叶龙武 - 厦门大学 - 固体表面物理化学国家重点实验室

个人简介

博士后 (University of California at Santa Barbara，2009/05－2011/07) 博士后 (The Scripps Research Institute，2008/09－2009/05) 博士 (中科院上海有机所，2003/09－2008/07) 学士 (浙江大学化学系，1999/09－2003/07) 荣誉与获奖中科院院长优秀奖 (2008), 中科院优秀毕业生 (2008), 上海市自然科学一等奖 (2011), 福建省杰出青年科学基金 (2015), Thieme Chemistry Journals Award (2016), 国家优秀青年科学基金(2016), 教育部青年长江学者 (2017), 福建省青年拔尖人才 (2017)，厦门大学“田昭武学科交叉奖”一等奖 (2019)，国家杰出青年科学基金 (2021)等。

研究领域

有机合成方法学：基于炔烃转化的选择性控制与多样性合成；功能分子合成：生物活性分子、天然产物及药物的合成

近期论文

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Asymmetric Büchner reaction and arene cyclopropanation via copper-catalyzed controllable cyclization of diynes.Yan-Xin Zheng,‡ Li-Gao Liu,‡ Tian-Qi Hu, Xiao Li, Zhou Xu, Xin Hong,* Xin Lu, Bo Zhou, Long-Wu Ye,* Nat. Commun. 2024, 15, 9227. Copper-Catalyzed Enantioselective Dehydro-Diels–Alder Reaction: Atom-Economical Synthesis of Axially Chiral Carbazoles.Hua-Hong Chen,‡ Yang-Bo Chen,‡ Jun-Zhe Gao, Long-Wu Ye, Bo Zhou,* Angew. Chem. Int. Ed. 2024, 63, e202411709. Asymmetric one-carbon ring expansion of diverse N-heterocycles via copper-catalyzed diyne cyclization.Fu-Shuai Li,‡ Xiu-Yuan Zou,‡ Tian-Qi Hu, Qing Sun,* Zhou Xu, Bo Zhou, Long-Wu Ye,* Sci. Adv. 2024, 10, eadq7767. Copper-catalyzed intermolecular formal [4 + 1] annulation of 1,5-diynes with benzocyclobutenones.Jia-Cheng Li, Tian-Qi Hu, Zhou Xu,* Bo Zhou, Long-Wu Ye,* Tetrahedron Chem. 2024, 12, 100090. Tandem asymmetric dearomatized functionalization reaction of phenols with Evans-ynamides enabled by divergent electrophiles.Ying-Qi Zhang,‡ Gan-Lu Qian,‡ Yun Liu, Jia-Hui Li, Xin Hong*, Zhou Xu*, Bo Zhou, Long-Wu Ye,* Sci. China Chem. 2024, 67, in press. Catalytic Cycloaddition Reactions of Ynol and Thioynol Ethers.Ming-Yu Teng,* Yin Xu, Xin-Qi Zhu, Bo Zhou, Long-Wu Ye,* Chin. J. Chem. 2024, 42, 3469. Chiral Brønsted Acid-Catalyzed Asymmetric Reaction via Vinylidene ortho-Quinone Methides.Xin-Qi Zhu,* Hai-Yu Yang, Long-Wu Ye,* Chem. Eur. J. 2024, 30, 30, e202402247. Photo-Promoted Cascade Sigmatropic Rearrangement Reaction for the Synthesis of Polysubstituted 1,3-Conjugated Dienes.Yi-Kao Xu,‡ Ze-Shu Wang,‡ Wei-Min He,* Long-Wu Ye,* Chin. J. Org. Chem. 2024, 44, 2024. Catalytic Epoxidation of Carbonyl Compounds via Carbonyl Ylides: from Racemic to Enantioselective.Lin-Jun Qi,* Bo Zhou, Long-Wu Ye,* Chem. Eur. J. 2024, 30, e202401389. Copper-Catalyzed [2 + 2] Cyclization/Ring Expansion of Ene-Ynamides: Construction of Medium- and Large-Sized Rings.Nan Wang,‡ Hao-Jin Xu,‡ Ting Li,* Long-Wu Ye, Bo Zhou,* Org. Lett. 2024, 26, 3861. Gold-catalyzed intermolecular amination reaction of allyl azides with ynamides: efficient construction of 3-azabicyclo[3.1.0] scaffold.Chong-Yang Shi, Jian-Xing Gong, Zhen Li, Chao Shu, Long-Wu Ye,* Qing Sun,* Bo Zhou, Xin-Qi Zhu,* Chin. Chem. Lett. 2024, 35, in press. Research progress on the hydroamination of o-alkynylanilines for the synthesis of axially chiral indoles.Jia-Sheng Wang, Ze-Shu Wang, Wei-Min He,* Long-Wu Ye,* Chin. J. Org. Chem. 2024, 44, 1786. Gold Catalysis, Asymmetric Friedel–Crafts Alkylation Cascade for One-Pot Synthesis of Chiral Dihydrocarbazoles and Dihydrodibenzofurans.Xuan Wang, Ai-Hua Zhou, Tian-Qi Hu, Zhou Xu,* Bo Zhou, Long-Wu Ye,* Org. Lett. 2024, 26, 2051. Copper-catalyzed enantioselective desymmetrizing C(sp2)–H functionalization of azide-ynamides via α-imino copper carbenes.En-He Huang,‡ Li-Gao Liu,‡ You-Wei Yin, Hao-Xuan Dong, Ji-Jia Zhou,* Xin Lu,* Bo Zhou, Long-Wu Ye,* Sci. China Chem. 2024, 67, 2982. Enantioselective functionalization of unactivated C(sp3)–H bonds through copper-catalyzed diyne cyclization by kinetic resolution.Yang-Bo Chen, Li-Gao Liu, Zhe-Qi Wang, Rong Chang, Xin Lu,* Bo Zhou Long-Wu Ye,* Nat. Commun. 2024, 15, 2232. Organocatalytic Atroposelective Reactions of Alkynes.Zhi-Xin Zhang, Tian-Qi Hu, Long-Wu Ye, Bo Zhou,* Synthesis 2024, 56, 2316. Enantioselective Reaction of Diynes and Multiynes for the Synthesis of Axially Chiral Compounds.Xin-Qi Zhu,* Yu-Chao Li, Long-Wu Ye,* Asian J. Org. Chem. 2024, 13, e202300554. Brønsted Acid-Catalyzed Enantioselective Desymmetrization of 1,3-Diols: Access to Chiral β-Amino Alcohol Derivatives.Da-Qiu Cui, Yu-Qi Wang, Bo Zhou, Long-Wu Ye,* Org. Lett. 2023, 25, 9130. Copper-catalyzed atroposelective formal [4+1] annulation of 1,2-diketones with vinyl cations.Ze-Shu Wang,‡ Hao-Jin Xu,‡ Yang-Bo Chen, Long-Wu Ye,* Bo Zhou,* Peng-Cheng Qian,* Chem. Commun. 2023, 59, 14831. Chiral Brønsted acid-catalyzed asymmetric dearomative spirocyclization of alkynyl thioethers.Xin-Yang Fan, Jia-Cheng Li, Ji-Jia Zhou,* Bo Zhou, Long-Wu Ye,* Green Chem. 2023, 25, 10638. Asymmetric formal C–C bond insertion into aldehydes via copper-catalyzed diyne cyclization.Cui-Ting Li, Lin-Jun Qi, Li-Gao Liu, Chang Ge, Xin Lu,* Long-Wu Ye, Bo Zhou,* Nat. Commun. 2023, 14, 7058. Radical strategies for chemodivergent cyclization reactions.Ling-Tao Wang,‡ Bo Zhou,‡ Fa-Liang Liu, Wen-Ting Wei,* Long-Wu Ye,* Trends Chem. 2023, 5, 906. Catalytic asymmetric reaction of isoxazoles and benzisoxazoles.Xin-Qi Zhu,* Jia-Juan He, Bo Zhou, Long-Wu Ye,* Cell Rep. Phy. Sci. 2023, 4, 101645. Copper-catalyzed intermolecular formal (5+1) annulation of 1,5-diynes with 1,2,5-oxadiazoles.Can-Ming Chen, Ye-Nan Yang, Yin-Zhu Kong, Bo-Han Zhu, Peng-Cheng Qian,* Bo Zhou, Long-Wu Ye,* Commun. Chem. 2023, 6, 194. Asymmetric Metal Carbene gem-Dialkylation for the Construction of Chiral Quaternary Carbon Centers.Xin-Qi Zhu, Long-Wu Ye,* Chin. J. Org. Chem. 2023, 43, 3323. Recent Advances in Asymmetric Doyle-Kirmse Reaction.Chong-Yang Shi, Bo Zhou, Ming-Yu Teng,* Long-Wu Ye,* Synthesis 2023, 55, 3895. Recent advances in the construction of axially chiral arylpyrroles.Yang-Bo Chen, Ye-Nan Yang, Xuan-Zhu Huo, Long-Wu Ye, Bo Zhou,* Sci. China Chem. 2023, 66, 2480. Brønsted Acid-Catalyzed Intramolecular Hydroalkoxylation/Claisen Rearrangement of Ynamides.Tong-Yi Zhai, Chang Ge, Peng-Cheng Qian,* Bo Zhou, Long-Wu Ye,* Acta Chim. Sinica 2023, 81, 1101. Enantioselective Desymmetrizing Hydroalkoxylation of 1,4- and 1,8-Diynes Enabled by Chiral Brønsted Acid Catalysis.Yin Xu,‡ Gan-Lu Qian,‡ Da-Qiu Cui, Peng-Cheng Qian,* Chao-Yue Zhao, Xin Hong,* Bo Zhou, Long-Wu Ye,* ACS Catal. 2023, 13, 8803. Formal [4+1] annulations based on metal carbenes.Can-Ming Chen, Yin-Zhu Kong, Peng-Cheng Qian*, Bo Zhou, Long-Wu Ye,* Sci. Sin. Chem. 2023, 1377. Organocatalytic intramolecular (4 + 2) annulation of enals with ynamides: atroposelective synthesis of axially chiral 7-aryl indolines.Zhi-Xin Zhang,‡ Li-Gao Liu,‡ Yi-Xi Liu, Jian Lin, Xin Lu,* Long-Wu Ye, and Bo Zhou,* Chem. Sci. 2023, 14, 5918. Controllable cyclization of alkynyl thioethers via Brønsted acid-catalyzed dearomatization.Xin-Yang Fan,‡ Xin Liu,‡ Yin-Zhu Kong, Bo-Han Zhu, Jian Lin, Peng-Cheng Qian,* Bo Zhou, Long-Wu Ye,* Org. Chem. Front. 2023, 10, 2766. Construction of Axially Chiral Arylpyrroles via Atroposelective Diyne Cyclization.Yang-Bo Chen, Li-Gao Liu, Can-Ming Chen, Yi-Xi Liu, Bo Zhou,* Xin Lu,* Zhou Xu, Long-Wu Ye,* Angew. Chem. Int. Ed. 2023, 62, e202303670. Recent Advances in Catalytic Asymmetric Büchner Reaction.Chong-Yang Shi, Guang-Yu Zhu, Yin Xu, Ming-Yu Teng, Long-Wu Ye,* Chin. Chem. Lett. 2023, 34, 108441. Recent Advances in Asymmetric [1,2]-Stevens-Type Rearrangement via Metal Carbenes.Chong-Yang Shi, Bo Zhou, Ming-Yu Teng,* Long-Wu Ye,* Synthesis 2023, 55, 2118. Construction of Spirolactams by Unexpected Oxidative Cyclization of Alkenyl Diynes via Copper Catalysis.Chong-Yang Shi, Tao Han, Feng-Lin Hong, Long-Wu Ye,* Qing Sun,* Ming-Yu Teng,* Org. Lett. 2023, 25, 1525. Copper-catalyzed enantioselective diyne cyclization via C(sp2)–O bond cleavage.Ji-Jia Zhou,‡ Ya-Nan Meng,‡ Li-Gao Liu, Yi-Xi Liu, Zhou Xu,* Xin Lu,* Bo Zhou, Long-Wu Ye,* Chem. Sci. 2023, 14, 3493. Brønsted acid-catalyzed asymmetric dearomatization for synthesis of chiral fused polycyclic enone and indoline scaffolds.Tong-De Tan,‡ Gan-Lu Qian,‡ Hao-Ze Su, Lu-Jing Zhu, Long-Wu Ye,* Bo Zhou, Xin Hong,* Peng-Cheng Qian,* Sci. Adv. 2023, 9, eadg4648. Chiral Brønsted acid-catalyzed asymmetric intermolecular [4 + 2] annulation of ynamides with para-quinone methides.Hang-Hao Li,‡ Ya-Nan Meng,‡ Can-Ming Chen, Yu-Qi Wang, Zhi-Xin Zhang*, Zhou Xu*, Bo Zhou, Long-Wu Ye,* Sci. China Chem. 2023, 66, 1467. Copper-Catalyzed Enantioselective Doyle−Kirmse Reaction of Azide-Ynamides via α-Imino Copper Carbenes.Xin Liu, Li-Gao Liu, Can-Ming Chen, Xiao Li, Zhou Xu, Xin Lu,* Bo Zhou, Long-Wu Ye,* Angew. Chem. Int. Ed. 2023, 62, e202216923. Copper-catalyzed formal [4 + 1] annulation of N-propargyl ynamides with diketones.Hao-Jin Xu,‡ Cui-Ting Li,‡ Can-Ming Chen, Jie Chen, Xin-Qi Zhu,* Bo Zhou, Long-Wu Ye,* Org. Chem. Front. 2023, 10, 203. Biocatalytic Aminohydroxylation of Styrenes for Efficient Synthesis of Enantiopure β-Amino alcohols.Ruiwen Hu,‡ Anjie Gong,‡ Langxing Liao,‡ Yan-Xin Zheng,‡ Xin Liu, Peng Wu, Fushuai Li, Huili Yu, Jing Zhao, Long-Wu Ye,* Binju Wang,* Aitao Li,* Chin. J. Catal. 2023, 44, 171. Brønsted acid-catalyzed asymmetric dearomatization of indolyl ynamides: practical and enantioselective synthesis of polycyclic indolines.Zhi-Xin Zhang, Xuan Wang, Jia-Tian Jiang, Jie Chen, Xin-Qi Zhu,* Long-Wu Ye,* Chin. Chem. Lett. 2023, 34, 107647.