The rise in global temperatures and environmental contamination resulting from traditional fossil fuel usage has prompted a search for alternative energy sources. Utilizing solar energy to drive the direct splitting of water for hydrogen production has emerged as a promising solution to these challenges. Covalent organic frameworks (COFs) are ordered, crystalline materials made up of organic molecules linked by covalent bonds, featuring permanent porosity and a wide range of structural topologies. COFs serve as suitable platforms for solar‐driven water splitting to produce hydrogen, as their building blocks can be tailored to possess adjustable band gaps, charge separation capabilities, porosity, wettability, and chemical stability. Here, the impact of the interface in the context of the photocatalytic reaction is focused and propose strategies to enhance the hydrogen production performance of COFs photocatalysis. In particular, how hybrid photocatalytic interfaces affect photocatalytic performance is focused.

中文翻译：

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界面对共价有机框架光催化制氢性能的影响


全球气温上升和传统化石燃料使用造成的环境污染促使人们寻找替代能源。利用太阳能驱动水的直接分解以生产氢气已成为应对这些挑战的有前途的解决方案。共价有机框架 （COF） 是由共价键连接的有机分子组成的有序结晶材料，具有永久孔隙率和广泛的结构拓扑结构。COF 可作为太阳能驱动水分解以产生氢气的合适平台，因为它们的构建单元可以定制为具有可调节的带隙、电荷分离能力、孔隙率、润湿性和化学稳定性。在这里，界面对光催化反应的影响受到关注，并提出了提高 COF 光催化产氢性能的策略。特别是，杂化光催化界面如何影响光催化性能是重点。