陆洲 - 安徽师范大学 - 物理与电子信息学院

个人简介

教育经历 1996年 - 2001年中国科学技术大学化学物理系理学学士 2001年 - 2007年 University of California, San Diego 化学与生物化学系博士工作经历 2007 - 2010 美国University of Southern California 化学系博士后 2010 - 2013 美国能源部太平洋西北国家实验室分子环境科学实验室博士后 2013 – 2019 中国科学院化学研究所分子反应动力学国家重点实验室研究员、博士生导师 2019 – 今安徽师范大学物理与电子信息学院教授、博士生导师人才入选情况 2013 中国科学院化学研究所“引进国外杰出青年人才”计划 2014 中国科学院“引进杰出技术人才”计划（中科院“技术百人”计划） 2020 安徽省“皖江学者”特聘教授

研究领域

（1）界面电荷转移动力学发展具有超快时间分辨的二阶非线性谱学新方法，拓展光谱检测范围，针对光电转换分子器件给-受体界面处的电子激发态行为进行原位测量，在分子与量子态层次上理解无机-有机杂化半导体以及低维材料界面分子的构象与光电性能之间的依赖关系，深入研究介电层-半导体层界面处的电荷注入和电荷传输等基本物理过程，揭示电荷分离与转移的驱动力。此外，发展兼具超快时间分辨与亚微米空间分辨的可视化动态荧光寿命成像技术，结合低温控制手段，探索半导体光电材料的温度依赖相变行为以及缺陷态分布对载流子动力学之间的影响；综合利用瞬态吸收、时间分辨荧光与界面非线性光谱等技术，研究外场对半导体器件晶格结构与性能的调控规律，为提高光电转换效率与光伏材料的使用寿命提供相关机理。（2）非均相界面反应动力学面向人工光合作用、有机污染物光降解治理、温和环境条件下电催化合成高附加值化工产品等重要应用领域，发展表面增强与相位敏感的二阶非线性光学新技术，提高非线性谱学探测灵敏度与适用范围，并结合多时域谱学表征手段，研究非均相光催化与电催化过程中的分子机制。主要关注半导体光催化体系中载流子的产生、扩散、捕获、复合以及分子在半导体界面的活化过程，探讨表面等离子体基元纳米催化体系与目标分子间的电子-振动态耦合机制，探究电场调控下电极表面不同动力学步骤之间相互竞争关系，捕获相关界面反应的瞬态物种，确定非均相反应的控速关键步骤。（3）分子基光敏剂的激发态动力学针对新型光敏材料制备和性能调控，设计并构筑具有独特光物理特性的有机共轭小分子与超分子光敏剂，利用飞秒-纳秒-微秒瞬态吸收、时间分辨荧光寿命、时间分辨电子自旋共振谱等技术，测量光敏分子或超分子结构中不同光敏单元的激发态寿命，确定分子内和分子间能量转移和转化的通道分支比与微观速率常数，探索分子间能量转移过程与分子构型以及能级结构等之间的内在联系，利用金属配位、超分子拓扑结构、自组装等方法对光敏剂能级范围与势能面进行人工调控，建立完善的激发态动力学过程机制，拓展有机共轭小分子与超分子光敏剂在光子上转换、光动力治疗、生物活体光学探针示踪等领域的实际应用价值。

近期论文

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Chunyi Zhao; Qi Sun*; Peng Xu; Longwen Chen; Rumeng Shi; Lingchen Meng; Yongfu Liang; Yanfeng Yin; Guanxin Yao; Xianyi Zhang; Zhou Lu*; Wenming Tian*; Shengye Jin. “Highly Diffusive Nonluminescent Carriers in Hybrid Phase Lead Triiodide Perovskite Nanowire”. Angewandte Chemie International Edition, DOI: 10.1002/anie.202411499, in press (2024). (Link) Yingcui Bu; Zhi-Peng Yu; Zhou Lu; Haoran Wang; Beibei Tian; Xiaojiao Zhu*; Hongping Zhou*. “In-Situ Self-Assembled Near-Infrared Phototherapeutic Agent: Unleashing Hydrogen Free Radicals and Coupling with NADPH Oxidation”. Chemical Science 15, 12559-12568 (2024). (Link) Min Zhou; Haozhi Wang; Rong Liu; Zheyang Liu; Xinyan Xiao; Weilin Li; Chao Gao; Zhou Lu; Zhifeng Jiang*; Weidong Shi*; Yujie Xiong*. “Construction of Frustrated Lewis Pairs in Poly(heptazine imide) Nanosheets via Hydrogen Bonds for Boosting CO2 Photoreduction”. Angewandte Chemie International Edition 63, e202407468 (2024). (Link) Guanlun Sun; Hong Li; Jian Hou; Hong Wang; Jinzhao Wang; Zhou Lu*; Xin Gao*. “Molecular Behavior of Ethylene Glycol/1,2-Butanediol Mixtures at the Vapor–Liquid Interface”. Industrial & Engineering Chemistry Research 63, 4853-4865 (2024). (Link) Daochuan Jiang; Zhongfei Li; Hao Li; Yingpeng Cheng; Haiwei Du; Chuhong Zhu; Lingchen Meng; Yuetong Fang; Chunyi Zhao; Zaizhu Lou*; Zhou Lu*; Yupeng Yuan*. “Achieving Long-Lived Charge Separated State through Ultrafast Interfacial Hole Transfer in Redox Sites-Isolated CdS Nanorods for Enhanced Photocatalysis”. Small 20, 202310414 (2024). (Link) Manman Shi: Dian Luo; Peng Wu; Yarong Shen; Jieding Wei; Saiya Guo; Zhou Lu*; Yucheng Huang*; Yonghong Ni*. “Manipulating the Electronic Structure of Platinum via Alloying with Ruthenium to Boost Photocatalytic Selective Hydrogenation with Water as a Proton Source”. Science China Materials 67, 824-832 (2024). (Link) Guiyuan Wu*; Huimin Zhu; Hao Li; Kai Zhang; Xianyi Zhang; Dong Yan; Xiudu Zhang; Lili Lin*; Zhou Lu*. “The Impact of Aggregation of AIE and ACQ Moiety-Integrating Material on the Excited State Dynamics”. RSC Advances 13, 33911-33917 (2023). (Link) Yan Gao; Kai Zhang*; Zhou Lu; Xiaojun Wu*. “Fluorination and Conjugation Engineering Synergistically Enhance the Optoelectronic Properties of Two-Dimensional Hybrid Organic-Inorganic Perovskites”. ACS Applied Materials and Interfaces 15, 46205-46212 (2023). (Link) Le Luo; Hao Li; Zhou Lu*; Zhenghua Wang*. “Boosting Carrier-Phonon Scattering in Cu2-xS Nanochains for 90.5% Photothermal Conversion Efficiency in Near-Infrared Ⅱ Region.” Journal of Physical Chemistry Letters 14, 5531-5536 (2023). (Link) Liang Zhu; Daochuan Jiang; Zhifu Liang; Hao Li; Haiwei Du; Chuhong Zhu; Huiquan Li*; Zhou Lu*; Yupeng Yuan*. “A π-Conjugated van der Waals Heterostructure between Single-Atom Ni-anchored Salphen-Based Covalent Organic Framework and Polymeric Carbon Nitride for High-Efficiency Charge Separation”. Small 19, 2301017, (2023). (Link) Yanan Bo; Pengye Du; Hao Li; Rong Liu; Chengming Wang; Hengjie Liu; Dong Liu; Tingting Kong*; Zhou Lu*; Chao Gao*; Yujie Xiong*. “Bridging Au Nanoclusters with Ultrathin LDH Nanosheets via Ligands for Enhanced Charge Transfer in Photocatalytic CO2 Reduction”. Applied Catalysis B – Environmental 330, 122667 (2023). (Link) Ziye Zhang; Liteng Ren; Hao Li; Daochuan Jiang; Yuetong Fang; Haiwei Du; Gengsheng Xu; Chuhong Zhu; Huiquan Li*; Zhou Lu*; and Yupeng Yuan*. “π-Conjugated In-Plane Heterostructure Enables Long-Lived Shallow Trapping in Graphitic Carbon Nitride for Increased Photocatalytic Hydrogen Generation”. Small 19, 2207173 (2023). (Link) Canyu Hu; Xing Chen; Jingxiang Low; Yaw-Wen Yang; Hao Li; Di Wu; Shuangming Chen; Jianbo Jin; He Li; Huan-Xin Ju; Chia-Hsin Wang; Zhou Lu; Ran Long*; Li Song; Yujie Xiong*. “Near-Infrared-Featured Broadband CO2 Reduction with Water to Hydrocarbons by Surface Plasmon”. Nature Communications 14, 221 (2023). (Link) Junjun Wang; Hao Li; Yicai Zhu; Mingdi Yang; Jing Huang; Xiaojiao Zhu; Zhipeng Yu*; Zhou Lu; Hongping Zhou*. “Unveiling Upsurge of Photogenerated ROS: Control of Intersystem Crossing through Tuning Aggregation Patterns”. Chemical Science 14, 323-330 (2023). (Link) Xiaotong Wang; Rong Liu; Limei Tian; Jingwen Bao; Chunyi Zhao; Fushuang Niu; Dajiao Cheng; Zhou Lu; Ke Hu*. “Highly Luminescent NHC-Stabilized Au13 Clusters as Efficient Excited State Electron Donors”. Journal of Physical Chemistry C 126, 18374-18382 (2022). (Link) Dian Luo; Yao Luo; Xiangyu Lu; Manman Shi; Jieding Wei; Zhou Lu*; Yucheng Huang*; Yonghong Ni*. “Cooperative Selective Benzyl Alcohol Oxidation and Hydrogen Production over Pd6(SC12H25)12 Cluster-Coupled CdS Nanorods: The Key Role of Water in Photocatalytic Benzyl Alcohol Splitting”. Journal of Materials Chemistry A 10, 15941-15948 (2022). (Link) Meilin Duan; Canyu Hu; Hao Li; Yihong Chen; Ruitian Chen; Wanbing Gong; Zhou Lu*; Ning Zhang*; Ran Long*; Li Song; Yujie Xiong*. “Synergizing Inter- and Intra-Band Transitions in Defective Tungsten Oxide for Efficient Photocatalytic Alcohol Dehydration to Alkene”. JACS Au 2, 1160-1168 (2022). (Link) Fuzhan Song; Tong Zhang; Dexia Zhou; Pengfei Sun; Zhou Lu*; Hongtao Bian*; Jingshuang Dang*; Hong Gao; Yuqin Qian; We Li; Nan Jiang; Haley Dummer; Jeremy Shaw; Shutang Chen; Gugang Chen*; Yujie Sun*; Yi Rao*. “Charge Transfer of Interfacial Catalysts for Hydrogen Energy”. ACS Materials Letters 4, 967-977 (2022). (Link) Xiangyu Lu; Aomei Tong; Dian Luo; Fan Jiang; Jieding Wei; Yucheng Huang*; Zheng Jiang; Zhou Lu*; Yonghong Ni*. “Confining Single Pt Atom from Pt Clusters CdS for Enhanced Photocatalytic Hydrogen Evolution”. Journal of Materials Chemistry A 10, 4594-4600 (2022). (Link) Tong Zhang; Zhichao Huangfu; Yuqin Qian; Zhou Lu*; Hong Gao*; and Yi Rao*. “Spectral Phase Measurements of Heterodyne Detection in Interfacial Broadband Electronic Spectroscopy”. Journal of Physical Chemistry C 126, 2823-2832 (2022). (Link) Shengnan Wang; Mengtao Rong; Hao Li; Tianren Xu; Yingcui Bu; Lei Chen; Xiaoqin Chen; Zhipeng Yu*; Xiaojiao Zhu; Zhou Lu*; Hongping Zhou*. “Unveiling Mechanism of Organic Photogenerator for Hydroxyl Radicals Generation by Molecular Modulation”. Small 18, 202104857 (2022). (Link) Guiyuan Wu*; Hongjuan Zhu; Fangfang Pan; Xiaowei Sheng; Mingrui Zhang; Xianyi Zhang; Guangxin Yao; Hang Qu*; Zhou Lu*. “Self-Assembly of [3]Catenane and [4]Catenane Based on Neutral Organometallic Scaffolds”, Frontiers in Chemistry 9, 805229 (2021). (Link) Guiyuan Wu*; Chao Liang; Hao Li; Xianyi Zhang; Guanxin Yao; Fanfan Zhu; Yixiong Hu; Guangqiang Yin; Wei Zheng*; Zhou Lu*. “Multi-Responsive Supramolecular Heparin-Based Biohybrid Metallogel Constructed by Controlled Self-Assembly Based on Metal–Ligand, Host-Guest and Electrostatic Interactions”. Organic Chemistry Frontiers 8, 4715-4722 (2021). (Link) Guiyuan Wu*; Chao Liang; Yixiong Hu; Xuqing Wang; Guangqiang Yin; Zhou Lu*. “Hierarchical Self-Assembly of Discrete Bis-[2]pseudorotaxanes Metallacycle with Bis-pillar[5]arene via Host-Guest Interactions and Their Redox-Responsive Behaviors”. RSC Advances 11, 1187-1193 (2021). (Link) Kaixi Sun; Tong Zhang; Liming Tan; Dexia Zhou; Yuqin Qian; Xiaoxia Gao; Fahui Song*; Hongtao Bian*; Zhou Lu*; Jingshuang Dang; Hong Gao; Jeremy Shaw; Shutang Chen; Gugang Chen; Yi Rao*. “Interface Catalysts of Ni/Co2N for Hydrogen Electrochemistry”. ACS Applied Materials and Interfaces 12, 29357-29364 (2020). (Link) Jian Hou; Guanlun Sun; Jianchuan Liu; Xin Gao*; Xianyi Zhang; Zhou Lu*. “Liquid/Vapor Interface of Dimethyl Carbonate−Methanol Binary Mixtures Investigated by Sum Frequency Generation Vibrational Spectroscopy and Molecular Dynamics Simulation”. Journal of Physical Chemistry B 124, 4211-4221 (2020). (Link) Jian Hou; Xianyi Zhang; Zhou Lu*. “Comparing Vibrational Sum Frequency Generation Responses at Fused Silica and Fluorite/Liquid Ethanol Interfaces”. Chemical Physics 536, 110814 (2020). (Link) Jean-Francois Boily*; Li Fu; Ashish Tuladhar; Zhou Lu; Benjamin A. Legg; Zheming Wang; Hongfei Wang. “Hydrogen Bonding and Molecular Orientations across Thin Water Films on Sapphire”. Journal of Colloid and Interface Science 555, 810-817 (2019). (Link) Jianchuan Liu; Xia Li; Jian Hou; Xun Li; Zhou Lu*. “The Influence of Sodium Iodide Salt on the Interfacial Properties of Aqueous Methanol Solution by a Combined Molecular Simulation and Sum Frequency Generation Vibrational Spectroscopy Study”. Langmuir 35, 7050-7059 (2019). (Link) Xia Li; Jianchuan Liu; Ke Lin; Yun Zhang; Yunhong Zhang; Renhui Zheng; Qiang Shi; Yuan Guo; Zhou Lu*. “Toward Unraveling the Puzzle of Sum Frequency Generation Spectra at Interface of Aqueous Methanol Solution: Effects of Concentration-Dependent Hyperpolarizability”. Journal of Physical Chemistry C 123, 12975-12983 (2019).