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Surface site design in photocatalytic carbon conversion applications
Coordination Chemistry Reviews ( IF 20.3 ) Pub Date : 2025-01-23 , DOI: 10.1016/j.ccr.2025.216459
Yi Zhang, Yixing Zhou, Molly Meng-Jung Li, Jun Di
Coordination Chemistry Reviews ( IF 20.3 ) Pub Date : 2025-01-23 , DOI: 10.1016/j.ccr.2025.216459
Yi Zhang, Yixing Zhou, Molly Meng-Jung Li, Jun Di
Photocatalysis offers innovative solutions to the pressing issues of energy scarcity and environmental pollution. Many photocatalytic reactions are related to the carbon conversion process. Therefore, the targeted construction of reaction-oriented photocatalysts is both meaningful but challenging. This review summarizes the most recent research achievements in the design of surface active sites on photocatalysts. The main functions of custom-made sites are described in details, such as light absorption, charge separation and interfacial reaction properties. Various methods for achieving precise site design on photocatalytic substrates are compiled, including surface exposure, interacting force, chemical bonding, multi-step integration and hybridization modification. Moreover, the review delves into the integral relationship between site design and photocatalytic applications, viewed through the lens of carbon atoms state transitions during reactions. Ultimately, we provide a prospective outline of the current challenges of site design and suggest potential trajectories for future investigations.
中文翻译:
光催化碳转化应用中的表面场地设计
光催化为能源稀缺和环境污染等紧迫问题提供创新解决方案。许多光催化反应与碳转化过程有关。因此,靶向构建反应导向的光催化剂既有意义又具有挑战性。本文总结了光催化剂表面活性位点设计的最新研究成果。详细描述了定制位点的主要功能,例如光吸收、电荷分离和界面反应特性。编译了在光催化底物上实现精确位点设计的各种方法,包括表面曝光、相互作用力、化学键合、多步整合和杂交修饰。此外,该综述通过反应过程中碳原子态转变的镜头深入探讨了位点设计和光催化应用之间的整体关系。最终,我们提供了场地设计当前挑战的前瞻性概述,并为未来的调查提出了潜在的轨迹。
更新日期:2025-01-23
中文翻译:
光催化碳转化应用中的表面场地设计
光催化为能源稀缺和环境污染等紧迫问题提供创新解决方案。许多光催化反应与碳转化过程有关。因此,靶向构建反应导向的光催化剂既有意义又具有挑战性。本文总结了光催化剂表面活性位点设计的最新研究成果。详细描述了定制位点的主要功能,例如光吸收、电荷分离和界面反应特性。编译了在光催化底物上实现精确位点设计的各种方法,包括表面曝光、相互作用力、化学键合、多步整合和杂交修饰。此外,该综述通过反应过程中碳原子态转变的镜头深入探讨了位点设计和光催化应用之间的整体关系。最终,我们提供了场地设计当前挑战的前瞻性概述,并为未来的调查提出了潜在的轨迹。