乐善堂 - 华南师范大学 - 化学与环境学院

研究领域

⑴ 金属-有机骨架多孔材料的合成及应用研究。利用刚性及柔性带有多节点羧基或胺基配体为有机构筑基元，以过渡金属离子、主族金属离子、稀土离子或金属氧簇为无机构筑单元，合成具有特殊孔道、高孔体积、高比表面积的金属有机刚性及柔性骨架多孔材料，并对其热稳定性、气体吸附性能、气体分离性能、催化性能、发光性能、磁性性能、分子识别性能等性质进行系统的研究。 ⑵ 风湿病及类风湿病中药新药的研究。痹证（痹有闭的含义，即痹有闭塞、闭阻、不畅通的意思）是以经脉、肌肉、筋骨、关节等部位疼痛、重着、顽麻不仁、屈伸不利或关节肿大、僵直、畸形、肌肉萎缩为临床特征的一类疾病。由人体营、卫、气、血失调或气血亏损，腠理疏豁，以致风、寒、湿、热之邪乘虚袭入，壅塞经络，深入骨骱，久而为痹。相当于现代医学的骨关节疾病和部分胶原性结缔组织一类疾病。风湿热、风湿性关节炎、类风湿性关节炎、增生性脊柱炎、强直性脊柱炎、坐骨神经痛、肩关节周围炎、骨质增生等病均属本病范畴。治痹用药，尤如用兵，功在审证求因，妙在配伍应证，若久痹顽证者，较为难治。该类疾病严重影响人们的健康和生活质量。因此，根据博大精深的中医理论研究开发服用方便、副作用小、效果显著的治疗风湿病及类风湿病的中药新药具有重要意义。

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C.J. Chen, N. Wang, Y. Long, S.T. Yue*, Y.L. Liu. Series of novel 3D microporous heterometallic 3d-4f coordination frameworks with unique (7,8)-connected topology: Synthesis, crystal structure and magnetic properties, CrystEngComm, 2013, in press J.Y. Gao, N Wang, X.H. Xiong, C.J. Chen, W.P. Xie, X.R. Ran, Y. Long, Y.L. Liu, S.T. Yue*. Syntheses, Structures and Photoluminescent Properties of a Series of Zinc(II)-3-amino-1,2,4- triazolate Coordination Polymers Constructed by Varying Carboxylate Anions, CrystEngComm, 2013, in press X.P. Ye, W.J. Liu, N. Wang, S.T. Yue*. Interesting structure of self-assembly of gadolinium coordination polymers with tuned stoichiometric ratios, J. Coord. Chem., 2013, 66(2), 191-205 J.Y. Gao, C.J. Chen, X.H. Xiong, W.P. Xie, X.R. Ran, S.T. Yue*. Syntheses, structures, and fluorescence of two novel 2D ZnII layered frameworks based on 3-amino-1,2,4-triazole, Z. Anorg. Allg. Chem., 2013, 639, (3-4), 582-586 J.Y. Gao, X.H. Xiong, C.J. Chen, W.P. Xie, X.R. Ran, S.T. Yue*. Three novel 3D complexes constructed by 1H-benzimidazole-5,6-dicarboxylic acid: syntheses, crystal structures and luminescence, Z. Anorg. Allg. Chem., 2013, 639, (3-4), 538-542 J.Y. Gao, X.H. Xiong, C.J. Chen. W.P. Xie. X.R. Ran. S.T. Yue*, Y.L. Liu, Y.P. Cai. Effect of lanthanide contraction on structures of 3D lanthanide organic frameworks from 5-nitroisophthalic acid and picolinic acid. Inorg. Chem. Commun., 2013, 31, 5-12 C.J. Chen, X.P. Ye, J.Y. Gao, W.P. Xie, X.R. Ran, S.T. Yue*, Y.P. Cai. Auxiliary ligand-directed synthesis of four novel functional supramolecular metal-organic frameworks from 1-D chains to 3-D architectures, Inorg. Chem. Commun., 2013, 29, 4-10 X. Zhao, X.P. Ye, L.M. Chang, C.J. Chen, J.Y. Gao, S.T. Yue*, Y.P. Cai. Ligand-directed and Solvent- controlled assembly of six novel functional supramolecular metal-organic frameworks, Inorg. Chem. Commun., 2012, 25, 96-102 X. Zhao, D.X. Wang, Q. Chen, J.B. Chen, G.Y. Lin, S.T. Yue*, Y.P. Cai. Effect of lanthanide contraction on structures of lanthanide coordination polymers based on 5-aminoisophthalic acid and oxalate, Inorg. Chem. Commun., 2012, 23, 127-131 X. Zhao, X.P. Ye, L.M. Chang, Z.Q. Wei, W.J. Liu, S.T. Yue*, Y.L. Liu, H.H. Mo, Y.P. Cai. Two novel 3D microporous heterometallic 3d-4f coordination frameworks with unique (7, 8) -connected topology: Synthesis, crystal structure and magnetic properties, Inorg. Chem. Commun., 2012, 16, 95-99 Z.Q. Wei, S.T. Yue *, N. Wang, W.J. Liu, Y.L. Liu. Construction of a porous Na-Cd mixed-metal-organic framework based on mixed biphenyl-4,4’-dicarboxylate and benzotriazole, Monatsh Chem, 2012, 143(3), 421-425 C.J. Chen, J.Y. Gao, X. Zhao, L.M. Chang, Y.L. Liu, H.H Mo, S.T. Yue*, 3D Coordination Polymers with Chiral Structures, [Ln2(tda)2(H2O)3]•5H2O: Hydrothermal Synthesis, Structural Characterization, and Luminescent Properties, Z. Anorg. Allg. Chem., 2012, 638(14), 2324-2328 L.M. Chang, X. Zhao, Z.G. Gu, W.J. Liu, Z.Q. Wei, Y.L. Liu, H.H. Mo, S.T.Yue*. Four Ln(Ⅲ)-Mg(Ⅱ) metal organic frameworks containing fan-like helices and independent [Mg(H2O)6]2+ units，Z. Anorg. Allg. Chem., 2012, 638, (3-4), 652-657 X.X. Li, Z.Q. Wei, S.T. Yue*, N. Wang, H.H. Mo, Y.L. Liu. A new lanthanide coordination polymer with 4, 4'-oxybis (benzoic acid) Ligand: Hydrothermal Synthesis, Crystal Structures and Photo- luminescence, J. Chem. Crystallogr., 2011, 41(5), 757-761 W.J. Liu, Z.Y. Li, N. Wang, X.X. Li, Z.Q. Wei, S.T. Yue*, Y.L. Liu. A new family of 3D heterometallic 3d-4f organodisulfonate complexes based on the linkages of 2D [Ln(nds)(H2O)]+ layers and [Cu(ina)2]- chains. CrystEngComm, 2011, 13(1), 138-144 W.J. Liu, S.T. Yue*, Z.Q. Wei. Controllable assembly of organodisulfonate complexes with tuned mole ratios: from 0D to 3D networks, Inorg. Chem. Commun., 2011, 14, 1807-1814 S.T. Yue*, Z.Q. Wei, N. Wang, W.J. Liu, X. Zhao, L.M. Chang, Y.L. Liu, H.H. Mo, Y.P. Cai. Three novel microporous 3D heterometallic 3d-4f coordination polymers: synthesis, crystal structures and photoluminescence properties, Inorg. Chem. Commun., 2011, 14, 1396-1399 Z.Y. Li, J.W. Dai, N. Wang, H.H. Qiu, S.T. Yue*, Y.L. Liu. A Series of Three-Dimensional 4d-4f Heterometallic Coordination Polymers with (2,6)-Connected Doubly Interpenetrated pcu Net Topology: Structural, Photoluminescent and Magnetic Properties. Cryst. Growth Des., 2010, 10(6), 2746- 2751 (被 Chem Soc Rev, 2011, 40(2), 926-940 (IF=26.583) 正面引用) Z.Y. Li, J.W. Dai, S.T. Yue*, Y.L. Liu. Novel three-dimensional Ln-Ag 4d-4f heteropenta- metallic helix-based microporous metal-organic frameworks with unprecedented (3,4,5,6)- connected topology constructed from isonicotinate ligand. CrystEngComm, 2010, 12(7), 2014-2017 X.X. Li, S.T. Yue*, N. Wang, Z.Y. Li, Y.L. Liu. Three New Supramolecular Complexes Based on 2-Propyl-1H- imidazole-4,5-dicarboxylate :Synthesis, Structures and Properties. Z. Anorg. Allg. Chem., 2010, 636, 2481-2486