<br>钙钛矿型 ABO3 氧化物在光催化、电催化和固体氧化物燃料电池中的应用：最新技术与未来展望,Chemical Reviews

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钙钛矿型 ABO3 氧化物在光催化、电催化和固体氧化物燃料电池中的应用：最新技术与未来展望
Chemical Reviews ( IF 51.4 ) Pub Date : 2025-03-12 , DOI: 10.1021/acs.chemrev.4c00553
Muhammad Humayun _{1,

2} , Zhishan Li ₃ , Muhammad Israr ₄ , Abbas Khan ₅ , Wei Luo ₁ , Chundong Wang _{1,

2} , Zongping Shao ₆

Affiliation

由于光催化和电催化技术对于应对能源和环境挑战至关重要，因此人们投入了大量精力来探索先进的催化剂。其中，钙钛矿型 ABO₃ 氧化物由于其灵活的物理和化学性质而显示出非常有前途的催化活性。本文综述了钙钛矿型 ABO₃ 氧化物合成的基本原理和最新进展。我们详细描述了电催化析氧反应（OER）、氧还原反应（ORR）、析氢反应（HER）、氮还原反应（NRR）、二氧化碳还原反应（CO₂RR）和金属-空气电池的机理。此外，还综述了光催化分解水、CO₂ 转化、污染物降解和固氮。我们还强调了钙钛矿型 ABO₃ 氧化物在固体氧化物燃料电池（SOF）中的应用。最后，描述了钙钛矿型 ABO₃ 氧化物在各个领域的应用优化，并展望了当前和未来的挑战。本文旨在全面概述钙钛矿型 ABO₃ 氧化物基催化剂开发的最新进展及其在能源转换和环境修复中的应用，并为这些热门研究领域的未来发展提供路线图。

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Perovskite Type ABO3 Oxides in Photocatalysis, Electrocatalysis, and Solid Oxide Fuel Cells: State of the Art and Future Prospects

Since photocatalytic and electrocatalytic technologies are crucial for tackling the energy and environmental challenges, significant efforts have been put into exploring advanced catalysts. Among them, perovskite type ABO₃ oxides show great promising catalytic activities because of their flexible physical and chemical properties. In this review, the fundamentals and recent progress in the synthesis of perovskite type ABO₃ oxides are considered. We describe the mechanisms for electrocatalytic oxygen evolution reactions (OER), oxygen reduction reactions (ORR), hydrogen evolution reactions (HER), nitrogen reduction reactions (NRR), carbon dioxide reduction reactions (CO₂RR), and metal–air batteries in details. Furthermore, the photocatalytic water splitting, CO₂ conversion, pollutant degradation, and nitrogen fixation are reviewed as well. We also stress the applications of perovskite type ABO₃ oxides in solid oxide fuel cells (SOFs). Finally, the optimization of perovskite type ABO₃ oxides for applications in various fields and an outlook on the current and future challenges are depicted. The aim of this review is to present a broad overview of the recent advancements in the development of perovskite type ABO₃ oxides-based catalysts and their applications in energy conversion and environmental remediation, as well as to present a roadmap for future development in these hot research areas.

更新日期：2025-03-12

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