis Liang Chang; Qing An; Lingfei Duan; Kaixuan Feng; Zhiwei Zuo* Chem. Rev., 2022, 122, 2, 2429– 2486. DOI: 10.1021/acs.chemrev.1c00256
Photocatalytic Dehydroxymethylative Arylation by Synergistic Cerium and Nickel Catalysis Yuegang Chen; Xin Wang; Xu He; Qing An; Zhiwei Zuo* J. Am. Chem. Soc., 2021, 143, 13, 4896– 4902. DOI: 10.1021/jacs.1c00618
Photocatalytic Aerobic Oxidative Ring Expansion of Cyclic Ketones to Macrolactones by Cerium and Cyanoanthracene Catalysis Jianbo Du†; Xiaokun Yang†; Xin Wang; Qing An; Xu He; Hui Pan; Zhiwei Zuo* Angew. Chem. Int. Ed., 2021,60, 5370– 5376. DOI: 10.1002/anie.202012720
Qing An‡, Ziyu Wang‡, Yuegang Chen‡, Xin Wang, Kaining Zhang, Hui Pan, Weimin Liu,* and Zhiwei Zuo* , “Cerium-Catalyzed C−H Functionalizations of Alkanes Utilizing Alcohols as Hydrogen Atom Transfer Agents.” J. Am. Chem. Soc. 2020, 142, 6216.
Yilin Chen, Jianbo Du, Zhiwei Zuo*, “Selective C-C Bond Scission of Ketones via Visible-Light-Mediated Cerium Catalysis.” Chem. 2020, 6, 266.
Hao Cheng, Xin Wang, Liang Chang, Yilin Chen, Lingling Chu*, Zhiwei Zuo*, “Bisphosphonium salt: an effective photocatalyst for the intramolecular hydroalkoxylation of olefins.”, Sci. Bull. 2019, 64, 1896.
Kaining Zhang‡, Liang Chang‡, Qing An, Xin Wang, Zhiwei Zuo*, “Dehydroxymethylation of Alcohols Enabled by Cerium Photocatalysis.” J. Am. Chem. Soc. 2019, 141, 10556.
Liang Chang, Yilin Chen, Zhiwei Zuo* , “Dearomative [4+2] Cycloaddition of Pyridine via Energy-Transfer Catalysis“, Chem, 2019, 5, 2744.
Anhua Hu‡, Jing-Jing Guo‡，Hui Pan,Zhiwei Zuo* , “Selective functionalization of methane, ethane, and higher alkanes by cerium photocatalysis” Science 2018, 361, 668.
Anhua Hu‡, Yilin Chen‡, Jing-Jing Guo, Na Yu, Qing An, and Zhiwei Zuo* , “Cerium-Catalyzed Formal Cycloaddition of Cycloalkanols with Alkenes through Dual Photoexcitation.”, J. Am. Chem. Soc. 2018, 140, 13580.
Anhua Hu‡, Jing-Jing Guo‡，Hui Pan, Haoming Tang, Zhaobo Gao,Zhiwei Zuo* , “-Selective functionalization of alkanols enabled by visible-light-induced ligand-to-metal charge transfer” J. Am. Chem. Soc. 2018, 140, 1612.
Jing-Jing Guo‡, Anhua Hu‡, Yiling Chen, Jianfeng Sun, Haoming Tang, Zhiwei Zuo* , “Photocatalytic C−C Bond Cleavage and Amination of Cycloalkanols by Cerium(III) Chloride Complex”, Angew. Chem. Int. Ed. 2016, 55, 15319.
Zhiwei Zuo‡, Huan Cong‡, Wei Li, Junwon Choi, Gregory C. Fu, David W. C. MacMillan “Enantioselective Decarboxylative Arylation of α-Amino Acids via the Merger of Photoredox and Nickel Catalysis”, J. Am. Chem. Soc. 2016, 138, 1832.
Weiwei Zi, Zhiwei Zuo, Dawei Ma. Acc. Chem. Res. 2015, 48, 702.
Lingling Chu, Chisa Ohta, Zhiwei Zuo, David W. C. MacMillan J. Am. Chem. Soc. 2014, 136, 10886.
Zhiwei Zuo, Derek Ahneman, Lingling Chu, Jack Terrett, Abigail G. Doyle and David W. C. MacMillan “Merging photoredox with nickel catalysis: Coupling of α-Carboxyl sp3-Carbons with Aryl Halides”, Science 2014, 345, 437.
Zhiwei Zuo and David W. C. MacMillan. “Decarboxylative Arylation of α-Amino Acids via Photoredox Catalysis: A One-Step Conversion of Biomass to Drug Pharmacophore”, J. Am. Chem. Soc. 2014, 136, 5257.
Zhiwei Zuo and Dawei Ma. “Enantioselective Total Syntheses of Communesins A and B”, Angew. Chem. Int. Ed. 2011, 50, 12008.
Zhiwei Zuo and Dawei Ma. “Synthetic Studies toward Communesins”, Isr. J. Chem. 2011, 51, 434.
Zhiwei Zuo, Weiqing Xie and Dawei Ma. “Total Synthesis and Absolute Stereochemical Assignment of (−)-Communesin F”, J. Am. Chem. Soc. 2010, 132, 13226.
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