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Tf2O-Mediated mild synthesis of 6H-chromeno[4,3-b]quinolines Li-Ning Chen,† Zhao-Ke Jin,† Jian-Liang Ye,* and Pei-Qiang Huang* Arkivoc 2024 (5) 202412191
Vaska’s complex–PMHS combination enabled mild and chemoselective reduction of sulfoxides to sulfides with low catalyst loading Fang-Fang Xu, Zhong-Lei Ruan and Pei-Qiang Huang * Org. Chem. Front., 2024, 11, 2448
Evans’ Chiral Auxiliary-Based Asymmetric Synthetic Methodology and Its Modern Extensions Ling-Yan Chen,* Pei-Qiang Huang,* Eur. J. Org. Chem. 2023, 26, e202301131.
Catalytic Enantioselective Reductive Alkynylation of Amides Enables One-Pot Syntheses of Pyrrolidine/ Piperidine and Indolizidine Alkaloids,Fang-Fang Xu, Jin-Quan Chen, Dong-Yang Shao, and Pei-Qiang Huang*, Nat. Commun. 2023, 14: 6251. Correction: Nat. Commun. 2024, 15: 1836.
Heteroaromatization and Nickel Catalysis Enabled Decarbamoylative Arylations and Borylations of Tertiary Amides Hang Chen, Dong-Huang Chen, and Pei-Qiang Huang, Cell Reports Physical Science 2023, 4: 101574. DOI: 10.1016/j.xcrp.2023.101574
Concise, three-step enantioselective total synthesis of (4S,5S)-4-hydroxy-5-octylpyrrolidin-2-one, a colibactin pathway metabolite Dong-Yang Shao and Pei-Qiang Huang*, Arkivoc 2023, ii, ii, 202312048. DOI: https://doi.org/10.24820/ark.5550190.p012.048
Concise Total Synthesis of (−)-Quinocarcin Enabled by Catalytic Enantioselective Reductive 1,3-Dipolar Cycloaddition of Secondary Amides Kan-Lei Ji†, Shu-Fan He†, Dong-Dong Xu, Wen-Xin He,Jian-Feng Zheng* and Pei-Qiang Huang* Angew. Chem. Int. Ed. 2023, e202302832.
One-pot synthesis of 1,3-oxazin-4-ones through an Ir-catalyzed mild formal condensation reaction of secondary amides with acyl chlorides Si-Jia Yu,‡ Jie Li,‡ Jian-Liang Ye * and Pei-Qiang Huang * Org. Chem. Front. 2023, 10, 1994-2001. DOI: 10.1039/d3qo00092c
Iridium and B(C6F5)3 co-catalyzed chemoselective deoxygenative reduction of tertiary amides: application to the efficient synthesis and late-stage modification of pharmaceuticals Feng Han†, Guang-Sheng Lu†, Dong-Ping Wu, Pei-Qiang Huang* SCIENCE CHINA Chemistry 2023, 66, 1094-1100. https://doi.org/10.1007/s11426-022-1501-y
Investigation of a novel approach to the core of stemofoline: enantioselective construction of a bicyclic intermediate with three contiguous chiral centers Long-Hui Gao, Jian-Liang Ye, Pei-Qiang Huang* Sci Sin Chim 2023, 53, 564–571.doi: 10.1360/SSC-2022-0237
Tf2O-Promoted Morgan–Walls Reaction: from A Flexible Approach to Functionalized Phenanthridines and Quinazolines to the Short and Divergent Total Syntheses of Alkaloids Xiao-Yu Su, Pei-Qiang Huang,* Synthesis 2023, 55, 877-891. DOI: 10.1055/a-1957-4343. Editor-in-Chief SYNTHESIS, Prof. Dr. Paul Knochel 邀稿：Feature Article栏目
Redox-Neutral Synthesis of α-Iminonitriles, α-Cyanoenamines, and N-Acyl Derivatives from Amides Ting-Ting Chen, Hui Geng, Zheng-Yun Weng, and Pei-Qiang Huang* ACS Earth Space Chem. 2023, 7, 243–251. 论文链接：https://doi.org/10.1021/acsearthspacechem.2c00315
Multicatalysis protocol enables direct and versatile enantioselective reductive transformations of secondary amides, Hang Chen,† Zhi-Zhong Wu,† Dong-Yang Shao, and Pei-Qiang Huang*, Sci. Adv. 2022, 8, eade3431.
A Flexible Enantioselective Synthesis Route Approach to 2,5-Disubstituted cis-Decahydroquinolines Qi-Wei Lang,a Xiang-Yang Qian,a Xiu-Lin He,a Hui Geng,a Jian-Feng Zheng*,a,b and Pei-Qiang Huang*,a Tetrahedron 2022, 122, 132935.
The Iridium-Catalyzed Chemoselective Deaminative Knoevenagel-type Reaction of Amides, Dong-Ping Wu1, Wei Ou1,2 and Pei-Qiang Huang1* Org. Lett. 2022, 24, 5366-5371.
Versatile One-Pot Synthesis of α-Amino Bisphosphonates from Nitriles via Tf2O/HC(OR)3-Mediated Interrupted Ritter-type Reaction, Ya-Cheng Hong, Jian-Liang Ye*, and Pei-Qiang Huang* J. Org. Chem. 2022, 87, 9044-9055.
Catalyst- and Solvent-Free Aminolysis of the Asymmetric Derivatives of Evans’ Chiral N-Acyloxazolidinones: Enantioselective Synthesis of Chiral Amides and Its Applications Hui-Rong Lu,†,a Hui Geng,†,a Guan-Tian Ding,†,a and Pei-Qiang Huang*,aGreen Chem. 2022, 24, 4405. DOI: 10.1039/D2GC00662F https://doi.org/10.1039/D2GC00662F
Tandem Catalysis Enabled Highly Chemoselective Deoxygenative Alkynylation and Alkylation of Tertiary Amides: A Versatile Entry to Functionalized a-Substituted Amines Xiao-Gang Wang,a,† Wei Ou,a,b,† Mu-Han Liu,a Zhan-Jiang Liua and Pei-Qiang Huanga,*, Org. Chem. Front. 2022, 9, 3237. DOI: 10.1039/D2QO00335J
Enantioselective Total Syntheses of Marine Natural Products (+)-Cylindricines C, D, E and Their 2-epi-Diastereomers, Ying-Hong Huang,§ Zhan-Jiang Liu,§ and Pei-Qiang Huang* Org. Chem. Front. 2022, 9, 58-63. 标注：21931010 and the National Key R&D Program of China (grant No. 2017YFA0207302).
Asymmetric Deoxygenative Alkynylation of Tertiary Amides Enabled by Iridium/Copper Bimetallic Relay Catalysis, Zhaokun Li,[a] Feng Zhao,[a] Wei Ou,[b] Pei-Qiang Huang,*[b] Xiaoming Wang*[a,c] Angew. Chem. Int. Ed. 2021, 60, 26604-26609. Angew. Chem. 2021, 133, 26808-26813. https://doi.org/10.1002/anie.202111029 First Published: 01 October 2021
Synthesis of 5-(1-Alkoxyalkylidene)tetronates by Direct Condensation Reactions of Tetronates with Thionolactones and Thionoesters Ya-Qing Huang,† Xiong-Zhi Huang,† and Pei-Qiang Huang* J. Org. Chem. 2021, 86, 16926-16939. https://doi.org/10.1021/acs.joc.1c02098 Dedicated to E. J. Baldwin
Tf2O/TTBP (2,4,6-tri-tert-Butylpyrimidine): An Alternative Amide Activation System for the Direct Transformations of Both Tertiary and Secondary Amides, Qian He, Jian-Liang Ye, Fang-Fang Xu, Hui Geng, Ting-Ting Chen, Hang Chen, and Pei-Qiang Huang*, J. Org. Chem. 2021, 86, 16300-16314. 内封面
SmI2/Sm-Arylboronic Esters Combination for the Reductive Arylation of Aromatic Tertiary Amides Wang, A. E and Huang, P. Q. Chin. J. Org. Chem. 2021, 41, 3738-3739.
Enantioselective Total Syntheses of the Proposed and Revised Structures of Methoxystemofoline: A Stereochemical Revision, Su-Yu Huang, Long-Hui Gao, Xiong-Zhi Huang, and Pei-Qiang Huang* J. Org. Chem. 2021, 86, 11053-11071. https://dx.doi.org/10.1021/acs.joc.0c02667
Biomimetic Total Synthesis of Natural Products: Retrospect and Prospect, J Xiamen Univ. Nat. Sci., 2021, 60, 149-159. (in Chinese)
A versatile approach to functionalized cyclic ketones bearing quaternary carbon stereocenters via organocatalytic asymmetric conjugate addition of nitroalkanes to cyclic b-substituted a,b-Enones, Si-Jia Yu, Ya-Nan Zhu, Jian-Liang Ye*, Pei-Qiang Huang, ** Tetrahedron 2021, 84, 132005.
Chemoselective Reactions of Isocyanates with Secondary Amides: One-Pot Construction of 2,3-Dialkyl-Substituted Quinazolinones, Yi Lin, Shu-Fan He, Hui Geng, Yu-Chen Xiao, Kan-Lei Ji, Jian-Feng Zheng,* and Pei-Qiang Huang* J. Org. Chem. 2021, 86, 5345−5353.
Enantioselective Reductive Cyanation and Phosphonylation of Secondary Amides by Iridium and Chiral Thiourea Sequential Catalysis, Dong-Huang Chen+, Wei-Ting Sun+, Cheng-Jie Zhu+, Guang-Sheng Lu, Dong-Ping Wu, Ai-E Wang,* and Pei-Qiang Huang* Angew. Chem. Int. Ed. 2021, 60, 8827-8831. Angew. Chem. 2021, 133, 8909-8913. DOI: 10.1002/anie.202015898
Synthesis of 5-(1-Alkoxyalkylidene)tetronates by Direct Condensation Reactions of Tetronates with Thionolactones and Thionoesters Ya-Qing Huang,† Xiong-Zhi Huang,† and Pei-Qiang Huang* J. Org. Chem. 2021, 86, 2359-2368. https://dx.doi.org/10.1021/acs.joc.0c02502
Photoredox-Catalyzed Decarboxylative Cross-Coupling of α-Amino acids with Nitrones Heng-Hui Li,† Jia-Qi Li,† Xiao Zheng*, and Pei-Qiang Huang* Org. Lett. 2021, 23, 876-880. https://dx.doi.org/10.1021/acs.orglett.0c04101
Organocatalytic Asymmetric Synthesis of an Advanced Intermediate of (+)-Sarain A Xiu-Ning Hu, Dong-Ping Wu,‡ Ye-Peng Xu,‡ and Pei-Qiang Huang* Chem. Eur. J. 2021, 27, 609-613.oi.org/10.1002/chem.202004261
Enantioselective total syntheses of (+)-stemofoline and three congeners based on a biogenetic hypothesis Xiong-Zhi Huang, Long-Hui Gao, Pei-Qiang Huang* Nature Commun. 2020, 11: 5314. https://doi.org/10.1038/s41467-020-19163-4
Catalytic Asymmetric Total Synthesis of Macrocyclic Marine Natural Product (-)-Haliclonin A Shi-Peng Luo,†,a,b Xiong-Zhi Huang,† Lian-Dong Guo,† and Pei-Qiang Huang,* Chin. J. Chem. 2020, 38, 1723-1736
Procedure-Economical, Enantioselective Total Syntheses of Polycyclic Natural Products and Analogs Containing a 3a-Hydroxyhexahydropyrrolo[2,3-b]indole-2-carboxylic Acid Residue Huang Pei-Qiang,* Synlett 2020, 31, 1681-1690. DOI: 10.1055/s-0040-1707164.
Catalytic Diastereoselective and Enantioconvergent C(sp3)–C(sp3) Cross-Coupling of Racemic Partners Wang Ai-E,* Huang Pei-Qiang,* Sci. China-Chem. 2020, 63, 871-872. https://doi.org/10.1007/s11426-020-9745-1
Ni-Catalyzed Direct Alcoholysis of N-Acylpyrrole-Type Tertiary Amides under Mild Conditions Hang Chen, Dong-Huang Chen and Pei-Qiang Huang, Sci. China-Chem. 2020, 63, 370-376. doi: 10.1007/s11426-019-9665-5
Amides as Surrogates of Aldehydes for C-C Bond Formation: Amide-Based Direct Knoevenagel-Type Condensation Reaction and Related Reactions Ou W.; Huang P.-Q. Sci. China-Chem. 2020, 63, 11-15. doi: 10.1007/s11426-019-9586-3
Two-step Catalytic Transformation of N-Benzyllactams to Alkaloids (±)-Solenopsin, (±)-Solenopsin A, and (+)-Julifloridine Wei Ou, Guang-Sheng Lu, Dong An, Feng Han, and Pei-Qiang Huang, Eur. J. Org. Chem. 2020, 52-56. DOI: 10.1002/ejoc.201901752 Dedicated to the memory of the late Professor Michel Che for his contribution to catalysis Featured in Org. Chem. Portal Highlights: Alkaloid Synthesis: https://www.organic-chemistry.org/Highlights/2020/16November.shtm
Concise, Enantioselective Total Syntheses of both Proposed and Revised Structures of (-)-Versiquinazoline H, Jiang-Feng Wu and Pei-Qiang Huang* Chin. Chem. Lett. 2020, 31, 61-63. DOI: 10.1016/j.cclet.2019.06.043
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