路军岭 - 中国科学技术大学 - 化学与材料科学学院

个人简介

2007年获中科院物理研究所博士学位。在攻读博士期间，曾赴德国弗里茨-哈伯马普所工作访问两年（2004至2006年）。2007至2013年，先后在美国西北大学表面与催化中心和美国阿贡国家实验室从事博士后研究工作。2013年3月，受聘为中国科学技术大学化学与材料科学学院、化学物理系教授，博士生导师。目前是《Chinese Chemical Letters》的青年编委。

研究领域

Atomic-Level Catalyst Smart Design Atomically-precise smart design of new catalytic materials using a combined wet-chemistry and ALD method Chemical Upgrading 1. Selective hydrogenation of dienes, unsaturated aldehydes, alkynes 2. Aerobic oxidation of alcohols 3. Biomass conversions 4. Alkenes epoxidation Clean Energy: Hydrogen production Hydrogen as a great clean energy source has attracted tremendous interest. The Lu research group is currently focusing on developing new generation of high performance catalysts in the application of CO-free hydrogen production for fuel cell applications. 1. Preferential CO oxidation in hydrogen (PROX) 2. Formic acid decomposition 3. Hydrolytic dehydrogenation of ammonia borane Clean Environment: CO2 utilization Global warming due to the accumulation of atmospheric CO2 has received widespread attention in recent years. Various techniques related to utilization of CO2 have been proposed. The Lu research group is currently focusing on the conversion of CO2 to valuable chemicals and energy products in the following two ways: 1. CO2 hydrogenation 2. CO2 reforming of methane

近期论文

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Q.M. Sun#, X.Y. Liu#, Q.Q. Gu, Z.H. Sun, H.W. Wang, L.N. Cao, Y.X. Xu, S. Li, B. Yang, S.Q. Wei, and J. L. Lu*Breaking the Conversion-Selectivity Trade-Off in Methanol Synthesis from CO2 Using Dual Intimate Oxide/Metal Interfaces J. Am. Chem. Soc. https://doi.org/10.1021/jacs.4c09106 (2024) L.H. Cai, L.N. Cao, and J. L. Lu* Confining volatile boron oxide species for stable oxidative dehydrogenation of propane Chem Catal. 4, 101067 (2024) Y. Li#, Y.X. Xu#, S. Chen#, X.X. Shi, Q.Q. Gu, L.L. Wang, M.H. Gu, B.T. Teng, B. Yang, Z.H. Sun, J. L. Lu*Tuning the Electronic Structures of Anchor Sites to Achieve Zero-Valence Single-Atom Catalysts for Advanced Hydrogenation Angew. Chem. Int. Ed. DOI: 10.1002/anie.202406262 (2024) X.Y. Liu, H.W. Wang*, J. L. Lu*Recent progress in understanding the nature of active sites for methanol synthesis over Cu/ZnO catalysts J. Catal. 436, 115561 (2024) L.H. Cai, S.L. Han, W.L. Xu, S. Chen, X.X. Shi, J. L. Lu*Formation of a Porous Crystalline Mg1‒x Al2Oy Overlayer on Metal Catalysts via Controlled Solid-State Reactions for High-temperature Stable Catalysis Angew. Chem. Int. Ed. 63, e202404398 (2024) H. Ye, L. N. Cao,* M.H. Gu, H. Nie, Q.Q. Gu, B. Yang, Y.X. Bai, Q.X. Nie, W.X. Huang, J. L. Lu* Atomically precise design of PtSn catalyst for the understanding of the role of Sn in propane dehydrogenation Precis. Chem., 2, 245–255 (2024) Q.Y. Wang, Y.D. Zhang, M.X. Lin, H.W. Wang, Y. Bai, C. Y. Liu, J. L. Lu, Q.Q. Luo, G. M. Wang, H.-L. Jiang, T. Yao, X. S. Zheng Photoinduced Metastable Asymmetric Cu Single Atoms for Photoreduction of CO2 to Ethylene Adv. Energy Mater., 13, 2302692 (2023) R. Jin, H.W. Wang*, J. L. Lu*Design of advanced energy-related materials via atomic layer deposition Sci. China Press., 68, 3670-3690 (2023) Q.Q.Guan, J. L. Lu*Degree-of-isolation shapes the catalytic performance of single-site alloy catalysts Sci. China Chem. 66, 2443-2444 (2023) (Invited highlight) C.W. Zhu#, W.L. Xu#, F. Liu, J. Luo, J. L. Lu*, and W.-X. Li*Molecule Saturation Boosts Acetylene Semihydrogenation Activity and Selectivity on a Core-Shell Ruthenium@Palladium Catalyst Angew. Chem. Int. Ed. 62, e202300110 (2023) J. Gu, Y.X. Xu and J. L. Lu* Atom-Precise Low-Nuclearity Cluster Catalysis: Opportunities and Challenges ACS Catal. 13, 5609-5634 (2023) X.Y. Liu#, Q.Q. Gu#, Y.F. Zhang, X.Y. Xu, H.W. Wang, Z.H. Sun, L.N. Cao, Q.M. Sun, L.L. Xu, L.L. Wang, S. Li, S.Q. Wei, B. Yang,* and J. L. Lu* Atomically thick oxide overcoating stimulates low–temperature reactive metal–support interactions for enhanced catalysis J. Am. Chem. Soc. Accepted (2023) X.X. Shi, S. Chen, S. Li, Y.Q. Yang, Q.Q. Guan, J.N. Ding, X.Y. Liu, Q. Liu, W.L. Xu, J. L. Lu*Particle size effect of SiO2-supported ZnO catalysts in propane dehydrogenation Catal.Sci.Technol. DOI : 10.1039/D2CY02131E (2023) X. H. Zhang,# Z.H. Sun,# R. Jin,# C.W. Zhu,# C.L. Zhao, Y. Lin, Q.Q. Guan, L.N. Cao, H.W. Wang, S. Li, H.C. Yu, X.Y. Liu, L.L. Wang, S.Q. Wei,* W.-X. Li,* J. L. Lu*Conjugated dual size effect of core-shell particles synergizes bimetallic catalysis Nat. Commun. 14, 530 (2023) L.L. Wang, H.W. Wang, and J. L. Lu*Local Chemical Environment Effect in Single-Atom Catalysis Chem Catal. 3, 100492 (2023) S. Li#, Y.X. Xu#, H.W. Wang*, B.T. Teng, Q. Liu, Q.H. Li, L.L. Xu, X.Y. Liu and J. L. Lu*Tuning the CO2 Hydrogenation Selectivity of Rhodium Single-Atom Catalysts on Zirconium Dioxide with Alkali Ions Angew. Chem. Int. Ed. 62, e202218167 (2023) Y.J. Zhao, Q.Q. Guan, H.Wang, Y. Li, J. L. Lu, R.-J. Xie*Waterproof surface passivation of K2GeF6:Mn4+ by a dense Al2O3 layer via atomic layer deposition J. Mater. Chem. C 10, 9867-9874 (2022) M.H. Gu, L.N. Cao*, H. Ye, J. L. Lu*Support effect and Stability of Inverse Fe1(OH)x/Pt Single-Site Interfacial Structured Catalysts for Preferential CO Oxidation in H2 J. Phys. Chem. C 126, 19676-19684 (2022) S. Chen,# B.B. Gong#, J. Gu#, Y. Lin, B. Yang, Q.Q. Gu, R. Jin, Q. Liu, W. X. Ying, X.X. Shi, W.L. Xu, L.H. Cai, Y. Li, Z.H. Sun,* S.Q. Wei, W.H. Zhang,* and J. L. Lu*Dehydrogenation of Ammonia Borane by Platinum-Nickel Dimers: Regulation of Heteroatom Interspace Boosts Bifunctional Synergetic Catalysis Angew. Chem. Int. Ed. 61, e202211919 (2022) X.H. Zhang#, Q.Q. Guan#, M. Sun, J. L. Lu*A comparison study of the structural thermostability of SiO2 supported Au@Pt and Au@Pd core-shell nanoparticles Chinese J. Chem. Phys. DOI: 10.1063/1674-0068/cjcp2204065 (2022) H.W. Wang, Y. Lin, J. L. Lu*Ultra-thin nickel oxide overcoating of noble metal catalysts for directing selective hydrogenation of nitriles to secondary amines Catal. Today 410, 253-263 (2023) X.Y. Liu#; J. Luo#; H.W. Wang#; L. Huang; S.S. Wang; S. Li; Z.H. Sun; F.F. Sun; Z. Jiang; S.Q. Wei*; W.-X. Li*; J. L. Lu*In Situ Spectroscopic Characterization and Theoretical Calculations Identify Partially Reduced ZnO1-x/Cu Interfaces for Methanol Synthesis from CO2 Angew. Chem. Int. Ed.134, e202202330 (2022) Y.D. Zhang, Q.Y. Wang, S.K. Yang, H.W. Wang, D.W. Rao, T. Chen, G.M. Wang, J. L. Lu, J.F. Zhu, S.Q. Wei, X.S. Zheng*, J. Zeng Tuning the Interaction between Ruthenium Single Atoms and the Second Coordination Sphere for Efficient Nitrogen Photofixation Adv. Funct. Mater. 2112452 (2022) J. L. Lu*Atomic Lego Catalysts Synthesized by Atomic Layer Deposition Acc. Mater. Res. 3, 358-368 (2022) L. L. Wang,# C. Z. Zhu,# C. L. Zhao, J. Gu, L. N. Cao, X. H. Zhang, Z. H. Sun, S. Q. Wei, W.-X. Li,* J. L. Lu*Boosting Activity and Stability of Metal Single-Atom Catalysts via Regulation of Coordination Number and Local Composition J. Am. Chem. Soc. 143, 45, 18854-18858 (2021) Q. Q. Guan#, C. W. Zhu#, Y. Lin, E. I. Vovk, X. H. Zhou, Y. Yang, H. C.Yu, L. N. Cao, H. W. Wang, X. H. Zhang, X. Y. Liu, S. Q. Wei, W. -X. Li*, J. L. Lu* Bimetallic monolayer catalyst breaks the activity–selectivity trade-off on metal particle size for efficient chemoselective hydrogenations Nat. Catal. 4, 840-849 (2021) D.-Y. Zhang, F. Liu, P.-F. Du, M.-W. Li, Z.X. Wu, Y. B. Feng, Y. Zhao, X.Y. Xu, X.X. Zhang, J. L. Lu, B. Yang Dynamic Formation of Pdδ+-Fe2+ Interface Promoting Reverse Water Gas Shift Reaction over Pd/FeOx Catalyst Chinese J. Inorg. Chem. 37, 140-150 (2021) C. Chen, W. Ou, K.-M. Yam, S.B. Xi, X.X. Zhao, S. Chen, J. Li, P. Lyu, L. Ma, Y.H. Du, W. Yu, H. Y. Fang, C.H. Yao, X. Hai, H. M. Xu, M. J. Koh, S. J. Pennycook, J. L. Lu, M. Lin, C. L. Su, C. Zhang, J. Lu Zero-Valent Palladium Single-Atoms Catalysts Confined in Black Phosphorus for Efficient Semi-Hydrogenation Adv. Mater. 33, 2008471 (2021) H. Zhang#, L.N. Cao#, Y.L. Wang, Z.D. Gan, F.F. Sun, M.L. Xiao, Y.Q. Yang, B.B. Mei, D.S. Wu,* J. L. Lu, H.Y. He,* Z. Jiang*Interfacial Proton Transfer for Hydrogen Evolution at the Sub-nanometric Platinum/Electrolyte Interface ACS Appl. Mater. & Inter., 13, 39, 47252-47261 (2021) J. Gu#, M. Z. Jian#, L. Huang#, Z. H. Sun, A. W. Li, Y. Pan, J. Z. Yang, W. Wen, W. Zhou, Y. Lin, H. J. Wang, X. Y. Liu, L. L. Wang, X. X. Shi, X. H. Huang, L. N. Cao, S. Chen, X. S. Zheng, H. B. Pan, J. F. Zhu, S. Q. Wei, W.-X. Li*, J. L. Lu*Synergizing metal-support interactions and spatial confinement boosts dynamics of atomic nickel for hydrogenations Nat. Nanotechnol. 16, 1141-1149 (2021) F. Liu#, Y.J. Xia#, W.L. Xu, L.N. Cao, Q.Q. Guan Q.Q. Gu, B. Yang, and J. L. Lu*Integration of Bimetallic Electronic Synergy with Oxide Site Isolation for Boosting Selective Hydrogenation of Acetylene Angew. Chem. Int. Ed. 60, 19324 (2021)