Craig, Stephen L - Duke University - Department of Chemistry

个人简介

Steve Craig received his undergraduate degrees (B.S. in Chemistry, A.B. in Math) from Duke in 1991. After a year at Cambridge (M. Phil.), he began doctoral work at Stanford, where he received his Ph.D. in 1997. Following his Ph.D., he took a position as a Research Chemist in DuPont Central Research until early 1999, when he moved to a postdoctoral position at The Scripps Research Institute. In 2000, he joined the Department of Chemistry at Duke, where he is now William T. Miller Professor of Chemistry.

研究领域

Our research interests bridge synthetic organic, physical, and materials chemistry. A primary theme is that of the rational, molecular design of materials — using the principles of physical organic and/or supramolecular chemistry to develop new materials. Current interests include using chemistry to guide the design and synthesis of stress-responsive and self-healing polymers and using new polymer architectures as a mechanism to create new reactivity and catalysts through mechanochemical coupling.

近期论文

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Horst, Matías, Jinghui Yang, Jan Meisner, Tatiana B. Kouznetsova, Todd J. Martínez, Stephen L. Craig, and Yan Xia. “Understanding the Mechanochemistry of Ladder-Type Cyclobutane Mechanophores by Single Molecule Force Spectroscopy.” Journal of the American Chemical Society, July 26, 2021. https://doi.org/10.1021/jacs.1c05857. Cha, Yujin, Tianyu Zhu, Ye Sha, Huina Lin, JiHyeon Hwang, Matthew Seraydarian, Stephen L. Craig, and Chuanbing Tang. “Mechanochemistry of Cationic Cobaltocenium Mechanophore.” Journal of the American Chemical Society, July 20, 2021. https://doi.org/10.1021/jacs.1c05233. Bowser, Brandon H., Shu Wang, Tatiana B. Kouznetsova, Haley K. Beech, Bradley D. Olsen, Michael Rubinstein, and Stephen L. Craig. “Single-Event Spectroscopy and Unravelling Kinetics of Covalent Domains Based on Cyclobutane Mechanophores.” Journal of the American Chemical Society 143, no. 13 (April 2021): 5269–76. https://doi.org/10.1021/jacs.1c02149. Brown, Cameron L., Brandon H. Bowser, Jan Meisner, Tatiana B. Kouznetsova, Stefan Seritan, Todd J. Martinez, and Stephen L. Craig. “Substituent Effects in Mechanochemical Allowed and Forbidden Cyclobutene Ring-Opening Reactions.” Journal of the American Chemical Society 143, no. 10 (March 5, 2021): 3846–55. https://doi.org/10.1021/jacs.0c12088. Wang, Shu, Haley K. Beech, Brandon H. Bowser, Tatiana B. Kouznetsova, Bradley D. Olsen, Michael Rubinstein, and Stephen L. Craig. “Mechanism Dictates Mechanics: A Molecular Substituent Effect in the Macroscopic Fracture of a Covalent Polymer Network.” Journal of the American Chemical Society 143, no. 10 (March 2, 2021): 3714–18. https://doi.org/10.1021/jacs.1c00265. Lin, Tzyy-Shyang, Nathan J. Rebello, Haley K. Beech, Zi Wang, Bassil El-Zaatari, David J. Lundberg, Jeremiah A. Johnson, Julia A. Kalow, Stephen L. Craig, and Bradley D. Olsen. “PolyDAT: A Generic Data Schema for Polymer Characterization.” Journal of Chemical Information and Modeling 61, no. 3 (March 2021): 1150–63. https://doi.org/10.1021/acs.jcim.1c00028. Razgoniaev, Anton O., Logan M. Glasstetter, Tatiana B. Kouznetsova, Kacey C. Hall, Matias Horst, Stephen L. Craig, and Katherine J. Franz. “Single-Molecule Activation and Quantification of Mechanically Triggered Palladium-Carbene Bond Dissociation.” Journal of the American Chemical Society 143, no. 4 (February 2021): 1784–89. https://doi.org/10.1021/jacs.0c13219. Ghanem, M. A., A. Basu, R. Behrou, N. Boechler, A. J. Boydston, S. L. Craig, Y. Lin, et al. “The role of polymer mechanochemistry in responsive materials and additive manufacturing.” Nature Reviews Materials 6, no. 1 (January 1, 2021): 84–98. https://doi.org/10.1038/s41578-020-00249-w. Shannahan, Logan S., Yangju Lin, James F. Berry, Meredith H. Barbee, Müge Fermen-Coker, and Stephen L. Craig. “Onset of Mechanochromic Response in the High Strain Rate Uniaxial Compression of Spiropyran Embedded Silicone Elastomers.” Macromolecular Rapid Communications 42, no. 1 (January 2021): e2000449. https://doi.org/10.1002/marc.202000449. Zhang, Yudi, Ethen Lund, Gregory R. Gossweiler, Bobin Lee, Zhenbin Niu, Constantine Khripin, Etienne Munch, Marc Couty, and Stephen L. Craig. “Molecular Damage Detection in an Elastomer Nanocomposite with a Coumarin Dimer Mechanophore.” Macromolecular Rapid Communications 42, no. 1 (January 2021): e2000359. https://doi.org/10.1002/marc.202000359. Zhang, Yudi, Zi Wang, Tatiana B. Kouznetsova, Ye Sha, Enhua Xu, Logan Shannahan, Muge Fermen-Coker, Yangju Lin, Chuanbing Tang, and Stephen L. Craig. “Distal conformational locks on ferrocene mechanophores guide reaction pathways for increased mechanochemical reactivity.” Nature Chemistry 13, no. 1 (January 2021): 56–62. https://doi.org/10.1038/s41557-020-00600-2. Lin, Yangju, Tatiana B. Kouznetsova, Chia-Chih Chang, and Stephen L. Craig. “Enhanced polymer mechanical degradation through mechanochemically unveiled lactonization.” Nature Communications 11, no. 1 (October 5, 2020): 4987. https://doi.org/10.1038/s41467-020-18809-7. Lin, Yangju, and Stephen L. Craig. “Oxidative regulation of the mechanical strength of a C-S bond.” Chemical Science 11, no. 38 (September 14, 2020): 10444–48. https://doi.org/10.1039/d0sc04381h. Lin, Yangju, Tatiana B. Kouznetsova, and Stephen L. Craig. “Mechanically Gated Degradable Polymers.” Journal of the American Chemical Society 142, no. 5 (February 2020): 2105–9. https://doi.org/10.1021/jacs.9b13359. Oldenhuis, Nathan J., K Peter Qin, Shu Wang, Hong-Zhou Ye, Eric A. Alt, Adam P. Willard, Troy Van Voorhis, Stephen L. Craig, and Jeremiah A. Johnson. “Photoswitchable Sol-Gel Transitions and Catalysis Mediated by Polymer Networks with Coumarin-Decorated Cu24 L24 Metal-Organic Cages as Junctions.” Angewandte Chemie (International Ed. in English) 59, no. 7 (February 2020): 2784–92. https://doi.org/10.1002/anie.201913297. Lin, Yangju, Tatiana B. Kouznetsova, and Stephen L. Craig. “A Latent Mechanoacid for Time-Stamped Mechanochromism and Chemical Signaling in Polymeric Materials.” Journal of the American Chemical Society 142, no. 1 (January 8, 2020): 99–103. https://doi.org/10.1021/mcs.9b12861. Lin, Yangju, Tatiana B. Kouznetsova, and Stephen L. Craig. “A Latent Mechanoacid for Time-Stamped Mechanochromism and Chemical Signaling in Polymeric Materials.” Journal of the American Chemical Society 142, no. 1 (January 2020): 99–103. https://doi.org/10.1021/jacs.9b12861. Bowser, B. H., and S. L. Craig. “Correction: Empowering mechanochemistry with multi-mechanophore polymer architectures (Polymer Chemistry (2018) 9 (3583-3593) DOI: 10.1039/C8PY00720A).” Polymer Chemistry 10, no. 47 (December 21, 2019): 6523. https://doi.org/10.1039/c9py90180a. Rohde, R. C., A. Basu, L. B. Okello, M. H. Barbee, Y. Zhang, O. D. Velev, A. Nelson, and S. L. Craig. “Mechanochromic composite elastomers for additive manufacturing and low strain mechanophore activation.” Polymer Chemistry 10, no. 44 (November 28, 2019): 5985–91. https://doi.org/10.1039/c9py01053j. Bowser, B. H., C. H. Ho, and S. L. Craig. “High Mechanophore Content, Stress-Relieving Copolymers Synthesized via RAFT Polymerization.” Macromolecules 52, no. 22 (November 26, 2019): 9032–38. https://doi.org/10.1021/acs.macromol.9b01792.