梁云 - 湖南师范大学 - 化学化工学院

研究领域

1. 通过构建碳硫键合成有机含硫化合物 2. 通过构建碳硅键合成有机硅化合物 3. 发展过渡金属催化的交叉偶联-串联反应策略

近期论文

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Yang, Y.; Zhou, L.; Yang, X.; Luo, X.; Deng, G.;Yang, Y.*;Liang, Y.* Synthesis of Phenanthrenes via Palladium-Catalyzed Three-Component Domino Reaction of Aryl Iodides, Internal Alkynes, ando-Bromobenzoic Acids, Synthesis 2020, 52, 1223-1230. Luo, X.; Li, W.; Lu, H.; Deng, G.;Yang, Y.*; Yang, C.*;Liang, Y.* Palladium-catalyzed cascade synthesis of spirocyclic oxindoles via regioselective C2-H arylation and C8-H alkylation of naphthalene ring, Chin. Chem. Lett. 2020, DOI: 10.1016/j.cclet.2020.07.005. Li, W.; Zhang, C.; Lu, H.; Wang, Y.; Deng, G.;Liang, Y.*;Yang, Y.*Pd-Catalyzed one-pot synthesis of vinylsilanes via a three-component tandem reaction. Org. Chem. Front. 2020, 7, 2075-2081. Lu, H.; Yang, X.; Zhou, L.; Li, W.; Deng, G.; Yang, Y.*;Liang, Y.* Palladium-catalyzed domino Heck-disilylation and -borylation of alkene-tethered 2-(2-halophenyl)-1H-indoles: access to diverse disilylated and borylated indolo[2,1-a]isoquinolines, Org. Chem. Front. 2020, 7, 2016-2021. Xiaoming Zhu,* Fuxing Zhang, Daizhi Kuang, Guobo Deng, Yuan Yang, Jiangxi Yu,* andYun Liang*, K2S as Sulfur Source and DMSO as Carbon Source for the Synthesis of 2‑Unsubstituted Benzothiazoles, Org.Lett., 2020, 22, 3789-3793. Xiaoming Zhu, Fengru Zhou, Yuan Yang, Guobo Deng,* andYun Liang*, Catalyst- and Additive-Free Method for the Synthesis of 2‑Substituted Benzothiazoles from Aromatic Amines, Aliphatic Amines, and Elemental Sulfur, ACS Omega 2020, 5, 13136-13147. Wenqi Chen, Xiaoming Zhu, Fei Wang, Yuan Yang, Guobo Deng,* andYun Liang*, Iodine-Catalyzed Three-Component Cascade Reaction for the Synthesis of Substituted 2‑Phenylnaphtho[1,3]selenazoles under Transition-Metal-Free Conditions, J. Org. Chem., 2020, 85, 3349-3357. Luo, X.; Zhou, L.; Lu, H.; Deng, G.;Liang, Y.*; Yang, C.*;Yang, Y.*Palladium-Catalyzed Domino Heck/C-H Activation/Decarboxylation: A Rapid Entry to Fused Isoquinolinediones and Isoquinolinones, Org. Lett. 2019,21, 9960. Li, W.; Chen, W.; Zhou, B.; Xu, Y.; Deng, G.;Liang, Y.*; Yang, Y.*NBE-Controlled Palladium-Catalyzed Interannular Selective C−H Silylation: Access to Divergent Silicon-Containing 1,1′-Biaryl-2- Acetamides, Org. Lett. 2019, 21, 2718. Yang, X.; Lu, H.; Zhu, X.; Zhou, L.; Deng, G.; Yang, Y.*;Liang, Y.*Palladium-Catalyzed Cascade Cyclization of Alkene-Tethered Aryl Halides with o‑Bromobenzoic Acids: Access to Diverse Fused Indolo[2,1‑a]isoquinolines, Org. Lett. 2019, 21, 7284. Chen, L.; Min, H.; Zeng, W.; Zhu, X.;Liang, Y.*; Deng, G.*; Yang, Y.*Transition-Metal-Free Sulfuration/Annulation of Alkenes: Economical Access to Thiophenes Enabled by the Cleavage of Multiple C−H Bonds, Org. Lett. 2018, 20, 7392. Yang, Y.; Zhou, B.; Zhu, X.; Deng, G.;Liang, Y.*; Yang, Y.*Palladium-Catalyzed Synthesis of Triphenylenes via Sequential C−H Activation and Decarboxylation, Org. Lett. 2018, 20, 5402. Luo, X.; Xu, Y.; Xiao, G.; Liu, W.; Qian, C.; Deng, G.; Song, J.;Liang, Y.*; Yang, C.*Palladium-Catalyzed Tandem Reaction of Three Aryl Iodides Involving Triple C−H Activation, Org. Lett. 2018, 20, 2997. Zhu, X.; Li, W.; Luo, X.; Deng, G.;Liang, Y.*; Liu, J.*A catalyst-free and additive-free method for the synthesis of benzothiazolethiones from o-iodoanilines, DMSO and potassium sulfide, Green Chem. 2018, 20, 1970. Xiao, G.; Chen, L.; Zhou, B.; Deng, G.; Gong, J.;Liang, Y.*Palladium-Catalyzed Domino Heck/Silylation Reaction for the Synthesis of (2-Oxoindolin-3-yl)methylsilanes via Trapping of the s-Alkylpalladium Intermediates with Disilanes, Adv. Synth. Catal. 2018, 360, 3477. Li, W.; Xiao, G.; Deng, G.;Liang, Y.*Pd-Catalyzed disilylation: an efficient route to 2,2’-bis(trimethylsilyl)biphenyls via trapping transient dibenzopalladacyclopentadienes with hexamethyldisilane, Org. Chem. Front. 2018, 5, 1488. Xu, Y.; Liu, X.; Chen, W.; Deng, G.;Liang, Y.*; Yang, Y.*Palladium/Norbornene Chemistry: Synthesis of Norbornene-Containing Arylsilanes Involving Double C−Si Bond Formation, J. Org. Chem. 2018, 83, 13930. Zheng, Z.; Chen, L.; Qian, C.; Zhu, X.; Yang, X.; Liu, J.*; Yang, Y.*;Liang, Y.*Copper-catalyzed synthesis of 2-acylbenzo[b]thiophenes from 3-(2-iodophenyl)-1-arylpropan-1-ones and potassium sulfide under aerobic conditions, Org. Biomol. Chem. 2018, 16, 8020. Zhou, B.; Chen, W.; Yang, Y.; Yang, Y.; Deng, G.*;Liang, Y.*A radical cyclization cascade of 2-alkynylbenzonitriles with sodium arylsulfinates, Org. Biomol. Chem. 2018, 16, 7959. Xiao, G.; Min, H.; Zheng, Z.; Deng, G.*;Liang, Y.*Copper-catalyzed three-component reaction of imidazo[1,2-a]pyridine with elemental sulfur and arylboronic acid to produce sulfenylimidazo[1,2-a]pyridines, Chin. Chem. Lett. 2018, 29, 1363. Xiao, G.; Chen, L.; Deng, G.; Liu, J.*;Liang, Y.*Disilylation of N-(2-Halophenyl)-2-phenylacrylamides with hexamethyldisilane via trapping the spirocyclic palladacycles, Tetrahedron Lett. 2018, 58, 1836. Liu, X.; Deng, G.*;Liang, Y.*Selective synthesis of benzo[4,5]imidazo[2,1-a]isoquinolines via coppercatalyzed tandem annulation of alkynylbenzonitriles with 2-Iodoanilines, Tetrahedron Lett. 2018, 58, 2844. Liu, W.; Min, H.; Zhu, X.; Deng, G.*;Liang, Y.*Copper-catalyzed highly selective synthesis of 2-benzyl- and 2-benzylidene-substituted benzo[b]thiazinones from 2-iodophenylcinnamamides and potassium sulfide, Org. Biomol. Chem., 2017, 15, 9804. Zhu, X.; Yang, Y.; Xiao, G.; Song, J.;Liang, Y.*; Deng, G.* Double C-S bond formation via C-H bond functionalization: synthesis of benzothiazoles and naphtho[2,1-d]thiazoles from N-substituted arylamines and elemental sulfur, Chem. Comm. 2017, 53, 11917. Dang, P.; Zheng, Z.;Liang, Y.*Copper-Catalyzed C(sp3)−S Bond and C(sp2)−S Bond Cross-Coupling of 2‑(2-Iodobenzoyl) Substituted or 2‑(2-Iodobenzyl) Substituted 1,2,3,4-Tetrahydroisoquinolines with Potassium Sulfide: Synthesis of Isoquinoline-Fused 1,3-Benzothiazine Scaffolds, J. Org. Chem. 2017, 82, 2263. Wu, L.; Deng, G.*;Liang, Y.* Synthesis of dibenzo[a,c]carbazoles from 2-(2-halophenyl)-indoles and iodobenzenes via palladium-catalyzed dual C–H functionalization, Org. Biomol. Chem., 2017, 15, 6808. Zhou, S.; Xia, G.;Liang, Y.*Copper-catalyzed synthesis of 2-sulfenylindoles from indoline-2-thiones and aryl iodides, Tetrahedron, Lett. 2017, 58, 338. Huang, H.; Dang, P.; Wu, L.;Liang, Y.*; Liu, J.*Copper-catalyzed synthesis of benzo[b]thiophene-fused imidazopyridines via the cleavage of C–H bond and C–X bond, Tetrahedron Lett. 2016, 57, 574. Zheng, Z.; Deng, G.;*Liang, Y.*Synthesis of quinolines through copper-catalyzed intermolecular cyclization reaction from anilines and terminal acetylene esters, RSC Adv. 2016, 6, 103478. Min, H.; Xiao, G.; Liu, W.;Liang, Y.*Copper-catalyzed synthesis of 2-aminobenzothiazoles from 2-iodophenyl isocyanides, potassium sulfide and amines, Org. Biomol. Chem., 2016, 14, 11088.