赵永生 - 中国科学院化学研究所 -

个人简介

2009年中国科学院化学研究所研究员，博士生导师 2011年国家杰出青年科学基金（2015年结题优秀） 2015年中国科学院大学岗位教授 2017年国家重点研发计划首席科学家教育背景 2008.4－2009.9 美国西北大学博士后 2007.3－2008.3 加州大学洛杉矶分校博士后 2003.9－2007.3 中科院化学所理学博士 2000.9－2003.7 北京化工大学理学硕士 1996.9－2000.7 青岛大学工学学士

研究领域

本课题组的研究方向是有机纳米光子学材料与器件，以新型可穿戴器件和下一代显示技术的关键需求为导向，用化学思想发展了新型光子学材料，同时以有机材料的光子学特异性为突破口，揭示分子在凝聚态下特殊的激发态动力学过程，发展传统的光化学理论。重点关注特定结构与功能的有机纳米光子学材料与器件的可控构筑，有机微纳晶体材料中的激发态过程与光子学功能的构效关系，以及有机柔性光子学集成器件等研究方向。 1. 通过有机材料特殊的激发态过程构筑了一系列全新性能的有机纳米激光器，阐明了有机材料全新的粒子数翻转机理与受激状态下的光化学和光物理过程，通过电荷转移、能量转移、激发态质子转移等过程得到了多波长、波长可调、单模激光等特殊性能微纳激光，并实现了全可见光范围的波长覆盖。 2. 揭示了有机材料的Frenkel激子与光子耦合形成激子极化激元（EP），利用这种半光半物质的准粒子，解决了传统光学器件中光子行为操纵的难题；在有机微纳体系中首次实现了室温下的激子极化激元玻色-爱因斯坦凝聚，在凝聚态下得到了与传统气、液、固态显著不同的激发态过程。 3. 发展了有机柔性光子器件加工技术，突破了有机材料集成化面临的关键技术瓶颈，构筑了集成光子回路以及大面积有机激光阵列，推动了有机激光材料在全色平板激光显示、可穿戴光子皮肤、光子学信息编码等领域的应用。 4. 针对本领域的研究需求，发展了多项具有自主知识产权的纳米光子学表征技术，相关仪器设备在多家高校、研究所及企业进行推广，极大提升了我国在纳米光电子领域的整体创新能力。

近期论文

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S. Ren, Z. F. Liu, P. Li, H. Liu, M. Lu, K. Wang, J. Yao, H. Dong, Q. Yang, Y. S. Zhao. "Steric engineering of HOF hierarchical branched homostructures for 3D photonic logic processing." Angew. Chem. Int. Ed. 2024, 63, e202415092. Y. Yao, Y. S. Zhao, L. Guan. "Steric engineering of HOF hierarchical branched homostructures for 3D photonic logic processing" Adv. Opt. Mater. 2024, 12, 2402260. K. Wang, Z. Y. Lin, A. De, C. A. Kocoj, W. Shao, H. Yang, Z. He, A. H. Coffey, C. B. Fruhling, Y. Tang, D. Varadharajan, C. Zhu, Y. S. Zhao, A. Boltasseva, V. M. Shalaev, P. Guo, B. M. Savoie, L. Dou. "Two-dimensional lattice confined single-molecule-like aggregates." Nature 2024, 633, 567-574. Q. Wang, Y. Niu, S. Zhang, Y. Hu, Z. Lou, Y. Hou, Y. S. Zhao, F. Teng, Q. Cui. "Micro-nano lasers based on aggregation-induced emission molecules: diverse resonant cavities investigation." ACS Appl. Mater. Interfaces 2024, 16, 44026-44032. S. Ji, M. Zeng, X. Zhan, H. Liu, Y. Zhou, K. Wang, Y. Yan, J. Yao, Y. S. Zhao. "Trion-triggered continuous-wave lasing in lithium ion-doped cuboidal perovskite microcrystals." CCS Chem. 2024, in press. S. Ji, M. Zeng, X. Zhan, H. Liu, Y. Zhou, K. Wang, Y. Yan, J. Yao, Y. S. Zhao. "Exceptionally high-glum circularly polarized lasers empowered by strong 2D-chiroptical response in a host-guest supramolecular microcrystal." J. Am. Chem. Soc. 2024, 146, 22583-22589. M. Lu, P. Li, X. Dong, Z. Jiang, S. Ren, J. Yao, H. Dong, Y. S. Zhao. "Adaptive Helical Chirality in Supramolecular Microcrystals for Circularly Polarized Lasing." Angew. Chem. Int. Ed. 2024, 63, e202408619. X. Liu, H. Liu, T. Zhang, K. Wang, J. Yao, H. Dong, Y. S. Zhao. "Continuous-wave organic Raman microlaser arrays for laser displays." Adv. Opt. Mater. 2024, 12, in press. J. Wang, T. Zhang, Z. Gao, M. Wei, Y. Jia, X. Tong, F. Hu, Y. S. Zhao. "Two-Dimensional Lanthanide-Metal Organic Framework Heterostructures for Noninvasively Photoresponsive High-Security Photonic Barcodes." ACS Appl. Mater. Interfaces 2024, 16, 23576-23584. K. Wang, J. H. Kim, J. Yang, X. Liu, Y. Dou, Y. Li, W. Tao, H. Dong, H. Zhu, K. Wu, L. N. Quan, F. Gao, J. Wang, L. Dou, Y. S. Zhao. "Luminesent metal-halide perovskites: fundamentals, synthesis, and light-emitting devices." Sci. China Chem. 2024, 67, 1766-1838. Y. Yao, Y. S. Zhao, L. Guan. "Dimension evolution of self-assembled organic microcrystal for laser and polarization-rotation function." Small 2024, 20, 2307661. J. Y. Park, R. Song, J. Liang, L. Jin, K. Wang, S. Li, E. Shi, Y. Gao, M. Zeller, S. T. Teat, P. Guo, L. Huang, Y. S. Zhao, V. Blum, L. Dou. "Thickness control of organic semiconductor-incorporated perovskites." Nat. Chem. 2023, in press. X. Liu, K. Wang, A. Ren. T. Zhang, S. Ren, J. Yao, H. Dong, Y. S. Zhao. "Continuous-wave Raman lasing from metal-linked organic dimer microcrystals." Angew. Chem. Int. Ed. 2023, 62, e202309386. X. Feng, R. Lin, S. Yang, Y. Xu, T. Zhang, S. Chen, Y. Ji, Z. Wang, S. Chen, C. Zhu, Z. Gao, Y. S. Zhao. "Spatially Resolved Organic Whispering-Gallery-Mode Hetero-Microrings for High-Security Photonic Barcodes." Angew. Chem. Int. Ed. 2023, 62, e202310263. J. Wang, J. Li, S. Sun, H. Dong, L. Wu, E. Zhao, F. He, X. Ma, Y. S. Zhao. "Revealing molecular diffusion dynamics in polymer microspheres by optical resonances." Science Advances 2023, 9, adf1725. C. Zhang, F. J. Shu, C. L. Zou, H. Dong, J. Yao, Y. S. Zhao. "Organic synthetic photonic systems with reconfigurable parity-time symmetry breaking for tunable single-mode microlasers." Adv. Mater. 2023, 35, 2300054. Y. Zhao, Z. Zhou, X. Liu, A. Ren, S. Ji, Y. Guan, Z. Liu, H. Liu, P. Li, F. Hu, Y. S. Zhao. "Chiral 2D/quasi-2D perovskite heterojunction nanowire arrays for high-performance full-Stokes polarization detection." Adv. Opt. Mater. 2023, 11, 2301239. W. Zhou, C. Zhang, A. Ren, H. Dong, J. Yao, Y. S. Zhao. "Smart liquid-crystal microlaser arrays with tactile perception." Adv. Opt. Mater. 2023, 11, 2202879. X. Zhan, Z. Zhou, W. Zhou, Y. Yan, J. Yao, Y. S. Zhao. "Wavelength-tunable circularly polarized laser arrays for multidimensional information encryption." Adv. Opt. Mater. 2023, 11, 2200872. S. Wen, W. Zhou, Z. Tian, Y. Yan, Y. S. Zhao. "Photoisomerization-controlled wavelength-tunable plasmonic lasers." Chem. Commun. 2023, 59, 7631-7634. Z. Gu, Y. Zhao, Y. Zhang, Z. Huang, Z. Zhou, K. Wang, L. Li, Y. S. Zhao, Q. Xu, Y. Song. "Ion aggregation-induced crystallization strategy for printing morphology-controllable perovskite single-crystal arrays and integrated devices." Chem. Mater. 2023, 35, 5127-5134. B. Xu, S. Yang, X. Feng, T. Zhang, Z. Gao, Y. S. Zhao. "Dual-stimuli responsive photonic barcodes based on perovskite quantum dots encapsulated in whispering-gallery-mode microspheres." Journal of Materiomics 2023, 9, 423-430. Z. Qu, P. Zhou, F. Min, S. Chen, M. Guo, Z. Huang, S. Ji, Y. Yan, X. Yin, H. Jiang, Y. Ke, Y. S. Zhao, X. Yan, Y. Qiao, Y. Song. "Bubble wall confinement-driven molecular assembly towards sub-12 nm and beyond precision patterning." Science Advances 2023, 9, eadf3567. B. Yin, H. Jia, H. Wang, R. Chen, L. Xu, Y. S. Zhao, C. Zhang, J. Yao. "Magnetic-Field-Driven Reconfigurable Microsphere Arrays for Laser Display Pixels." ACS Nano 2023, 17, 1187-1195. B. Yin, J. Liang, J. Hao, C. Dai, H. Jia, H. Wang, D. Wang, F. J. Shu, C. Zhang, J. Gu, Y. S. Zhao. "Nonconfinement growth of edge-curved molecular crystals for self-focused microlasers." Science Advances 2022, 8, eabn8106. Y. Guan, C. Zhang, Z. Liu, Y. Zhao, A. Ren, J. Liang, F. Hu, Y. S. Zhao. "Single-crystalline perovskite p-n junction nanowire arrays for ultrasensitive photodetection." Adv. Mater. 2022, 34, 2203201. H. Dong, C. Zhang, W. Zhou, J. Yao, Y. S. Zhao. "Differential polymer chain scission enables free-standing microcavity laser arrays." Adv. Mater. 2022, 34, 2107611. Z. Jiang, A. Ren, Y. Yan, J. Yao, Y. S. Zhao. "Exciton-polaritons and their Bose-Einstein condensates in organic semiconductor microcavities." Adv. Mater. 2022, 34, 2106095. H. Dong, C. Zhang, W. Nie, S. Duan, C. N. Saggau, M. Tang, M. Zhu, Y. S. Zhao, L. Ma, O. G. Schmidt. "Interfacial chemistry triggers ultrafast radiative recombination in metal halide perovskites." Angew. Chem. Int. Ed. 2022, 61, e202115875. X. T. Liu, B. B. Qian, T. Zhang, H. X. Nie, N. N. Xiao, H. Y. Shi, Z. Chang, Y. S. Zhao, X. H. Bu. "Programmable assembly of multiple donor-acceptor systems in metal-organic framework for heterogeneity manipulation and functions integration." Matter 2022, 5, 2918-2932. C. Qiao, C. Zhang, Z. Zhou, J. Yao, Y. S. Zhao. "Optically reconfigurable FRET process for broadband switchable organic single-mode microlasers." CCS Chem. 2022, 4, 250-258. A. Ren, J. Tang, Z. Jiang, Y. Yan, J. Yao, Y. S. Zhao. "Energy-controllable exciton–polariton Bose–Einstein condensation in perovskite microstrip cavities." Adv. Opt. Mater. 2022, 10, 2201126. J. Liang, Y. Du, K. Wang, A. Ren, X. Dong, C. Zhang, J. Tang, Y. Yan, Y. S. Zhao. "Ultrahigh color rendering in RGB perovskite micro-light-emitting diode arrays with resonance-enhanced photon recycling for next generation displays." Adv. Opt. Mater. 2022, 10, 2101642. Z. Liu, X. Qin, Q. H. Chen, Q. S. Chen, Y. Jing, Z. Zhou, Y. S. Zhao, J. Chen, X. Liu. "Highly Stable Lead-Free Perovskite Single Crystals with NIR Emission Beyond 1100 nm." Adv. Opt. Mater. 2022, 10, 2201254. X. Lin, W. Zhou, Y. Liu, F. J. Shu, C. L. Zou, C. Dong, C. Wei, H. Dong, C. Zhang, J. Yao, Y. S. Zhao. "3D-Printed Möbius Microring Lasers: Topology Engineering in Photonic Microstructures." Small 2022, 18, 2202812. W. Dong, C. Zhang, H. Dong, Z. Zhou, J. Yao, Y. S. Zhao. "Realization of Single-Crystal Dye Lasers by Taming Charge Transfer in Molecular Self-Assemblies." ACS Nano 2022, 16, 12345-12351. J. Liang, K. Wang, Y. Du, C. Zhang, Y. Yan, Y. S. Zhao. "Screen overprinted perovskite RGB microlaser arrays based on wet-solute-dynamics for full-color laser displays." ACS Appl. Mater. Interfaces 2022, 14, 1774-1782. Y. Guan, J. Liang, Y. Zhao, Z. Liu, Z. Zhou, S. Ji, Y. Jia, F. Hu, Y. S. Zhao. "Defect engineering in two-dimensional perovskite nanowire arrays by Europium (III) doping towards high-performance photodetection." Chem. Commun. 2022, 58, 7829-7832. Z. Zhou, C. Qiao, Y. Yan, J. Yao, Y. S. Zhao. "Exciton Funneling Amplified Photoluminescence Anisotropy in Organic Radical-Doped Microcrystals." J. Mater. Chem. C 2022, 10, 2551-2555. K. Wang, X. Gong, Y. S. Zhao, S. Makarov, B, P. Rand, L. Dou. "Halide Perovskites for Photonics and Optoelectronics: introduction to special issue." Opt. Mater. Express. 2022, 12, 1764-1766. L. Lian, T. Zhang, H. Ding, P. Zhang, X. Zhang, Y. B. Zhao, J. Gao, D. Zhang, Y. S. Zhao, J. Zhang. "Highly Luminescent Zero-Dimensional Organic Copper Halide with Low-Loss Optical Waveguides and Highly Polarized Emission." ACS Materials Lett. 2022, 4, 1446-1452. Y. Lv, Z. Xiong, Y. Li, D. Li, J. Liang, Y. Yang, F. Xiang, S. Xiang, Y. S. Zhao, Z. Zhang. "Framework-shrinkage-induced wavelength-switchable lasing from a single hydrogen-bonded organic framework microcrystal." J. Phys. Chem. Lett. 2022, 13, 130-135. D. Lin, J. Liu, H. Zhang, Y. Qian, H. Yang, L. Liu, A. Ren, Y. S. Zhao, X. Yu, Y. Wei, S. Hu, L. Li, S. Li, C. Sheng, J. Shen, H. Liu, Q. Feng, S. Wang, L. Xie, W. Huang. "Gridization-driven mesoscale self-assembly of conjugated nanopolymers into luminescence-anisotropic photonic crystals." Adv. Mater. 2022, 34, 2109399. F. F. Xu, W. Zeng, M J. Sun, Z. L. Gong, Z. Q. Li, Y. S. Zhao, J. Yao, Y. W. Zhong. "Organoplatinum(II) Cruciform: A Versatile Building Block to Fabricate 2D Microcrystals with Full-Color and White Phosphorescence and Anisotropic Photon Transport." Angew. Chem. Int. Ed. 2022, 61, e202116603. J. Yang, L. Guo, X. Yong, T. Zhang, B. Wang, H. Song, Y. S. Zhao, H. Hou, B. Yang, J. Ding, S. Lu. "Simulating the Structure of Carbon Dots via Crystalline π-Aggregated Organic Nanodots Prepared by Kinetically Trapped Self-Assembly." Angew. Chem. Int. Ed. 2022, 61, e202207817. D. Zhu, W. Jiang, Z. Ma, J. Feng, X. Zhan, C. Lu, J. Liu, J. Liu, Y. Hu, D. Wang, Y. S. Zhao, J. Wang, Z. Wang, L. Jiang. "Organic donor-acceptor heterojunctions for high performance circularly polarized light detection." Nat. Commun. 2022, 13, 3454. R. Chen, W. Zhou, Y. Gong, Z. Zhou, H. Wang, C. Dai, Y. S. Zhao, Y. Che, C. Zhang, J. Yao. "Accumulating bright excitons on the hybridized local and charge transfer excited state for organic semiconductor lasers." J. Mater. Chem. C 2022, 10, 9945-9952. K. Wang, Y. S. Zhao. "Pursuing electrically pumped lasing with organic semiconductors." Chem 2021, 7, 3221-3231. J. Tang, J. Zhang, Y. Lv, H. Wang, F. F. Xu, C. Zhang, L. Sun, J. Yao, Y. S. Zhao. "Room temperature exciton-polariton Bose-Einstein condensation in organic single-crystal microribbon cavities." Nat. Commun. 2021, 12, 3265. C. Zhang, H. Dong, C. Zhang, Y. Fan, J. Yao, Y. S. Zhao. "Photonic skins based on flexible organic microlaser arrays." Science Advances 2021, 7, eabh3530. J. Liang, Y. Yan, Y. S. Zhao. "Organic microlaser arrays: from materials engineering to optoelectronic applications." Acc. Mater. Res. 2021, 2, 340-351. T. Zhang, Z. Zhou, X. Liu, K. Wang, Y. Fan, C. Zhang, J. Yao, Y. Yan, Y. S. Zhao. "Thermally activated lasing in organic microcrystals towards laser displays." J. Am. Chem. Soc. 2021, 143, 20249-20255. H. Huang, H. Sato, J. Pirillo, Y. Hijikata, Y. S. Zhao, S. Z. D. Cheng, T. Aida. "Accumulated Lattice Strain as an Internal Trigger for Spontaneous Pathway Selection." J. Am. Chem. Soc. 2021, 143, 15319-15325. Y. Fan, C. Zhang, Z. Gao, Z. Zhou, J. Yao, Y. S. Zhao. "Randomly induced phase transformation in silk protein-based microlaser arrays for anti-counterfeiting." Adv. Mater. 2021, 33, 2102586. X. Zhan, F. F. Xu, Z. Zhou, Y. Yan, J. Yao, Y. S. Zhao. "3D Laser Displays Based on Circularly Polarized Lasing from Cholesteric Liquid Crystal Arrays." Adv. Mater. 2021, 33, 2104418. H. Dong, C. Zhang, F. Shu, C.-L. Zou, Y. Yan, J. Yao, Y. S. Zhao. "Superkinetic growth of oval organic semiconductor microcrystals for chaotic lasing." Adv. Mater. 2021, 33, 2100484. Z. Gao, S. Yang, B. Xu, T. Zheng, S. Chen, W. Zhang, X. Xu, Z. Wang, X. Wang, X. Meng, Y. S. Zhao. "Laterally Engineering Ln-MOFs Epitaxial Heterostructures for Spatially Resolved Planar 2D Photonic Barcoding." Angew. Chem. Int. Ed. 2021, 60, 24519-24525. F. Liu, T. Zhang, D. Mondal, S. Teng, Y. Zhang, K. Huang, D. Wang, W. Yang, P. Mahadevan, Y. S. Zhao, R. Xie, N. Pradhan. "Light emitting metal‐organic halide 1D and 2D structures: near‐unity quantum efficiency, low‐loss optical waveguide and highly polarized emission." Angew. Chem. Int. Ed. 2021, 60, 13548-13553. Z. Gao, B. Xu, Y. Fan, T. Zhang, S. Chen, S. Yang, W. Zhang, X. Sun, Y. Wei, Z. Wang, X. Wang, X. Meng, Y. S. Zhao. "Toplolgical distortion driven amorphous spherical MOFs for high quality single-mode microlasers." Angew. Chem. Int. Ed. 2021, 60, 6362-6366. Z. Gao, K. Wang, Y. Yan, J. Yao, Y. S. Zhao. "Smart responsive organic microlasers with multiple emission states for high-security optical encryption." Natl. Sci. Rev. 2021, 8, nwaa162. Z. Gong, X. Zhu, Z. Zhou, S. Zhang, D. Yang, B. Zhao, Y. Zhang, J. Deng, Y. Cheng, Y. Zheng, S. Zang, H. Kuang, P. Duan, M. Yuan, C. Chen, Y. S. Zhao, Y. Zhong, B. Z. Tang, M. Liu, "Frontiers in circularly polarized luminescence: molecular design, self-assembly, nanomaterials, and applications." Sci. China Chem. 2021, 64, 2060-2104. H. Dong, Y. S. Zhao. "Triplet management for room-temperature continuous-wave perovskite." Sci. China Chem. 2021, 64, 1-2. M. Wang, H. Li, C. Dai, J. Tang, B. Yin, H. Wang, J. Li, Y. Wu, C. Zhang, Y. S. Zhao, "Large-area periodic lead halide perovskite nanostructures for lenticular printing laser displays." Sci. China Chem. 2021, 64, 629-635. Y. Hou, Z. Zhou, C. Zhang, J. Tang, Y. Fan, F. F. Xu, Y. S. Zhao. "Full-color flexible laser displays based on random laser arrays." Sci. China Mater. 2021, 64, 2805-2812. Z. Liu, C. Zhang, X. Liu, A. Ren, Z. Zhou, C. Qiao, Y. Guan, Y. Fan, F. Hu, Y. S. Zhao. "Chiral hybrid perovskite single-crystal nanowire arrays for high-performance circularly polarized light detection." Adv. Sci. 2021, 8, 2102065. K. Wang, J. Liang, R. Chen, Z. Gao, C. Zhang, Y. Yan, J. Yao, Y. S. Zhao. "Geometry-Programmable Perovskite Microlaser Patterns for Two-Dimensional Optical Encryption." Nano Lett. 2021, 21, 6792-6799. H. Dong, C. N. Saggau, M. Zhu, J. Liang, S. Duan, X. Wang, H. Tang, Y. Yin, X. Wang, J. Wang, C. Zhang, Y. S. Zhao, L. Ma, O. G. Schmidt. "Perovskite origami for programmable microtube lasing." Adv. Funct. Mater. 2021, 31, 2109080. Y. Fan, C. Zhang, Y. Du, C. Qiao, K. Wang, Y. Hou, J. Yao, Y. S. Zhao. "A universal in situ cross-linking strategy enables orthogonal processing of full-color organic microlaser arrays." Adv. Funct. Mater. 2021, 31, 2103031. K. Pei, S. Ji, M. Zhao, C. Li, P. Luo, L. Jiang, Y. S. Zhao, T. Zhai. "2D metal-organic comples luminescent crystals." Adv. Funct. Mater. 2021, 31, 2106160. J. Zhao, Y. Zhao, Y. Guo, X. Zhan, J. Feng, Y. Geng, M. Yuan, X. Fan, H. Gao, L. Jiang, Y. Yan, Y. Wu, "Layered metal-halide perovskite single-crystalline microwire arrays for anisotropic nonlinear opitcs." Adv. Funct. Mater. 2021, 31, 2105855. P. Li, Z. Zhou, Y. S. Zhao, Y. Yan. " Recent advances in luminescent metal-organic frameworks and their photonic applications." Chem. Commun. 2021, 57, 13678-13691. H. Dong, C. Zhang, J. Yao. Y. S. Zhao. "Organic composite materials: understanding and manipulating excited states towards higher light-emitting performances." Aggregate 2021, 2, e103. Y. Zhang, C. Zhang, Y. Fan, Z. Liu, F. Hu, Y. S. Zhao. "Smart protein-based biolasers: an alternative way to protein conformation detection." ACS Appl. Mater. Interfaces 2021, 13, 19187-19192. Y. Lv, D. Li, A. Ren, Z. Xiong, Y. Yao, K. Cai, S. Xiang, Z. Zhang, Y. S. Zhao. "Hydrogen-bonded organic framework microlasers with conformation-induced color-tunable output." ACS Appl. Mater. Interfaces 2021, 13, 28662-28667. Y. Lv, Z. Xiong, Y. Yao, A. Ren, S. Xiang, Y. S. Zhao, Z. Zhang. "Controlled shape evolution of pure-MOF microcrystals towards efficienet waveguide and laser applications." Chem. Eur. J. 2021, 27, 3297-3301. F. Song, C. Zhang, H. Dong, Y. Fan, M. Y. Wu, G. G. Shan, P. Lai, H. Gao, Y. S. Zhao, S. Chen. "Switchable multimode microlaser based on AIE microsphere." J. Mater. Chem. C 2021, 9, 11180-11188. S. Li, M. Chu, Y. Du, Y. Yan, J. Yao, Y. S. Zhao. "Red, green, and blue high-color purity light sources based on polymer light-emitting electrochemical cells embedded in distributed Bragg reflector mirror microcavities." Chemistry (huaxue tongbao), 2021, 84, 53-57.