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Research and progress in catalyst modification for ZSM-5 zeolite catalyzed ethanol-to hydrocarbon reaction
Journal of Industrial and Engineering Chemistry ( IF 5.9 ) Pub Date : 2024-11-17 , DOI: 10.1016/j.jiec.2024.11.031
Yiyang Lin, Haitao Yin, Shuang Chen, Jiaqi Wang, Wen Li, Yining Gao, Mingyuan Sheng, Nanzhe Jiang

Ethanol-to-hydrocarbons (ETH) conversion represents a pivotal reaction in non-homogeneous catalysis, offering a sustainable solution for the production of significant platform chemicals, including olefins, gasoline, and aromatics. However, it is imperative to continue enhancing the catalytic efficiency and extending the operational longevity of the catalysts. This review presents a comprehensive overview of the latest research developments in the field of catalytic conversion of ethanol to hydrocarbons. It emphasizes the pivotal role of zeolite catalysts in the conversion of ethanol to hydrocarbons and offers insights into the recent scientific discoveries pertaining to the reaction mechanism of ETH conversion. In addition, we investigate the catalyst optimization and design, with the objective of enhancing the selectivity of the target product and prolonging the catalyst life. This topic has not been fully addressed in recent reviews. The aim of this review is to offer theoretical insights into the ETH reaction mechanism and to guide the development of more efficient ETH catalysts.

中文翻译:


ZSM-5 分子筛催化乙醇制烃反应催化剂改性的研究进展



乙醇制碳氢化合物 (ETH) 转化是非均相催化中的关键反应,为烯烃、汽油和芳烃等重要平台化学品的生产提供了可持续的解决方案。然而,必须继续提高催化效率并延长催化剂的使用寿命。本文全面概述了乙醇催化转化为碳氢化合物领域的最新研究进展。它强调了沸石催化剂在乙醇转化为碳氢化合物中的关键作用,并提供了对与 ETH 转化反应机制有关的最新科学发现的见解。此外,我们还研究了催化剂的优化和设计,以提高目标产品的选择性并延长催化剂的使用寿命。在最近的综述中,该主题尚未得到充分讨论。本文的目的是为 ETH 反应机理提供理论见解,并指导开发更高效的 ETH 催化剂。
更新日期:2024-11-17
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