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Tuning interfacial charge transport via Ti–O–Sn bonds for efficient CO2 conversion
Chemical Communications ( IF 4.3 ) Pub Date : 2024-12-18 , DOI: 10.1039/d4cc05929h
Shikang Yin, Fan Zhou, Yiying Zhou, Yuming Sun, Binrong Li, Yingying Qin, Yan Yan, Pengwei Huo

Here, the clever design of forming an ohmic contact between SnS2 and MXene can regulate interfacial electron transport through Ti–O–Sn chemical bonds. This fast directional charge transport kinetics is attributed to the built-in electric field formed by the ohmic contact. As expected, the photoreduction CO2 activity of the optimized SSTC-5 catalyst is 10.4 times that of the original SnS2.

中文翻译:


通过 Ti-O-Sn 键调整界面电荷传输以实现高效的 CO2 转化



在这里,在 SnS 2 和 MXene 之间形成欧姆接触的巧妙设计可以调节通过 Ti-O-Sn 化学键的界面电子传递。这种快速定向电荷传输动力学归因于欧姆接触形成的内置电场。正如预期的那样,优化的 SSTC-5 催化剂的光还原 CO 2 活性是原始 SnS 2 的 10.4 倍。
更新日期:2024-12-19
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