梁子骐 - 复旦大学 - 材料科学系

个人简介

教育和科研背景 2012年9月--至今复旦大学材料科学系教授博士生导师 2008年6月-2012年6月美国国家可再生能源实验室博士后、科学家III 2006年5月-2008年5月英国剑桥大学博士后 2006年春季美国宾夕法尼亚州立大学材料科学与工程系高分子科学专业博士 2002年夏季美国加州大学河滨分校化学系硕士 1999年春季华东理工大学/上海交通大学高分子材料科学与工程系本科/硕士研究生奖励和荣誉美国宾夕法尼亚州立大学（研究生）杰出科研奖上海市浦江人才计划入选者上海市优秀学术带头人

研究领域

从事有机/钙钛矿半导体材料光+热—电能源转换研究，主要开展以下工作：（1）π-共轭高分子：设计、合成、功能与器件（2）光电能量转换：有机/钙钛矿太阳能电池及其关键物理化学问题研究（3）热电能量转换：有机半导体材料、有机/无机纳米复合材料及元件的热电性能研究

近期论文

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R. Chen, Y. Yan, Y. Ma, L. Chen,* Z. Liang,* Light/Heat-Driven Modulation of Carrier Transportation in Tin Halide Perovskites to Maximize Output Voltages (Submitted). J. Tang, Z. Wu, W. Li, G. Zuo, Y. Zhao,* Z. Liang,* Learning From Polymeric π-Backbone to Film Sequences Unravels that A Coexistence of Bilayered and Mixed Morphologies Optimally Strengthens Thermoelectrics. Adv. Energy Mater. 14, 2303494 (2024). K. Liao, Y. Yan, Z. Liang,* In-Situ Ligand-Exchanged 2D Halide Perovskites onto PbS Quantum Dots Reinforce Colloidal and Device Stabilities via Inward Coordination and Outward Hydrophobicity (Submitted). J. Ji, Z. Wu, J. Xie, W.-Y. Wang, H. Qian, Z. Liang,* Dual Polymerized Y-Acceptors of Distinct-Dimensionality Create Neuron-Like Interpenetrating Hierarchical Network towards Efficient and Stable All-Polymer Solar Cells. Adv. Mater. 2313237 (2024). J. Xie, W. Lin, D. Wang, Z.-H. Lu,* K. Zheng,* Z. Liang,* Sequentially N-Doped Acceptor Primer Layer Facilitates Electron Collection of Inverted Non-fullerene Organic Solar Cells. Adv. Funct. Mater. 2309511 (2023). R. Chen, L. Chen,* Z. Liang,* Strategic Doping in Metal Halide Perovskites for Thermoelctrics. Adv. Funct. Mater. 33, 2303774 (2023). J. Tang, Y.-H. Pai, Z. Liang,* Strategic Insights into Semiconducting Polymer Thermoelectrics by Leveraging Between Molecular Structures and Chemical Doping. ACS Energy Lett. 7, 4299?4324 (2022). Y.-H. Pai, J. Tang, Y. Zhao,* Z. Liang,* Ionic Organic Thermoelectrics with Impressively High Thermopower for Sensitive Heat Harvesting Scenarios. Adv. Energy Mater. 13, 2202507 (2023). J. Xie, W. Lin, G. C. Bazan, T. Pullerits, K. Zheng,* Z. Liang,* N-Doping of Nonfullerene Bulk-Heterojunction Organic Solar Cells Strengthens Photogeneration and Exciton Dissociation. J. Mater. Chem. A 10, 18845?18855 (2022). S. Yu, J. Meng, Q. Pan, Q. Zhao, T. Pullerits, Y. Yang,* K. Zheng,* Z. Liang,* Imidazole Additives in 2D Halide Perovskites: Impacts of ?CN versus ?CH3 Substituents Reveal the Mediation of Crystal Growth by Phase Buffering. Energy Environ. Sci. 15, 3321?3330 (2022). R. Chen, Y. Yan, J. Tang, Q. Yao,* L. Chen, Z. Liang,* Efficient P-Type Doping of Tin Halide Perovskite via Sequential Diffusion for Thermoelectrics. Small Sci. 2, 2200004 (2022). J. Ji, L. Zhu, X. Xiong, K. Zheng, F. Liu, Z. Liang,* Developing Y-Branched Polymer Acceptor with 3D Architectures to Reconcile Between Crystallinity and Miscibility Yielding >15% Efficient All-Polymer Solar Cells. Adv. Sci. 9, 2200864 (2022). K. Ba, D. Pu, X. Yang, T. Ye, J. Chen, X. Wang, T. Xiao, T. Duan,* Y. Sun, B. Ge, P. Zhang, Z, Liang,* Z. Sun,* Billiard Catalysis at Ti3C2Tx MXene/MAX Heterostructure for Efficient Nitrogen Fixation. Appl. Catal. B Environ. 317, 121755 (2022). J. Tang, J. Ji, R. Chen, Y. Yan, Y. Zhao, Z. Liang,* Achieving Efficient p-Type Organic Thermoelectrics by Modulation of Acceptor Unit in Photovoltaic π-Conjugated Copolymers. Adv. Sci. 9,2103646 (2022). J. Sun, S. Yang,* J. Wu, X. He, Y. Zhang, J. Ji, C. Zhang, Z. Liang,* In-Situ Electro-Polymerization of Fluorescent Electrochromic Thin Films Based on Charge-Transfer Complexes. Chem. Eng. J. 428, 132625 (2022). Y. Yan, Y. Yang,* M. Liang, M. Abdellah, T. Pullerits, K. Zheng,* Z. Liang,* Implementing An Intermittent Spin-Coating Strategy to Enable Bottom-up Crystallization in Layered Halide Perovskites. Nat. Commun. 12, 6603 (2021). S. Yu, M. Abdellah, T. Pullerits, K. Zheng,* Z. Liang,* Asymmetric Spacer in Dion-Jacobson Halide Perovskites Induces Staggered Alignment to Direct Out-of-Plane Carrier Tansport and Enhance Ambient Stability Simultaneously. Adv. Funct. Mater. 31, 2104342 (2021). J. Ji, J. Xie, J. Tang, K. Zheng,* Z. Liang,* Developing Halogen-Free Polymer Donors for Efficient Nonfullerene Organic Solar Cells by Addition of Highly Electron-Deficient Diketopyrrolopyrrole Unit. Sol. RRL 5, 2100142 (2021). R. Chen, J. Tang, Y. Yan, Z. Liang,* Solvent‐Mediated n‐Type Doping of SWCNTs to Achieve Superior Thermoelectric Power Factor. Adv. Mater. Technol. 5, 2000288 (2020). Y. Yan, T. Pullerits, K. Zheng,* Z. Liang,* Advancing Strategies in Tin Halide Perovskites for Desirable Optoelectronic Performance and Durability. ACS Energy Letters 5, 2052?2086 (2020). J. Tang, R. Chen, L. Chen, G. C. Bazan, Z. Liang,* Semiconducting Polymer Contributes Favorably to the Seebeck Coefficient in Multi-component, High-performance n-type Thermoelectric Nano-composites. J. Mater. Chem. A 8, 9797?9805 (2020). Z. Wang, J. Ji, W. Lin, Y. Yao, K. Zheng,* Z. Liang,* Mechanistic Investigation into Dynamic Function of Third-Component Incorporated in Ternary Near Infrared Nonfullerene Organic Solar Cells. Adv. Funct. Mater. 30, 2001564 (2020). S. Yu, Y. Yan, M. Abdellah, T. Pullerits, K. Zheng,* Z. Liang,* Non-Confinement Structure Revealed in Dion-Jacobson Type Quasi-2D Perovskite Expedites Interlayer Charge Transport. Small 15, 1905081 (2019). Y. Yan, S. Yu, A. Honarfar, T. Pullerits, K. Zheng,* Z. Liang,* Benefiting from Spontaneously Generated 2D/3D Bulk-Heterojunctions in Ruddlesden?Popper Perovskite by Incorporation of S-Bearing Spacer Cation. Adv. Sci. 6, 1900548 (2019). J. Tang, Y. Chen, S. R. McCuskey, L. Chen,* G. C. Bazan,* Z. Liang,* Recent Advances in n-Type Thermoelectric Nanocomposites. Adv. Electron. Mater. 5, 1800943 (2019). Z. Liang,* L. Chen,* G. C. Bazan,* Editorial in Organic and Hybrid Thermoelectrics Special Issue. Adv. Electron. Mater. 5, 1900650 (2019). X. Liu, Y. Yan, Y. Yao, A. Honarfar, K. Zheng*, Z. Liang,* Unveiling Excitonic Dynamics in High-Efficiency Nonfullerene Organic Solar Cells to Direct Morphological Optimization for Suppressing Charge Recombination. Adv. Sci. 6, 1802103 (2019). S. Yu, Y. Yan, Y. Chen, P. Chábera, K. Zheng,* Z. Liang,* Enabling Room-Temperature Processed Highly Efficient 2D Ruddlesden?Popper Perovskite Solar Cells with Eliminated Hysteresis by Synergistic Exploitation of Additive and Solvent. J. Mater. Chem. A 7, 2015?2021 (2019). Y. Yan, Q. Wu, Y. Zhao, S. Chen, S. Hu, J. Zhu, J. Huang,* Z. Liang,* Air-Stable and Self-Driven Perovskite Photodiodes with High ON/OFF Ratio and Swift Photoresponse. Small 14, 1802764 (2018). Y. Chen, M. He, J. Tang, G. C. Bazan, Z. Liang,* Flexible Thermoelectric Generators with Ultra-High Output Power Enabled by Magnetic Field Aligned Metallic Nanowires. Adv. Electron. Mater. 4, 1800200 (2018). X. Gao, M. He, B. Liu, J. Hu, Y. Wang,* Z. Liang,* J. Zhou,* Topological Design of Inorganic-Organic Thermoelectric Nanocomposites Based on 'Electron-Percolation Phonon-Insulator' Concept. ACS Appl. Energy Mater. 1, 2927?2933 (2018). Y. Chen, Y. Sun, J. Peng, P. Cha?bera, A. Honarfar, K. Zheng,* Z. Liang,* Composition Engineering in Two-Dimensional Pb-Sn Alloyed Perovskites for Efficient and Stable Solar Cells. ACS Appl. Mater. Interfaces 10, 21343?21348 (2018). Y. Chen, S. Yu, Y. Sun, Z. Liang,* Phase Engineering in Quasi-2D Ruddlesden–Popper Perovskites. J. Phys. Chem. Lett. 9, 2627–2631 (2018). X. Liu, Y. Yan, Y. Yao,* Z. Liang,* Ternary Blend Strategy for Achieving High-Efficiency Organic Solar Cells with Nonfullerene Acceptors Involved. Adv. Funct. Mater. 28, 1802004 (2018). K. Zheng,* Y. Chen, Y. Sun, J. Chen, P. Chábera, R. Schaller, M. J. Al-Marri, S. E Canton, Z. Liang,* T. Pullerits,* Inter-Phase Charge and Energy Transfer in Ruddlesden–Popper 2D Perovskites: Critical Role of the Spacing Cations. J. Mater. Chem. A 6, 6244–6250 (2018). Y. Chen, Y. Sun, J. Peng, K. Zheng, Z. Liang,* Two-Dimensional Ruddlesden?Popper Perovskites for Optoelectronics. Adv. Mater. 30, 1703487 (2018). M. He, X. Gao, B. Liu, J. Zhou,* Z. Liang,* Ultra-High Electrical Conductivity and Superior Bendability Simultaneously Enabled in Ag Nanowire Based Nanocomposites. RSC Adv. 7, 44254–44258 (2017). Y. Jin, Z. Chen, M. Xiao, J. Peng, B. Fan, L. Ying, G. Zhang, X.-F. Jiang, Q. Yin, Z. Liang, F. Huang, Y. Cao, Thick Film Polymer Solar Cells Based on Naphtho[1,2-c:5,6-c]bis[1,2,5]thiadiazole Conjugated Polymers with Efficiency over 11%. Adv. Energy Mater. 7, 1700944 (2017). X. Liu, J. Wang, J. Peng, Z. Liang,* 2D/1A Strategy to Regulate Film Morphology for Highly Efficient and Stable Nonfullerene Organic Solar Cells. Macromolecules 50, 6954–6960 (2017). J. Peng, Y. Chen, K. Zheng,* T. Pullerits, Z. Liang,* Insights into Charge Carrier Dynamics in Organo-Metal Halide Perovskites: From Neat Films to Solar Cells. Chem. Soc. Rev. 46, 5714–5729 (2017). J. Wang, J. Peng, X. Liu, Z. Liang,* Efficient and Stable Ternary Organic Solar Cells Based on Two Planar Nonfullerene Acceptors with Tunable Crystallinity and Phase Miscibility. ACS Appl. Mater. Interfaces 9, 20704–20710 (2017). Y. Sun, D. Chen, Z. Liang,* Two-Dimensional MXenes for Energy Storage and Conversion Applications. Materials Today Energy 5, 22–36 (2017). J. Sun,* H. Sun, Z. Liang,* Nanomaterials in Electrochemiluminescence Sensors. ChemElectroChem 4, 1651–1662 (2017). Y. Chen, Y. Sun, J. Peng, W. Zhang, X. Su, K. Zheng, T. Pullerits, Z. Liang,* Tailoring Organic Cation of Two-Dimensional Air-Stable Organometal Halide Perovskites for Highly Efficient Planar Solar Cells. Adv. Energy Mater. 7, 1700162 (2017). Y. Sun, J. Peng, Y. Chen, Y. Yao, Z. Liang,* Triple-cation Mixed-halide Perovskites: towards Efficient, Annealing-free and Air-stable Solar Cells Enabled by Pb(SCN)2 Additive. Sci. Rep. 7, 46193 (2017). M. Li , K. Gao , X. Wan,* Q. Zhang, B. Kan, R. Xia, F. Liu, X. Yang, H. Feng, W. Ni, Y. Wang, J. Peng, H. Zhang, Z. Liang, H.-L. Yip, X. Peng,* Y. Cao, Y. Chen,* Solution-Processed Organic Tandem Solar Cells with Power Efficiencies >12%. Nature Photonics 11, 85–90 (2017). Y. Chen, M. He, B. Liu, G. C. Bazan,* J. Zhou,* Z. Liang,* Bendable n-Type Metallic Nanocomposites with Large Thermoelectric Power Factor. Adv. Mater. 29, 1604752 (2017). J. Peng, Y. Sun, Y. Chen, Y. Yao,* Z. Liang,* Light and Thermally Induced Evolutional Charge Transport in CH3NH3PbI3 Perovskite Solar Cells. ACS Energy Lett. 1, 1000–1006 (2016). J. Wang, J. Peng, Y. Sun, X. Liu, Y. Chen, Z. Liang,* FAPbCl3 Perovskite as Alternative Interfacial Layer for Highly Efficient and Stable Polymer Solar Cells. Adv. Electron. Mater. 2, 1600329 (2016). J. Wang, Z. Liang,* Synergetic Solvent Engineering of Film Nanomorphology to Enhance Planar Perylene Diimide Based Organic Photovoltaics. ACS Appl. Mater. Interfaces 8, 22418–22424 (2016). J. Sun, Z. Liang,* Swift Electrofluorochromism Based on Donor-Acceptor Conjugated Polytriarylamines. ACS Appl. Mater. Interfaces 8, 18301–18308 (2016). J. Wang, L. Kong, Z. Liang,* Fine Control of Side Chains in Random π-Conjugated Terpolymers for Organic Photovoltaics. Macromol. Chem. Phys. 217, 1513–1520 (2016). D. Chen, Y. Zhao, Y. Chen, T. Lu, Y. Wang,* J. Zhou,* Z. Liang,* Thermoelectric Enhancement of Cu3SbS4 Nanocrystals by Magnetic Nickel Doping. Adv. Electron. Mater. 2, 1500473 (2016). J. Sun, Y. Chen, Z. Liang,* Electroluminochromic Materials and Devices. Adv. Funct. Mater. 26, 2783–2799 (2016). Y. Chen, M. He, J. Peng, Y. Sun, Z. Liang,* Structure and Growth Control of Organic-Inorganic Halide Perovskites for Optoelectronics: From Polycrystalline Films to Single Crystals. Adv. Sci. 3, 1500392 (2016). J. Peng, Y. Chen, X. Zhang, A. Dong, Z. Liang,* Solid-State Ligand-Exchange Fabrication of CH3NH3PbI3 Capped PbS Quantum Dot Solar Cells. Adv. Sci. 3, 1500432 (2016). J. Peng, X. Chen, Y. Chen, O. Sandberg, R. ?sterbacka,* Z. Liang,* Transient Extraction of Holes and Electrons Separately Reveals the Transport Dynamics in Organic Photovoltaics. Adv. Electron. Mater. 2, 1500333 (2016). D. Su, Y. Yao, Y. Chen, J. Peng, Z. Liang,* Conjugated Polymers Based Chemical and Biological Sensors. (Book Chapter) in Smart Nanomaterials for Sensors and Transducers, World Scientific Publishers (2016). B. Li, Y. Chen, Z. Liang,* D. Gao,*, W. Huang,* Interfacial Engineering by Using Self-Assembled Monolayer in Mesoporous Perovskite Solar Cell. RSC Adv. 5, 94290–94295 (2015). M. He, Y. Zhao, B. Wang, Q. Xi, J. Zhou,* Z. Liang,* 3D Printing Fabrication of Amorphous Thermoelectric Materials with Ultralow Thermal Conductivity. Small 11, 5889–5894 (2015). (Frontispiece). Y. Zhang, J. Du, X. Wu, G. Zhang, Y. Chu, D. Liu, Y. Zhao,*, Y. Zhao,* Z. Liang,* J. Huang,* Ultrasensitive Phototransistors Based on Island-Structured CH3NH3PbI3 Thin Films. ACS Appl. Mater. Interfaces 7, 21634–21638 (2015). K. Wang, Z. Liang, X. Wang, X. Cui,* Lead Replacement in CH3NH3PbI3 Perovskites. Adv. Electron. Mater. 1, 1500089 (2015). J. Peng, Y. Chen, X. Wu, Q. Zhang, X. Chen, Y. Chen, J. Huang, Z. Liang,* Correlating Molecular Structures with Transport Dynamics in High-Efficiency Small Molecule Organic Photovoltaics. ACS Appl. Mater. Interfaces 7, 13137–13141 (2015). Y. Chen, B. Li, W. Huang, D. Gao,* Z. Liang,* Efficient and Reproducible Mixed Perovskite based Planar Solar Cells. Chem. Commun. 51, 11997–11999 (2015). M. He, Y. Chen, H. Liu, J. Wang, X. Fang, Z. Liang,* Chemical Decoration of CH3NH3PbI3 Perovskite with Graphene Oxides for Photodetector Applications. Chem. Commun. 51, 9659–9661 (2015). Chen, Y. Zhao, Y. Chen, B. Wang, Y. Wang, J. Zhou,* Z. Liang,* Hot-Injection Synthesis of Cu-doped Cu2ZnSnSe4Nanocrystals to Reach Thermoelectric Figure of Merit of 0.70. ACS Appl. Mater. Interfaces 7, 24403–24408 (2015). X. Chen, Z. He, Y. Hu, Y. He, H. Peng, Z. Liang,* Tunable Exciton Dissociation at the Organic/Metal Electrode Interface. J. Phys. Chem. C 119, 7039–7046 (2015). Y. Chen, Y. Zhao, Z. Liang,* Nonvolatile Chlorinated Additives Adversely Influence CH3NH3PbI3 Based Planar Solar Cells. J. Mater. Chem. A 3, 9137–9140 (2015). Y. Chen, J. Peng, D. Su, X. Chen, Z. Liang,* Efficient and Balanced Charge Transport Revealed in Planar Perovskite Solar Cells. ACS Appl. Mater. Interfaces 7, 4471–4475 (2015). Y. Chen, Y. Zhao, Z. Liang,* Non-Thermal Annealing Fabrication of Efficient Planar Perovskite Solar Cells with Inclusion of NH4Cl. Chem. Mater. 27, 1448–1451 (2015). M. He, K. Song, H. Mo, J. Li, D. Pan, Z. Liang,* Progress on Photosensitive Resins for 3D Printing. J. Funct. Polym. 28, 102–108 (2015). D. Chen, Y. Zhao, Y. Chen, B. Wang, H. Chen, J. Zhou, Z. Liang,* One-Step Chemical Synthesis of ZnO/Graphene Oxide Molecular Hybrids for High-Temperature Thermoelectric Applications. ACS Appl. Mater. Interfaces 7, 3224–3230 (2015). Y. Chen, Y. Zhao, Z. Liang,* Solution Processed Organic Thermoelectrics: Towards Flexible Thermoelectric Modules. Energy Environ. Sci. 8, 401–422 (2015). (Review article, Back Cover). Q. Zhang, B. Kan, G. Long, X. Wan, F. Liu, X. Chen, Y. Zuo, W. Ni, H. Zhang, M. Li, Z. Hu, F. Huang, Y. Cao, T. P. Russell, Z. Liang, M. Zhang, Y. Chen, Over 9% Efficiency of Small Molecule Based Solar Cells with Nanoscale Fibrillar Morphology. Nature Photonics 9, 35–41 (2015). S. Han, L. Hu, Z. Liang, S. Wageh, A. A. Al-Ghamdi, Y. Chen, X. Fang, One-Step Hydrothermal Synthesis of 2D Hexagonal Nanoplates of a-Fe2O3/Graphene Composites with Enhanced Photocatalytic Activity. Adv. Funct. Mater. 24, 5719–5727 (2014). X. Chen, B. Wu, Z. He, H. Xuxie, Z. Liang,* X. Hou,* Transient Photovoltage Study on the Dynamics of Excitons and Carriers in Tris-(8-hydroxyquinolinato)aluminum (AlQ). J. Appl. Phys. 116, 153704 (2014).