当前位置: X-MOL 学术Nano-Micro Lett. › 论文详情
Our official English website, www.x-mol.net, welcomes your feedback! (Note: you will need to create a separate account there.)
Deciphering Water Oxidation Catalysts: The Dominant Role of Surface Chemistry over Reconstruction Degree in Activity Promotion
Nano-Micro Letters ( IF 31.6 ) Pub Date : 2024-11-26 , DOI: 10.1007/s40820-024-01562-7
Li An, Jianyi Li, Yuanmiao Sun, Jiamin Zhu, Justin Zhu Yeow Seow, Hong Zhang, Nan Zhang, Pinxian Xi, Zhichuan J. Xu, Chun-Hua Yan

  • Demonstrate that the key factor to determine the activity of reconstructed surfaces is the surface chemistry, instead of reconstruction degree using the popular perovskite LaNi1-xFexO3 oxides as model materials.

  • Fe content can influence both the surface reconstruction degree, the activation degree, and the activity of reconstructed surfaces.

  • The oxygen evolution reaction activity of reconstructed catalysts is primarily governed by the chemistry of the reconstructed surface species.



中文翻译:


破译水氧化催化剂:表面化学在活性促进中的主导作用超过重建度



  • 证明决定重建表面活性的关键因素是表面化学,而不是使用流行的钙钛矿 LaNi1-xFexO3 氧化物作为模型材料的重建程度。


  • Fe 含量可以影响表面重建程度、活化程度和重建表面的活性。


  • 重构催化剂的析氧反应活性主要受重构表面物质的化学性质控制。

更新日期:2024-11-26
down
wechat
bug